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Taprogge, J. et al, Gadea, A., & Montaner-Piza, A. (2014). Identification of a millisecond isomeric state in Cd-129(81) via the detection of internal conversion and Compton electrons. Phys. Lett. B, 738, 223–227.
Abstract: The decay of an isomeric state in the neutron-rich nucleus Cd-129 has been observed via the detection of internal conversion and Compton electrons providing first experimental information on excited states in this nucleus. The isomer was populated in the projectile fission of a U-238 beam at the Radioactive Isotope Beam Factory at RIKEN. From the measured yields of gamma-rays and internal conversion electrons, a multipolarity of E3 was tentatively assigned to the isomeric transition. A half-life of T-1/2 = 3.6(2) ms was determined for the new state which was assigned a spin of (21/2(+)), based on a comparison to shell model calculations performed using state-of-the-art realistic effective interactions.
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Kucuk, L. et al, Orrigo, S. E. A., Montaner-Piza, A., Rubio, B., Gelletly, W., Algora, A., et al. (2017). Half-life determination of T-z =-1 and T-z =-1/2 proton-rich nuclei and the beta decay of Zn-58. Eur. Phys. J. A, 53(6), 134–10pp.
Abstract: We have measured the beta-decay half-lives of 16 neutron-deficient nuclei with T-z = -1/2 and -1, ranging from chromium to germanium. They were produced in an experiment carried out at GANIL and optimized for the production of Zn-58, for which in addition we present the decay scheme and absolute Fermi and Gamow-Teller transition strengths. Since all of these nuclei lie on the rp-process pathway, the T-1/2 values are important ingredients for the rp-process reaction flow calculations and for models of X-ray bursters.
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Jungclaus, A. et al, Gadea, A., & Montaner-Piza, A. (2016). First observation of gamma rays emitted from excited states south-east of Sn-132: The pi g(9/2)(-1) circle times nu f(7/2) multiplet of In-132(83). Phys. Rev. C, 93(4), 041301–6pp.
Abstract: For the first time, the gamma decay of excited states has been observed in a nucleus situated in the quadrant south-east of doubly magic Sn-132, a region in which experimental information so far is limited to ground-state properties. Six gamma rays with energies of 50, 86, 103, 227, 357, and 602 keV were observed following the beta-delayed neutron emission from Cd-133(85), populated in the projectile fission of a U-238 beam at the Radioactive Isotope Beam Factory at RIKEN within the EURICA project. The new experimental information is compared to the results of a modern realistic shell-model calculation, the first one in this region very far from stability, focusing in particular on the pi 0g(9/2)(-1) circle times nu 1f(7/2) particle-hole multiplet in In-132(83). In addition, theoretical estimates based on a scaling of the two-body matrix elements for the pi h(11/2)(-1) circle times nu g(9/2) analog multiplet in Tl-208(127), one major proton and one major neutron shell above, are presented.
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Caballero-Folch, R. et al, Agramunt, J., Tain, J. L., Algora, A., Domingo-Pardo, C., Guadilla, V., et al. (2018). First determination of beta-delayed multiple neutron emission beyond A=100 through direct neutron measurement: The P-2n value of Sb-136. Phys. Rev. C, 98(3), 034310–10pp.
Abstract: Background: beta-delayed multiple neutron emission has been observed for some nuclei with A <= 100 being the Rb-100 the heaviest beta 2n emitter measured to date. So far only 25 P-2n values have been determined for the approximate to 300 nuclei that may decay in this way. Accordingly it is of interest to measure P-2n values for the other possible multiple neutron emitters throughout the chart of the nuclides. It is of particular interest to make such a measurement for nuclei with A > 100 to test the predictions of theoretical models and simulation tools for the decays of heavy nuclei in the region of very neutron-rich nuclei. In addition the decay properties of these nuclei are fundamental for the understanding of astrophysical nucleosynthesis processes such as the r-process and safety inputs for nuclear reactors. Purpose: To determine for the first time the two-neutron branching ratio the P-2n value for Sb-136 through a direct neutron measurement and to provide precise P-1n values for Sb-136 and Te-136. Method: A pure beam of each isotope of interest was provided by the JYFLTRAP Penning trap at the Ion Guide Isotope Separator On-Line (IGISOL) facility of the University of Jyvaskyla Finland. The purified ions were implanted into a moving tape at the end of the beam line. The detection setup consisted of a plastic scintillator placed right behind the implantation point after the tape to register the beta decays and the BELEN detector based on neutron counters embedded in a polyethylene matrix. The analysis was based on the study of the beta- and neutron-growth-and-decay curves and the beta-one-neutron and beta-two-neutron time correlations which allowed us the determination of the neutron branching ratios. Results: The P-2n value of Sb-136 was found to be 0.14(3)% and the measured P-1n values for Sb-136 and Te-136 were found to be 32.2(15)% and 1.47(6)% respectively. Conclusions: The measured P-2n value is a factor 44 smaller than predicted by the finite-range droplet model plus the quasiparticle random-phase approximation (FRDM+QRPA) model used for r-process calculations.
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Guadilla, V. et al, Algora, A., Tain, J. L., Agramunt, J., Jordan, M. D., Montaner-Piza, A., et al. (2017). Experimental study of Tc-100 beta decay with total absorption gamma-ray spectroscopy. Phys. Rev. C, 96(1), 014319–10pp.
Abstract: The beta decay of Tc-100 has been studied by using the total absorption gamma-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility in Jyvaskyla. In this work the new Decay Total Absorption gamma-ray Spectrometer in coincidence with a cylindrical plastic beta detector has been employed. The beta intensity to the ground state obtained from the analysis is in good agreement with previous high-resolution measurements. However, differences in the feeding to the first-excited state as well as weak feeding to a new level at high excitation energy have been deduced from this experiment. Theoretical calculations performed in the quasiparticle random-phase approximation framework are also reported. Comparison of these calculations with our measurement serves as a benchmark for calculations of the double beta decay of Mo-100.
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Jungclaus, A. et al, Gadea, A., & Montaner-Piza, A. (2024). Excited-State Half-Lives in 130 Cd and the Isospin Dependence of Effective Charges. Phys. Rev. Lett., 132(22), 222501–7pp.
Abstract: The known I pi = 8 & thorn; 1 , E x = 2129-keV isomer in the semimagic nucleus 130 Cd 82 was populated in the projectile fission of a 238 U beam at the Radioactive Isotope Beam Factory at RIKEN. The high counting statistics of the accumulated data allowed us to determine the excitation energy, E x = 2001.2(7) keV, and half-life, T 1 =2 = 57(3) ns, of the I pi = 6 & thorn; 1 state based on gamma gamma coincidence information. Furthermore, the halflife of the 8 & thorn; 1 state, T 1 =2 = 224(4) ns, was remeasured with high precision. The new experimental information, combined with available data for 134 Sn and large-scale shell model calculations, allowed us to extract proton and neutron effective charges for 132 Sn, a doubly magic nucleus far -off stability. A comparison to analogous information for 100 Sn provides first reliable information regarding the isospin dependence of the isoscalar and isovector effective charges in heavy nuclei.
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Jungclaus, A. et al, & Montaner-Piza, A. (2020). Evolution of proton single-particle states in neutron-rich Sb isotopes beyond N=82. Phys. Rev. C, 102(3), 034324–11pp.
Abstract: The beta decay of the semimagic Sn isotopes Sn-136,Sn-137,Sn-138 has been studied at the Radioactive Isotope Beam Factory at the RIKEN Nishina Center. The first experimental information on excited states was obtained for Sb-137 while, in the case of Sb-136, the established excitation scheme could be extended by ten previously unidentified levels. In the decay of the most-neutron-rich isotope Sn-138, two gamma rays were observed for the first time. The new experimental results, in combination with state-of-the-art shell-model calculations, provide the first information with respect to the evolution of the Og(7/2) and 1d(5/2) proton single-particle states with increasing neutron number beyond N = 84.
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Guadilla, V. et al, Tain, J. L., Algora, A., Agramunt, J., Jordan, D., Monserrate, M., et al. (2020). Determination of beta-decay ground state feeding of nuclei of importance for reactor applications. Phys. Rev. C, 102(6), 064304–12pp.
Abstract: In beta-decay studies the determination of the decay probability to the ground state (g.s.) of the daughter nucleus often suffers from large systematic errors. The difficulty of the measurement is related to the absence of associated delayed gamma-ray emission. In this work we revisit the 4 pi gamma – beta method proposed by Greenwood and collaborators in the 1990s, which has the potential to overcome some of the experimental difficulties. Our interest is driven by the need to determine accurately the beta-intensity distributions of fission products that contribute significantly to the reactor decay heat and to the antineutrinos emitted by reactors. A number of such decays have large g.s. branches. The method is relevant for nuclear structure studies as well. Pertinent formulas are revised and extended to the special case of beta-delayed neutron emitters, and the robustness of the method is demonstrated with synthetic data. We apply it to a number of measured decays that serve as test cases and discuss the features of the method. Finally, we obtain g.s. feeding intensities with reduced uncertainty for four relevant decays that will allow future improvements in antineutrino spectrum and decay heat calculations using the summation method.
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Guadilla, V. et al, Algora, A., Tain, J. L., Agramunt, J., Jordan, D., Monserrate, M., et al. (2017). Characterization of a cylindrical plastic beta-detector with Monte Carlo simulations of optical photons. Nucl. Instrum. Methods Phys. Res. A, 854, 134–138.
Abstract: In this work we report on the Monte Carlo study performed to understand and reproduce experimental measurements of a new plastic beta-detector with cylindrical geometry. Since energy deposition simulations differ from the experimental measurements for such a geometry, we show how the simulation of production and transport of optical photons does allow one to obtain the shapes of the experimental spectra. Moreover, taking into account the computational effort associated with this kind of simulation, we develop a method to convert the simulations of energy deposited into light collected, depending only on the interaction point in the detector. This method represents a useful solution when extensive simulations have to be done, as in the case of the calculation of the response function of the spectrometer in a total absorption gamma-ray spectroscopy analysis.
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Guadilla, V. et al, Tain, J. L., Algora, A., Agramunt, J., Gelletly, W., Jordan, D., et al. (2018). Characterization and performance of the DTAS detector. Nucl. Instrum. Methods Phys. Res. A, 910, 79–89.
Abstract: DTAS is a segmented total absorption y-ray spectrometer developed for the DESPEC experiment at FAIR. It is composed of up to eighteen NaI(Tl) crystals. In this work we study the performance of this detector with laboratory sources and also under real experimental conditions. We present a procedure to reconstruct offline the sum of the energy deposited in all the crystals of the spectrometer, which is complicated by the effect of NaI(Tl) light-yield non-proportionality. The use of a system to correct for time variations of the gain in individual detector modules, based on a light pulse generator, is demonstrated. We describe also an event-based method to evaluate the summing-pileup electronic distortion in segmented spectrometers. All of this allows a careful characterization of the detector with Monte Carlo simulations that is needed to calculate the response function for the analysis of total absorption gamma-ray spectroscopy data. Special attention was paid to the interaction of neutrons with the spectrometer, since they are a source of contamination in studies of beta-delayed neutron emitting nuclei.
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