|
|
n_TOF Collaboration(Bacak, M. et al), Domingo-Pardo, C., & Tain, J. L. (2020). A compact fission detector for fission-tagging neutron capture experiments with radioactive fissile isotopes. Nucl. Instrum. Methods Phys. Res. A, 969, 163981–10pp.
Abstract: In the measurement of neutron capture cross-sections of fissile isotopes, the fission channel is a source of background which can be removed efficiently using the so-called fission-tagging or fission-veto technique. For this purpose a new compact and fast fission chamber has been developed. The design criteria and technical description of the chamber are given within the context of a measurement of the U-233(n, gamma) cross-section at the nTOF facility at CERN, where it was coupled to the nTOF Total Absorption Calorimeter. For this measurement the fission detector was optimized for time resolution, minimization of material in the neutron beam and for alpha-fission discrimination. The performance of the fission chamber and its application as a fission tagging detector are discussed.
|
|
|
|
Ciemala, M. et al, Domingo-Pardo, C., & Perez-Vidal, R. M. (2020). Testing ab initio nuclear structure in neutron-rich nuclei: Lifetime measurements of second 2(+) state in C-16 and O-20. Phys. Rev. C, 101(2), 021303–7pp.
Abstract: To test the predictive power of ab initio nuclear structure theory, the lifetime of the second 2(+) state in neutron-rich O-20, tau(2(2)(+)) = 150(-30)(+80) fs, and an estimate for the lifetime of the second 2(+) state in C-16 have been obtained for the first time. The results were achieved via a novel Monte Carlo technique that allowed us to measure nuclear state lifetimes in the tens-to-hundreds of femtoseconds range by analyzing the Doppler-shifted gamma-transition line shapes of products of low-energy transfer and deep-inelastic processes in the reaction O-18 (7.0 MeV/u) + Ta-181. The requested sensitivity could only be reached owing to the excellent performances of the Advanced gamma-Tracking Array AGATA, coupled to the PARIS scintillator array and to the VAMOS++ magnetic spectrometer. The experimental lifetimes agree with predictions of ab initio calculations using two- and three-nucleon interactions, obtained with the valence-space in-medium similarity renormalization group for O-20 and with the no-core shell model for C-16. The present measurement shows the power of electromagnetic observables, determined with high-precision gamma spectroscopy, to assess the quality of first-principles nuclear structure calculations, complementing common benchmarks based on nuclear energies. The proposed experimental approach will be essential for short lifetime measurements in unexplored regions of the nuclear chart, including r-process nuclei, when intense beams, produced by Isotope Separation On-Line (ISOL) techniques, become available.
|
|
|
|
AGATA Collaboration(Cederwall, B. et al), Gadea, A., Jurado, M., Domingo-Pardo, C., Huyuk, T., & Perez-Vidal, R. M. (2020). Isospin Properties of Nuclear Pair Correlations from the Level Structure of the Self-Conjugate Nucleus Ru-88. Phys. Rev. Lett., 124(6), 062501–6pp.
Abstract: The low-lying energy spectrum of the extremely neutron-deficient self-conjugate (N = Z) nuclide Ru-88(44)44 has been measured using the combination of the Advanced Gamma Tracking Array (AGATA) spectrometer, the NEDA and Neutron Wall neutron detector arrays, and the DIAMANT charged particle detector array. Excited states in Ru-88 were populated via the Fe-54(Ar-36, 2n gamma)Ru-88* fusion-evaporation reaction at the Grand Accelerateur National d'Ions Lourds (GANIL) accelerator complex. The observed gamma-ray cascade is assigned to Ru-88 using clean prompt gamma-gamma-2-neutron coincidences in anticoincidence with the detection of charged particles, confirming and extending the previously assigned sequence of low-lying excited states. It is consistent with a moderately deformed rotating system exhibiting a band crossing at a rotational frequency that is significantly higher than standard theoretical predictions with isovector pairing, as well as observations in neighboring N > Z nuclides. The direct observation of such a “delayed” rotational alignment in a deformed N = Z nucleus is in agreement with theoretical predictions related to the presence of strong isoscalar neutron-proton pair correlations.
|
|
|
|
Babiano, V., Balibrea, J., Caballero, L., Calvo, D., Ladarescu, I., Mira Prats, S., et al. (2020). First i-TED demonstrator: A Compton imager with Dynamic Electronic Collimation. Nucl. Instrum. Methods Phys. Res. A, 953, 163228–9pp.
Abstract: i-TED consists of both a total energy detector and a Compton camera primarily intended for the measurement of neutron capture cross sections by means of the simultaneous combination of neutron time-of-flight (TOF) and gamma-ray imaging techniques. TOF allows one to obtain a neutron-energy differential capture yield, whereas the imaging capability is intended for the discrimination of radiative background sources, that have a spatial origin different from that of the capture sample under investigation. A distinctive feature of i-TED is the embedded Dynamic Electronic Collimation (DEC) concept, which allows for a trade-off between efficiency and image resolution. Here we report on some general design considerations and first performance characterization measurements made with an i-TED demonstrator in order to explore its gamma-ray detection and imaging capabilities.
|
|
|
|
AGATA Collaboration(Goldkuhle, A. et al), Perez-Vidal, R. M., Domingo-Pardo, C., & Gadea, A. (2019). Lifetime measurements in Ti-52,Ti-54 to study shell evolution toward N=32. Phys. Rev. C, 100(5), 054317–12pp.
Abstract: Lifetimes of the excited states in the neutron-rich Ti-52,Ti-54 nuclei, produced in a multinucleon-transfer reaction, were measured by employing the Cologne plunger device and the recoil-distance Doppler-shift method. The experiment was performed at the Grand Accelerateur National d'Ions Lourds facility by using the Advanced Gamma Tracking Array for the gamma-ray detection, coupled to the large-acceptance variable mode spectrometer for an event-by-event particle identification. A comparison between the transition probabilities obtained from the measured lifetimes of the 2(1)(+) to 8(1)(+) yrast states in Ti-52,Ti-54 and that from the shell-model calculations based on the well-established GXPF1A, GXPF1B, and KB3G fp shell interactions support the N = 32 subshell closure. The B(E2) values for Ti-52 determined in this work are in disagreement with the known data, but are consistent with the predictions of the shell-model calculations and reduce the previously observed pronounced staggering across the even-even titanium isotopes.
|
|
|
|
n_TOF Collaboration(Gawlik, A. et al), Domingo-Pardo, C., Tain, J. L., & Tarifeño-Saldivia, A. (2019). Measurement of the Ge-70(n, gamma) cross section up to 300 keV at the CERN n_TOF facility. Phys. Rev. C, 100(4), 045804–10pp.
Abstract: Neutron capture data on intermediate mass nuclei are of key importance to nucleosynthesis in the weak component of the slow neutron capture processes, which occurs in massive stars. The (n,gamma) cross section on Ge-70, which is mainly produced in the s process, was measured at the neutron time-of-flight facility n_TOF at CERN. Resonance capture kernels were determined up to 40 keV neutron energy and average cross sections up to 300 keV. Stellar cross sections were calculated from kT = 5 keV to kT = 100 keV and are in very good agreement with a previous measurement by Walter and Beer (1985) and recent evaluations. Average cross sections are in agreement with Walter and Beer (1985) over most of the neutron energy range covered, while they are systematically smaller for neutron energies above 150 keV. We have calculated isotopic abundances produced in s-process environments in a 25 solar mass star for two initial metallicities (below solar and close to solar). While the low metallicity model reproduces best the solar system germanium isotopic abundances, the close to solar model shows a good global match to solar system abundances in the range of mass numbers A = 60-80.
|
|
|
|
Guerrero, C., Tessler, M., Paul, M., Lerendegui-Marco, J., Heinitz, S., Maugeri, E. A., et al. (2019). The s-process in the Nd-Pm-Sm region: Neutron activation of Pm-147. Phys. Lett. B, 797, 134809–6pp.
Abstract: The Nd-Pm-Sm branching is of interest for the study of the s-process, related to the production of heavy elements in stars. As Sm-148 and Sm-150 are s-only isotopes, the understanding of the branching allows constraining the s-process neutron density. In this context the key physics input needed is the cross section of the three unstable nuclides in the region: Nd-147 (10.98 d half-life), Pm-147 (2.62 yr) and Pm-148 (5.37 d). This paper reports on the activation measurement of Pm-147, the longest-lived of the three nuclides. The cross section measurement has been carried out by activation at the SARAF LiLiT facility using a 56(2) μg target. Compared to the single previous measurement of Pm-147, the measurement presented herein benefits from a target 2000 times more massive. The resulting Maxwellian Averaged Cross Section (MACS) to the ground and metastable states in Pm-148 are 469(50) mb and 357(27) mb. These values are 41% higher (to the ground state) and 15% lower (to the metastable state) than the values reported so far, leading however to a total cross section of 826(107) mb consistent within uncertainties with the previous result and hence leaving unchanged the previous calculation of the s-process neutron density.
|
|
|
|
Boso, A. et al, Domingo-Pardo, C., & Perez-Vidal, R. M. (2019). Isospin dependence of electromagnetic transition strengths among an isobaric triplet. Phys. Lett. B, 797, 134835–6pp.
Abstract: Electric quadrupole matrix elements, M-p, for the J(pi) = 2(+) -> 0(+), Delta T = 0, T = 1 transitions across the A = 46 isobaric multiplet Cr-46-V-46-Ti-46 have been measured at GSI with the FRS-LYCCA-AGATA setup. This allows direct insight into the isospin purity of the states of interest by testing the linearity of M-p with respect to T-z. Pairs of nuclei in the T = 1 triplet were studied using identical reaction mechanisms in order to control systematic errors. The M-p values were obtained with two different methodologies: (i) a relativistic Coulomb excitation experiment was performed for Cr-46 and Ti-46; (ii) a “stretched target” technique was adopted here, for the first time, for lifetime measurements in V-46 and Ti-46. A constant value of M-p across the triplet has been observed. Shell-model calculations performed within the fp shell fail to reproduce this unexpected trend, pointing towards the need of a wider valence space. This result is confirmed by the good agreement with experimental data achieved with an interaction which allows excitations from the underlying sd shell. A test of the linearity rule for all published data on complete T = 1 isospin triplets is presented.
|
|
|
|
Yokoyama, R. et al, Tain, J. L., Algora, A., Agramunt, J., Domingo-Pardo, C., Morales, A. I., et al. (2019). Strong one-neutron emission from two-neutron unbound states in beta decays of the r-process nuclei Ga-86,Ga-87. Phys. Rev. C, 100(3), 031302–6pp.
Abstract: beta-delayed one-neutron and two-neutron branching ratios (P-1n and P-2n) have been measured in the decay of A = 84 to 87 Ga isotopes at the Radioactive-Isotope Beam Factory (RIBF) at the RIKEN Nishina Center using a high-efficiency array of He-3 neutron counters (BRIKEN). Two-neutron emission was observed in the decay of Ga-84,Ga-85,Ga-87 for the first time and the branching ratios were measured to be P-2n = 1.6(2)%, 1.3(2)%, and 10.2(28)(stat)(5)(sys)%, respectively. One-neutron branching ratio of Ga-87 (P-1n = 81(9)(stat)(8)(sys)%) and half-life of 29(4) ms were measured for the first time. The branching ratios of Ga-86 were also measured to be P-1n = 74(2)(stat)(8)(sys)% and 16.2(9)(stat)(6)(sys)% with better precision than a previous study. The observation that P-1n > P-2n for both Ga-86,Ga-87 was unexpected and is interpreted as a signature of dominating one-neutron emission from the two-neutron unbound excited states in Ge-86,Ge-87. In order to interpret the experimental results, shell-model and Hauser-Feshbach statistical model calculations of delayed particle and gamma-ray emission probabilities were performed. This model framework reproduces the experimental results. The shell model alone predicts P-2n significantly larger than P-1n for the Ga-87 decay, and it is necessary to invoke a statistical description to successfully explain the observation that P-1n > P-2n. Our new results demonstrate the relevance and importance of a statistical description of neutron emission for the prediction of the decay properties of multineutron emitters and that it must be included in the r-process modeling.
|
|
|
|
n_TOF Collaboration(Amaducci, S. et al), Domingo-Pardo, C., & Tain, J. L. (2019). Measurement of the U-235(n, f) cross section relative to the Li-6(n, t) and B-10(n,alpha) standards from thermal to 170 keV neutron energy range at n_TOF. Eur. Phys. J. A, 55(7), 120–19pp.
Abstract: .The U-235(n, f ) cross section was measured at n_TOF relative to Li-6(n, t) and B-10(n,alpha) , with high resolution ( L=183.49(2) m) and in a wide energy range (25meV-170keV) with 1.5% systematic uncertainty, making use of a stack of six samples and six silicon detectors placed in the neutron beam. This allowed us to make a direct comparison of the yields of the U-235(n, f ) and of the two reference reactions under the same experimental conditions, and taking into account the forward/backward emission asymmetry. A hint of an anomaly in the 10-30keV neutron energy range had been previously observed in other experiments, indicating a cross section systematically lower by several percent relative to major evaluations. The present results indicate that the cross section in the 9-18keV neutron energy range is indeed overestimated by almost 5% in the recently released evaluated data files ENDF/B-VIII.0 and JEFF3.3, as a consequence of a 7% overestimate in a single GMA node in the IAEA reference file. Furthermore, these new high-resolution data confirm the existence of resonance-like structures in the keV neutron energy region. The results here reported may lead to a reduction of the uncertainty in the 1-100keV neutron energy region. Finally, from the present data, a value of 249.7 +/- 1.4( stat )+/- 0.94( syst ) b<bold>eV has been extracted for the cross section integral between </bold>7.8 and 11eV, confirming the value of 247.5 +/- 3 b<bold>eV recently established as a standard</bold>.
|
|
