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n_TOF Collaboration(Mazzone, A. et al), Babiano-Suarez, V., Caballero, L., Domingo-Pardo, C., Ladarescu, I., & Tain, J. L. (2020). Measurement of the Gd-154(n, gamma) cross section and its astrophysical implications. Phys. Lett. B, 804, 135405–6pp.
Abstract: The neutron capture cross section of Gd-154 was measured from 1 eV to 300 keV in the experimental area located 185 m from the CERN n_TOF neutron spallation source, using a metallic sample of gadolinium, enriched to 67% in Gd-154. The capture measurement, performed with four C6D6 scintillation detectors, has been complemented by a transmission measurement performed at the GELINA time-of-flight facility (JRC-Geel), thus minimising the uncertainty related to sample composition. An accurate Maxwellian averaged capture cross section (MACS) was deduced over the temperature range of interest for s process nucleosynthesis modelling. We report a value of 880(50) mb for the MACS at kT = 30 keV, significantly lower compared to values available in literature. The new adopted Gd-154(n, gamma) cross section reduces the discrepancy between observed and calculated solar s-only isotopic abundances predicted by s-process nucleosynthesis models.
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Babiano, V., Balibrea, J., Caballero, L., Calvo, D., Ladarescu, I., Mira Prats, S., et al. (2020). First i-TED demonstrator: A Compton imager with Dynamic Electronic Collimation. Nucl. Instrum. Methods Phys. Res. A, 953, 163228–9pp.
Abstract: i-TED consists of both a total energy detector and a Compton camera primarily intended for the measurement of neutron capture cross sections by means of the simultaneous combination of neutron time-of-flight (TOF) and gamma-ray imaging techniques. TOF allows one to obtain a neutron-energy differential capture yield, whereas the imaging capability is intended for the discrimination of radiative background sources, that have a spatial origin different from that of the capture sample under investigation. A distinctive feature of i-TED is the embedded Dynamic Electronic Collimation (DEC) concept, which allows for a trade-off between efficiency and image resolution. Here we report on some general design considerations and first performance characterization measurements made with an i-TED demonstrator in order to explore its gamma-ray detection and imaging capabilities.
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Babiano, V., Caballero, L., Calvo, D., Ladarescu, I., Olleros, P., & Domingo-Pardo, C. (2019). gamma-Ray position reconstruction in large monolithic LaCl3(Ce) crystals with SiPM readout. Nucl. Instrum. Methods Phys. Res. A, 931, 1–22.
Abstract: We report on the spatial response characterization of large LaCl3(Ce) monolithic crystals optically coupled to 8 x 8 pixel silicon photomultiplier (SiPM) sensors. A systematic study has been carried out for 511 keV gamma-rays using three different crystal thicknesses of 10 mm, 20 mm and 30 mm, all of them with planar geometry and a base size of 50 x 50 mm(2). In this work we investigate and compare two different approaches for the determination of the main gamma-ray hit location. On one hand, methods based on the fit of an analytical model for the scintillation light distribution provide the best results in terms of linearity and field of view, with spatial resolutions close to similar to 1 mm FWHM. On the other hand, position reconstruction techniques based on neural networks provide similar linearity and field-of-view, becoming the attainable spatial resolution similar to 3 mm FWHM. For the third space coordinate z or depth-of-interaction we have implemented an inverse linear calibration approach based on the cross-section of the measured scintillation-light distribution at a certain height. The detectors characterized in this work are intended for the development of so-called Total Energy Detectors with Compton imaging capability (i-TED), aimed at enhanced sensitivity and selectivity measurements of neutron capture cross sections via the time-of-flight (TOF) technique.
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Olleros, P., Caballero, L., Domingo-Pardo, C., Babiano, V., Ladarescu, I., Calvo, D., et al. (2018). On the performance of large monolithic LaCl3(Ce) crystals coupled to pixelated silicon photosensors. J. Instrum., 13, P03014–17pp.
Abstract: We investigate the performance of large area radiation detectors, with high energy-and spatial-resolution, intended for the development of a Total Energy Detector with gamma-ray imaging capability, so-called i-TED. This new development aims for an enhancement in detection sensitivity in time-of-flight neutron capture measurements, versus the commonly used C6D6 liquid scintillation total-energy detectors. In this work, we study in detail the impact of the readout photosensor on the energy response of large area (50 x 50 mm(2)) monolithic LaCl3(Ce) crystals, in particular when replacing a conventional mono-cathode photomultiplier tube by an 8 x 8 pixelated silicon photomultiplier. Using the largest commercially available monolithic SiPM array (25 cm(2)), with a pixel size of 6 x 6 mm(2), we have measured an average energy resolution of 3.92% FWHM at 662 keV for crystal thick-nesses of 10, 20 and 30 mm. The results are confronted with detailed Monte Carlo (MC) calculations, where optical processes and properties have been included for the reliable tracking of the scintillation photons. After the experimental validation of the MC model, we use our MC code to explore the impact of a smaller photosensor segmentation on the energy resolution. Our optical MC simulations predict only a marginal deterioration of the spectroscopic performance for pixels of 3 x 3 mm(2).
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Caballero, L., Albiol, F., Corbi Bellot, A., Domingo-Pardo, C., Leganes Nieto, J. L., Agramunt Ros, J., et al. (2018). Gamma-ray imaging system for real-time measurements in nuclear waste characterisation. J. Instrum., 13, P03016–23pp.
Abstract: Acompact, portable and large field-of-viewgamma camera that is able to identify, locate and quantify gamma-ray emitting radioisotopes in real-time has been developed. The device delivers spectroscopic and imaging capabilities that enable its use it in a variety of nuclear waste characterisation scenarios, such as radioactivity monitoring in nuclear power plants and more specifically for the decommissioning of nuclear facilities. The technical development of this apparatus and some examples of its application in field measurements are reported in this article. The performance of the presented gamma-camera is also benchmarked against other conventional techniques.
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