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n_TOF Collaboration(Guerrero, C. et al), Domingo-Pardo, C., & Tain, J. L. (2011). Study of Photon Strength Function of Actinides: the Case of (235)U, (238)Np and (241)Pu. J. Korean Phys. Soc., 59(2), 1510–1513.
Abstract: The decay from excited levels in medium and heavy nuclei can be described in a statistical approach by means of Photon Strength Functions and Level Density distributions. The study of electromagnetic cascades following neutron capture based on the use of high efficiency detectors has been shown to be well suited for probing the properties of the Photon Strength Function of heavy (high level density) and/or radioactive (high background) nuclei. In this work we have investigated for the first time the validity of the recommended PSF of actinides, in particular (235)U, (238)Np and (241)Pu. Our study includes the search for resonance structures in the PSF below S(n) and draws conclusions regarding their existence and their characteristics in terms of energy, width and electromagnetic nature.
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n_TOF Collaboration, Gunsing, F., Berthoumieux, E., Borella, A., Belgya, T., Szentmiklosi, L., et al. (2011). Neutron Capture on (209)Bi: Determination of the Production Ratio of (210m)Bi/(210g)Bi. J. Korean Phys. Soc., 59(2), 1670–1675.
Abstract: Neutron capture on (209)Bi produces either an isomeric state (210m)Bi with a half life of 3 x 106 years, or the ground state (210g)Bi which decays with a half life of 5 days to the alpha emitter (210)Po. Therefore the neutron capture cross section ratio (209)Bi(n,gamma)(210m)Bi/(210g)Bi plays an important role in predicting the short- and long-term radio-toxicity produced by (209)Bi under neutron irradiation. This ratio is dependent on the neutron energy. We have measured this ratio for cold neutrons at the cold neutron beam facility of the Budapest Neutron Centre by observing the population of the ground-and the metastable state using high resolution gamma-ray spectroscopy. The same technique has been used at the pulsed white neutron source GELINA of the IRMM, Geel in combination with the neutron time-of-flight technique. Results for the neutron-energy dependent branching ratio will be presented. In addition we performed simulations using a statistical decay code.
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n_TOF Collaboration(Cano-Ott, D. et al), Domingo-Pardo, C., & Tain, J. L. (2011). Neutron Capture Measuremetns on Minor Actinides at the n_TOF Facility at CERN: Past, Present and Future. J. Korean Phys. Soc., 59(2), 1809–1812.
Abstract: The successful development of advanced nuclear systems for sustainable energy production and nuclear waste management depends on high quality nuclear data libraries. Recent sensitivity studies and reports [1-3] have identified the need for substantially improving the accuracy of neutron cross-section data for minor actinides. The n_TOF collaboration has initiated an ambitious experimental program for the measurement of neutron capture cross sections of minor actinides. Two experimental setups have been constructed for this purpose: a Total Absorption Calorimeter (TAC) [4] for measuring neutron capture cross-sections of low-mass and/or radioactive samples and a set of two low neutron sensitivity C(6)D(6) detectors for the less radioactive materials.
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n_TOF Collaboration(Tarrio, D. et al), Domingo-Pardo, C., Plag, R., Plompen, A., & Tain, J. L. (2011). High-energy Neutron-induced Fission Cross Sections of Natural Lead and Bismuth-209. J. Korean Phys. Soc., 59(2), 1904–1907.
Abstract: The CERN Neutron Time-Of-Flight (n_TOF) facility is well suited to measure small neutron-induced fission cross sections, as those of subactinides. The cross section ratios of (nat)Pb and (209)Bi relative to (235)U and (238)U were measured using PPAC detectors. The fragment coincidence method allows to unambiguously identify the fission events. The present experiment provides the first results for neutron-induced fission up to 1 GeV for (nat)Pb and (209)Bi. A good agreement with previous experimental data below 200 MeV is shown. The comparison with proton-induced fission indicates that the limiting regime where neutron-induced and proton-induced fission reach equal cross section is close to 1 GeV.
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n_TOF Collaboration(Paradela, C. et al), Domingo-Pardo, C., Plag, R., Plompen, A., & Tain, J. L. (2011). (237)Np(n,f) Cross Section: New Data and Present Status. J. Korean Phys. Soc., 59(2), 1908–1911.
Abstract: In this document, we present the final result obtained at the nTOF experiment; for the neutron-induced fission cross section of the (237)Np, from the fission threshold up to 1 GeV. The method applied to get tins result is briefly discussed. nTOF data are compared to the last experimental measurements using other TOF facilities or the surrogate method, reported experiments performed with monoenergetic sources and the FISCAL systematic, including a discussion about the existing discrepancies.
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n_TOF Collaboration(Calviani, M. et al), Domingo-Pardo, C., & Tain, J. L. (2011). Fission Cross-section Measurements of (233)U, (245)Cm and (241,243)Am at CERN n_TOF Facility. J. Korean Phys. Soc., 59(2), 1912–1915.
Abstract: Neutron-induced fission cross-sections of minor actinides have been measured using the nTOF white neutron source at CERN. Geneva, as part of a large experimental program aiming at collecting new data relevant for nuclear astrophysics and for the design of advanced reactor systems. The measurements at nTOF take advantage of the innovative features of the n_TOF facility, namely the wide energy range, high instantaneous neutron flux and good energy resolution. Final results on the fission cross-section of (233)U, (245)cm and (243)Am from thermal to 20 MeV are here reported, together with preliminary results for (241)Am. The measurement have been performed with a dedicated Fast Ionization Chamber (FIC), a fission fragment detector with a very high efficiency, relative to the very well known cross-section of (235)U, measured simultaneously with the same detector.
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n_TOF Collaboration, Kappeler, F., Mengoni, A., Mosconi, M., Fujii, K., Heil, M., et al. (2011). Neutron Studies for Dating the Universe. J. Korean Phys. Soc., 59(2), 2094–2099.
Abstract: The neutron capture cross sections of (186)Os and (187)Os are of key importance for defining the 8-process abundance of (187)Os at the formation of the solar system. This quantity can be used to determine the radiogenic abundance component of (187)Os from the decay of (187)Re (t(1/2) = 41.2 Gyr) and to infer the time-duration of the nucleosynthesis in our galaxy (Re/Os cosmochronometer). The neutron capture cross sections of (186)Os, (187)Os, and (188)Os have been measured at the CERN nTOF facility from 1 eV to 1 MeV, covering the entire energy range of astrophysical interest. From these data Maxwellian averaged capture cross sections have been calculated with uncertainties between 3.3 and 4.7%. Additional information was obtained by measuring the inelastic scattering cross section of (187)Os at the Karlsruhe 3.7 MV Van de Graaff accelerator and by neutron resonance analyses of the nTOF capture data to establish a comprehensive experimental basis for the Hauser-Feshbach statistical model. Consistent I-IF calculations for the capture and inelastic reaction channels were performed to determine the stellar enhancement factors, which are required to correct the Maxwellian averaged cross sections for the effect of thermally populated excited states. The consequences of this analysis for the s-process component of the (187)Os abundance and the related impact on the evaluation of the time-duration of Galactic nucleosynthesis via the Re/Os cosmo-chronometer are discussed.
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n_TOF Collaboration(Belloni, F. et al), Domingo-Pardo, C., & Tain, J. L. (2012). Neutron-induced fission cross section measurement of U-233, Am-241 and Am-243 in the energy range 0.5 MeV <= E-n <= 20 MeV at n_TOF at CERN. Phys. Scr., T150, 014005–4pp.
Abstract: Neutron-induced fission cross section measurements of U-233, Am-243 and Am-241 relative to U-235 have been carried out at the neutron time-of-flight facility n_TOF at CERN. A fast ionization chamber has been employed. All samples were located in the same detector; therefore the studied elements and the reference U-235 target are subject to the same neutron beam.
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BRIKEN Collaboration(Tarifeño-Saldivia, A. et al), Tain, J. L., Domingo-Pardo, C., Agramunt, J., Algora, A., Morales, A. I., et al. (2017). Conceptual design of a hybrid neutron-gamma detector for study of beta-delayed neutrons at the RIB facility of RIKEN. J. Instrum., 12, P04006–22pp.
Abstract: BRIKEN is a complex detection system to be installed at the RIB-facility of the RIKEN Nishina Center. It is aimed at the detection of heavy-ion implants, β-particles, γ-rays and β-delayed neutrons. The whole detection setup involves the Advanced Implantation Detection Array (AIDA), two HPGe Clover detectors and a large set of 166 counters of 3He embedded in a high-density polyethylene matrix. This article reports on a novel methodology developed for the conceptual design and optimisation of the 3He-tubes array, aiming at the best possible performance in terms of neutron detection. The algorithm is based on a geometric representation of two selected parameters of merit, namely, average neutron detection efficiency and efficiency flatness, as a function of a reduced number of geometric variables. The response of the detection system itself, for each configuration, is obtained from a systematic MC-simulation implemented realistically in Geant4. This approach has been found to be particularly useful. On the one hand, due to the different types and large number of 3He-tubes involved and, on the other hand, due to the additional constraints introduced by the ancillary detectors for charged particles and gamma-rays. Empowered by the robustness of the algorithm, we have been able to design a versatile detection system, which can be easily re-arranged into a compact mode in order to maximize the neutron detection performance, at the cost of the gamma-ray sensitivity. In summary, we have designed a system which shows, for neutron energies up to 1(5) MeV, a rather flat and high average efficiency of 68.6%(64%) and 75.7%(71%) for the hybrid and compact modes, respectively. The performance of the BRIKEN system has been also quantified realistically by means of MC-simulations made with different neutron energy distributions.
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AGATA Collaboration(Lalovic, N. et al), Gadea, A., & Domingo-Pardo, C. (2018). Study of isomeric states in Pb-198, Pb-200, Pb-202, Pb-206 and Hg-206 populated in fragmentation reactions. J. Phys. G, 45(3), 035105–27pp.
Abstract: Isomeric states in isotopes in the vicinity of doubly-magic Pb-208 were populated following reactions of a relativistic Pb-208 primary beam impinging on a Be-9 fragmentation target. Secondary beams of Pb-198,Pb-200,Pb-202,Pb-206 and Hg-206 were isotopically separated and implanted in a passive stopper positioned in the focal plane of the GSI Fragment Separator. Delayed gamma rays were detected with the Advanced Gamma Tracking Array (AGATA). Decay schemes were reevaluated and interpreted with shell-model calculations. The momentum-dependent population of isomeric states in the two-nucleon hole nuclei Pb-206/Hg-206 was found to differ from the population of multi neutron-hole isomeric states in Pb-198,Pb-200,Pb-202.
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