Abstract: The beta decay of the semimagic Sn isotopes Sn-136,Sn-137,Sn-138 has been studied at the Radioactive Isotope Beam Factory at the RIKEN Nishina Center. The first experimental information on excited states was obtained for Sb-137 while, in the case of Sb-136, the established excitation scheme could be extended by ten previously unidentified levels. In the decay of the most-neutron-rich isotope Sn-138, two gamma rays were observed for the first time. The new experimental results, in combination with state-of-the-art shell-model calculations, provide the first information with respect to the evolution of the Og(7/2) and 1d(5/2) proton single-particle states with increasing neutron number beyond N = 84.

Abstract: Excited states of neutron-rich iodine isotopes I130-134 above the high-spin isomers have been identified using prompt-delayed gamma-ray spectroscopy. The iodine isotopes were produced as fission fragments of fusion-fission and transfer induced fission of 9Be(U-238, f) at a beam energy of 6.2 MeV/u. The complete (A, Z) identification was obtained using the large acceptance magnetic spectrometer VAMOS++. The AGATA gamma-ray tracking array was used to detect the prompt gamma rays while the delayed gamma rays (in the time range of 100 ns to 200 μs) from the isomeric states were identified by the EXOGAM segmented clover detectors, placed behind the focal plane of the VAMOS++ spectrometer. The high-spin states above the (8(-)) isomers in I-130,I-132 were populated for the first time, and a new isomer in I-132 was identified. A new gamma-ray transition was also assigned to the level structure of I-134. Prompt transitions above the 19/2- isomer were identified in I-131,I-133, for the first time. The level structures are interpreted in terms of the systematics of odd-Z nuclei above the Z = 50 shell closure and large-scale shell model calculations.

Abstract: In beta-decay studies the determination of the decay probability to the ground state (g.s.) of the daughter nucleus often suffers from large systematic errors. The difficulty of the measurement is related to the absence of associated delayed gamma-ray emission. In this work we revisit the 4 pi gamma – beta method proposed by Greenwood and collaborators in the 1990s, which has the potential to overcome some of the experimental difficulties. Our interest is driven by the need to determine accurately the beta-intensity distributions of fission products that contribute significantly to the reactor decay heat and to the antineutrinos emitted by reactors. A number of such decays have large g.s. branches. The method is relevant for nuclear structure studies as well. Pertinent formulas are revised and extended to the special case of beta-delayed neutron emitters, and the robustness of the method is demonstrated with synthetic data. We apply it to a number of measured decays that serve as test cases and discuss the features of the method. Finally, we obtain g.s. feeding intensities with reduced uncertainty for four relevant decays that will allow future improvements in antineutrino spectrum and decay heat calculations using the summation method.

Abstract: Prompt and delayed gamma-ray spectroscopy of the neutron-rich Kr-94 was performed, as part of the fission campaign at the ALTO facility of the IPN Orsay, using the fast-neutron-induced fission reaction U-238(n, f) in combination with the nu-Ball array, a novel hybrid gamma spectrometer for energy and lifetime measurements. Several new yrast and nonyrast transitions were observed for the first time, extending the previously known level scheme. Additionally, we report on the observation of a new short-lived isomer at 3444 keV with a half-life of 32(3) ns. The analysis of the Nilsson orbitals obtained from Gogny cranked Hartree-Fock-Bogoliubov calculations suggests a (9(-)) spin and an oblate deformation for this isomer corresponding to a two-quasineutron state, indicating an isomeric structure very similar to that of the neighboring isotones Sr-96 and Se-92.

Abstract: The beta decay of Zr-101,Zr-102 and Tc-109 was studied using the technique of total absorption spectroscopy. The experiment was performed at the National Superconducting Cyclotron Laboratory using the Summing NaI(Tl) (SuN) detector in the first-ever application of total absorption spectroscopy with a fast beam produced via projectile fragmentation. The beta-decay feeding intensity and Gamow-Teller transition strength distributions were extracted for these three decays. The extracted distributions were compared to three different quasiparticle random-phase approximation (QRPA) models based on different mean-field potentials. A comparison with calculations from one of the QRPA models was performed to learn about the ground-state shape of the parent nucleus. For Zr-101 and Zr-102, calculations assuming a pure shape configuration (oblate or prolate) were not able to reproduce the extracted distributions. These results may indicate that some type of mixture between oblate and prolate shapes is necessary to reproduce the extracted distributions. For Tc-109, a comparison of the extracted distributions with QRPA calculations suggests a dominant oblate configuration. The other two QRPA models are commonly used to provide beta-decay properties in r-process network calculations. This work shows the importance of making comparisons between the experimental and theoretical beta-decay distributions, rather than just half-lives and beta-delayed neutron emission probabilities, as close to the r-process path as possible.