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n_TOF Collaboration (Stamatopoulos, A. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Investigation of the Pu-240(n, f) reaction at the n_TOF/EAR2 facility in the 9 meV-6 MeV range |
Type |
Journal Article |
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Year |
2020 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
102 |
Issue |
1 |
Pages |
014616 - 23pp |
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Abstract |
Background: Nuclear waste management is considered amongst the major challenges in the field of nuclear energy. A possible means of addressing this issue is waste transmutation in advanced nuclear systems, whose operation requires a fast neutron spectrum. In this regard, the accurate knowledge of neutron-induced reaction cross sections of several (minor) actinide isotopes is essential for design optimization and improvement of safety margins of such systems. One such case is Pu-240, due to its accumulation in spent nuclear fuel of thermal reactors and its usage in fast reactor fuel. The measurement of the Pu-240(n, f) cross section was previously attempted at the CERN nTOF facility EAR1 measuring station using the time-of-flight technique. Due to the low amount of available material and the given flux at EAR1, the measurement had to last several months to achieve a sufficient statistical accuracy. This long duration led to detector deterioration due to the prolonged exposure to the high alpha activity of the fission foils, therefore the measurement could not be successfully completed. Purpose: It is aimed to determine whether it is feasible to study neutron-induced fission at nTOF/EAR2 and provide data on the Pu-240(n, f) reaction in energy regions requested for applications. Methods: The study of the Pu-240(n, f) reaction was made at a new experimental area (EAR2) with a shorter flight path which delivered on average 30 times higher flux at fast neutron energies. This enabled the measurement to be performed much faster, thus limiting the exposure of the detectors to the intrinsic activity of the fission foils. The experimental setup was based on microbulk Micromegas detectors and the time-of-flight data were analyzed with an optimized pulse-shape analysis algorithm. Special attention was dedicated to the estimation of the non-negligible counting loss corrections with the development of a new methodology, and other corrections were estimated via Monte Carlo simulations of the experimental setup. Results: This new measurement of the Pu-240(n, f) cross section yielded data from 9 meV up to 6 MeV incident neutron energy and fission resonance kernels were extracted up to 10 keV. Conclusions: Neutron-induced fission of high activity samples can be successfully studied at the n_TOF/EAR2 facility at CERN covering a wide range of neutron energies, from thermal to a few MeV. |
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Address |
[Stamatopoulos, A.; Tsinganis, A.; Kokkoris, M.; Vlastou, R.; Diakaki, M.] Natl Tech Univ Athens, Athens, Greece, Email: athanasios.stamatopoulos@cern.ch |
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Amer Physical Soc |
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0556-2813 |
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Notes |
WOS:000551057500002 |
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no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4466 |
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Author |
n_TOF Collaboration (Balibrea-Correa, J. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Measurement of the alpha ratio and (n, gamma) cross section of U-235 from 0.2 to 200 eV at n_TOF |
Type |
Journal Article |
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Year |
2020 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
102 |
Issue |
4 |
Pages |
044615 - 18pp |
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Abstract |
We measured the neutron capture-to-fission cross-section ratio (alpha ratio) and the capture cross section of U-235 between 0.2 and 200 eV at the nTOF facility at CERN. The simultaneous measurement of neutron-induced capture and fission rates was performed by means of the nTOF BaF2 Total Absorption Calorimeter (TAC), used for detection of gamma rays, in combination with a set of micromegas detectors used as fission tagging detectors. The energy dependence of the capture cross section was obtained with help of the Li-6(n, t) standard reaction determining the n_TOF neutron fluence; the well-known integral of the U-235(n, f) cross section between 7.8 and 11 eV was then used for its absolute normalization. The alpha ratio, obtained with slightly higher statistical fluctuations, was determined directly, without need for any reference cross section. To perform the analysis of this measurement we developed a new methodology to correct the experimentally observed effect that the probabilities of detecting a fission reaction in the TAC and the micromegas detectors are not independent. The results of this work have been used in a new evaluation of U-235 performed within the scope of the Collaborative International Evaluated Library Organisation (CIELO) Project, and are consistent with the ENDF/B-VIII.0 and JEFF-3.3 capture cross sections below 4 eV and above 100 eV. However, the measured capture cross section is on average 10% larger between 4 and 100 eV. |
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Address |
[Balibrea-Correa, J.; Mendoza, E.; Cano-Ott, D.] Ctr Invest Energet Medioambientales & Tecnol, CIEMAT, Madrid, Spain, Email: emilio.mendoza@ciemat.es |
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Amer Physical Soc |
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0556-2813 |
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Conference |
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Notes |
WOS:000579839000003 |
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no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4575 |
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Author |
n_TOF Collaboration (Gawlik, A. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Measurement of the Ge-76(n, gamma) cross section at the n_TOF facility at CERN |
Type |
Journal Article |
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Year |
2021 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
104 |
Issue |
4 |
Pages |
044610 - 7pp |
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Abstract |
The Ge-76(n, gamma) reaction has been measured at the n_TOF facility at CERN via the time-of-flight technique. Neutron capture cross sections on Ge-76 are of interest to a variety of low-background experiments, such as neutrinoless double beta decay searches, and to nuclear astrophysics. We have determined resonance capture kernels up to 52 keV neutron energy and used the new data to calculate Maxwellian-averaged neutron capture cross sections for k(B)T values of 5 to 100 keV. |
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Address |
[Gawlik-Ramiega, A.; Andrzejewski, J.; Perkowski, J.] Univ Lodz, Lodz, Poland, Email: aleksandra.gawlik@uni.lodz.pl |
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Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
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Notes |
WOS:000707420400002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5003 |
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Author |
n_TOF Collaboration (Tagliente, G. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Zr-92(n, gamma) and (n,tot) measurements at the GELINA and n_TOF facilities |
Type |
Journal Article |
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Year |
2022 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
105 |
Issue |
2 |
Pages |
025805 - 14pp |
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Keywords |
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Abstract |
Background: Stellar nucleosynthesis of elements heavier than iron is driven by neutron capture processes. Zr-92 is positioned at a strategic point along the slow nucleosynthesis path, given its proximity to the neutron magic number N = 50 and its position at the matching region between the weak and main slow processes. Purpose: In parallel with recent improved astronomical data, the extraction of accurate Maxwellian averaged cross sections (MACSs) derived from a more complete and accurate set of resonance parameters should allow for a better understanding of the stellar conditions at which nucleosynthesis takes place. Methods: Transmission and capture cross section measurements using enriched Zr-92 metallic samples were performed at the time-of flight facilities GELINA of JRC-Geel (BE) and nTOF of CERN (CH). The neutron beam passing through the samples was investigated in transmission measurements at GELINA using a Li-glass scintillator. The gamma rays emitted during the neutron capture reactions were detected by C6D6 detectors at both GELINA and nTOF. Results: Resonance parameters of individual resonances up to 81 keV were extracted from a combined resonance shape analysis of experimental transmissions and capture yields. For the majority of the resonances the parity was determined from an analysis of the transmission data obtained with different sample thicknesses. Average resonance parameters were calculated. Conclusions: Maxwellian averaged cross sections were extracted from resonances observed up to 81 keV. The MACS for kT = 30 keV is fully consistent with experimental data reported in the literature. The MACSs for kT less than or similar to 15 keV are in good agreement with those derived from the ENDF/B-VIII.0 library and recommended in the KADoNTS database. For kT higher than 30 keV differences are observed. A comparison with MACSs obtained with the cross sections recommended in the JEFF-3.3 and JENDL-4.0 libraries shows discrepancies even for kT less than or similar to 15 keV. |
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Address |
[Tagliente, G.; Barbagallo, M.; Colonna, N.; Mastromarco, M.; Variale, V.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: giuseppe.tagliente@ba.infn.it |
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Amer Physical Soc |
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English |
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2469-9985 |
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Notes |
WOS:000766732800002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5163 |
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Author |
Wu, J. et al; Algora, A.; Agramunt, J.; Morales, A.I.; Orrigo, S.E.A.; Tain, J.L.; Tarifeño-Saldivia, A.; Tolosa-Delgado, A. |
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Title |
First observation of isomeric states in 111Zr, 113Nb, and 115Mo |
Type |
Journal Article |
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Year |
2022 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
106 |
Issue |
6 |
Pages |
064328 - 5pp |
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Keywords |
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Abstract |
Isomeric states in the neutron-rich nuclei 111Zr [T1/2 = 0.10(7) μs], 113Nb [T1/2 = 0.7(4) μs], 115Mo [T1/2 = 46(3) μs] were first identified at the Radioactive Ion Beam Factory (RIBF) of RIKEN by using in-flight fission and fragmentation of a 238U beam at an energy of 345 MeV/u. This is a brief report of the gamma transitions de -exciting from isomeric states and half-lives measurements, which provides the first spectroscopy in the nuclear region of prolate-to-oblate shape-phase transition around mass A approximate to 110. |
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Address |
[Wu, J.] Brookhaven Natl Lab, Natl Nucl Data Ctr, Upton, NY 11973 USA, Email: jwu2@bnl.gov |
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Amer Physical Soc |
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English |
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Abbreviated Series Title |
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ISSN |
2469-9985 |
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Conference |
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Notes |
WOS:000906391600002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5452 |
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Author |
Phong, V.H. et al; Agramunt, J.; Algora, A.; Domingo-Pardo, C.; Morales, A.I.; Rubio, B.; Tain, J.L.; Tarifeño-Saldivia, A.; Tolosa-Delgado, A. |
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Title |
Beta-Delayed One and Two Neutron Emission Probabilities South-East of Sn-132 and the Odd-Even Systematics in r-Process Nuclide Abundances |
Type |
Journal Article |
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Year |
2022 |
Publication |
Physical Review Letters |
Abbreviated Journal |
Phys. Rev. Lett. |
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Volume |
129 |
Issue |
18 |
Pages |
172701 - 7pp |
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Keywords |
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Abstract |
The beta-delayed one- and two-neutron emission probabilities (P-1n and P-2n) of 20 neutron-rich nuclei with N >= 82 have been measured at the RIBF facility of the RIKEN Nishina Center. P-1n of Ag-130;131, Cd-133;134, In-135;136, and (138;13)9Sn were determined for the first time, and stringent upper limits were placed on P-2n for nearly all cases. beta-delayed two-neutron emission (beta 2n) was unambiguously identified in Cd-133 and In-135;136, and their P-2n were measured. Weak beta 2n was also detected from Sn-137;138. Our results highlight the effect of the N = 82 and Z = 50 shell closures on beta-delayed neutron emission probability and provide stringent benchmarks for newly developed macroscopic-microscopic and self-consistent global models with the inclusion of a statistical treatment of neutron and. emission. The impact of our measurements on r-process nucleosynthesis was studied in a neutron star merger scenario. Our P-1n and P-2n have a direct impact on the |
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Address |
[Phong, V. H.; Nishimura, S.; Lorusso, G.; Liu, J.; Nishimura, N.; Ahn, D. S.; Baba, H.; Fukuda, N.; Go, S.; Ha, J.; Isobe, T.; Kiss, G. G.; Kubono, S.; Matsui, K.; Sakurai, H.; Shimizu, Y.; Sumikama, T.; Suzuki, H.; Takeda, H.] RIKEN, Nishina Ctr, Wako, Saitama 3510198, Japan, Email: phong@ribf.riken.jp; |
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Amer Physical Soc |
Place of Publication |
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English |
Summary Language |
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Abbreviated Series Title |
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Series Issue |
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Edition |
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ISSN |
0031-9007 |
ISBN |
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Conference |
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Notes |
WOS:000910940600006 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5458 |
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Author |
n_TOF Collaboration (Amaducci, S. et al); Babiano-Suarez, V.; Caballero-Ontanaya, L.; Domingo-Pardo, C.; Ladarescu, I.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Measurement of the 140Ceðn;γþ Cross Section at n_TOF and Its Astrophysical Implications for the Chemical Evolution of the Universe |
Type |
Journal Article |
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Year |
2024 |
Publication |
Physical Review Letters |
Abbreviated Journal |
Phys. Rev. Lett. |
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Volume |
132 |
Issue |
12 |
Pages |
122701 - 8pp |
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Keywords |
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Abstract |
140Ce(n, gamma) is a key reaction for slow neutron -capture (s -process) nucleosynthesis due to being a bottleneck in the reaction flow. For this reason, it was measured with high accuracy (uncertainty approximate to 5%) at the n_TOF facility, with an unprecedented combination of a high purity sample and low neutron -sensitivity detectors. The measured Maxwellian averaged cross section is up to 40% higher than previously accepted values. Stellar model calculations indicate a reduction around 20% of the s -process contribution to the Galactic cerium abundance and smaller sizeable differences for most of the heavier elements. No variations are found in the nucleosynthesis from massive stars. |
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Address |
[Amaducci, S.; Cosentino, L.; Finocchiaro, P.; Brown, A.] INFN, Lab Nazl Sud, Catania, Italy |
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Amer Physical Soc |
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English |
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0031-9007 |
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Notes |
WOS:001202102900011 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
6074 |
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Author |
Balibrea-Correa, J.; Lerendegui-Marco, J.; Calvo, D.; Caballero, L.; Babiano, V.; Ladarescu, I.; Redondo, M.L.; Tain, J.L.; Tolosa, A.; Domingo-Pardo, C.; Calvino, F.; Casanovas, A.; Tarifeño-Saldivia, A.; Alcayne, V.; Cano-Ott, D.; Martinez, T.; Guerrero, C.; Barbagallo, M.; Macina, D.; Bacak, M. |
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Title |
A first prototype of C6D6 total-energy detector with SiPM readout for neutron capture time-of-flight experiments |
Type |
Journal Article |
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Year |
2021 |
Publication |
Nuclear Instruments & Methods in Physics Research A |
Abbreviated Journal |
Nucl. Instrum. Methods Phys. Res. A |
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Volume |
985 |
Issue |
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Pages |
164709 - 8pp |
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Keywords |
Silicon photomultiplier; Radiation detectors; Time-of-flight; Radiative capture; Total energy detector; Pulse-height weighting technique |
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Abstract |
Low efficiency total-energy detectors (TEDs) are one of the main tools for neutron capture cross section measurements utilizing the time-of-flight (TOF) technique. State-of-the-art TEDs are based on a C6D6 liquid-scintillation cell optically coupled to a fast photomultiplier tube. The large photomultiplier tube represents yet a significant contribution to the so-called neutron sensitivity background, which is one of the most conspicuous sources of uncertainty in this type of experiments. Here we report on the development of a first prototype of a TED based on a silicon-photomultiplier (SiPM) readout, thus resulting in a lightweight and much more compact detector. Apart from the envisaged improvement in neutron sensitivity, the new system uses low voltage (+28 V) and low current supply (-50 mA), which is more practical than the-kV supply required by conventional photomultipliers. One important difficulty hindering the earlier implementation of SiPM readout for this type of detector was the large capacitance for the output signal when all pixels of a SiPM array are summed together. The latter leads to long pulse rise and decay times, which are not suitable for time-of-flight experiments. In this work we demonstrate the feasibility of a Schottky-diode multiplexing readout approach, that allows one to preserve the excellent timing properties of SiPMs, hereby paving the way for their implementation in future neutron TOF experiments. |
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Address |
[Balibrea-Correa, J.; Lerendegui-Marco, J.; Calvo, D.; Caballero, L.; Babiano, V; Ladarescu, I; Redondo, M. Lopez; Tain, J. L.; Tolosa, A.; Domingo-Pardo, C.] Univ Valencia, Inst Fis Corpuscular, CSIC, Valencia, Spain, Email: dacaldia@ific.uv.es; |
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Publisher |
Elsevier |
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English |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0168-9002 |
ISBN |
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Conference |
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Notes |
WOS:000592358200019 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4638 |
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Author |
n_TOF Collaboration (Weiss, C. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
The new vertical neutron beam line at the CERN n_TOF facility design and outlook on the performance |
Type |
Journal Article |
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Year |
2015 |
Publication |
Nuclear Instruments & Methods in Physics Research A |
Abbreviated Journal |
Nucl. Instrum. Methods Phys. Res. A |
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Volume |
799 |
Issue |
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Pages |
90-98 |
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Keywords |
n_TOF facility; Neutron time-of-flight; FLUKA; Neutron cross-section measurement |
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Abstract |
At the neutron Lime-of-flight facility n_TOF at CERN a new vertical beam line was constructed in 2014, in order to extend the experimental possibilities at this facility to an even wider range of challenging cross-section measurements of interest in astrophysics, nuclear technology and medical physics. The design of the beam line and the experimental hall was based on FLUKA Monte Carlo simulations, aiming at maximizing the neutron flux, reducing the beam halo and minimizing the background from neutrons interacting with the collimator or back-scattered in the beam dump. The present paper gives an overview on the design of the beam line and the relevant elements and provides an outlook on the expected performance regarding the neutron beam intensity, shape and energy resolution, as well as the neutron and photon backgrounds. |
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Address |
[Weiss, C.; Chiaveri, E.; Girod, S.; Vlachoudis, V.; Aberle, O.; Bergstroem, I.; Calviani, M.; Guerrero, C.; Sabate-Gilarte, M.; Tsinganis, A.; Brugger, M.; Cerutti, F.; Ferrari, A.; Hernandez-Prieto, A.; Kadi, Y.; Leal-Cidoncha, E.; Losito, R.; Macina, D.; Montesano, S.; Porras, I.; Rubbia, C.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland |
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Publisher |
Elsevier Science Bv |
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English |
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ISSN |
0168-9002 |
ISBN |
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Conference |
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Notes |
WOS:000361877300015 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
2392 |
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Author |
Agramunt, J. et al; Tain, J.L.; Albiol, F.; Algora, A.; Domingo-Pardo, C.; Jordan, M. D.; Rubio, B.; Tarifeño-Saldivia, A.; Valencia, E. |
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Title |
Characterization of a neutron-beta counting system with beta-delayed neutron emitters |
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Journal Article |
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Year |
2016 |
Publication |
Nuclear Instruments & Methods in Physics Research A |
Abbreviated Journal |
Nucl. Instrum. Methods Phys. Res. A |
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Volume |
807 |
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Pages |
69-78 |
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Keywords |
Beta-delayed neutron emission probability; Neutron and beta counters; Self-triggered digital data acquisition system; Geant4 simulations |
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Abstract |
A new detection system for the measurement of beta-delayed neutron emission probabilities has been characterized using fission products with well known beta-delayed neutron emission properties. The setup consists of BELEN-20, a 4 pi-neutron counter with twenty He-3 proportional tubes arranged inside a large polyethylene neutron moderator, a thin Si detector for beta counting and a self-triggering digital data acquisition system. The use of delayed-neutron precursors with different neutron emission windows allowed the study of the effect of energy dependency on neutron, beta and beta-neutron rates. The observed effect is well reproduced by Monte Carlo simulations. The impact of this dependency on the accuracy of neutron emission probabilities is discussed. A new accurate value of the neutron emission probability for the important delayed-neutron precursor I-137 was obtained, P-n = 7.76(14)%. |
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Address |
[Agramunt, J.; Tain, J. L.; Albiol, E.; Algora, A.; Domingo-Pardo, C.; Jordan, M. D.; Rubio, B.; Tarifeno-Saldivia, A.; Valencia, E.] Univ Valencia, CSIC, Inst Fis Corpuscular, E-46071 Valencia, Spain, Email: Tain@ific.uv.es |
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Publisher |
Elsevier Science Bv |
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Language |
English |
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ISSN |
0168-9002 |
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Notes |
WOS:000365596200010 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
2481 |
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