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n_TOF Collaboration(Massimi, C. et al), Domingo-Pardo, C., & Tain, J. L. (2010). Au-197(n,gamma) cross section in the resonance region. Phys. Rev. C, 81(4), 044616–22pp.
Abstract: The (n,gamma) cross section of Au-197 has been measured at nTOF in the resolved resonance region, up to 5 keV, with the aim of improving the accuracy in an energy range where it is not yet considered standard. The measurements were performed with two different experimental setup and detection techniques, the total energy method based on C6D6 detectors, and the total absorption calorimetry based on a 4 pi BaF2 array. By comparing the data collected with the two techniques, two accurate sets of neutron-capture yields have been obtained, which could be the basis for a new evaluation leading to an extended cross-section standard. Overall good agreement is found between the n_TOF results and evaluated cross sections, with some significant exceptions for small resonances. A few resonances not included in the existing databases have also been observed.
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n_TOF Collaboration(Tagliente, G. et al.), Domingo-Pardo, C., & Tain, J. L. (2011). Neutron capture on (94)Zr: Resonance parameters and Maxwellian-averaged cross sections. Phys. Rev. C, 84(1), 015801–9pp.
Abstract: The neutron capture cross sections of the Zr isotopes play an important role in nucleosynthesis studies. The s-process reaction flow between the Fe seed and the heavier isotopes passes through the neutron magic nucleus (90)Zr and through (91,92,93,94)Zr, but only part of the flow extends to (96)Zr because of the branching point at (95)Zr. Apart from their effect on the s-process flow, the comparably small isotopic (n, gamma) cross sections make Zr also an interesting structural material for nuclear reactors. The (94)Zr (n, gamma) cross section has been measured with high resolution at the spallation neutron source n_TOF at CERN and resonance parameters are reported up to 60 keV neutron energy.
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Dillmann, I., Coquard, L., Domingo-Pardo, C., Kappeler, F., Marganiec, J., Uberseder, E., et al. (2011). Cross sections for proton-induced reactions on Pd isotopes at energies relevant for the gamma process. Phys. Rev. C, 84(1), 015802–11pp.
Abstract: Proton-activation reactions on natural and enriched palladium samples were investigated via the activation technique in the energy range of E(p) = 2.75-9 MeV, close to the upper end of the respective Gamow window of the. process. We have determined cross sections for (102)Pd(p,gamma)(103)Ag, (104)Pd(p,gamma)(105)Ag, and (105)Pd(p,n)(105)Ag, as well as partial cross sections of (104)Pd(p,n)(104)Ag(g), (105)Pd(p,gamma)(106)Ag(m), (106)Pd(p,n)(106)Ag(m), and (110)Pd(p,n)(110)Ag(m) with uncertainties between 3% and 15% for constraining theoretical Hauser-Feshbach rates and for direct use in gamma-process calculations.
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n_TOF Collaboration(Tagliente, G. et al.), Domingo-Pardo, C., & Tain, J. L. (2011). (96)Zr(n,gamma) measurement at the n_TOF facility at CERN. Phys. Rev. C, 84(5), 055802–8pp.
Abstract: The (n,gamma) cross section of (96)Zr has been investigated at the CERN n_TOF spallation neutron source. High-resolution time-of-flight measurements using an enriched ZrO(2) sample allowed us to analyze 15 resonances below 40 keV with improved accuracy. On average, the capture widths were found to be 25% smaller than reported in earlier experiments. If complemented with the contribution by direct radiative capture, the derived Maxwellian averaged cross sections are consistent with activation data at kT = 25 keV. The present results confirm the astrophysical implications for the s-process branching at (95)Zr.
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n_TOF Collaboration(Sarmento, R. et al), Domingo-Pardo, C., & Tain, J. L. (2011). Measurement of the (236)U(n, f) cross section from 170 meV to 2 MeV at the CERN n_TOF facility. Phys. Rev. C, 84(4), 044618–10pp.
Abstract: The neutron-induced fission cross section of (236)U was measured at the neutron Time-of-Flight (nTOF) facility at CERN relative to the standard (235)U(n, f) cross section for neutron energies ranging from above thermal to several MeV. The measurement, covering the full range simultaneously, was performed with a fast ionization chamber, taking advantage of the high resolution of the nTOF spectrometer. The n_TOF results confirm that the first resonance at 5.45 eV is largely overestimated in some nuclear data libraries. The resonance triplet around 1.2 keV was measured with high resolution and resonance parameters were determined with good accuracy. Resonances at high energy have also been observed and characterized and different values for the cross section are provided for the region between 10 keV and the fission threshold. The present work indicates various shortcomings of the current nuclear data libraries in the subthreshold region and provides the basis for an accurate re-evaluation of the (236)U(n, f) cross section, which is of great relevance for the development of emerging or innovative nuclear reactor technologies.
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n_TOF Collaboration(Guerrero, C. et al), Domingo-Pardo, C., & Tain, J. L. (2012). Measurement and resonance analysis of the Np-237 neutron capture cross section. Phys. Rev. C, 85(4), 044616–15pp.
Abstract: The neutron capture cross section of Np-237 was measured between 0.7 and 500 eV at the CERN n_TOF facility using the 4 pi BaF2 Total Absorption Calorimeter. The experimental capture yield was extracted minimizing all the systematic uncertainties and was analyzed together with the most reliable transmission data available using the SAMMY code. The result is a complete set of individual as well as average resonance parameters [D-0 = 0.56(2) eV, <Gamma(gamma)> = 40.9(18) meV, 10(4)S(0) = 0.98(6), R' = 9.8(6) fm]. The capture cross section obtained in this work is in overall agreement with the evaluations and the data of Weston and Todd [Nucl. Sci. Eng. 79, 184 (1981)], thus showing sizable differences with respect to previous data from Scherbakov et al. [J. Nucl. Sci. Technol. 42, 135 (2005)] and large discrepancies with data Kobayashi et al. [J. Nucl. Sci. Technol. 39, 111 (2002)]. The results indicate that a new evaluation combining the present capture data with reliable transmission data would allow reaching an accuracy better than 4%, in line with the uncertainty requirements of the nuclear data community for the design and operation of current and future nuclear devices.
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n_TOF Collaboration(Massimi, C. et al), Domingo-Pardo, C., & Tain, J. L. (2012). Resonance neutron-capture cross sections of stable magnesium isotopes and their astrophysical implications. Phys. Rev. C, 85(4), 044615–15pp.
Abstract: We have measured the neutron capture cross sections of the stable magnesium isotopes Mg-24,Mg-25,Mg-26 in the energy range of interest to the s process using the neutron time-of-flight facility n_TOF at CERN. Capture events from a natural metal sample and from samples enriched in Mg-25 and Mg-26 were recorded using the total energy method based on (C6H6)-H-2 detectors. Neutron resonance parameters were extracted by a simultaneous resonance shape analysis of the present capture data and existing transmission data on a natural isotopic sample. Maxwellian-averaged capture cross sections for the three isotopes were calculated up to thermal energies of 100 keV and their impact on s-process analyses was investigated. At 30 keV the new values of the stellar cross section for Mg-24, Mg-25, and Mg-26 are 3.8 +/- 0.2 mb, 4.1 +/- 0.6 mb, and 0.14 +/- 0.01 mb, respectively.
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n_TOF Collaboration(Gunsing, F. et al), Domingo-Pardo, C., & Tain, J. L. (2012). Measurement of resolved resonances of Th-232(n, gamma) at the n_TOF facility at CERN. Phys. Rev. C, 85(6), 064601–17pp.
Abstract: The yield of the neutron capture reaction Th-232(n, gamma) has been measured at the neutron time-of-flight facility n_TOF at CERN in the energy range from 1 eV to 1 MeV. The reduction of the acquired data to the capture yield for resolved resonances from 1 eV to 4 keV is described and compared to a recent evaluated data set. The resonance parameters were used to assign an orbital momentum to each resonance. A missing level estimator was used to extract the s-wave level spacing of D-0 = 17.2 +/- 0.9 eV.
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n_TOF Collaboration(Tagliente, G. et al.), Domingo-Pardo, C., & Tain, J. L. (2013). The Zr-93(n, gamma) reaction up to 8 keV neutron energy. Phys. Rev. C, 87(1), 014622–7pp.
Abstract: The (n, gamma) reaction of the radioactive isotope Zr-93 has been measured at the n_TOF high-resolution time-of-flight facility at CERN. Resonance parameters have been extracted in the neutron energy range up to 8 keV, yielding capture widths smaller (14%) than reported in an earlier experiment. These results are important for detailed nucleosynthesis calculations and for refined studies of waste transmutation concepts. DOI: 10.1103/PhysRevC.87.014622
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n_TOF Collaboration(Zugec, P. et al), Domingo-Pardo, C., Giubrone, G., & Tain, J. L. (2014). Experimental neutron capture data of Ni-58 from the CERN n_TOF facility. Phys. Rev. C, 89(1), 014605–9pp.
Abstract: The Ni-58(n,gamma) cross section has been measured at the neutron time of flight facility n_TOF at CERN, in the energy range from 27 meV up to 400 keV. In total, 51 resonances have been analyzed up to 122 keV. Maxwellian averaged cross sections (MACS) have been calculated for stellar temperatures of kT = 5-100 keV with uncertainties of less than 6%, showing fair agreement with recent experimental and evaluated data up to kT = 50 keV. The MACS extracted in the present work at 30 keV is 34.2 +/- 0.6(stat) +/- 1.8(sys) mb, in agreement with latest results and evaluations, but 12% lower relative to the recent KADoNIS compilation of astrophysical cross sections. When included in models of the s-process nucleosynthesis in massive stars, this change results in a 60% increase of the abundance of Ni-58, with a negligible propagation on heavier isotopes. The reason is that, using both the old or the new MACS, Ni-58 is efficiently depleted by neutron captures.
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