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Yoshida, T., Hagura, N., Umezu, R., Algora, A., Tain, J. L., Jordan, D., et al. (2011). Impact of TAGS Measurement on FP Decay Data and Decay Heat Calculations. J. Korean Phys. Soc., 59(2), 1543–1546.
Abstract: Nuclear level schemes are usually constructed from the high-resolution data of the gamma-ray transitions which immediately follow the beta-decay of their parents. It is recognized that this procedure may lead to the “pandemonium problem”. If we use the decay data suffering from the pandemonium problem for the decay heat calculations the beta-ray component will be overestimated and the gamma-ray component underestimated. The beta-feeding data obtained by the total absorption gamma-ray spectroscopy (TAGS) is proved to be free from this problem. In the case of the Japanese data base for the FP decay heat calculation, the theoretical values based on the gross theory of beta-decay are widely introduced to circumvent the pandemonium problem. The gross theory, however, is not good at describing any beta-transition exclusively concentrating to a single level in the daughter nucleus. The TAGS method is also proved to be able to save this situation. Further, we have to change our comprehension over the currently published decay schemes.
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Agramunt, J. et al, Algora, A., Domingo-Pardo, C., Jordan, D., Rubio, B., Tain, J. L., et al. (2014). New Beta-delayed Neutron Measurements in the Light-mass Fission Group. Nucl. Data Sheets, 120, 74–77.
Abstract: A new accurate determination of beta-delayed neutron emission probabilities from nuclei in the low mass region of the light fission group has been performed. The measurements were carried out using the BELEN 4 pi neutron counter at the IGISOL-JYFL mass separator in combination with a Penning trap. The new results significantly improve the uncertainties of neutron emission probabilities for Br-91, As-86, As-85, and Ge-85 nuclei.
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Estienne, M., Fallot, M., Cormon, S., Algora, A., Bui, V. M., Cucoanes, A., et al. (2014). Contribution of Recently Measured Nuclear Data to Reactor Antineutrino Energy Spectra Predictions. Nucl. Data Sheets, 120, 149–152.
Abstract: The aim of this work is to study the impact of the inclusion of the recently measured beta decay properties of the Tc-102,Tc-104,Tc-105,Tc-106,Tc-107, Mo-105, and Nb-101 nuclei in the calculation of the antineutrino (anti-nu) energy spectra arising after the fissions of the four main fissile isotopes U-235,U-238, and (PU)-P-239,241 in PWRs. These beta feeding probabilities, measured using the Total Absorption Technique (TAS) at the JYFL facility of Jyvaskyla, have been found to play a major role in the gamma component of the decay heat for Pu-239 in the 4-3000 s range. Following the fission product summation method, the calculation was performed using the MCNP Utility Reactor Evolution code (MURE) coupled to the experimental spectra built from beta decay properties of the fission products taken from evaluated databases. These latest TAS data are found to have a significant effect on the Pu isotope energy spectra and on the spectrum of U-238 showing the importance of their measurement for a better assessment of the reactor anti-nu energy spectrum, as well as importance for fundamental neutrino physics experiments and neutrino applied physics.
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Guerrero, C., Cano-Ott, D., Mendoza, E., Tain, J. L., Algora, A., Berthoumieux, E., et al. (2012). Monte Carlo simulation of the n_TOF Total Absorption Calorimeter. Nucl. Instrum. Methods Phys. Res. A, 671, 108–117.
Abstract: The n_TOF Total Absorption Calorimeter (TAC) is a 4 pi BaF2 segmented detector used at CERN for measuring neutron capture cross-sections of importance for the design of advanced nuclear reactors. This work presents the simulation code that has been developed in GEANT4 for the accurate determination of the detection efficiency of the TAC for neutron capture events. The code allows to calculate the efficiency of the TAC for every neutron capture state, as a function of energy, crystal multiplicity, and counting rate. The code includes all instrumental effects such as the single crystal detection threshold and energy resolution, finite size of the coincidence time window, and signal pile-up. The results from the simulation have been validated with experimental data for a large set of electromagnetic de-excitation patterns: beta-decay of well known calibration sources, neutron capture reactions in light nuclei with well known level schemes like Ti-nat, reference samples used in (n,gamma) measurements like Au-197 and experimental data from an actinide sample like Pu-240. The systematic uncertainty in the determination of the detection efficiency has been estimated for all the cases. As a representative example, the accuracy reached for the case of Au-197(n,gamma) ranges between 0.5% and 2%, depending on the experimental and analysis conditions. Such a value matches the high accuracy required for the nuclear cross-section data needed in advanced reactor design.
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Magan, D. L. P., Caballero, L., Domingo-Pardo, C., Agramunt-Ros, J., Albiol, F., Casanovas, A., et al. (2016). First tests of the applicability of gamma-ray imaging for background discrimination in time-of-flight neutron capture measurements. Nucl. Instrum. Methods Phys. Res. A, 823, 107–119.
Abstract: In this work we explore for the first time the applicability of using gamma-ray imaging in neutron capture measurements to identify and suppress spatially localized background. For this aim, a pinhole gamma camera is assembled, tested and characterized in terms of energy and spatial performance. It consists of a monolithic CeBr3 scintillating crystal coupled to a position-sensitive photomultiplier and readout through an integrated circuit AMIC2GR. The pinhole collimator is a massive carven block of lead. A series of dedicated measurements with calibrated sources and with a neutron beam incident on a Au-197 sample have been carried out at n_TOF, achieving an enhancement of a factor of two in the signal-to-background ratio when selecting only those events coming from the direction of the sample.
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