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Author |
Yokoyama, R. et al; Tain, J.L.; Algora, A.; Agramunt, J.; Domingo-Pardo, C.; Morales, A.I.; Rubio, B.; Tolosa-Delgado, A. |
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Title |
Strong one-neutron emission from two-neutron unbound states in beta decays of the r-process nuclei Ga-86,Ga-87 |
Type |
Journal Article |
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Year |
2019 |
Publication  |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
100 |
Issue |
3 |
Pages |
031302 - 6pp |
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Keywords |
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Abstract |
beta-delayed one-neutron and two-neutron branching ratios (P-1n and P-2n) have been measured in the decay of A = 84 to 87 Ga isotopes at the Radioactive-Isotope Beam Factory (RIBF) at the RIKEN Nishina Center using a high-efficiency array of He-3 neutron counters (BRIKEN). Two-neutron emission was observed in the decay of Ga-84,Ga-85,Ga-87 for the first time and the branching ratios were measured to be P-2n = 1.6(2)%, 1.3(2)%, and 10.2(28)(stat)(5)(sys)%, respectively. One-neutron branching ratio of Ga-87 (P-1n = 81(9)(stat)(8)(sys)%) and half-life of 29(4) ms were measured for the first time. The branching ratios of Ga-86 were also measured to be P-1n = 74(2)(stat)(8)(sys)% and 16.2(9)(stat)(6)(sys)% with better precision than a previous study. The observation that P-1n > P-2n for both Ga-86,Ga-87 was unexpected and is interpreted as a signature of dominating one-neutron emission from the two-neutron unbound excited states in Ge-86,Ge-87. In order to interpret the experimental results, shell-model and Hauser-Feshbach statistical model calculations of delayed particle and gamma-ray emission probabilities were performed. This model framework reproduces the experimental results. The shell model alone predicts P-2n significantly larger than P-1n for the Ga-87 decay, and it is necessary to invoke a statistical description to successfully explain the observation that P-1n > P-2n. Our new results demonstrate the relevance and importance of a statistical description of neutron emission for the prediction of the decay properties of multineutron emitters and that it must be included in the r-process modeling. |
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Address |
[Yokoyama, R.; Grzywacz, R.; Rasco, B. C.; Brewer, N.; Heideman, J.; King, T. T.; Madurga, M.; Singh, M.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA, Email: ryokoyam@utk.edu |
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Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
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Conference |
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Notes |
WOS:000486641000001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4145 |
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Author |
Guadilla, V. et al; Tain, J.L.; Algora, A.; Agramunt, J.; Jordan, D.; Monserrate, M.; Montaner-Piza, A.; Nacher, E.; Orrigo, S.E.A.; Rubio, B.; Valencia, E. |
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Title |
Total absorption gamma-ray spectroscopy of the beta-delayed neutron emitters I-137 and Rb-95 |
Type |
Journal Article |
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Year |
2019 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
100 |
Issue |
4 |
Pages |
044305 - 17pp |
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Keywords |
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Abstract |
The decays of the beta-delayed neutron emitters( 137)I and Rb-95 have been studied with the total absorption gamma-ray spectroscopy technique. The purity of the beams provided by the JYFLTRAP Penning trap at the ion guide isotope separator on-line facility in Jyvaskyla allowed us to carry out a campaign of isotopically pure measurements with the decay total absorption gamma-ray spectrometer, a segmented detector composed of 18 NaI(T1) modules. The contamination coming from the interaction of neutrons with the spectrometer has been carefully studied, and we have tested the use of time differences between prompt gamma rays and delayed neutron interactions to eliminate this source of contamination. Due to the sensitivity of our spectrometer, we have found a significant amount of beta intensity to states above the neutron separation energy that deexcite by gamma rays, comparable to the neutron emission probability. The competition between gamma deexcitation and neutron emission has been compared with Hauser-Feshbach calculations, and it can be understood as a nuclear structure effect. In addition, we have studied the impact of the beta-intensity distributions determined in this work on reactor decay heat and reactor antineutrino spectrum summation calculations. The robustness of our results is demonstrated by a thorough study of uncertainties and with the reproduction of the spectra of the individual modules and the module-multiplicity gated spectra. This work represents the state-of-the-art of our analysis methodology for segmented total absorption spectrometers. |
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Address |
[Guadilla, V; Tain, J. L.; Algora, A.; Agramunt, J.; Jordan, D.; Monserrate, M.; Montaner-Piza, A.; Nacher, E.; Orrigo, S. E. A.; Rubio, B.; Valencia, E.] Univ Valencia, Inst Fis Corpuscular, CSIC, E-46071 Valencia, Spain, Email: guadilla@ific.uv.es |
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Amer Physical Soc |
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English |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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ISSN |
2469-9985 |
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Conference |
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Notes |
WOS:000489250100001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4169 |
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Author |
n_TOF Collaboration (Gawlik, A. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Measurement of the Ge-70(n, gamma) cross section up to 300 keV at the CERN n_TOF facility |
Type |
Journal Article |
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Year |
2019 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
100 |
Issue |
4 |
Pages |
045804 - 10pp |
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Keywords |
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Abstract |
Neutron capture data on intermediate mass nuclei are of key importance to nucleosynthesis in the weak component of the slow neutron capture processes, which occurs in massive stars. The (n,gamma) cross section on Ge-70, which is mainly produced in the s process, was measured at the neutron time-of-flight facility n_TOF at CERN. Resonance capture kernels were determined up to 40 keV neutron energy and average cross sections up to 300 keV. Stellar cross sections were calculated from kT = 5 keV to kT = 100 keV and are in very good agreement with a previous measurement by Walter and Beer (1985) and recent evaluations. Average cross sections are in agreement with Walter and Beer (1985) over most of the neutron energy range covered, while they are systematically smaller for neutron energies above 150 keV. We have calculated isotopic abundances produced in s-process environments in a 25 solar mass star for two initial metallicities (below solar and close to solar). While the low metallicity model reproduces best the solar system germanium isotopic abundances, the close to solar model shows a good global match to solar system abundances in the range of mass numbers A = 60-80. |
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Address |
[Gawlik, A.; Andrzejewski, J.; Perkowski, J.; Marganiec, J.] Univ Lodz, Lodz, Poland, Email: claudia.lederer-woods@ed.ac.uk |
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Publisher |
Amer Physical Soc |
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English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
2469-9985 |
ISBN |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000490751000004 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4174 |
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Author |
n_TOF Collaboration (Stamatopoulos, A. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Investigation of the Pu-240(n, f) reaction at the n_TOF/EAR2 facility in the 9 meV-6 MeV range |
Type |
Journal Article |
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Year |
2020 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
102 |
Issue |
1 |
Pages |
014616 - 23pp |
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Keywords |
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Abstract |
Background: Nuclear waste management is considered amongst the major challenges in the field of nuclear energy. A possible means of addressing this issue is waste transmutation in advanced nuclear systems, whose operation requires a fast neutron spectrum. In this regard, the accurate knowledge of neutron-induced reaction cross sections of several (minor) actinide isotopes is essential for design optimization and improvement of safety margins of such systems. One such case is Pu-240, due to its accumulation in spent nuclear fuel of thermal reactors and its usage in fast reactor fuel. The measurement of the Pu-240(n, f) cross section was previously attempted at the CERN nTOF facility EAR1 measuring station using the time-of-flight technique. Due to the low amount of available material and the given flux at EAR1, the measurement had to last several months to achieve a sufficient statistical accuracy. This long duration led to detector deterioration due to the prolonged exposure to the high alpha activity of the fission foils, therefore the measurement could not be successfully completed. Purpose: It is aimed to determine whether it is feasible to study neutron-induced fission at nTOF/EAR2 and provide data on the Pu-240(n, f) reaction in energy regions requested for applications. Methods: The study of the Pu-240(n, f) reaction was made at a new experimental area (EAR2) with a shorter flight path which delivered on average 30 times higher flux at fast neutron energies. This enabled the measurement to be performed much faster, thus limiting the exposure of the detectors to the intrinsic activity of the fission foils. The experimental setup was based on microbulk Micromegas detectors and the time-of-flight data were analyzed with an optimized pulse-shape analysis algorithm. Special attention was dedicated to the estimation of the non-negligible counting loss corrections with the development of a new methodology, and other corrections were estimated via Monte Carlo simulations of the experimental setup. Results: This new measurement of the Pu-240(n, f) cross section yielded data from 9 meV up to 6 MeV incident neutron energy and fission resonance kernels were extracted up to 10 keV. Conclusions: Neutron-induced fission of high activity samples can be successfully studied at the n_TOF/EAR2 facility at CERN covering a wide range of neutron energies, from thermal to a few MeV. |
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Address |
[Stamatopoulos, A.; Tsinganis, A.; Kokkoris, M.; Vlastou, R.; Diakaki, M.] Natl Tech Univ Athens, Athens, Greece, Email: athanasios.stamatopoulos@cern.ch |
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Publisher |
Amer Physical Soc |
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English |
Summary Language |
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Original Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0556-2813 |
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Conference |
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Notes |
WOS:000551057500002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4466 |
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Author |
n_TOF Collaboration (Balibrea-Correa, J. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Measurement of the alpha ratio and (n, gamma) cross section of U-235 from 0.2 to 200 eV at n_TOF |
Type |
Journal Article |
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Year |
2020 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
102 |
Issue |
4 |
Pages |
044615 - 18pp |
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Keywords |
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Abstract |
We measured the neutron capture-to-fission cross-section ratio (alpha ratio) and the capture cross section of U-235 between 0.2 and 200 eV at the nTOF facility at CERN. The simultaneous measurement of neutron-induced capture and fission rates was performed by means of the nTOF BaF2 Total Absorption Calorimeter (TAC), used for detection of gamma rays, in combination with a set of micromegas detectors used as fission tagging detectors. The energy dependence of the capture cross section was obtained with help of the Li-6(n, t) standard reaction determining the n_TOF neutron fluence; the well-known integral of the U-235(n, f) cross section between 7.8 and 11 eV was then used for its absolute normalization. The alpha ratio, obtained with slightly higher statistical fluctuations, was determined directly, without need for any reference cross section. To perform the analysis of this measurement we developed a new methodology to correct the experimentally observed effect that the probabilities of detecting a fission reaction in the TAC and the micromegas detectors are not independent. The results of this work have been used in a new evaluation of U-235 performed within the scope of the Collaborative International Evaluated Library Organisation (CIELO) Project, and are consistent with the ENDF/B-VIII.0 and JEFF-3.3 capture cross sections below 4 eV and above 100 eV. However, the measured capture cross section is on average 10% larger between 4 and 100 eV. |
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Address |
[Balibrea-Correa, J.; Mendoza, E.; Cano-Ott, D.] Ctr Invest Energet Medioambientales & Tecnol, CIEMAT, Madrid, Spain, Email: emilio.mendoza@ciemat.es |
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Corporate Author |
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Thesis |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0556-2813 |
ISBN |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000579839000003 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4575 |
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| Permanent link to this record |
