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n_TOF Collaboration(Amaducci, S. et al), Babiano-Suarez, V., Caballero-Ontanaya, L., Domingo-Pardo, C., Ladarescu, I., & Tain, J. L. (2021). First Results of the Ce-140(n,gamma)Ce-141 Cross-Section Measurement at n_TOF. Universe, 7(6), 200–11pp.
Abstract: An accurate measurement of the Ce-140(n,gamma) energy-dependent cross-section was performed at the n_TOF facility at CERN. This cross-section is of great importance because it represents a bottleneck for the s-process nucleosynthesis and determines to a large extent the cerium abundance in stars. The measurement was motivated by the significant difference between the cerium abundance measured in globular clusters and the value predicted by theoretical stellar models. This discrepancy can be ascribed to an overestimation of the Ce-140 capture cross-section due to a lack of accurate nuclear data. For this measurement, we used a sample of cerium oxide enriched in Ce-140 to 99.4%. The experimental apparatus consisted of four deuterated benzene liquid scintillator detectors, which allowed us to overcome the difficulties present in the previous measurements, thanks to their very low neutron sensitivity. The accurate analysis of the p-wave resonances and the calculation of their average parameters are fundamental to improve the evaluation of the Ce-140 Maxwellian-averaged cross-section.
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Massimi, C., Cristallo, S., Domingo-Pardo, C., & Lederer-Woods, C. (2022). n_TOF: Measurements of Key Reactions of Interest to AGB Stars. Universe, 8(2), 100–19pp.
Abstract: In the last 20 years, the neutron time-of-flight facility nTOF at CERN has been providing relevant data for the astrophysical slow neutron capture process (s process). At nTOF, neutron-induced radiative capture (n,gamma) as well as (n,p) and (n,alpha) reaction cross sections are measured as a function of energy, using the time-of-flight method. Improved detection systems, innovative ideas and collaborations with other neutron facilities have lead to a considerable contribution of the n_TOF collaboration to studying the s process in asymptotic giant branch stars. Results have been reported for stable and radioactive samples, i.e.,Mg- 24,Mg-25,Mg-26, Al-26, S-33,Fe- 54,Fe-57, Ni-58,Ni-59,Ni-62,Ni-63, Ge-70,Ge-72,Ge-73, Zr-90,Zr-91,Zr-92,Zr-93,Zr-94,Zr-96, La-139, Ce-140, Pm-147, Sm-151,Gd- 154,Gd-155,Gd-157, Tm-171, Os-186,Os-187,Os-188, Au-197, Tl-203,Tl-204,Pb- 204,Pb-206,Pb-207 and Bi-209 isotopes, while others are being studied or planned to be studied in the near future. In this contribution, we present an overview of the most successful achievements, and an outlook of future challenging measurements, including ongoing detection system developments.
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Lerendegui-Marco, J., Balibrea-Correa, J., Babiano-Suarez, V., Ladarescu, I., & Domingo-Pardo, C. (2022). Towards machine learning aided real-time range imaging in proton therapy. Sci Rep, 12(1), 2735–17pp.
Abstract: Compton imaging represents a promising technique for range verification in proton therapy treatments. In this work, we report on the advantageous aspects of the i-TED detector for proton-range monitoring, based on the results of the first Monte Carlo study of its applicability to this field. i-TED is an array of Compton cameras, that have been specifically designed for neutron-capture nuclear physics experiments, which are characterized by gamma-ray energies spanning up to 5-6 MeV, rather low gamma-ray emission yields and very intense neutron induced gamma-ray backgrounds. Our developments to cope with these three aspects are concomitant with those required in the field of hadron therapy, especially in terms of high efficiency for real-time monitoring, low sensitivity to neutron backgrounds and reliable performance at the high gamma-ray energies. We find that signal-to-background ratios can be appreciably improved with i-TED thanks to its light-weight design and the low neutron-capture cross sections of its LaCl3 crystals, when compared to other similar systems based on LYSO, CdZnTe or LaBr3. Its high time-resolution (CRT similar to 500 ps) represents an additional advantage for background suppression when operated in pulsed HT mode. Each i-TED Compton module features two detection planes of very large LaCl3 monolithic crystals, thereby achieving a high efficiency in coincidence of 0.2% for a point-like 1 MeV gamma-ray source at 5 cm distance. This leads to sufficient statistics for reliable image reconstruction with an array of four i-TED detectors assuming clinical intensities of 10(8) protons per treatment point. The use of a two-plane design instead of three-planes has been preferred owing to the higher attainable efficiency for double time-coincidences than for threefold events. The loss of full-energy events for high energy gamma-rays is compensated by means of machine-learning based algorithms, which allow one to enhance the signal-to-total ratio up to a factor of 2.
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n_TOF Collaboration(Alcayne, V. et al), Balibrea-Correa, J., Domingo-Pardo, C., Lerendegui-Marco, J., Babiano-Suarez, V., & Ladarescu, I. (2024). A Segmented Total Energy Detector (sTED) optimized for (n,γ) cross-section measurements at n_TOF EAR2. Radiat. Phys. Chem., 217, 11pp.
Abstract: The neutron time-of-flight facility nTOF at CERN is a spallation source dedicated to measurements of neutroninduced reaction cross-sections of interest in nuclear technologies, astrophysics, and other applications. Since 2014, Experimental ARea 2 (EAR2) is operational and delivers a neutron fluence of similar to 4 center dot 10(7) neutrons per nominal proton pulse, which is similar to 50 times higher than the one of Experimental ARea 1 (EAR1) of similar to 8 center dot 10(5) neutrons per pulse. The high neutron flux at EAR2 results in high counting rates in the detectors that challenged the previously existing capture detection systems. For this reason, a Segmented Total Energy Detector (sTED) has been developed to overcome the limitations in the detector's response, by reducing the active volume per module and by using a photo-multiplier (PMT) optimized for high counting rates. This paper presents the main characteristics of the sTED, including energy and time resolution, response to gamma-rays, and provides as well details of the use of the Pulse Height Weighting Technique (PHWT) with this detector. The sTED has been validated to perform neutron-capture cross-section measurements in EAR2 in the neutron energy range from thermal up to at least 400 keV. The detector has already been successfully used in several measurements at nTOF EAR2.
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n_TOF Collaboration(Massimi, C. et al.), Domingo-Pardo, C., Giubrone, G., & Tain, J. L. (2017). Neutron spectroscopy of Mg-26 states: Constraining the stellar neutron source Ne-22(alpha, n)Mg-25. Phys. Lett. B, 768, 1–6.
Abstract: This work reports on accurate, high-resolution measurements of the Mg-25(n, gamma)Mg-26 and Mg-25(n, tot) cross sections in the neutron energy range from thermal to about 300 keV, leading to a significantly improved Mg-25(n, gamma)Mg-26 parametrization. The relevant resonances for n+Mg-25 were characterized from a combined R-matrix analysis of the experimental data. This resulted in an unambiguous spin/parity assignment of the corresponding excited states in Mg-26. With this information experimental upper limits of the reaction rates for Ne-22(alpha, n)Mg-25 and Ne-22(alpha, gamma)Mg-26 were established, potentially leading to a significantly higher (alpha, n)/(alpha, gamma) ratio than previously evaluated. The impact of these results has been studied for stellar models in the mass range 2 to 25 M-circle dot. (C) 2017 The Author(s). Published by Elsevier B.V.
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n_TOF Collaboration(Lederer-Woods, C. et al), Domingo-Pardo, C., Tain, J. L., & Tarifeño-Saldivia, A. (2019). Measurement of Ge-73(n, gamma) cross sections and implications for stellar nucleosynthesis. Phys. Lett. B, 790, 458–465.
Abstract: Ge-73(n, gamma) cross sections were measured at the neutron time-of-flight facility n_TOF at CERN up to neutron energies of 300 keV, providing for the first time experimental data above 8 keV. Results indicate that the stellar cross section at kT = 30 keV is 1.5 to 1.7 times higher than most theoretical predictions. The new cross sections result in a substantial decrease of Ge-73 produced in stars, which would explain the low isotopic abundance of Ge-73 in the solar system.
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Boso, A. et al, Domingo-Pardo, C., & Perez-Vidal, R. M. (2019). Isospin dependence of electromagnetic transition strengths among an isobaric triplet. Phys. Lett. B, 797, 134835–6pp.
Abstract: Electric quadrupole matrix elements, M-p, for the J(pi) = 2(+) -> 0(+), Delta T = 0, T = 1 transitions across the A = 46 isobaric multiplet Cr-46-V-46-Ti-46 have been measured at GSI with the FRS-LYCCA-AGATA setup. This allows direct insight into the isospin purity of the states of interest by testing the linearity of M-p with respect to T-z. Pairs of nuclei in the T = 1 triplet were studied using identical reaction mechanisms in order to control systematic errors. The M-p values were obtained with two different methodologies: (i) a relativistic Coulomb excitation experiment was performed for Cr-46 and Ti-46; (ii) a “stretched target” technique was adopted here, for the first time, for lifetime measurements in V-46 and Ti-46. A constant value of M-p across the triplet has been observed. Shell-model calculations performed within the fp shell fail to reproduce this unexpected trend, pointing towards the need of a wider valence space. This result is confirmed by the good agreement with experimental data achieved with an interaction which allows excitations from the underlying sd shell. A test of the linearity rule for all published data on complete T = 1 isospin triplets is presented.
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Guerrero, C., Tessler, M., Paul, M., Lerendegui-Marco, J., Heinitz, S., Maugeri, E. A., et al. (2019). The s-process in the Nd-Pm-Sm region: Neutron activation of Pm-147. Phys. Lett. B, 797, 134809–6pp.
Abstract: The Nd-Pm-Sm branching is of interest for the study of the s-process, related to the production of heavy elements in stars. As Sm-148 and Sm-150 are s-only isotopes, the understanding of the branching allows constraining the s-process neutron density. In this context the key physics input needed is the cross section of the three unstable nuclides in the region: Nd-147 (10.98 d half-life), Pm-147 (2.62 yr) and Pm-148 (5.37 d). This paper reports on the activation measurement of Pm-147, the longest-lived of the three nuclides. The cross section measurement has been carried out by activation at the SARAF LiLiT facility using a 56(2) μg target. Compared to the single previous measurement of Pm-147, the measurement presented herein benefits from a target 2000 times more massive. The resulting Maxwellian Averaged Cross Section (MACS) to the ground and metastable states in Pm-148 are 469(50) mb and 357(27) mb. These values are 41% higher (to the ground state) and 15% lower (to the metastable state) than the values reported so far, leading however to a total cross section of 826(107) mb consistent within uncertainties with the previous result and hence leaving unchanged the previous calculation of the s-process neutron density.
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n_TOF Collaboration(Mazzone, A. et al), Babiano-Suarez, V., Caballero, L., Domingo-Pardo, C., Ladarescu, I., & Tain, J. L. (2020). Measurement of the Gd-154(n, gamma) cross section and its astrophysical implications. Phys. Lett. B, 804, 135405–6pp.
Abstract: The neutron capture cross section of Gd-154 was measured from 1 eV to 300 keV in the experimental area located 185 m from the CERN n_TOF neutron spallation source, using a metallic sample of gadolinium, enriched to 67% in Gd-154. The capture measurement, performed with four C6D6 scintillation detectors, has been complemented by a transmission measurement performed at the GELINA time-of-flight facility (JRC-Geel), thus minimising the uncertainty related to sample composition. An accurate Maxwellian averaged capture cross section (MACS) was deduced over the temperature range of interest for s process nucleosynthesis modelling. We report a value of 880(50) mb for the MACS at kT = 30 keV, significantly lower compared to values available in literature. The new adopted Gd-154(n, gamma) cross section reduces the discrepancy between observed and calculated solar s-only isotopic abundances predicted by s-process nucleosynthesis models.
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AGATA Collaboration(Siciliano, M. et al), Gadea, A., Perez-Vidal, R. M., & Domingo-Pardo, C. (2020). Pairing-quadrupole interplay in the neutron-deficient tin nuclei: First lifetime measurements of low-lying states in Sn-106,Sn-108. Phys. Lett. B, 806, 135474–7pp.
Abstract: The lifetimes of the low-lying excited states 2(+) and 4(+) have been directly measured in the neutron-deficient Sn-106,Sn-108 isotopes. The nuclei were populated via a deep-inelastic reaction and the lifetime measurement was performed employing a differential plunger device. The emitted gamma rays were detected by the AGATA array, while the reaction products were uniquely identified by the VAMOS++ magnetic spectrometer. Large-Scale Shell-Model calculations with realistic forces indicate that, independently of the pairing content of the interaction, the quadrupole force is dominant in the B(E2; 2(1)(+) -> 0(g.s)(+)) values and it describes well the experimental pattern for Sn104-114 ; the B(E2;(+)(4) -> 2(1)(+)) values, measured here for the first time, depend critically on a delicate pairing-quadrupole balance, disclosed by the very precise results in Sn-108.
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