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Algora, A. et al, Valencia, E., Tain, J. L., Jordan, M. D., Agramunt, J., Rubio, B., et al. (2014). Total Absorption Study of Beta Decays Relevant for Nuclear Applications and Nuclear Structure. Nucl. Data Sheets, 120, 12–15.
Abstract: An overview is given of our activities related to the study of the beta decay of neutron rich nuclei relevant for nuclear applications. Recent results of the study of the beta decay of Br-87,Br-88 using a new segmented total absorption spectrometer are presented. The measurements were performed at the IGISOL facility using trap-assisted total absorption spectroscopy.
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Tain, J. L., Algora, A., Agramunt, J., Guadilla, V., Jordan, M. D., Montaner-Piza, A., et al. (2015). A decay total absorption spectrometer for DESPEC at FAIR. Nucl. Instrum. Methods Phys. Res. A, 803, 36–46.
Abstract: This paper presents the design of a total absorption gamma-ray spectrometer for the determination of beta-decay intensity distributions of exotic nuclear species at the focal plane of the FAIR-NUSTAR Super Fragment Separator. The spectrometer is a key instrument in the DESPEC experiment and the proposed implementation follows extensive design studies and prototype tests. Two options were contemplated, based on Nal(TI) and LaBr3:Ce inorganic scintillation crystals respectively. Monte Carlo simulations and technical considerations determined the optimal configurations consisting of sixteen 15 x 15 x 25 cm(3) crystals for the Nal(Tl) option and one hundred and twenty-eight 5.5 x 5.5 x 11 cm(3) crystals for the LaBr3:Ce option. Minimization of dead material was crucial for maximizing the spectrometer full-energy peak efficiency. Module prototypes were build to verify constructional details and characterize their performance. The measured energy and timing resolution was found to agree rather well with estimates based on simulations of scintillation light transport and collection. The neutron sensitivity of the spectrometer, important when measuring beta-delayed neutron emitters, was investigated by means of Monte Carlo simulations.
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IGISOL Collaboration(Briz, J. A. et al), Algora, A., Tain, J. L., Guadilla, V., Agramunt, J., Estevez, E., et al. (2016). Total absorption spectroscopy of fission fragments relevant for reactor antineutrino spectra determination. Acta Phys. Pol. B, 47(3), 755–762.
Abstract: The contribution of each fission fragment to the reactor antineutrino spectra was determined using the summation method based on the existing information on fission yields and decay data contained in nuclear databases and the reactor evolution code MURE. The beta decay of some of the main contributors has been studied using the Total Absorption Spectroscopy (TAS) technique during two experimental campaigns at the IGISOL facility, in Jyvaskyla (Finland). Results on the decay of Rb-92, the most important contributor in the 4-8 MeV energy region are reported. The status of the analysis of the second experiment is presented as well.
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Blank, B. et al, Agramunt, J., Algora, A., Guadilla, V., Montaner-Piza, A., Morales, A. I., et al. (2016). New neutron-deficient isotopes from Kr-78 fragmentation. Phys. Rev. C, 93(6), 061301–5pp.
Abstract: In an experiment with the RIKEN projectile fragment separator called BigRIPS at the RIKEN Nishina Center, the fragmentation of a Kr-78 beam allowed the observation of new neutron-deficient isotopes at the proton drip line. Clean identification spectra could be produced and Se-63, Kr-67, and Kr-68 were identified for the first time. In addition, Ge-59 was also observed. Three of these isotopes, Ge-59, Se-63, and Kr-67, are potential candidates for ground-state two-proton radioactivity. In addition, the isotopes Ge-58, Se-62, and Kr-66 were also sought but without success. The present experiment also allowed the determination of production cross sections for some of the most exotic isotopes. These measurements confirm the trend already observed that the empirical parametrization of fragmentation cross sections, EPAX, significantly overestimates experimental cross sections in this mass region.
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Goigoux, T. et al, Algora, A., Guadilla, V., Montaner-Piza, A., Morales, A. I., Orrigo, S. E. A., et al. (2016). Two-Proton Radioactivity of Kr-67. Phys. Rev. Lett., 117(16), 162501–6pp.
Abstract: In an experiment with the BigRIPS separator at the RIKEN Nishina Center, we observed two-proton (2p) emission from Kr-67. At the same time, no evidence for 2p emission of Ge-59 and Se-63, two other potential candidates for this exotic radioactivity, could be observed. This observation is in line with Q value predictions which pointed to Kr-67 as being the best new candidate among the three for two-proton radioactivity. Kr-67 is only the fourth 2p ground-state emitter to be observed with a half-life of the order of a few milliseconds. The decay energy was determined to be 1690(17) keV, the 2p emission branching ratio is 37(14)%, and the half-life of Kr-67 is 7.4(30) ms.
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Guadilla, V. et al, Algora, A., Tain, J. L., Agramunt, J., Jordan, D., Monserrate, M., et al. (2017). Characterization of a cylindrical plastic beta-detector with Monte Carlo simulations of optical photons. Nucl. Instrum. Methods Phys. Res. A, 854, 134–138.
Abstract: In this work we report on the Monte Carlo study performed to understand and reproduce experimental measurements of a new plastic beta-detector with cylindrical geometry. Since energy deposition simulations differ from the experimental measurements for such a geometry, we show how the simulation of production and transport of optical photons does allow one to obtain the shapes of the experimental spectra. Moreover, taking into account the computational effort associated with this kind of simulation, we develop a method to convert the simulations of energy deposited into light collected, depending only on the interaction point in the detector. This method represents a useful solution when extensive simulations have to be done, as in the case of the calculation of the response function of the spectrometer in a total absorption gamma-ray spectroscopy analysis.
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Morales, A. I. et al, Algora, A., Rubio, B., Orrigo, S. E. A., Agramunt, J., Gelletly, W., et al. (2017). Simultaneous investigation of the T=1(J(pi)=0(+)) and T=0(J(pi)=9(+)) beta decays in Br-70. Phys. Rev. C, 95(6), 064327–11pp.
Abstract: The beta decay of the odd-odd nucleus Br-70 has been investigated with the BigRIPS and EURICA setups at the Radioactive Ion Beam Factory (RIBF) of the RIKEN Nishina Center. The T = 0(J(pi) = 9(+)) and T = 1(J(pi) = 0(+)) isomers have both been produced in in-flight fragmentation of Kr-78 with ratios of 41.6(8)% and 58.4(8)%, respectively. A half-life of t(1/2) = 2157(-49)(+53) ms has been measured for the J pi = 9(+) isomer from gamma-ray time decay analysis. Based on this result, we provide a new value of the half-life for the J pi = 0(+) ground state of Br-70, t(1/2) = 78.42 +/- 0.51 ms, which is slightly more precise, and in excellent agreement, with the best measurement reported hitherto in the literature. For this decay, we provide the first estimate of the total branching fraction decaying through the 2(1)(+) state in the daughter nucleus Se-70, R(2(1)(+)) = 1.3 +/- 1.1%. We also report four new low-intensity gamma-ray transitions at 661, 1103, 1561, and 1749 keV following the beta decay of the J pi = 9(+) isomer. Based on their coincidence relationships, we tentatively propose two new excited states at 3945 and 4752 keV in 70Se with most probable spins and parities of J(pi) = (6(+)) and (8(+)), respectively. The observed structure is interpreted with the help of shell-model calculations, which predict a complex interplay between oblate and prolate configurations at low excitation energies.
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Guadilla, V. et al, Algora, A., Tain, J. L., Agramunt, J., Jordan, M. D., Montaner-Piza, A., et al. (2017). Experimental study of Tc-100 beta decay with total absorption gamma-ray spectroscopy. Phys. Rev. C, 96(1), 014319–10pp.
Abstract: The beta decay of Tc-100 has been studied by using the total absorption gamma-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility in Jyvaskyla. In this work the new Decay Total Absorption gamma-ray Spectrometer in coincidence with a cylindrical plastic beta detector has been employed. The beta intensity to the ground state obtained from the analysis is in good agreement with previous high-resolution measurements. However, differences in the feeding to the first-excited state as well as weak feeding to a new level at high excitation energy have been deduced from this experiment. Theoretical calculations performed in the quasiparticle random-phase approximation framework are also reported. Comparison of these calculations with our measurement serves as a benchmark for calculations of the double beta decay of Mo-100.
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Caballero-Folch, R. et al, Agramunt, J., Tain, J. L., Algora, A., Domingo-Pardo, C., Guadilla, V., et al. (2018). First determination of beta-delayed multiple neutron emission beyond A=100 through direct neutron measurement: The P-2n value of Sb-136. Phys. Rev. C, 98(3), 034310–10pp.
Abstract: Background: beta-delayed multiple neutron emission has been observed for some nuclei with A <= 100 being the Rb-100 the heaviest beta 2n emitter measured to date. So far only 25 P-2n values have been determined for the approximate to 300 nuclei that may decay in this way. Accordingly it is of interest to measure P-2n values for the other possible multiple neutron emitters throughout the chart of the nuclides. It is of particular interest to make such a measurement for nuclei with A > 100 to test the predictions of theoretical models and simulation tools for the decays of heavy nuclei in the region of very neutron-rich nuclei. In addition the decay properties of these nuclei are fundamental for the understanding of astrophysical nucleosynthesis processes such as the r-process and safety inputs for nuclear reactors. Purpose: To determine for the first time the two-neutron branching ratio the P-2n value for Sb-136 through a direct neutron measurement and to provide precise P-1n values for Sb-136 and Te-136. Method: A pure beam of each isotope of interest was provided by the JYFLTRAP Penning trap at the Ion Guide Isotope Separator On-Line (IGISOL) facility of the University of Jyvaskyla Finland. The purified ions were implanted into a moving tape at the end of the beam line. The detection setup consisted of a plastic scintillator placed right behind the implantation point after the tape to register the beta decays and the BELEN detector based on neutron counters embedded in a polyethylene matrix. The analysis was based on the study of the beta- and neutron-growth-and-decay curves and the beta-one-neutron and beta-two-neutron time correlations which allowed us the determination of the neutron branching ratios. Results: The P-2n value of Sb-136 was found to be 0.14(3)% and the measured P-1n values for Sb-136 and Te-136 were found to be 32.2(15)% and 1.47(6)% respectively. Conclusions: The measured P-2n value is a factor 44 smaller than predicted by the finite-range droplet model plus the quasiparticle random-phase approximation (FRDM+QRPA) model used for r-process calculations.
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Guadilla, V. et al, Tain, J. L., Algora, A., Agramunt, J., Gelletly, W., Jordan, D., et al. (2018). Characterization and performance of the DTAS detector. Nucl. Instrum. Methods Phys. Res. A, 910, 79–89.
Abstract: DTAS is a segmented total absorption y-ray spectrometer developed for the DESPEC experiment at FAIR. It is composed of up to eighteen NaI(Tl) crystals. In this work we study the performance of this detector with laboratory sources and also under real experimental conditions. We present a procedure to reconstruct offline the sum of the energy deposited in all the crystals of the spectrometer, which is complicated by the effect of NaI(Tl) light-yield non-proportionality. The use of a system to correct for time variations of the gain in individual detector modules, based on a light pulse generator, is demonstrated. We describe also an event-based method to evaluate the summing-pileup electronic distortion in segmented spectrometers. All of this allows a careful characterization of the detector with Monte Carlo simulations that is needed to calculate the response function for the analysis of total absorption gamma-ray spectroscopy data. Special attention was paid to the interaction of neutrons with the spectrometer, since they are a source of contamination in studies of beta-delayed neutron emitting nuclei.
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