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Rasco, B. C., Brewer, N. T., Yokoyama, R., Grzywacz, R., Rykaczewski, K. P., Tolosa-Delgado, A., et al. (2018). The ORNL analysis technique for extracting beta-delayed multi-neutron branching ratios with BRIKEN. Nucl. Instrum. Methods Phys. Res. A, 911, 79–86.
Abstract: Many choices are available in order to evaluate large radioactive decay networks. There are many parameters that influence the calculated beta-decay delayed single and multi-neutron emission branching fractions. We describe assumptions about the decay model, background, and other parameters and their influence on beta-decay delayed multi-neutron emission analysis. An analysis technique, the ORNL BRIKEN analysis procedure, for determining beta-delayed multi-neutron branching ratios in beta-neutron precursors produced by means of heavy-ion fragmentation is presented. The technique is based on estimating the initial activities of zero, one, and two neutrons occurring in coincidence with an ion-implant and beta trigger. The technique allows one to extract beta-delayed multi-neutron decay branching ratios measured with the He-3 BRIKEN neutron counter. As an example, two analyses of the beta-neutron emitter Cu-77 based on different a priori assumptions are presented along with comparisons to literature values.
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Wimmer, K. et al, Algora, A., & Rubio, B. (2018). Shape coexistence and isospin symmetry in A=70 nuclei: Spectroscopy of the T-z =-1 nucleus Kr-70. Phys. Lett. B, 785, 441–446.
Abstract: Excited states in the T-z = -1 nucleus Kr-70 have been populated using inelastic scattering of a radioactive Kr-70 beam as well as one- and two-neutron removal reactions from Kr-71,Kr-72 at intermediate beam energies. The level scheme of Kr-70 was constructed from the observed gamma-ray transitions and coincidences. Tentative spin and parity assignments were made based on comparison with the mirror nucleus Se-70. Asecond 2(+) state and a candidate for the corresponding 4(2)(+) state suggest shape coexistence in Kr-70.
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Caballero-Folch, R. et al, Agramunt, J., Tain, J. L., Algora, A., Domingo-Pardo, C., Guadilla, V., et al. (2018). First determination of beta-delayed multiple neutron emission beyond A=100 through direct neutron measurement: The P-2n value of Sb-136. Phys. Rev. C, 98(3), 034310–10pp.
Abstract: Background: beta-delayed multiple neutron emission has been observed for some nuclei with A <= 100 being the Rb-100 the heaviest beta 2n emitter measured to date. So far only 25 P-2n values have been determined for the approximate to 300 nuclei that may decay in this way. Accordingly it is of interest to measure P-2n values for the other possible multiple neutron emitters throughout the chart of the nuclides. It is of particular interest to make such a measurement for nuclei with A > 100 to test the predictions of theoretical models and simulation tools for the decays of heavy nuclei in the region of very neutron-rich nuclei. In addition the decay properties of these nuclei are fundamental for the understanding of astrophysical nucleosynthesis processes such as the r-process and safety inputs for nuclear reactors. Purpose: To determine for the first time the two-neutron branching ratio the P-2n value for Sb-136 through a direct neutron measurement and to provide precise P-1n values for Sb-136 and Te-136. Method: A pure beam of each isotope of interest was provided by the JYFLTRAP Penning trap at the Ion Guide Isotope Separator On-Line (IGISOL) facility of the University of Jyvaskyla Finland. The purified ions were implanted into a moving tape at the end of the beam line. The detection setup consisted of a plastic scintillator placed right behind the implantation point after the tape to register the beta decays and the BELEN detector based on neutron counters embedded in a polyethylene matrix. The analysis was based on the study of the beta- and neutron-growth-and-decay curves and the beta-one-neutron and beta-two-neutron time correlations which allowed us the determination of the neutron branching ratios. Results: The P-2n value of Sb-136 was found to be 0.14(3)% and the measured P-1n values for Sb-136 and Te-136 were found to be 32.2(15)% and 1.47(6)% respectively. Conclusions: The measured P-2n value is a factor 44 smaller than predicted by the finite-range droplet model plus the quasiparticle random-phase approximation (FRDM+QRPA) model used for r-process calculations.
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Ertoprak, A. et al, Algora, A., Gadea, A., & Huyuk, T. (2018). M1 and E2 transition rates from core-excited states in semi-magic Ru-94. Eur. Phys. J. A, 54(9), 145–9pp.
Abstract: Lifetimes of high-spin states have been measured in the semi-magic (N = 50) nucleus Ru-94. Excited states in Ru-94 were populated in the Ni-58(Ca-40, 4p)Ru-94* fusion-evaporation reaction at the Grand Accelerateur National d'Ions Lourds (GANIL) accelerator complex. DSAM lifetime analysis was performed on the Doppler broadened line shapes in energy spectra obtained from gamma-rays emitted while the residual nuclei were slowing down in a thick 6 mg/cm(2) metallic Ni-58 target. In total eight excited-state lifetimes in the angular momentum range I = (13-20)h have been measured, five of which were determined for the first time. The corresponding B(M1) and B(E2) reduced transition strengths are discussed within the framework of large-scale shell model calculations to study the contribution of different particle-hole configurations, in particular for analyzing contributions from core-excited configurations.
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Sarriguren, P., Algora, A., & Kiss, G. (2018). beta-decay properties of neutron-rich Ca, Ti, and Cr isotopes. Phys. Rev. C, 98(2), 024311–10pp.
Abstract: beta-decay properties of neutron-rich Ca, Ti, and Cr isotopes are studied within a deformed proton-neutron quasiparticle random-phase approximation. The underlying mean field is described self-consistently from deformed Skyrme Hartree-Fock calculations with pairing correlations. Residual spin-isospin interactions in the particle-hole and particle-particle channels are also included in the formalism. The energy distributions of the Gamow-Teller strength, the beta-decay feedings, the beta-decay half-lives, and the beta-delayed neutron emission probabilities are discussed and compared with other theoretical results, as well as with the available experimental information. The evolution of these nuclear beta-decay properties is investigated in isotopic chains in a search for structural changes. A reliable estimate of the beta-decay properties in this mass region is valuable information for evaluating decay rates in astrophysical scenarios.
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Garcia, A. R., Mendoza, E., Cano-Ott, D., Nolte, R., Martinez, T., Algora, A., et al. (2017). New physics model in GEANT4 for the simulation of neutron interactions with organic scintillation detectors. Nucl. Instrum. Methods Phys. Res. A, 868, 73–81.
Abstract: The accurate determination of the response function of organic scintillation neutron detectors complements their experimental characterization. Monte Carlo simulations with GEANT4 can reduce the effort and cost implied, especially for complex detection systems for which the characterization is more challenging. Previous studies have reported on the inaccuracy of GEANT4 in the calculation of the neutron response of organic scintillation detectors above 6 MeV, due to an incomplete description of the neutron-induced alpha production reactions on carbon. We have improved GEANT4 in this direction by incorporating models and data from NRESP, an excellent Monte Carlo simulation tool developed at the Physikalisch-Technische Bundesanstalt (PTB), Germany, for the specific purpose of calculating the neutron response function of organic scintillation detectors. The results have been verified against simulations with NRESP and validated against Time-Of-Flight measurements with an NE213 detector at PTB. This work has potential applications beyond organic scintillation detectors, to other types of detectors where reactions induced by fast neutrons on carbon require an accurate description.
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Rice, S. et al, Algora, A., Tain, J. L., Valencia, E., Agramunt, J., Rubio, B., et al. (2017). Total absorption spectroscopy study of the beta decay of Br-86 and Rb-91. Phys. Rev. C, 96(1), 014320–10pp.
Abstract: The beta decays of Br-86 and Rb-91 have been studied using the total absorption spectroscopy technique. The radioactive nuclei were produced at the Ion Guide Isotope Separator On-Line facility in Jyvaskyla and further purified using the JYFLTRAP. Br-86 and Rb-91 are considered to be major contributors to the decay heat in reactors. In addition, Rb-91 was used as a normalization point in direct measurements of mean gamma energies released in the beta decay of fission products by Rudstam et al. assuming that this decaywas well known from high-resolution measurements. Our results show that both decays were suffering from the Pandemonium effect and that the results of Rudstam et al. should be renormalized. The relative impact of the studied decays in the prediction of the decay heat and antineutrino spectrum from reactors has been evaluated.
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Guadilla, V. et al, Algora, A., Tain, J. L., Agramunt, J., Jordan, M. D., Montaner-Piza, A., et al. (2017). Experimental study of Tc-100 beta decay with total absorption gamma-ray spectroscopy. Phys. Rev. C, 96(1), 014319–10pp.
Abstract: The beta decay of Tc-100 has been studied by using the total absorption gamma-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility in Jyvaskyla. In this work the new Decay Total Absorption gamma-ray Spectrometer in coincidence with a cylindrical plastic beta detector has been employed. The beta intensity to the ground state obtained from the analysis is in good agreement with previous high-resolution measurements. However, differences in the feeding to the first-excited state as well as weak feeding to a new level at high excitation energy have been deduced from this experiment. Theoretical calculations performed in the quasiparticle random-phase approximation framework are also reported. Comparison of these calculations with our measurement serves as a benchmark for calculations of the double beta decay of Mo-100.
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BRIKEN Collaboration(Tarifeño-Saldivia, A. et al), Tain, J. L., Domingo-Pardo, C., Agramunt, J., Algora, A., Morales, A. I., et al. (2017). Conceptual design of a hybrid neutron-gamma detector for study of beta-delayed neutrons at the RIB facility of RIKEN. J. Instrum., 12, P04006–22pp.
Abstract: BRIKEN is a complex detection system to be installed at the RIB-facility of the RIKEN Nishina Center. It is aimed at the detection of heavy-ion implants, β-particles, γ-rays and β-delayed neutrons. The whole detection setup involves the Advanced Implantation Detection Array (AIDA), two HPGe Clover detectors and a large set of 166 counters of 3He embedded in a high-density polyethylene matrix. This article reports on a novel methodology developed for the conceptual design and optimisation of the 3He-tubes array, aiming at the best possible performance in terms of neutron detection. The algorithm is based on a geometric representation of two selected parameters of merit, namely, average neutron detection efficiency and efficiency flatness, as a function of a reduced number of geometric variables. The response of the detection system itself, for each configuration, is obtained from a systematic MC-simulation implemented realistically in Geant4. This approach has been found to be particularly useful. On the one hand, due to the different types and large number of 3He-tubes involved and, on the other hand, due to the additional constraints introduced by the ancillary detectors for charged particles and gamma-rays. Empowered by the robustness of the algorithm, we have been able to design a versatile detection system, which can be easily re-arranged into a compact mode in order to maximize the neutron detection performance, at the cost of the gamma-ray sensitivity. In summary, we have designed a system which shows, for neutron energies up to 1(5) MeV, a rather flat and high average efficiency of 68.6%(64%) and 75.7%(71%) for the hybrid and compact modes, respectively. The performance of the BRIKEN system has been also quantified realistically by means of MC-simulations made with different neutron energy distributions.
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Rubio, B., Gelletly, W., Algora, A., Nacher, E., & Tain, J. L. (2017). Beta decay studies with total absorption spectroscopy and the Lucrecia spectrometer at ISOLDE. J. Phys. G, 44(8), 084004–25pp.
Abstract: Here we present the experimental activities carried out at ISOLDE with the total absorption spectrometer Lucrecia, a large 4 pi scintillator detector designed to absorb a full gamma cascade following beta decay. This spectrometer is designed to measure beta-feeding to excited states without the systematic error called Pandemonium. The set up allows the measurement of decays of very short half life. Experimental results from several campaigns, that focus on the determination of the shapes of beta-decaying nuclei by measuring their beta decay strength distributions as a function of excitation energy in the daughter nucleus, are presented.
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