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Ong, W. J. et al, & Domingo-Pardo, C. (2017). Low-lying level structure of Cu-56 and its implications for the rp process. Phys. Rev. C, 95(5), 055806–8pp.
Abstract: The low-lying energy levels of proton-rich Cu-56 have been extracted using in-beam gamma-ray spectroscopy with the state-of-the-art gamma-ray tracking array GRETINA in conjunction with the S800 spectrograph at the National Superconducting Cyclotron Laboratory at Michigan State University. Excited states in Cu-56 serve as resonances in the Ni-55(p,gamma)Cu-56 reaction, which is a part of the rp process in type-I x-ray bursts. To resolve existing ambiguities in the reaction Q value, a more localized isobaric multiplet mass equation (IMME) fit is used, resulting in Q = 639 +/- 82 keV. We derive the first experimentally constrained thermonuclear reaction rate for Ni-55(p,.) Cu-56. We find that, with this newrate, the rp processmay bypass the (56)Niwaiting point via the Ni-55(p,gamma) reaction for typical x-ray burst conditions with a branching of up to similar to 40%. We also identify additional nuclear physics uncertainties that need to be addressed before drawing final conclusions about the rp-process reaction flow in the Ni-56 region.
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Caballero-Folch, R. et al, Domingo-Pardo, C., Agramunt, J., Algora, A., Rubio, B., & Tain, J. L. (2017). beta-decay half-lives and beta-delayed neutron emission probabilities for several isotopes of Au, Hg, Tl, Pb, and Bi, beyond N=126. Phys. Rev. C, 95(6), 064322–16pp.
Abstract: Background: There have been measurements on roughly 230 nuclei that are beta-delayed neutron emitters. They range from He-8 up to La-150. Apart from 210Tl, with a branching ratio of only 0.007%, no other neutron emitter has been measured beyond A = 150. Therefore, new data are needed, particularly in the region of heavy nuclei around N = 126, in order to guide theoretical models and help understand the formation of the third r-process peak at A similar to 195. Purpose: To measure both beta-decay half-lives and neutron branching ratios of several neutron-rich Au, Hg, Tl, Pb, and Bi isotopes beyond N = 126. Method: Ions of interest were produced by fragmentation of a U-238 beam, selected and identified via the GSI-FRS fragment separator. A stack of segmented silicon detectors (SIMBA) was used to measure ion implants and beta decays. An array of 30 He-3 tubes embedded in a polyethylene matrix (BELEN) was used to detect neutrons with high efficiency and selectivity. A self-triggered digital system is employed to acquire data and to enable time correlations. The latter were analyzed with an analytical model and results for the half-lives and neutron-branching ratios were derived by using the binned maximum-likelihood method. Results: Twenty new beta-decay half-lives are reported for Au204-206, Hg208-211, Tl211-216, Pb215-218, and Bi218-220, nine of them for the first time. Neutron emission probabilities are reported for Hg-210,Hg-211 and Tl211-216. Conclusions: The new beta-decay half-lives are in good agreement with previous measurements on nuclei in this region. The measured neutron emission probabilities are comparable to or smaller than values predicted by global models such as relativistic Hartree Bogoliubov plus the relativistic quasi-particle random phase approximation (RHB + RQRPA).
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n_TOF Collaboration(Sabate-Gilarte et al.), Domingo-Pardo, C., Tain, J. L., & Tarifeño-Saldivia, A. (2017). High-accuracy determination of the neutron flux in the new experimental area n_TOF-EAR2 at CERNx. Eur. Phys. J. A, 53(10), 210–13pp.
Abstract: A new high flux experimental area has recently become operational at the nTOF facility at CERN. This new measuring station, nTOF-EAR2, is placed at the end of a vertical beam line at a distance of approximately 20m from the spallation target. The characterization of the neutron beam, in terms of flux, spatial profile and resolution function, is of crucial importance for the feasibility study and data analysis of all measurements to be performed in the new area. In this paper, the measurement of the neutron flux, performed with different solid-state and gaseous detection systems, and using three neutronconverting reactions considered standard in different energy regions is reported. The results of the various measurements have been combined, yielding an evaluated neutron energy distribution in a wide energy range, from 2meV to 100MeV, with an accuracy ranging from 2%, at low energy, to 6% in the high-energy region. In addition, an absolute normalization of the n_TOF-EAR2 neutron flux has been obtained by means of an activation measurement performed with 197 Au foils in the beam.
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n_TOF Collaboration(Wright, T. et al), Domingo-Pardo, C., Giubrone, G., Tain, J. L., & Tarifeño-Saldivia, A. (2017). Measurement of the U-238(n,gamma) cross section up to 80 keV with the Total Absorption Calorimeter at the CERN n_TOF facility. Phys. Rev. C, 96(6), 064601–11pp.
Abstract: The radiative capture cross section of a highly pure (99.999%), 6.125(2) grams and 9.56(5) x 10(-4) atoms/barn areal density U-238 sample has been measured with the Total Absorption Calorimeter (TAC) in the 185 m flight path at the CERN neutron time-of-flight facility n_TOF. This measurement is in response to the NEA High Priority Request list, which demands an accuracy in this cross section of less than 3% below 25 keV. These data have undergone careful background subtraction, with special care being given to the background originating from neutrons scattered by the 238U sample. Pileup and dead-time effects have been corrected for. The measured cross section covers an energy range between 0.2 eV and 80 keV, with an accuracy that varies with neutron energy, being better than 4% below 25 keV and reaching at most 6% at higher energies.
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n_TOF Collaboration(Lerendegui-Marco, J. et al.), Domingo-Pardo, C., Tain, J. L., & Tarifeño-Saldivia, A. (2018). Radiative neutron capture on Pu-242 in the resonance region at the CERN n_TOF-EAR1 facility. Phys. Rev. C, 97(2), 024605–21pp.
Abstract: The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with uranium to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. However, an extensive use of MOX fuels, in particular in fast reactors, requires more accurate capture and fission cross sections for some Pu isotopes. In the case of Pu-242 there are sizable discrepancies among the existing capture cross-section measurements included in the evaluations (all from the 1970s) resulting in an uncertainty as high as 35% in the fast energy region. Moreover, postirradiation experiments evaluated with JEFF-3.1 indicate an overestimation of 14% in the capture cross section in the fast neutron energy region. In this context, the Nuclear Energy Agency (NEA) requested an accuracy of 8% in this cross section in the energy region between 500 meV and 500 keV. This paper presents a new time-of-flight capture measurement on Pu-242 carried out at nTOF-EAR1 (CERN), focusing on the analysis and statistical properties of the resonance region, below 4 keV. The Pu-242(n, gamma) reaction on a sample containing 95(4) mg enriched to 99.959% was measured with an array of four C6D6 detectors and applying the total energy detection technique. The high neutron energy resolution of nTOF-EAR1 and the good statistics accumulated have allowed us to extend the resonance analysis up to 4 keV, obtaining new individual and average resonance parameters from a capture cross section featuring a systematic uncertainty of 5%, fulfilling the request of the NEA.
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