Huyuk, T. et al, Gadea, A., Aliaga-Varea, R. J., & Domingo-Pardo, C. (2016). Conceptual design of the early implementation of the NEutron Detector Array (NEDA) with AGATA. Eur. Phys. J. A, 52(3), 55–8pp.
Abstract: The NEutron Detector Array (NEDA) project aims at the construction of a new high-efficiency compact neutron detector array to be coupled with large gamma-ray arrays such as AGATA. The application of NEDA ranges from its use as selective neutron multiplicity filter for fusion-evaporation reaction to a large solid angle neutron tagging device. In the present work, possible configurations for the NEDA coupled with the Neutron Wall for the early implementation with AGATA has been simulated, using Monte Carlo techniques, in order to evaluate their performance figures. The goal of this early NEDA implementation is to improve, with respect to previous instruments, efficiency and capability to select multiplicity for fusion-evaporation reaction channels in which 1, 2 or 3 neutrons are emitted. Each NEDA detector unit has the shape of a regular hexagonal prism with a volume of about 3.23 l and it is filled with the EJ301 liquid scintillator, that presents good neutron-gamma discrimination properties. The simulations have been performed using a fusion-evaporation event generator that has been validated with a set of experimental data obtained in the Ni-58 + Fe-56 reaction measured with the Neutron Wall detector array.
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Domingo-Pardo, C. (2016). Beta-delayed neutron emission: first measurements in the heavy mass region and future prospects. Acta Phys. Pol. B, 47(3), 729–737.
Abstract: Beta-delayed neutrons play a key role in the formation of heavy elements in explosive stellar environments. The final r-process abundance distribution, including the rare-earth peak, is tailored to a large extent by the neutrons released after the beta decay of very exotic neutron-rich nuclei encountered along the r-process path and during the freeze-out phase. Such scenarios involve a vast amount of – yet undiscovered – nuclei, and most of them are expected to be neutron emitters. In this respect, existing beta-delayed neutron emission data is rather scarce, spanning from the lightest isotopes up to the region of the fission-fragments with masses up to A similar to 150. This contribution gives an overview on the latest measurements of neutron branching ratios in the heavy mass region around N = 126, which was practically unexplored in the past. Present plans to access very exotic nuclei at the RIB-facility of RIKEN in the framework of the BRIKEN project, are presented, together with the expected impact in r-process nucleosynthesis studies.
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n_TOF Collaboration(Zugec, P. et al), Domingo-Pardo, C., Giubrone, G., & Tain, J. L. (2016). Integral measurement of the C-12(n, p)B-12 reaction up to 10 GeV. Eur. Phys. J. A, 52(4), 101–13pp.
Abstract: The integral measurement of the C-12(n, p)B-12 reaction was performed at the neutron time-of-flight facility nTOF at CERN. The total number of B-12 nuclei produced per neutron pulse of the nTOF beam was determined using the activation technique in combination with a time-of-flight technique. The cross section is integrated over the n_TOF neutron energy spectrum from reaction threshold at 13.6 MeV to 10 GeV. Having been measured up to 1 GeV on basis of the U-235(n, f) reaction, the neutron energy spectrum above 200 MeV has been re-evaluated due to the recent extension of the cross section reference for this particular reaction, which is otherwise considered a standard up to 200 MeV. The results from the dedicated GEANT4 simulations have been used to evaluate the neutron flux from 1 GeV up to 10 GeV. The experimental results related to the C-12(n, p)B-12 reaction are compared with the evaluated cross sections from major libraries and with the predictions of different GEANT4 models, which mostly underestimate the B-12 production. On the contrary, a good reproduction of the integral cross section derived from measurements is obtained with TALYS-1.6 calculations, with optimized parameters.
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Caballero-Folch, R. et al, Domingo-Pardo, C., Agramunt, J., Algora, A., Rubio, B., & Tain, J. L. (2016). First Measurement of Several beta-Delayed Neutron Emitting Isotopes Beyond N=126. Phys. Rev. Lett., 117(1), 012501–6pp.
Abstract: The beta-delayed neutron emission probabilities of neutron rich Hg and Tl nuclei have been measured together with beta-decay half-lives for 20 isotopes of Au, Hg, Tl, Pb, and Bi in the mass region N greater than or similar to 126. These are the heaviest species where neutron emission has been observed so far. These measurements provide key information to evaluate the performance of nuclear microscopic and phenomenological models in reproducing the high-energy part of the beta-decay strength distribution. This provides important constraints on global theoretical models currently used in r-process nucleosynthesis.
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n_TOF Collaboration(Barbagallo, M. et al), Domingo-Pardo, C., Tain, J. L., & Tarifeño-Saldivia, A. (2016). Be-7(n,alpha)He-4 Reaction and the Cosmological Lithium Problem: Measurement of the Cross Section in a Wide Energy Range at n_TOF at CERN. Phys. Rev. Lett., 117(15), 152701–7pp.
Abstract: The energy-dependent cross section of the (7)Bed(n,alpha)He-4 reaction, of interest for the so-called cosmological lithium problem in big bang nucleosynthesis, has been measured for the first time from 10 meV to 10 keV neutron energy. The challenges posed by the short half-life of Be-7 and by the low reaction cross section have been overcome at nTOF thanks to an unprecedented combination of the extremely high luminosity and good resolution of the neutron beam in the new experimental area (EAR2) of the nTOF facility at CERN, the availability of a sufficient amount of chemically pure Be-7, and a specifically designed experimental setup. Coincidences between the two alpha particles have been recorded in two Si-Be-7-Si arrays placed directly in the neutron beam. The present results are consistent, at thermal neutron energy, with the only previous measurement performed in the 1960s at a nuclear reactor. The energy dependence reported here clearly indicates the inadequacy of the cross section estimates currently used in BBN calculations. Although new measurements at higher neutron energy may still be needed, the n_TOF results hint at a minor role of this reaction in BBN, leaving the long-standing cosmological lithium problem unsolved.
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n_TOF Collaboration(Gunsing, F. et al), Domingo-Pardo, C., Tain, J. L., & Tarifeño-Saldivia, A. (2016). Nuclear data activities at the n_TOF facility at CERN. Eur. Phys. J. Plus, 131(10), 371–13pp.
Abstract: Nuclear data in general, and neutron-induced reaction cross sections in particular, are important for a wide variety of research fields. They play a key role in the safety and criticality assessment of nuclear technology, not only for existing power reactors but also for radiation dosimetry, medical applications, the transmutation of nuclear waste, accelerator-driven systems, fuel cycle investigations and future reactor systems as in Generation IV. Applications of nuclear data are also related to research fields as the study of nuclear level densities and stellar nucleosynthesis. Simulations and calculations of nuclear technology applications largely rely on evaluated nuclear data libraries. The evaluations in these libraries are based both on experimental data and theoretical models. Experimental nuclear reaction data are compiled on a worldwide basis by the international network of Nuclear Reaction Data Centres (NRDC) in the EXFOR database. The EXFOR database forms an important link between nuclear data measurements and the evaluated data libraries. CERN's neutron time-of-flight facility nTOF has produced a considerable amount of experimental data since it has become fully operational with the start of the scientific measurement programme in 2001. While for a long period a single measurement station (EAR1) located at 185 m from the neutron production target was available, the construction of a second beam line at 20 m (EAR2) in 2014 has substantially increased the measurement capabilities of the facility. An outline of the experimental nuclear data activities at CERN's neutron time-of-flight facility nTOF will be presented.
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n_TOF Collaboration(Mingrone, F. et al), Domingo-Pardo, C., Giubrone, G., & Tain, J. L. (2017). Neutron capture cross section measurement of U-238 at the CERN n_TOF facility in the energy region from 1 eV to 700 keV. Phys. Rev. C, 95(3), 034604–14pp.
Abstract: The aim of this work is to provide a precise and accurate measurement of the U-238(n,gamma) reaction cross section in the energy region from 1 eV to 700 keV. This reaction is of fundamental importance for the design calculations of nuclear reactors, governing the behavior of the reactor core. In particular, fast reactors, which are experiencing a growing interest for their ability to burn radioactive waste, operate in the high energy region of the neutron spectrum. In this energy region most recent evaluations disagree due to inconsistencies in the existing measurements of up to 15%. In addition, the assessment of nuclear data uncertainty performed for innovative reactor systems shows that the uncertainty in the radiative capture cross section of U-238 should be further reduced to 1-3% in the energy region from 20 eV to 25 keV. To this purpose, addressed by the Nuclear Energy Agency as a priority nuclear data need, complementary experiments, one at the GELINA and two at the nTOF facility, were proposed and carried out within the 7th Framework Project ANDES of the European Commission. The results of one of these U-238(n, gamma) measurements performed at the nTOF CERN facility are presented in this work. The gamma-ray cascade following the radiative neutron capture has been detected exploiting a setup of two C6D6 liquid scintillators. Resonance parameters obtained from this work are on average in excellent agreement with the ones reported in evaluated libraries. In the unresolved resonance region, this work yields a cross section in agreement with evaluated libraries up to 80 keV, while for higher energies our results are significantly higher.
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PreSPEC and AGATA Collaborations(Ralet, D. et al), Domingo-Pardo, C., Gadea, A., & Huyuk, T. (2017). Lifetime measurement of neutron-rich even-even molybdenum isotopes. Phys. Rev. C, 95(3), 034320–11pp.
Abstract: Background: In the neutron-rich A approximate to 100 mass region, rapid shape changes as a function of nucleon number as well as coexistence of prolate, oblate, and triaxial shapes are predicted by various theoretical models. Lifetime measurements of excited levels in the molybdenum isotopes allow the determination of transitional quadrupole moments, which in turn provides structural information regarding the predicted shape change. Purpose: The present paper reports on the experimental setup, the method that allowed one to measure the lifetimes of excited states in even-even molybdenum isotopes from mass A = 100 up to mass A = 108, and the results that were obtained. Method: The isotopes of interest were populated by secondary knock-out reaction of neutron-rich nuclei separated and identified by the GSI fragment separator at relativistic beam energies and detected by the sensitive PreSPEC-AGATA experimental setup. The latter included the Lund-York-Cologne calorimeter for identification, tracking, and velocity measurement of ejectiles, and AGATA, an array of position sensitive segmented HPGe detectors, used to determine the interaction positions of the gamma ray enabling a precise Doppler correction. The lifetimes were determined with a relativistic version of the Doppler-shift-attenuation method using the systematic shift of the energy after Doppler correction of a gamma-ray transition with a known energy. This relativistic Doppler-shift-attenuation method allowed the determination of mean lifetimes from 2 to 250 ps. Results: Even-even molybdenum isotopes from mass A = 100 to A = 108 were studied. The decays of the low-lying states in the ground-state band were observed. In particular, two mean lifetimes were measured for the first time: tau = 29.7(-9.1)(+11.3) ps for the 4(+) state of Mo-108 and tau = 3.2(-0.7)(+ 0.7) ps for the 6(+) state of Mo-102. Conclusions: The reduced transition strengths B(E2), calculated from lifetimes measured in this experiment, compared to beyond-mean-field calculations, indicate a gradual shape transition in the chain of molybdenum isotopes when going from A = 100 to A = 108 with a maximum reached at N = 64. The transition probabilities decrease for Mo-108 which may be related to its well-pronounced triaxial shape indicated by the calculations.
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Dudouet, J. et al, Domingo-Pardo, C., Gadea, A., & Perez-Vidal, R. M. (2017). Kr-96(36)60-Low-Z Boundary of the Island of Deformation at N=60. Phys. Rev. Lett., 118(16), 162501–6pp.
Abstract: Prompt.-ray spectroscopy of the neutron-rich Kr-96, produced in transfer-and fusion-induced fission reactions, has been performed using the combination of the Advanced Gamma Tracking Array and the VAMOS + +spectrometer. A second excited state, assigned to J pi = 4(+), is observed for the first time, and a previously reported level energy of the first 2+ excited state is confirmed. The measured energy ratio R-4/2 = E(4(+))/E(2(+)) = 2.12(1) indicates that this nucleus does not show a well-developed collectivity contrary to that seen in heavier N = 60 isotones. This new measurement highlights an abrupt transition of the degree of collectivity as a function of the proton number at Z = 36, of similar amplitude to that observed at N = 60 at higher Z values. A possible reason for this abrupt transition could be related to the insufficient proton excitations in the g(9/2), d(5/2), and s(1/2) orbitals to generate strong quadrupole correlations or to the coexistence of competing different shapes. An unexpected continuous decrease of R-4/2 as a function of the neutron number up to N = 60 is also evidenced. This measurement establishes the Kr isotopic chain as the low-Z boundary of the island of deformation for N = 60 isotones. A comparison with available theoretical predictions using different beyond mean-field approaches shows that these models fail to reproduce the abrupt transitions at N = 60 and Z = 36.
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Guerrero, C., Domingo-Pardo, C., Kappeler, F., Lerendegui-Marco, J., Palomo, F. R., Quesada, J. M., et al. (2017). Prospects for direct neutron capture measurements on s-process branching point isotopes. Eur. Phys. J. A, 53(5), 87–5pp.
Abstract: The neutron capture cross sections of several unstable key isotopes acting as branching points in the s-process are crucial for stellar nucleosynthesis studies, but they are very challenging to measure directly due to the difficult production of sufficient sample material, the high activity of the resulting samples, and the actual (n, gamma) measurement, where high neutron fluxes and effective background rejection capabilities are required. At present there are about 21 relevant s-process branching point isotopes whose cross section could not be measured yet over the neutron energy range of interest for astrophysics. However, the situation is changing with some very recent developments and upcoming technologies. This work introduces three techniques that will change the current paradigm in the field: the use of gamma-ray imaging techniques in (n,gamma) experiments, the production of moderated neutron beams using high-power lasers, and double capture experiments in Maxwellian neutron beams.
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