Watanabe, H. et al, & Montaner-Piza, A. (2019). New isomers in (125)Pd(79)( )and Pd-127(81): Competing proton and neutron excitations in neutron-rich palladium nuclides towards the N=82 shell closure. Phys. Lett. B, 792, 263–268.
Abstract: The neutron-rich isotopes of palladium have attracted considerable interest in terms of the evolution of the N = 82 neutron shell closure and its influence on the r-process nucleosynthesis. In this Letter, we present the first spectroscopic information on the excited states in Pd-125(79) and Pd-127(81) studied using the EURICA gamma-ray spectrometer, following production via in-flight fission of a high-intensity U-238 beam at the RIBF facility. New isomeric states with half-lives of 144(4) ns and 39(6) μs have been assigned spins and parities of (23/2(+)) and (19/2(+)) in Pd-125 and Pd-127, respectively. The observed level properties are compared to a shell-model calculation, suggesting the competition between proton excitations and neutron excitations in the proton-hole and neutron-hole systems in the vicinity of the doubly magic nucleus Sn-132.
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Chen, Z. Q. et al, & Montaner-Piza, A. (2019). Proton Shell Evolution below Sn-132: First Measurement of Low-Lying beta-Emitting Isomers in Ag-123,Ag-325. Phys. Rev. Lett., 122(21), 212502–6pp.
Abstract: The beta-delayed gamma-ray spectroscopy of neutron-rich Ag-123,Ag-325 isotopes is investigated at the Radioactive Isotope Beam Factory of RIKEN, and the long-predicted 1/2(-) beta-emitting isomers in Ag-123,Ag-325 are identified for the first time. With the new experimental results, the systematic trend of energy spacing between the lowest 9/2(+) and 1/2(-) levels is extended in Ag isotopes up to N = 78, providing a clear signal for the reduction of the Z = 40 subshell gap in Ag towards N = 82. Shell-model calculations with the state-of-the-art V-MU plus M3Y spin-orbit interaction give a satisfactory description of the low-lying states in Ag-123,Ag-325. The tensor force is found to play a crucial role in the evolution of the size of the Z = 40 subshell gap. The observed inversion of the single-particle levels around Ag-123 can be well interpreted in terms of the monopole shift of the pi 1g(9/2) orbitals mainly caused by the increasing occupation of nu 1h(11/2) orbitals.
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Guadilla, V., Algora, A., Tain, J. L., Agramunt, J., Jordan, D., Monserrate, M., et al. (2019). Total absorption gamma-ray spectroscopy of niobium isomers. Phys. Rev. C, 100(2), 024311–15pp.
Abstract: The beta-intensity distributions of the decays of Nb-100gs,Nb-100m and Nb-102gs,Nb-102m have been determined using the total absorption gamma-ray spectroscopy technique. The JYFLTRAP double Penning trap system was employed in a campaign of challenging measurements performed with the decay total absorption gamma-ray spectrometer at the Ion Guide Isotope Separator On-Line facility in Jyvaskyla. Different strategies were applied to disentangle the isomeric states involved, lying very close in energy. The low-spin component of each niobium case was populated through the decay of the zirconium parent, which was treated as a contaminant. We have applied a method to extract this contamination, and additionally we have obtained beta-intensity distributions for these zirconium decays. The beta-strength distributions evaluated with these results were compared with calculations in a quasiparticle random-phase approximation, suggesting a prolate configuration for the ground states of Zr-100,Zr-102. The footprint of the Pandemonium effect was found when comparing our results for the analyses of the niobium isotopes with previous decay data. The beta-intensities of the decay of Nb-102m, for which there were no previous data, were obtained. A careful evaluation of the uncertainties was carried out, and the consistency of our results was validated taking advantage of the segmentation of our spectrometer. The final results were used as input in reactor summation calculations. A large impact on antineutrino spectrum calculations was already reported, and here we detail the significant impact on decay heat calculations.
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Guadilla, V. et al, Tain, J. L., Algora, A., Agramunt, J., Jordan, D., Monserrate, M., et al. (2019). Total absorption gamma-ray spectroscopy of the beta-delayed neutron emitters I-137 and Rb-95. Phys. Rev. C, 100(4), 044305–17pp.
Abstract: The decays of the beta-delayed neutron emitters( 137)I and Rb-95 have been studied with the total absorption gamma-ray spectroscopy technique. The purity of the beams provided by the JYFLTRAP Penning trap at the ion guide isotope separator on-line facility in Jyvaskyla allowed us to carry out a campaign of isotopically pure measurements with the decay total absorption gamma-ray spectrometer, a segmented detector composed of 18 NaI(T1) modules. The contamination coming from the interaction of neutrons with the spectrometer has been carefully studied, and we have tested the use of time differences between prompt gamma rays and delayed neutron interactions to eliminate this source of contamination. Due to the sensitivity of our spectrometer, we have found a significant amount of beta intensity to states above the neutron separation energy that deexcite by gamma rays, comparable to the neutron emission probability. The competition between gamma deexcitation and neutron emission has been compared with Hauser-Feshbach calculations, and it can be understood as a nuclear structure effect. In addition, we have studied the impact of the beta-intensity distributions determined in this work on reactor decay heat and reactor antineutrino spectrum summation calculations. The robustness of our results is demonstrated by a thorough study of uncertainties and with the reproduction of the spectra of the individual modules and the module-multiplicity gated spectra. This work represents the state-of-the-art of our analysis methodology for segmented total absorption spectrometers.
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Jungclaus, A. et al, & Montaner-Piza, A. (2020). Evolution of proton single-particle states in neutron-rich Sb isotopes beyond N=82. Phys. Rev. C, 102(3), 034324–11pp.
Abstract: The beta decay of the semimagic Sn isotopes Sn-136,Sn-137,Sn-138 has been studied at the Radioactive Isotope Beam Factory at the RIKEN Nishina Center. The first experimental information on excited states was obtained for Sb-137 while, in the case of Sb-136, the established excitation scheme could be extended by ten previously unidentified levels. In the decay of the most-neutron-rich isotope Sn-138, two gamma rays were observed for the first time. The new experimental results, in combination with state-of-the-art shell-model calculations, provide the first information with respect to the evolution of the Og(7/2) and 1d(5/2) proton single-particle states with increasing neutron number beyond N = 84.
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Guadilla, V. et al, Tain, J. L., Algora, A., Agramunt, J., Jordan, D., Monserrate, M., et al. (2020). Determination of beta-decay ground state feeding of nuclei of importance for reactor applications. Phys. Rev. C, 102(6), 064304–12pp.
Abstract: In beta-decay studies the determination of the decay probability to the ground state (g.s.) of the daughter nucleus often suffers from large systematic errors. The difficulty of the measurement is related to the absence of associated delayed gamma-ray emission. In this work we revisit the 4 pi gamma – beta method proposed by Greenwood and collaborators in the 1990s, which has the potential to overcome some of the experimental difficulties. Our interest is driven by the need to determine accurately the beta-intensity distributions of fission products that contribute significantly to the reactor decay heat and to the antineutrinos emitted by reactors. A number of such decays have large g.s. branches. The method is relevant for nuclear structure studies as well. Pertinent formulas are revised and extended to the special case of beta-delayed neutron emitters, and the robustness of the method is demonstrated with synthetic data. We apply it to a number of measured decays that serve as test cases and discuss the features of the method. Finally, we obtain g.s. feeding intensities with reduced uncertainty for four relevant decays that will allow future improvements in antineutrino spectrum and decay heat calculations using the summation method.
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Orrigo, S. E. A. et al, Rubio, B., Gelletly, W., Aguilera, P., Algora, A., Morales, A. I., et al. (2021). beta decay of the very neutron-deficient Ge-60 and Ge-62 nuclei. Phys. Rev. C, 103(1), 014324–12pp.
Abstract: We report here the results of a study of the beta decay of the proton-rich Ge isotopes, Ge-60 and Ge-62, produced in an experiment at the RIKEN Nishina Center. We have improved our knowledge of the half-lives of Ge-62 [73.5(1) ms] and Ge-60 [25.0(3) ms] and its daughter nucleus, Ga-60 [69.4(2) ms]. We measured individual beta-delayed proton and gamma emissions and their related branching ratios. Decay schemes and absolute Fermi and Gamow-Teller transition strengths have been determined. The mass excesses of the nuclei under study have been deduced. A total beta-delayed proton-emission branching ratio of 67(3)% has been obtained for Ge-60. New information has been obtained on the energy levels populated in Ga-60 and on the 1/2(-) excited state in the beta p daughter Zn-59. We extracted a ground state-to-ground state feeding of 85.3(3)% for the decay of Ge-62. Eight new y lines have been added to the deexcitation of levels populated in the Ga-62 daughter.
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Moon, B. et al, & Montaner-Piza, A. (2021). Nuclear structure of Te isotopes beyond neutron magic number N=82. Phys. Rev. C, 103(3), 034320–15pp.
Abstract: Newly observed decay schemes of the nuclei Sb-137 and Sb-138 are reported. The neutron-rich Sb isotopes were produced by the in-flight fragmentation of a U-238 primary beam with an energy of 345 MeV/nucleon. Several new excited states of Te-137 with tentatively assigned spin-parities of (5/2(-)), (9/2(-)), and (7/2) have been established which play an important role in the evolution of neutron levels beyond N = 82. The study of the beta decay of Sb-138 led to a considerable extension of the level scheme of Te-138 including the identification of several nonyrast states. The structure of Te-137 and Te-138 is discussed on the basis of large-scale shell-model calculations performed using two different effective interactions.
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Guadilla, V. et al, Algora, A., Tain, J. L., Agramunt, J., Jordan, D., Monserrate, M., et al. (2022). Total absorption gamma-ray spectroscopy of the ss decays of Y-96gs,Y-m. Phys. Rev. C, 106(1), 014306–14pp.
Abstract: The ss decays of the ground state (gs) and isomeric state (m) of Y-96 have been studied with the total absorption gamma-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility. The separation of the 8(+) isomeric state from the 0(-) ground state was achieved thanks to the purification capabilities of the JYFLTRAP double Penning trap system. The ss-intensity distributions of both decays have been independently determined. In the analyses the deexcitation of the 1581.6 keV level in Zr-96, in which conversion electron emission competes with pair production, has been carefully considered and found to have significant impact on the ss-detector efficiency, influencing the ss-intensity distribution obtained. Our results for Y-96gs (0(-)) confirm the large ground state to ground state ss-intensity probability, although a slightly larger value than reported in previous studies was obtained, amounting to 96.6(-2.1)(+0.3) % of the total ss intensity. Given that the decay of Y-96gs is the second most important contributor to the reactor antineutrino spectrum between 5 and 7 MeV, the impact of the present results on reactor antineutrino summation calculations has been evaluated. In the decay of Y-96m (8(+)), previously undetected ss intensity in transitions to states above 6 MeV has been observed. This shows the importance of total absorption gamma-ray spectroscopy measurements of ss decays with highly fragmented deexcitation patterns. Y-96m (8(+)) is a major contributor to reactor decay heat in uranium-plutonium and thorium-uranium fuels around 10 s after fission pulses, and the newly measured average ss and gamma energies differ significantly from the previous values in evaluated databases. The discrepancy is far above the previously quoted uncertainties. Finally, we also report on the successful implementation of an innovative total absorption gamma-ray spectroscopy analysis of the module-multiplicity gated spectra, as a first proof of principle to distinguish between decaying states with very different spin-parity values.
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Vitez-Sveiczer, A. et al, Algora, A., Morales, A. I., Rubio, B., Agramunt, J., Guadilla, V., et al. (2022). The beta-decay of Kr-70 into Br-70: Restoration of the pseudo-SU(4) symmetry. Phys. Lett. B, 830, 137123–8pp.
Abstract: The beta-decay of the even-even nucleus Kr-70 with Z=N+2, has been investigated at the Radioactive Ion Beam Factory (RIBF) of the RIKEN Nishina Center using the BigRIPS fragment separator, the ZeroDegree Spectrometer, the WAS3ABI implantation station and the EURICA HPGe cluster array. Fifteen gamma-rays associated with the beta-decay of( 70)Kr into Br-70 have been identified for the first time, defining ten populated states below E-exc=3300 keV. The half-life of Kr-70 was derived with increased precision and found to be t(1/2)=45.19 +/- 0.14 ms. The beta-delayed proton emission probability has also been determined as epsilon(p)=0.545(23)%. An increase in the beta-strength to the yrast 1(+) state in comparison with the heaviest Z=N+2 system studied so far (Ge-62 decay) is observed that may indicate increased np correlations in the T=0 channel. The beta-decay strength deduced from the results is interpreted in terms of the proton-neutron quasiparticle random-phase approximation (pnQRPA) and also with a schematic model that includes isoscalar and isovector pairing in addition to quadrupole deformation. The application of this last model indicates an approximate realization of pseudo-SU(4) symmetry in this system.
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