n_TOF Collaboration, Gunsing, F., Berthoumieux, E., Borella, A., Belgya, T., Szentmiklosi, L., et al. (2011). Neutron Capture on (209)Bi: Determination of the Production Ratio of (210m)Bi/(210g)Bi. J. Korean Phys. Soc., 59(2), 1670–1675.
Abstract: Neutron capture on (209)Bi produces either an isomeric state (210m)Bi with a half life of 3 x 106 years, or the ground state (210g)Bi which decays with a half life of 5 days to the alpha emitter (210)Po. Therefore the neutron capture cross section ratio (209)Bi(n,gamma)(210m)Bi/(210g)Bi plays an important role in predicting the short- and long-term radio-toxicity produced by (209)Bi under neutron irradiation. This ratio is dependent on the neutron energy. We have measured this ratio for cold neutrons at the cold neutron beam facility of the Budapest Neutron Centre by observing the population of the ground-and the metastable state using high resolution gamma-ray spectroscopy. The same technique has been used at the pulsed white neutron source GELINA of the IRMM, Geel in combination with the neutron time-of-flight technique. Results for the neutron-energy dependent branching ratio will be presented. In addition we performed simulations using a statistical decay code.
|
Jordan, D., Tain, J. L., Algora, A., Agramunt, J., Domingo-Pardo, C., Gomez-Hornillos, M. B., et al. (2013). Measurement of the neutron background at the Canfranc Underground Laboratory LSC. Astropart Phys., 42, 1–6.
Abstract: The energy distribution of the neutron background was measured for the first time at Hall A of the Canfranc Underground Laboratory. For this purpose we used a novel approach based on the combination of the information obtained with six large high-pressure He-3 proportional counters embedded in individual polyethylene blocks of different size. In this way not only the integral value but also the flux distribution as a function of neutron energy was determined in the range from 1 eV to 10 MeV. This information is of importance because different underground experiments show different neutron background energy dependence. The high sensitivity of the setup allowed to measure a neutron flux level which is about four orders of magnitude smaller that the neutron background at sea level. The integral value obtained is Phi(Hall A) = (3.44 +/- 0.35) x 10(-6) cm(-2) s(-1).
|
n_TOF Collaboration, Kappeler, F., Mengoni, A., Mosconi, M., Fujii, K., Heil, M., et al. (2011). Neutron Studies for Dating the Universe. J. Korean Phys. Soc., 59(2), 2094–2099.
Abstract: The neutron capture cross sections of (186)Os and (187)Os are of key importance for defining the 8-process abundance of (187)Os at the formation of the solar system. This quantity can be used to determine the radiogenic abundance component of (187)Os from the decay of (187)Re (t(1/2) = 41.2 Gyr) and to infer the time-duration of the nucleosynthesis in our galaxy (Re/Os cosmochronometer). The neutron capture cross sections of (186)Os, (187)Os, and (188)Os have been measured at the CERN nTOF facility from 1 eV to 1 MeV, covering the entire energy range of astrophysical interest. From these data Maxwellian averaged capture cross sections have been calculated with uncertainties between 3.3 and 4.7%. Additional information was obtained by measuring the inelastic scattering cross section of (187)Os at the Karlsruhe 3.7 MV Van de Graaff accelerator and by neutron resonance analyses of the nTOF capture data to establish a comprehensive experimental basis for the Hauser-Feshbach statistical model. Consistent I-IF calculations for the capture and inelastic reaction channels were performed to determine the stellar enhancement factors, which are required to correct the Maxwellian averaged cross sections for the effect of thermally populated excited states. The consequences of this analysis for the s-process component of the (187)Os abundance and the related impact on the evaluation of the time-duration of Galactic nucleosynthesis via the Re/Os cosmo-chronometer are discussed.
|
Magan, D. L. P., Caballero, L., Domingo-Pardo, C., Agramunt-Ros, J., Albiol, F., Casanovas, A., et al. (2016). First tests of the applicability of gamma-ray imaging for background discrimination in time-of-flight neutron capture measurements. Nucl. Instrum. Methods Phys. Res. A, 823, 107–119.
Abstract: In this work we explore for the first time the applicability of using gamma-ray imaging in neutron capture measurements to identify and suppress spatially localized background. For this aim, a pinhole gamma camera is assembled, tested and characterized in terms of energy and spatial performance. It consists of a monolithic CeBr3 scintillating crystal coupled to a position-sensitive photomultiplier and readout through an integrated circuit AMIC2GR. The pinhole collimator is a massive carven block of lead. A series of dedicated measurements with calibrated sources and with a neutron beam incident on a Au-197 sample have been carried out at n_TOF, achieving an enhancement of a factor of two in the signal-to-background ratio when selecting only those events coming from the direction of the sample.
|
n_TOF Collaboration(Alcayne, V. et al), Balibrea-Correa, J., Domingo-Pardo, C., Lerendegui-Marco, J., Babiano-Suarez, V., & Ladarescu, I. (2024). A Segmented Total Energy Detector (sTED) optimized for (n,γ) cross-section measurements at n_TOF EAR2. Radiat. Phys. Chem., 217, 11pp.
Abstract: The neutron time-of-flight facility nTOF at CERN is a spallation source dedicated to measurements of neutroninduced reaction cross-sections of interest in nuclear technologies, astrophysics, and other applications. Since 2014, Experimental ARea 2 (EAR2) is operational and delivers a neutron fluence of similar to 4 center dot 10(7) neutrons per nominal proton pulse, which is similar to 50 times higher than the one of Experimental ARea 1 (EAR1) of similar to 8 center dot 10(5) neutrons per pulse. The high neutron flux at EAR2 results in high counting rates in the detectors that challenged the previously existing capture detection systems. For this reason, a Segmented Total Energy Detector (sTED) has been developed to overcome the limitations in the detector's response, by reducing the active volume per module and by using a photo-multiplier (PMT) optimized for high counting rates. This paper presents the main characteristics of the sTED, including energy and time resolution, response to gamma-rays, and provides as well details of the use of the Pulse Height Weighting Technique (PHWT) with this detector. The sTED has been validated to perform neutron-capture cross-section measurements in EAR2 in the neutron energy range from thermal up to at least 400 keV. The detector has already been successfully used in several measurements at nTOF EAR2.
|
