Guadilla, V. et al, Algora, A., Tain, J. L., Agramunt, J., Aysto, J., Jordan, D., et al. (2019). Large Impact of the Decay of Niobium Isomers on the Reactor (v)over-bar(e) Summation Calculations. Phys. Rev. Lett., 122(4), 042502–6pp.
Abstract: Even mass neutron-rich niobium isotopes are among the principal contributors to the reactor antineutrino energy spectrum. They are also among the most challenging to measure due to the refractory nature of niobium, and because they exhibit isomeric states lying very close in energy. The beta-intensity distributions of Nb-100gs,Nb-100m and Nb-102gs,Nb-02m beta decays have been determined using the total absorption.-ray spectroscopy technique. The measurements were performed at the upgraded Ion Guide Isotope Separator On-Line facility at the University of Jyvaskyla. Here, the double Penning trap system JYFLTRAP was employed to disentangle the beta decay of the isomeric states. The new data obtained in this challenging measurement have a large impact in antineutrino summation calculations. For the first time the discrepancy between the summation model and the reactor antineutrino measurements in the region of the shape distortion has been reduced.
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Estienne, M., Fallot, M., Algora, A., Briz-Monago, J., Bui, V. M., Cormon, S., et al. (2019). Updated Summation Model: An Improved Agreement with the Daya Bay Antineutrino Fluxes. Phys. Rev. Lett., 123(2), 022502–6pp.
Abstract: A new summation method model of the reactor antineutrino energy spectrum is presented. It is updated with the most recent evaluated decay databases and with our total absorption gamma-ray spectroscopy measurements performed during the last decade. For the first time, the spectral measurements from the Daya Bay experiment are compared with the antineutrino energy spectrum computed with the updated summation method without any renormalization. The results exhibit a better agreement than is obtained with the Huber-Mueller model in the 2-5 MeV range, the region that dominates the detected flux. A systematic trend is found in which the antineutrino flux computed with the summation model decreases with the inclusion of more pandemonium-free data. The calculated flux obtained now lies only 1.9% above that detected in the Daya Bay experiment, a value that may be reduced with forthcoming new pandemonium-free data, leaving less room for a reactor anomaly. Eventually, the new predictions of individual antineutrino spectra for the U-235, Pu-239, Pu-241, and U-238 are used to compute the dependence of the reactor antineutrino spectral shape on the fission fractions.
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Phong, V. H. et al, Agramunt, J., Algora, A., Domingo-Pardo, C., Morales, A. I., Tain, J. L., et al. (2019). Observation of a μs isomer in In-134(49)85: Proton-neutron coupling “southeast” of Sn-132(50)82. Phys. Rev. C, 100(1), 011302–6pp.
Abstract: We report on the observation of a microsecond isomeric state in the single-proton-hole, three-neutron-particle nucleus In-134. The nuclei of interest were produced by in-flight fission of a U-238 beam at the Radioactive Isotope Beam Factory at RIKEN. The isomer depopulates through a gamma ray of energy 56.7(1) keV and with a half-life of T-1/2 = 3.5(4) μs. Based on the comparison with shell-model calculations, we interpret the isomer as the I-pi = 5(-) member of the pi 0g(9/2)(-1) circle times nu 1f(7/2)(3) multiplet, decaying to the I-pi = 7(-) ground state with a reduced-transition probability of B(E2; 5(-) -> 7(-)) = 0.53(6) W.u. Observation of this isomer, and lack of evidence in the current work for a I-pi = 5(-) isomer decay in In-132, provides a benchmark of the proton-neutron interaction in the region of the nuclear chart “southeast” of Sn-132, where experimental information on excited states is sparse.
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n_TOF Collaboration(Amaducci, S. et al), Domingo-Pardo, C., & Tain, J. L. (2019). Measurement of the U-235(n, f) cross section relative to the Li-6(n, t) and B-10(n,alpha) standards from thermal to 170 keV neutron energy range at n_TOF. Eur. Phys. J. A, 55(7), 120–19pp.
Abstract: .The U-235(n, f ) cross section was measured at n_TOF relative to Li-6(n, t) and B-10(n,alpha) , with high resolution ( L=183.49(2) m) and in a wide energy range (25meV-170keV) with 1.5% systematic uncertainty, making use of a stack of six samples and six silicon detectors placed in the neutron beam. This allowed us to make a direct comparison of the yields of the U-235(n, f ) and of the two reference reactions under the same experimental conditions, and taking into account the forward/backward emission asymmetry. A hint of an anomaly in the 10-30keV neutron energy range had been previously observed in other experiments, indicating a cross section systematically lower by several percent relative to major evaluations. The present results indicate that the cross section in the 9-18keV neutron energy range is indeed overestimated by almost 5% in the recently released evaluated data files ENDF/B-VIII.0 and JEFF3.3, as a consequence of a 7% overestimate in a single GMA node in the IAEA reference file. Furthermore, these new high-resolution data confirm the existence of resonance-like structures in the keV neutron energy region. The results here reported may lead to a reduction of the uncertainty in the 1-100keV neutron energy region. Finally, from the present data, a value of 249.7 +/- 1.4( stat )+/- 0.94( syst ) b<bold>eV has been extracted for the cross section integral between </bold>7.8 and 11eV, confirming the value of 247.5 +/- 3 b<bold>eV recently established as a standard</bold>.
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Guadilla, V., Algora, A., Tain, J. L., Agramunt, J., Jordan, D., Monserrate, M., et al. (2019). Total absorption gamma-ray spectroscopy of niobium isomers. Phys. Rev. C, 100(2), 024311–15pp.
Abstract: The beta-intensity distributions of the decays of Nb-100gs,Nb-100m and Nb-102gs,Nb-102m have been determined using the total absorption gamma-ray spectroscopy technique. The JYFLTRAP double Penning trap system was employed in a campaign of challenging measurements performed with the decay total absorption gamma-ray spectrometer at the Ion Guide Isotope Separator On-Line facility in Jyvaskyla. Different strategies were applied to disentangle the isomeric states involved, lying very close in energy. The low-spin component of each niobium case was populated through the decay of the zirconium parent, which was treated as a contaminant. We have applied a method to extract this contamination, and additionally we have obtained beta-intensity distributions for these zirconium decays. The beta-strength distributions evaluated with these results were compared with calculations in a quasiparticle random-phase approximation, suggesting a prolate configuration for the ground states of Zr-100,Zr-102. The footprint of the Pandemonium effect was found when comparing our results for the analyses of the niobium isotopes with previous decay data. The beta-intensities of the decay of Nb-102m, for which there were no previous data, were obtained. A careful evaluation of the uncertainties was carried out, and the consistency of our results was validated taking advantage of the segmentation of our spectrometer. The final results were used as input in reactor summation calculations. A large impact on antineutrino spectrum calculations was already reported, and here we detail the significant impact on decay heat calculations.
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