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Author n_TOF Collaboration (Tagliente, G. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A.
Title Zr-92(n, gamma) and (n,tot) measurements at the GELINA and n_TOF facilities Type Journal Article
Year 2022 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 105 Issue (up) 2 Pages 025805 - 14pp
Keywords
Abstract Background: Stellar nucleosynthesis of elements heavier than iron is driven by neutron capture processes. Zr-92 is positioned at a strategic point along the slow nucleosynthesis path, given its proximity to the neutron magic number N = 50 and its position at the matching region between the weak and main slow processes. Purpose: In parallel with recent improved astronomical data, the extraction of accurate Maxwellian averaged cross sections (MACSs) derived from a more complete and accurate set of resonance parameters should allow for a better understanding of the stellar conditions at which nucleosynthesis takes place. Methods: Transmission and capture cross section measurements using enriched Zr-92 metallic samples were performed at the time-of flight facilities GELINA of JRC-Geel (BE) and nTOF of CERN (CH). The neutron beam passing through the samples was investigated in transmission measurements at GELINA using a Li-glass scintillator. The gamma rays emitted during the neutron capture reactions were detected by C6D6 detectors at both GELINA and nTOF. Results: Resonance parameters of individual resonances up to 81 keV were extracted from a combined resonance shape analysis of experimental transmissions and capture yields. For the majority of the resonances the parity was determined from an analysis of the transmission data obtained with different sample thicknesses. Average resonance parameters were calculated. Conclusions: Maxwellian averaged cross sections were extracted from resonances observed up to 81 keV. The MACS for kT = 30 keV is fully consistent with experimental data reported in the literature. The MACSs for kT less than or similar to 15 keV are in good agreement with those derived from the ENDF/B-VIII.0 library and recommended in the KADoNTS database. For kT higher than 30 keV differences are observed. A comparison with MACSs obtained with the cross sections recommended in the JEFF-3.3 and JENDL-4.0 libraries shows discrepancies even for kT less than or similar to 15 keV.
Address [Tagliente, G.; Barbagallo, M.; Colonna, N.; Mastromarco, M.; Variale, V.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: giuseppe.tagliente@ba.infn.it
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:000766732800002 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 5163
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Author n_TOF Collaboration (Moreno-Soto, J. et al); Babiano-Suarez, V.; Caballero-Ontanaya, L.; Domingo-Pardo, C.; Ladarescu, I.; Tain, J.L.
Title Constraints on the dipole photon strength for the odd uranium isotopes Type Journal Article
Year 2022 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 105 Issue (up) 2 Pages 024618 - 14pp
Keywords
Abstract Background: The photon strength functions (PSFs) and nuclear level density (NLD) are key ingredients for calculation of the photon interaction with nuclei, in particular the reaction cross sections. These cross sections are important especially in nuclear astrophysics and in the development of advanced nuclear technologies. Purpose: The role of the scissors mode in the M1 PSF of (well-deformed) actinides was investigated by several experimental techniques. The analyses of different experiments result in significant differences, especially on the strength of the mode. The shape of the low-energy tail of the giant electric dipole resonance is uncertain as well. In particular, some works proposed a presence of the E1 pygmy resonance just above 7 MeV. Because of these inconsistencies additional information on PSFs in this region is of great interest. Methods: The gamma-ray spectra from neutron-capture reactions on the U-234, U-236, and U-238 nuclei have been measured with the total absorption calorimeter of the n_TOF facility at CERN. The background-corrected sum-energy and multi-step-cascade spectra were extracted for several isolated s-wave resonances up to about 140 eV. Results: The experimental spectra were compared to statistical model predictions coming from a large selection of models of photon strength functions and nuclear level density. No combination of PSF and NLD models from literature is able to globally describe our spectra. After extensive search we were able to find model combinations with modified generalized Lorentzian (MGLO) E1 PSF, which match the experimental spectra as well as the total radiative widths. Conclusions: The constant temperature energy dependence is favored for a NLD. The tail of giant electric dipole resonance is well described by the MGLO model of the E1 PSF with no hint of pygmy resonance. The M1 PSF must contain a very strong, relatively wide, and likely double-resonance scissors mode. The mode is responsible for about a half of the total radiative width of neutron resonances and significantly affects the radiative cross section.
Address [Moreno-Soto, J.; Berthoumieux, E.; Dupont, E.; Gunsing, F.; Bacak, M.] Univ Paris Saclay, CEA Irfu, F-91191 Gif Sur Yvette, France, Email: jmoreno53@us.es;
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:000810791100001 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 5278
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Author Kiss, G.G. et al; Tarifeño-Saldivia, A.; Tain, J.L.; Agramunt, J.; Algora, A.; Domingo-Pardo, C.; Morales, A.I.; Nacher, E.; Rubio, B.; Tolosa, A.
Title Measuring the beta-decay Properties of Neutron-rich Exotic Pm, Sm, Eu, and Gd Isotopes to Constrain the Nucleosynthesis Yields in the Rare-earth Region Type Journal Article
Year 2022 Publication Astrophysical Journal Abbreviated Journal Astrophys. J.
Volume 936 Issue (up) 2 Pages 107 - 18pp
Keywords
Abstract The beta-delayed neutron-emission probabilities of 28 exotic neutron-rich isotopes of Pm, Sm, Eu, and Gd were measured for the first time at RIKEN Nishina Center using the Advanced Implantation Detector Array (AIDA) and the BRIKEN neutron detector array. The existing beta-decay half-life (T (1/2)) database was significantly increased toward more neutron-rich isotopes, and uncertainties for previously measured values were decreased. The new data not only constrain the theoretical predictions of half-lives and beta-delayed neutron-emission probabilities, but also allow for probing the mechanisms of formation of the high-mass wing of the rare-earth peak located at A approximate to 160 in the r-process abundance distribution through astrophysical reaction network calculations. An uncertainty quantification of the calculated abundance patterns with the new data shows a reduction of the uncertainty in the rare-earth peak region. The newly introduced variance-based sensitivity analysis method offers valuable insight into the influence of important nuclear physics inputs on the calculated abundance patterns. The analysis has identified the half-lives of Sm-168 and of several gadolinium isotopes as some of the key variables among the current experimental data to understand the remaining abundance uncertainty at A = 167-172.
Address [Kiss, G. G.; Vitez-Sveiczer, A.; Algora, A.; Szegedi, T. N.] Inst Nucl Res ATOMKI, Bem Ter 18-c, H-4026 Debrecen, Hungary, Email: ggkiss@atomki.hu;
Corporate Author Thesis
Publisher IOP Publishing Ltd Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0004-637x ISBN Medium
Area Expedition Conference
Notes WOS:000850804600001 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 5353
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Author Algora, A. et al; Jordan, D.; Tain, J.L.; Rubio, B.; Agramunt, J.; Perez-Cerdan, A.B.; Molina, F.; Caballero, L.; Nacher, E.
Title Reactor Decay Heat in Pu-239: Solving the gamma Discrepancy in the 4-3000-s Cooling Period Type Journal Article
Year 2010 Publication Physical Review Letters Abbreviated Journal Phys. Rev. Lett.
Volume 105 Issue (up) 20 Pages 202501 - 4pp
Keywords
Abstract The beta feeding probability of Tc-102,Tc- 104,Tc- 105,Tc- 106,Tc- 107, Mo-105, and Nb-101 nuclei, which are important contributors to the decay heat in nuclear reactors, has been measured using the total absorption technique. We have coupled for the first time a total absorption spectrometer to a Penning trap in order to obtain sources of very high isobaric purity. Our results solve a significant part of a long-standing discrepancy in the gamma component of the decay heat for Pu-239 in the 4-3000 s range.
Address [Algora, A.; Jordan, D.; Tain, J. L.; Rubio, B.; Agramunt, J.; Perez-Cerdan, A. B.; Molina, F.; Caballero, L.; Nacher, E.] Univ Valencia, IFIC, CSIC, Valencia, Spain, Email: algora@ific.uv.es
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0031-9007 ISBN Medium
Area Expedition Conference
Notes ISI:000283927700004 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ elepoucu @ Serial 328
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Author Fallot, M.; Cormon, S.; Estienne, M.; Algora, A.; Bui, V.M.; Cucoanes, A.; Elnimr, M.; Giot, L.; Jordan, D.; Martino, J.; Onillon, A.; Porta, A.; Pronost, G.; Remoto, A.; Tain, J.L.; Yermia, F.; Zakari-Issoufou, A.A.
Title New Antineutrino Energy Spectra Predictions from the Summation of Beta Decay Branches of the Fission Products Type Journal Article
Year 2012 Publication Physical Review Letters Abbreviated Journal Phys. Rev. Lett.
Volume 109 Issue (up) 20 Pages 202504 - 5pp
Keywords
Abstract In this Letter, we study the impact of the inclusion of the recently measured beta decay properties of the Tc-102;104;105;106;107, Mo-105, and Nb-101 nuclei in an updated calculation of the antineutrino energy spectra of the four fissible isotopes U-235,U-238 and Pu-239,Pu-241. These actinides are the main contributors to the fission processes in pressurized water reactors. The beta feeding probabilities of the above-mentioned Tc, Mo, and Nb isotopes have been found to play a major role in the gamma component of the decay heat of Pu-239, solving a large part of the gamma discrepancy in the 4-3000 s range. They have been measured by using the total absorption technique, insensitive to the pandemonium effect. The calculations are performed by using the information available nowadays in the nuclear databases, summing all the contributions of the beta decay branches of the fission products. Our results provide a new prediction of the antineutrino energy spectra of U-235, Pu-239,Pu-241, and, in particular, U-238 for which no measurement has been published yet. We conclude that new total absorption technique measurements are mandatory to improve the reliability of the predicted spectra.
Address [Fallot, M.; Cormon, S.; Estienne, M.; Bui, V. M.; Cucoanes, A.; Elnimr, M.; Giot, L.; Martino, J.; Onillon, A.; Porta, A.; Pronost, G.; Remoto, A.; Yermia, F.; Zakari-Issoufou, A. -A.] Univ Nantes, Ecole Mines Nantes, CNRS, IN2P3,SUBATECH, F-44307 Nantes, France
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0031-9007 ISBN Medium
Area Expedition Conference
Notes WOS:000310991700009 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 1250
Permanent link to this record