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Rice, S. et al, Algora, A., Tain, J. L., Valencia, E., Agramunt, J., Rubio, B., et al. (2017). Total absorption spectroscopy study of the beta decay of Br-86 and Rb-91. Phys. Rev. C, 96(1), 014320–10pp.
Abstract: The beta decays of Br-86 and Rb-91 have been studied using the total absorption spectroscopy technique. The radioactive nuclei were produced at the Ion Guide Isotope Separator On-Line facility in Jyvaskyla and further purified using the JYFLTRAP. Br-86 and Rb-91 are considered to be major contributors to the decay heat in reactors. In addition, Rb-91 was used as a normalization point in direct measurements of mean gamma energies released in the beta decay of fission products by Rudstam et al. assuming that this decaywas well known from high-resolution measurements. Our results show that both decays were suffering from the Pandemonium effect and that the results of Rudstam et al. should be renormalized. The relative impact of the studied decays in the prediction of the decay heat and antineutrino spectrum from reactors has been evaluated.
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IGISOL Collaboration(Zakari-Issoufou, A. A. et al), Algora, A., Tain, J. L., Valencia, E., Agramunt, J., Estevez, E., et al. (2015). Total Absorption Spectroscopy Study of Rb-92 Decay: A Major Contributor to Reactor Antineutrino Spectrum Shape. Phys. Rev. Lett., 115(10), 102503–6pp.
Abstract: The antineutrino spectra measured in recent experiments at reactors are inconsistent with calculations based on the conversion of integral beta spectra recorded at the ILL reactor. Rb-92 makes the dominant contribution to the reactor antineutrino spectrum in the 5-8 MeV range but its decay properties are in question. We have studied Rb-92 decay with total absorption spectroscopy. Previously unobserved beta feeding was seen in the 4.5-5.5 region and the GS to GS feeding was found to be 87.5(25)%. The impact on the reactor antineutrino spectra calculated with the summation method is shown and discussed.
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Valencia, E. et al, Tain, J. L., Algora, A., Agramunt, J., Estevez, E., Jordan, M. D., et al. (2017). Total absorption gamma-ray spectroscopy of the beta-delayed neutron emitters Br-87, Br-88, and Rb-94. Phys. Rev. C, 95(2), 024320–18pp.
Abstract: We investigate the decay of Br-87,Br-88 and Rb-94 using total absorption gamma-ray spectroscopy. These important fission products are beta-delayed neutron emitters. Our data show considerable beta gamma intensity, so far unobserved in high-resolution gamma-ray spectroscopy, from states at high excitation energy. We also find significant differences with the beta intensity that can be deduced from existing measurements of the beta spectrum. We evaluate the impact of the present data on reactor decay heat using summation calculations. Although the effect is relatively small it helps to reduce the discrepancy between calculations and integral measurements of the photon component for U-235 fission at cooling times in the range 1-100 s. We also use summation calculations to evaluate the impact of present data on reactor antineutrino spectra. We find a significant effect at antineutrino energies in the range of 5 to 9 MeV. In addition, we observe an unexpected strong probability for. emission from neutron unbound states populated in the daughter nucleus. The. branching is compared to Hauser-Feshbach calculations, which allow one to explain the large value for bromine isotopes as due to nuclear structure. However the branching for Rb-94, although much smaller, hints of the need to increase the radiative width gamma by one order of magnitude. This increase in gamma would lead to a similar increase in the calculated (n, gamma) cross section for this very neutron-rich nucleus with a potential impact on r process abundance calculations.
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IGISOL Collaboration(Briz, J. A. et al), Algora, A., Tain, J. L., Guadilla, V., Agramunt, J., Estevez, E., et al. (2016). Total absorption spectroscopy of fission fragments relevant for reactor antineutrino spectra determination. Acta Phys. Pol. B, 47(3), 755–762.
Abstract: The contribution of each fission fragment to the reactor antineutrino spectra was determined using the summation method based on the existing information on fission yields and decay data contained in nuclear databases and the reactor evolution code MURE. The beta decay of some of the main contributors has been studied using the Total Absorption Spectroscopy (TAS) technique during two experimental campaigns at the IGISOL facility, in Jyvaskyla (Finland). Results on the decay of Rb-92, the most important contributor in the 4-8 MeV energy region are reported. The status of the analysis of the second experiment is presented as well.
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Tain, J. L. et al, Valencia, E., Algora, A., Agramunt, J., Rubio, B., Estevez, E., et al. (2015). Enhanced gamma-Ray Emission from Neutron Unbound States Populated in beta Decay. Phys. Rev. Lett., 115(6), 062502–5pp.
Abstract: Total absorption spectroscopy is used to investigate the beta-decay intensity to states above the neutron separation energy followed by gamma-ray emission in Br-87,Br-88 and Rb-94. Accurate results are obtained thanks to a careful control of systematic errors. An unexpectedly large. intensity is observed in all three cases extending well beyond the excitation energy region where neutron penetration is hindered by low neutron energy. The gamma branching as a function of excitation energy is compared to Hauser-Feshbach model calculations. For Br-87 and Br-88 the gamma branching reaches 57% and 20%, respectively, and could be explained as a nuclear structure effect. Some of the states populated in the daughter can only decay through the emission of a large orbital angular momentum neutron with a strongly reduced barrier penetrability. In the case of neutron-rich Rb-94 the observed 4.5% branching is much larger than the calculations performed with standard nuclear statistical model parameters, even after proper correction for fluctuation effects on individual transition widths. The difference can be reconciled by introducing an enhancement of 1 order of magnitude in the photon strength to neutron strength ratio. An increase in the photon strength function of such magnitude for very neutron-rich nuclei, if it proves to be correct, leads to a similar increase in the (n, gamma) cross section that would have an impact on r process abundance calculations.
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