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n_TOF Collaboration (Stamatopoulos, A. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Investigation of the Pu-240(n, f) reaction at the n_TOF/EAR2 facility in the 9 meV-6 MeV range |
Type |
Journal Article |
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Year |
2020 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
102 |
Issue  |
1 |
Pages |
014616 - 23pp |
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Keywords |
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Abstract |
Background: Nuclear waste management is considered amongst the major challenges in the field of nuclear energy. A possible means of addressing this issue is waste transmutation in advanced nuclear systems, whose operation requires a fast neutron spectrum. In this regard, the accurate knowledge of neutron-induced reaction cross sections of several (minor) actinide isotopes is essential for design optimization and improvement of safety margins of such systems. One such case is Pu-240, due to its accumulation in spent nuclear fuel of thermal reactors and its usage in fast reactor fuel. The measurement of the Pu-240(n, f) cross section was previously attempted at the CERN nTOF facility EAR1 measuring station using the time-of-flight technique. Due to the low amount of available material and the given flux at EAR1, the measurement had to last several months to achieve a sufficient statistical accuracy. This long duration led to detector deterioration due to the prolonged exposure to the high alpha activity of the fission foils, therefore the measurement could not be successfully completed. Purpose: It is aimed to determine whether it is feasible to study neutron-induced fission at nTOF/EAR2 and provide data on the Pu-240(n, f) reaction in energy regions requested for applications. Methods: The study of the Pu-240(n, f) reaction was made at a new experimental area (EAR2) with a shorter flight path which delivered on average 30 times higher flux at fast neutron energies. This enabled the measurement to be performed much faster, thus limiting the exposure of the detectors to the intrinsic activity of the fission foils. The experimental setup was based on microbulk Micromegas detectors and the time-of-flight data were analyzed with an optimized pulse-shape analysis algorithm. Special attention was dedicated to the estimation of the non-negligible counting loss corrections with the development of a new methodology, and other corrections were estimated via Monte Carlo simulations of the experimental setup. Results: This new measurement of the Pu-240(n, f) cross section yielded data from 9 meV up to 6 MeV incident neutron energy and fission resonance kernels were extracted up to 10 keV. Conclusions: Neutron-induced fission of high activity samples can be successfully studied at the n_TOF/EAR2 facility at CERN covering a wide range of neutron energies, from thermal to a few MeV. |
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Address |
[Stamatopoulos, A.; Tsinganis, A.; Kokkoris, M.; Vlastou, R.; Diakaki, M.] Natl Tech Univ Athens, Athens, Greece, Email: athanasios.stamatopoulos@cern.ch |
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Amer Physical Soc |
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English |
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0556-2813 |
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Notes |
WOS:000551057500002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4466 |
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Author |
Siciliano, M. et al; Gadea, A. |
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Title |
Shape coexistence in neutron-deficient Hg-188 investigated via lifetime measurements |
Type |
Journal Article |
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Year |
2020 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
102 |
Issue |
1 |
Pages |
014318 - 16pp |
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Keywords |
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Abstract |
Background: Shape coexistence in the Z approximate to 82 region has been established in mercury, lead, and polonium isotopes. For even-even mercury isotopes with 100 <= N <= 106 multiple fingerprints of this phenomenon are observed, which seems to be no longer present for N >= 110. According to a number of theoretical calculations, shape coexistence is predicted in the Hg-188 isotope. Purpose: The aim of this work was to measure lifetimes of excited states in Hg-188 to infer their collective properties, such as the deformation. Extending the investigation to higher-spin states, which are expected to be less affected by band-mixing effects, can provide additional information on the coexisting structures. Methods: The Hg-188 nucleus was populated using two different fusion-evaporation reactions with two targets, Gd-158 and Gd-160, and a beam of S-34 provided by the Tandem-ALPI accelerator complex at the Laboratori Nazionali di Legnaro. The channels of interest were selected using the information from the Neutron Wall array, while the gamma rays were detected using the GALILEO gamma-ray spectrometer. Lifetimes of excited states were determined using the recoil-distance Doppler-shift method, employing the dedicated GALILEO plunger device. Results: Lifetimes of the states up to spin 16 (h) over bar were measured and the corresponding reduced transition probabilities were calculated. Assuming two-band mixing and adopting, as done commonly, the rotational model, the mixing strengths and the deformation parameters of the unperturbed structures were obtained from the experimental results. In order to shed light on the nature of the observed configurations in the Hg-188 nucleus, the extracted transition strengths were compared with those resulting from state-of-the-art beyond-mean-field calculations using the symmetry-conserving configuration-mixing approach, limited to axial shapes, and the five-dimensional collective Hamiltonian, including the triaxial degree of freedom. Conclusions: The first lifetime measurement for states with spin >= 6 suggested the presence of an almost spherical structure above the 12(1)(+) isomer and allowed elucidating the structure of the intruder band. The comparison of the extracted B(E2) strengths with the two-band mixing model allowed the determination of the ground-state band deformation. Both beyond-mean-field calculations predict coexistence of a weakly deformed band with a strongly prolate-deformed one, characterized by elongation parameters similar to those obtained experimentally, but the calculated relative position of the bands and their mixing strongly differ. |
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[Siciliano, M.; Zanon, I; Cicerchia, M.; de Angelis, G.; Galtarossa, F.; Gozzelino, A.; Hadynska-Klek, K.; Jaworski, G.; Napoli, D. R.; Valiente-Dobon, J. J.] INFN, Lab Nazl Legnaro, I-35020 Legnaro, Italy, Email: marco.siciliano@lnl.infn.it |
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Amer Physical Soc |
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English |
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ISSN |
0556-2813 |
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Notes |
WOS:000551404600001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4471 |
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Author |
IDS Collaboration (Benito, J. et al); Nacher, E. |
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Title |
Detailed spectroscopy of doubly magic Sn-132 |
Type |
Journal Article |
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Year |
2020 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
102 |
Issue |
1 |
Pages |
014328 - 18pp |
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Abstract |
The structure of the doubly magic Sn-132(50)82 has been investigated at the ISOLDE facility at CERN, populated both by the beta(-) decay of In-132 and beta(-)-delayed neutron emission of In-133. The level scheme of Sn-13(2) is greatly expanded with the addition of 68 gamma transitions and 17 levels observed for the first time in the beta decay. The information on the excited structure is completed by new gamma transitions and states populated in the beta-n decay of In-133. Improved delayed neutron emission probabilities are obtained both for In-132 and In-133. Level lifetimes are measured via the advanced time-delayed beta gamma gamma(t) fast-timing method. An interpretation of the level structure is given based on the experimental findings and the particle-hole configurations arising from core excitations both from the N = 82 and Z = 50 shells, leading to positive- and negative-parity particle-hole multiplets. The experimental information provides new data to challenge the theoretical description of Sn-132. |
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[Benito, J.; Fraile, L. M.; Carmona, M.; Galve, P.; Garcia-Diez, M.; Ibanez, P.; Lopez-Montes, A.; Martinez, M. C.; Sanchez-Parcerisa, D.; Sanchez-Tembleque, V; Udias, J. M.; Vedia, V.; Villa-Abaunza, A.] Univ Complutense Madrid, Grp Fis Nucl, CEI Moncloa, E-28040 Madrid, Spain, Email: jabenito@ucm.es; |
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Amer Physical Soc |
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English |
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0556-2813 |
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Notes |
WOS:000556554700006 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4488 |
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Author |
Biswas, S. et al; Perez-Vidal, R.M. |
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Title |
Prompt-delayed gamma-ray spectroscopy of neutron-rich In-119, In-121 isotopes |
Type |
Journal Article |
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Year |
2020 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
102 |
Issue |
1 |
Pages |
014326 - 10pp |
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Abstract |
Background: The Z = 50 shell closure, near N = 82, is unique in the sense that it is the only shell closure with the spin-orbit partner orbitals, pi g(9/2) and pi g(7/2), enclosing the magic gap. The interaction of the proton hole/particle in the above-mentioned orbitals with neutrons in the nu h(11)(/2) orbital is an important prerequisite to the understanding of the nuclear structure near N = 82 and the nu pi interaction. Purpose: To explore the structural similarity between the high-spin isomeric states in In (Z = 49), Sn (Z = 50), and Sb (Z = 51) isotopes from a microscopic point of view. In addition, to understand the role of a proton hole or particle in the spin-orbit partner orbitals, pi g(9/2) and pi g(7/2), respectively, with neutron holes in the nu h(11)(/2) orbital on these aforementioned isomers. Methods: The fusion and transfer induced fission reaction Be-9(U-238, f) with 6.2 MeV/u beam energy, using a unique setup consisting of AGATA, VAMOS ++, and EXOGAM detectors, was used to populate through the fission process and study the neutron-rich In-119,In-121 isotopes. This setup enabled the prompt-delayed gamma-ray spectroscopy of isotopes in the time range of 100 ns-200 μs. Results: In the odd-A In-119,In-121 isotopes, indications of a short half-life 19/2(-) isomeric state, in addition to the previously known 25/2(+) isomeric state, were observed from the present data. Further, new prompt transitions above the 25/2(+) isomer in In-121 were identified along with reevaluation of its half-life. Conclusions: The experimental data were compared with the theoretical results obtained in the framework of large-scale shell-model calculations in a restricted model space. The <pi g(9/2)nu h(11/2); I vertical bar H vertical bar pi g(9/2) nu h(11/2);I > two-body matrix elements of residual interaction were modified to explain the excitation energies and the B(E2) transition probabilities in the neutron-rich In isotopes. The (i) decreasing trend of E(29/2(+))-E(25/2(+)) in odd-In (with dominant configuration pi g(9/)(2)(-1) nu h(11/2)(-2) and maximum aligned spin of 29/2+) and (ii) increasing trend of E(27/2(+)) – E(23/2(+)) in odd-Sb (with dominant configuration pi g(7/)(2)(+1) nu h(11/2)(-2) and maximum aligned spin of 27/2(+)) with increasing neutron number could be understood as a consequence of hole-hole and particle-hole interactions, respectively. |
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[Biswas, S.; Lemasson, A.; Rejmund, M.; Navin, A.; Kim, Y. H.; Michelagnoli, C.; Clement, E.; de France, G.; Fremont, G.; Goupil, J.; Jacquot, B.; Li, H. J.; Menager, L.; Morel, V; Ropert, J.] GANIL, CEA, DRF, CNRS,IN2P3, Bd Henri Becquerel,BP 55027, F-14076 Caen 05, France, Email: lemasson@ganil.fr |
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Amer Physical Soc |
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English |
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ISSN |
0556-2813 |
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Notes |
WOS:000556554700003 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4489 |
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Author |
Orrigo, S.E A. et al; Rubio, B.; Gelletly, W.; Aguilera, P.; Algora, A.; Morales, A.I.; Agramunt, J.; Guadilla, V.; Montaner-Piza, A. |
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Title |
beta decay of the very neutron-deficient Ge-60 and Ge-62 nuclei |
Type |
Journal Article |
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Year |
2021 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
103 |
Issue |
1 |
Pages |
014324 - 12pp |
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Keywords |
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Abstract |
We report here the results of a study of the beta decay of the proton-rich Ge isotopes, Ge-60 and Ge-62, produced in an experiment at the RIKEN Nishina Center. We have improved our knowledge of the half-lives of Ge-62 [73.5(1) ms] and Ge-60 [25.0(3) ms] and its daughter nucleus, Ga-60 [69.4(2) ms]. We measured individual beta-delayed proton and gamma emissions and their related branching ratios. Decay schemes and absolute Fermi and Gamow-Teller transition strengths have been determined. The mass excesses of the nuclei under study have been deduced. A total beta-delayed proton-emission branching ratio of 67(3)% has been obtained for Ge-60. New information has been obtained on the energy levels populated in Ga-60 and on the 1/2(-) excited state in the beta p daughter Zn-59. We extracted a ground state-to-ground state feeding of 85.3(3)% for the decay of Ge-62. Eight new y lines have been added to the deexcitation of levels populated in the Ga-62 daughter. |
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Address |
[Orrigo, S. E. A.; Rubio, B.; Gelletly, W.; Aguilera, P.; Algora, A.; Morales, A., I; Agramunt, J.; Guadilla, V; Montaner-Piza, A.] Univ Valencia, Inst Fis Corpuscular, CSIC, E-46071 Valencia, Spain, Email: sonja.orrigo@ific.uv.es |
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Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
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Notes |
WOS:000613141500002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4716 |
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