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Deo, A. Y., Podolyak, Z., Walker, P. M., Algora, A., Rubio, B., Agramunt, J., et al. (2010). Structures of Po-201 and Rn-205 from EC/beta(+)-decay studies. Phys. Rev. C, 81(2), 024322–8pp.
Abstract: Several low-lying excited states in Rn-205(86)119 and Po-201(84)117 were identified for the first time following EC/beta(+) decay of Fr-205 and At-201, respectively, using gamma-ray and conversion electron spectroscopy at the CERN isotope separator on-line (ISOLDE) facility. The EC/beta(+) branch from Fr-205 was measured to be 1.5(2)%. The excited states of the daughter nuclei are understood in terms of the odd nucleon coupling to the neighboring even-even core. The neutron single-particle energies of the p(3/2) orbital relative to the f(5/2) ground state in Rn-205, and the f(5/2) orbital relative to the p(3/2) ground state in Po-201, were determined to be 31.4(2) and 5.7(3) keV, respectively. We tentatively identify a 13/2(+) isomeric level at 657.1(5) keV in Rn-205. The systematic behavior of the 13/2(+) and 3/2(-) levels is also discussed.
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Algora, A. et al, Jordan, D., Tain, J. L., Rubio, B., Agramunt, J., Perez-Cerdan, A. B., et al. (2011). Improvements on Decay Heat Summation Calculations by Means of Total Absorption Gamma-ray Spectroscopy Measurements. J. Korean Phys. Soc., 59(2), 1479–1482.
Abstract: The decay heat of fission products plays an important role in predictions of the heat released by nuclear fuel in reactors. In this contribution we present results of the analysis of the measurement of the beta decay of some refractory isotopes that were considered possible important contributors to the decay heat in reactors. The measurements presented here were performed at the IGISOL facility of the University of Jyvaskyla, Finland. In our measurements we have combined for the first time a Penning trap (JYFLTRAP), which was used as a high resolution isobaric separator, with a total absorption spectrometer. The results of the measurements as well as their consequences for decay heat summation calculations are discussed.
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Hornillos, M. B. G., Gorlychev, V., Caballero, R., Cortes, G., Poch, A., Pretel, C., et al. (2011). Monte Carlo Simulations for the Study of a Moderated Neutron Detector. J. Korean Phys. Soc., 59(2), 1573–1576.
Abstract: This work presents the Monte Carlo simulations performed with the MCNPX and GEANT4 codes for the design of a BEta deLayEd Neutron detector, BELEN-20. This detector will be used for the study of beta delayed neutron emission and consists of a block of polyethylene with dimensions 90 x 90 x 80 cm(3) and 20 cylindrical (3)He gas counters. The results of these simulations have been validated experimentally with a (252)Cf source in the laboratory at UPC, Barcelona. Also the first experiment with this detector has been carried out in November 2009 in JYFL, Finland. In this experiment the neutron emission probability after beta decay of the fission products (88)Br, (94,95)Rb, and (138)I has been measured; this data is still under analysis. Simulations with MCNPX and GEANT4 have been performed in order to obtain the efficiency of the BELEN-20 detector for each of the above nuclei using the neutron energy distribution corresponding to each nucleus.
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Valencia, E. et al, Tain, J. L., Algora, A., Agramunt, J., Estevez, E., Jordan, M. D., et al. (2017). Total absorption gamma-ray spectroscopy of the beta-delayed neutron emitters Br-87, Br-88, and Rb-94. Phys. Rev. C, 95(2), 024320–18pp.
Abstract: We investigate the decay of Br-87,Br-88 and Rb-94 using total absorption gamma-ray spectroscopy. These important fission products are beta-delayed neutron emitters. Our data show considerable beta gamma intensity, so far unobserved in high-resolution gamma-ray spectroscopy, from states at high excitation energy. We also find significant differences with the beta intensity that can be deduced from existing measurements of the beta spectrum. We evaluate the impact of the present data on reactor decay heat using summation calculations. Although the effect is relatively small it helps to reduce the discrepancy between calculations and integral measurements of the photon component for U-235 fission at cooling times in the range 1-100 s. We also use summation calculations to evaluate the impact of present data on reactor antineutrino spectra. We find a significant effect at antineutrino energies in the range of 5 to 9 MeV. In addition, we observe an unexpected strong probability for. emission from neutron unbound states populated in the daughter nucleus. The. branching is compared to Hauser-Feshbach calculations, which allow one to explain the large value for bromine isotopes as due to nuclear structure. However the branching for Rb-94, although much smaller, hints of the need to increase the radiative width gamma by one order of magnitude. This increase in gamma would lead to a similar increase in the calculated (n, gamma) cross section for this very neutron-rich nucleus with a potential impact on r process abundance calculations.
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Guadilla, V., Algora, A., Tain, J. L., Agramunt, J., Jordan, D., Monserrate, M., et al. (2019). Total absorption gamma-ray spectroscopy of niobium isomers. Phys. Rev. C, 100(2), 024311–15pp.
Abstract: The beta-intensity distributions of the decays of Nb-100gs,Nb-100m and Nb-102gs,Nb-102m have been determined using the total absorption gamma-ray spectroscopy technique. The JYFLTRAP double Penning trap system was employed in a campaign of challenging measurements performed with the decay total absorption gamma-ray spectrometer at the Ion Guide Isotope Separator On-Line facility in Jyvaskyla. Different strategies were applied to disentangle the isomeric states involved, lying very close in energy. The low-spin component of each niobium case was populated through the decay of the zirconium parent, which was treated as a contaminant. We have applied a method to extract this contamination, and additionally we have obtained beta-intensity distributions for these zirconium decays. The beta-strength distributions evaluated with these results were compared with calculations in a quasiparticle random-phase approximation, suggesting a prolate configuration for the ground states of Zr-100,Zr-102. The footprint of the Pandemonium effect was found when comparing our results for the analyses of the niobium isotopes with previous decay data. The beta-intensities of the decay of Nb-102m, for which there were no previous data, were obtained. A careful evaluation of the uncertainties was carried out, and the consistency of our results was validated taking advantage of the segmentation of our spectrometer. The final results were used as input in reactor summation calculations. A large impact on antineutrino spectrum calculations was already reported, and here we detail the significant impact on decay heat calculations.
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Kiss, G. G. et al, Tarifeño-Saldivia, A., Tain, J. L., Agramunt, J., Algora, A., Domingo-Pardo, C., et al. (2022). Measuring the beta-decay Properties of Neutron-rich Exotic Pm, Sm, Eu, and Gd Isotopes to Constrain the Nucleosynthesis Yields in the Rare-earth Region. Astrophys. J., 936(2), 107–18pp.
Abstract: The beta-delayed neutron-emission probabilities of 28 exotic neutron-rich isotopes of Pm, Sm, Eu, and Gd were measured for the first time at RIKEN Nishina Center using the Advanced Implantation Detector Array (AIDA) and the BRIKEN neutron detector array. The existing beta-decay half-life (T (1/2)) database was significantly increased toward more neutron-rich isotopes, and uncertainties for previously measured values were decreased. The new data not only constrain the theoretical predictions of half-lives and beta-delayed neutron-emission probabilities, but also allow for probing the mechanisms of formation of the high-mass wing of the rare-earth peak located at A approximate to 160 in the r-process abundance distribution through astrophysical reaction network calculations. An uncertainty quantification of the calculated abundance patterns with the new data shows a reduction of the uncertainty in the rare-earth peak region. The newly introduced variance-based sensitivity analysis method offers valuable insight into the influence of important nuclear physics inputs on the calculated abundance patterns. The analysis has identified the half-lives of Sm-168 and of several gadolinium isotopes as some of the key variables among the current experimental data to understand the remaining abundance uncertainty at A = 167-172.
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Algora, A. et al, Jordan, D., Tain, J. L., Rubio, B., Agramunt, J., Perez-Cerdan, A. B., et al. (2010). Reactor Decay Heat in Pu-239: Solving the gamma Discrepancy in the 4-3000-s Cooling Period. Phys. Rev. Lett., 105(20), 202501–4pp.
Abstract: The beta feeding probability of Tc-102,Tc- 104,Tc- 105,Tc- 106,Tc- 107, Mo-105, and Nb-101 nuclei, which are important contributors to the decay heat in nuclear reactors, has been measured using the total absorption technique. We have coupled for the first time a total absorption spectrometer to a Penning trap in order to obtain sources of very high isobaric purity. Our results solve a significant part of a long-standing discrepancy in the gamma component of the decay heat for Pu-239 in the 4-3000 s range.
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Orrigo, S. E. A. et al, Rubio, B., Agramunt, J., Algora, A., & Molina, F. (2014). Observation of the beta-Delayed gamma-Proton Decay of Zn-56 and its Impact on the Gamow-Teller Strength Evaluation. Phys. Rev. Lett., 112(22), 222501–5pp.
Abstract: We report the observation of a very exotic decay mode at the proton drip line, the beta-delayed gamma-proton decay, clearly seen in the beta decay of the T-z = -2 nucleus Zn-56. Three gamma-proton sequences have been observed after the beta decay. Here this decay mode, already observed in the sd shell, is seen for the first time in the f p shell. Both. and proton decays have been taken into account in the estimation of the Fermi and Gamow-Teller strengths. Evidence for fragmentation of the Fermi strength due to strong isospin mixing is found.
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Estevez, E. et al, Algora, A., Rubio, B., Bernabeu, J., Nacher, E., Tain, J. L., et al. (2011). beta-decay study of (150)Er, (152)Yb, and (156)Yb: Candidates for a monoenergetic neutrino beam facility. Phys. Rev. C, 84(3), 034304–6pp.
Abstract: The beta decays of (150)Er, (152)Yb, and (156)Yb nuclei are investigated using the total absorption spectroscopy technique. These nuclei can be considered possible candidates for forming the beam of a monoenergetic neutrino beam facility based on the electron capture (EC) decay of radioactive nuclei. Our measurements confirm that for the cases studied the EC decay proceeds mainly to a single state in the daughter nucleus.
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Orrigo, S. E. A. et al, Rubio, B., Agramunt, J., Algora, A., & Molina, F. (2015). β-delayed γ-proton decay in 56Zn: analysis of the charged-particle spectrum. Acta Phys. Pol. B, 46(3), 709–712.
Abstract: A study of the beta decay of the proton-rich T-z = 2 nucleus Zn-56 has been reported in a recent publication. A rare and exotic decay mode, beta-delayed gamma-proton decay, has been observed there for the first time in the fp shell. Here, we expand on some of the details of the data analysis, focussing on the charged particle spectrum.
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