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Rasco, B. C., Brewer, N. T., Yokoyama, R., Grzywacz, R., Rykaczewski, K. P., Tolosa-Delgado, A., et al. (2018). The ORNL analysis technique for extracting beta-delayed multi-neutron branching ratios with BRIKEN. Nucl. Instrum. Methods Phys. Res. A, 911, 79–86.
Abstract: Many choices are available in order to evaluate large radioactive decay networks. There are many parameters that influence the calculated beta-decay delayed single and multi-neutron emission branching fractions. We describe assumptions about the decay model, background, and other parameters and their influence on beta-decay delayed multi-neutron emission analysis. An analysis technique, the ORNL BRIKEN analysis procedure, for determining beta-delayed multi-neutron branching ratios in beta-neutron precursors produced by means of heavy-ion fragmentation is presented. The technique is based on estimating the initial activities of zero, one, and two neutrons occurring in coincidence with an ion-implant and beta trigger. The technique allows one to extract beta-delayed multi-neutron decay branching ratios measured with the He-3 BRIKEN neutron counter. As an example, two analyses of the beta-neutron emitter Cu-77 based on different a priori assumptions are presented along with comparisons to literature values.
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Guadilla, V. et al, Tain, J. L., Algora, A., Agramunt, J., Gelletly, W., Jordan, D., et al. (2018). Characterization and performance of the DTAS detector. Nucl. Instrum. Methods Phys. Res. A, 910, 79–89.
Abstract: DTAS is a segmented total absorption y-ray spectrometer developed for the DESPEC experiment at FAIR. It is composed of up to eighteen NaI(Tl) crystals. In this work we study the performance of this detector with laboratory sources and also under real experimental conditions. We present a procedure to reconstruct offline the sum of the energy deposited in all the crystals of the spectrometer, which is complicated by the effect of NaI(Tl) light-yield non-proportionality. The use of a system to correct for time variations of the gain in individual detector modules, based on a light pulse generator, is demonstrated. We describe also an event-based method to evaluate the summing-pileup electronic distortion in segmented spectrometers. All of this allows a careful characterization of the detector with Monte Carlo simulations that is needed to calculate the response function for the analysis of total absorption gamma-ray spectroscopy data. Special attention was paid to the interaction of neutrons with the spectrometer, since they are a source of contamination in studies of beta-delayed neutron emitting nuclei.
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BRIKEN Collaboration(Tolosa-Delgado, A. et al), Agramunt, J., Tain, J. L., Algora, A., Domingo-Pardo, C., Morales, A. I., et al. (2019). Commissioning of the BRIKEN detector for the measurement of very exotic beta-delayed neutron emitters. Nucl. Instrum. Methods Phys. Res. A, 925, 133–147.
Abstract: A new detection system has been installed at the RIKEN Nishina Center (Japan) to investigate decay properties of very neutron-rich nuclei. The setup consists of three main parts: a moderated neutron counter, a detection system sensitive to the implantation and decay of radioactive ions, and gamma-ray detectors. We describe here the setup, the commissioning experiment and some selected results demonstrating its performance for the measurement of half-lives and beta-delayed neutron emission probabilities. The methodology followed in the analysis of the data is described in detail. Particular emphasis is placed on the correction of the accidental neutron background.
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Wimmer, K. et al, Algora, A., & Rubio, B. (2019). Discovery of Br-68 in secondary reactions of radioactive beams. Phys. Lett. B, 795, 266–270.
Abstract: The proton-rich isotope Br-68 was discovered in secondary fragmentation reactions of fast radioactive beams. Proton-rich secondary beams of (70,71,72) Kr and Br-70, produced at the RIKEN Nishina Center and identified by the BigRIPS fragment separator, impinged on a secondary Be-9 target. Unambiguous particle identification behind the secondary target was achieved with the ZeroDegree spectrometer. Based on the expected direct production cross sections from neighboring isotopes, the lifetime of the ground or long-lived isomeric state of Br-68 was estimated. The results suggest that secondary fragmentation reactions, where relatively few nucleons are removed from the projectile, offer an alternative way to search for new isotopes, as these reactions populate preferentially low-lying states.
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Kulikov, I., Algora, A., Atanasov, D., Ascher, P., Blaum, K., Cakirli, R. B., et al. (2020). Masses of short-lived Sc-49, Sc-50, As-70, Br-73 and stable Hg-196 nuclides. Nucl. Phys. A, 1002, 121990–15pp.
Abstract: Mass measurements of Sc-49,Sc-50, As-70, Br-73 and Hg-196 nuclides produced at CERN's radioactive-ion beam facility ISOLDE are presented. The measurements were performed at the ISOLTRAP mass spectrometer by use of the multi-reflection time-of-flight and the Penning-trap mass spectrometry techniques. The new results agree well with previously known literature values. The mass accuracy for all cases has been improved.
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Liang, J., Singh, B., McCutchan, E. A., Dillmann, I., Birch, M., Sonzogni, A. A., et al. (2020). Compilation and Evaluation of Beta-Delayed Neutron Emission Probabilities and Half-Lives for Z > 28 Precursors. Nucl. Data Sheets, 168, 1–116.
Abstract: We present a compilation and evaluation of experimental beta-delayed neutron emission probabilities (P-n) and half-lives (T-1/2) for known or potential beta-delayed neutron precursors with atomic number Z > 28 (Cu-73 – Fr-233). This article includes the recommended values of both of these quantities, together with a compilation of experimental measurements when available. Some notable cases, as well as proposed standards for beta-delayed neutron measurements are also discussed. Evaluated data has also been compared to systematics using three different approaches. The literature cut-off date for this work is August 15, 2020.
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Hall, O. et al, Agramunt, J., Algora, A., Domingo-Pardo, C., Morales, A. I., Rubio, B., et al. (2021). beta-delayed neutron emission of r-process nuclei at the N=82 shell closure. Phys. Lett. B, 816, 136266–7pp.
Abstract: Theoretical models of beta-delayed neutron emission are used as crucial inputs in r-process calculations. Benchmarking the predictions of these models is a challenge due to a lack of currently available experimental data. In this work the beta-delayed neutron emission probabilities of 33 nuclides in the important mass regions south and south-west of Sn-132 are presented, 16 for the first time. The measurements were performed at RIKEN using the Advanced Implantation Detector Array (AIDA) and the BRIKEN neutron detector array. The P-1n values presented constrain the predictions of theoretical models in the region, affecting the final abundance distribution of the second r-process peak at A approximate to 130.
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Valiente-Dobon, J. J. et al, Gadea, A., & Algora, A. (2021). Manifestation of the Berry phase in the atomic nucleus Pb-213. Phys. Lett. B, 816, 136183–5pp.
Abstract: The neutron-rich Pb-213 isotope was produced in the fragmentation of a primary 1 GeV A U-238 beam, separated in FRS in mass and atomic number, and then implanted for isomer decay gamma-ray spectroscopy with the RISING setup at GSI. A newly observed isomer and its measured decay properties indicate that states in Pb-213 are characterized by the seniority quantum number that counts the nucleons not in pairs coupled to angular momentum J = 0. The conservation of seniority is a consequence of a geometric phase associated with particle-hole conjugation, which becomes observable in semi-magic nuclei where nucleons half-fill the valence shell. The gamma-ray spectroscopic observables in Pb-213 are thus found to be driven by two mechanisms, particle-hole conjugation and seniority conservation, which are intertwined through a Berry phase.
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Dimitriou, P. et al, Tain, J. L., & Algora, A. (2021). Development of a Reference Database for Beta-Delayed Neutron Emission. Nucl. Data Sheets, 173, 144–238.
Abstract: Beta-delayed neutron emission is important for nuclear structure and astrophysics as well as for reactor applications. Significant advances in nuclear experimental techniques in the past two decades have led to a wealth of new measurements that remain to be incorporated in the databases. We report on a coordinated effort to compile and evaluate all the available beta-delayed neutron emission data. The different measurement techniques have been assessed and the data have been compared with semi-microscopic and microscopic-macroscopic models. The new microscopic database has been tested against aggregate total delayed neutron yields, time-dependent group parameters in 6-and 8-group re-presentation, and aggregate delayed neutron spectra. New recommendations of macroscopic delayed-neutron data for fissile materials of interest to applications are also presented.
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Algora, A., Ganioglu, E., Sarriguren, P., Guadilla, V., Fraile, L. M., Nacher, E., et al. (2021). Total absorption gamma-ray spectroscopy study of the beta-decay of Hg-186. Phys. Lett. B, 819, 136438–7pp.
Abstract: The Gamow-Teller strength distribution of the decay of Hg-186 into Au-186 has been determined for the first time using the total absorption gamma spectroscopy technique and has been compared with theoretical QRPA calculations using the SLy4 Skyrme force. The measured Gamow-Teller strength distribution and the half-life are described by mixing oblate and prolate configurations independently in the parent and daughter nuclei. In this theoretical framework the best description of the experimental beta strength is obtained with dominantly prolate components for both parent Hg-186 and daughter Au-186. The approach also allowed us to determine an upper limit of the oblate component in the parent state. The complexity of the analysis required the development of a new approach in the analysis of the X-ray gated total absorption spectrum.
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