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n_TOF Collaboration(Garcia-Infantes, F. et al), Babiano-Suarez, V., Balibrea-Correa, J., Casanovas-Hoste, A., Domingo-Pardo, C., Ladarescu, I., et al. (2024). Measurement of the 176Yb(n,γ) cross section at the n_TOF facility at CERN. Phys. Rev. C, 110(6), 064619–16pp.
Abstract: Background: The Yb-176(n, gamma)Yb-177 -> 177Lu reaction is of interest in nuclear medicine as it is the preferred production route for 177Lu. This radioisotope has seen a very fast growth of usage in nuclear medicine in recent years due to its outstanding properties. New data on this reaction could provide useful information for production at new facilities. Purpose: We aim to resolve resonances in the Yb-176(n, gamma)Yb-177 reaction for the first time. Previous capture measurement provided data at thermal point and encompassed integral measurements in the range from 3 keV to 1 MeV, where three time-of-flight measurements are available, but with low resolution to resolve the resonances. Transmission measurements from the 1970s resolved and analyzed some resonances. Method: We measure the neutron capture cross section of Yb-176(n, gamma)Yb-177 by means of the time-of-flight technique at the Experimental Area 1 of the n_TOF facility at CERN using an enriched (Yb2O3)-Yb-176 sample and an array of four C6D6 liquid scintillation detectors. Results: We have resolved 164 resonances up to 21 keV, including 96 new ones. We also provide new capture experimental data from 90 eV to 3 keV, and we extend the resolved resonance region up to 21 keV. In addition, resonance decay widths, Gamma(gamma) and Gamma(n), are provided for all resonances together with resonance energies. Conclusions: The Yb-176(n, gamma) Yb-177 reaction has been measured, providing resonance parameters for the first time from a few eV to 21 keV. The analysis of the resonances has been carried out and compared with previous works and existing libraries, revealing discrepancies due to the new information on Gamma(gamma) parameters. Our results are consistent with the Gamma(n) parameters obtained in transmission measurements.
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Lerendegui-Marco, J., Babiano-Suarez, V., Balibrea-Correa, J., Caballero, L., Calvo, D., Ladarescu, I., et al. (2024). Simultaneous Gamma-Neutron Vision device: a portable and versatile tool for nuclear inspections. EPJ Tech. Instrum., 11(1), 2–17pp.
Abstract: This work presents GN-Vision, a novel dual gamma-ray and neutron imaging system, which aims at simultaneously obtaining information about the spatial origin of gamma-ray and neutron sources. The proposed device is based on two position sensitive detection planes and exploits the Compton imaging technique for the imaging of gamma-rays. In addition, spatial distributions of slow- and thermal-neutron sources (<100 eV) are reconstructed by using a passive neutron pin-hole collimator attached to the first detection plane. The proposed gamma-neutron imaging device could be of prime interest for nuclear safety and security applications. The two main advantages of this imaging system are its high efficiency and portability, making it well suited for nuclear applications were compactness and real-time imaging is important. This work presents the working principle and conceptual design of the GN-Vision system and explores, on the basis of Monte Carlo simulations, its simultaneous gamma-ray and neutron detection and imaging capabilities for a realistic scenario where a Cf-252 source is hidden in a neutron moderating container.
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Balibrea-Correa, J., Lerendegui-Marco, J., Ladarescu, I., Guerrero, C., Rodriguez-Gonzalez, T., Jimenez-Ramos, M. C., et al. (2022). Hybrid in-beam PET- and Compton prompt-gamma imaging aimed at enhanced proton-range verification. Eur. Phys. J. Plus, 137(11), 1258–18pp.
Abstract: We report on a hybrid in-beam PET and prompt-gamma Compton imaging system aimed at quasi real-time ion-range verification in proton-therapy treatments. Proof-of-concept experiments were carried out at the radiobiology beam line of the CNA cyclotron facility using a set of two synchronous Compton imagers and different target materials. The time structure of the 18 MeV proton beam was shaped with a series of beam-on and beam-off intervals, thereby mimicking a pulsed proton beam on a long time scale. During beam-on intervals, Compton imagingwas performed utilizing the high energy. -rays promptly emitted from the nuclear reactions occurring in the targets. In the course of the beam-off intervals in situ positron-emission tomography was accomplished with the same imagers using the beta+ decay of activated nuclei. The targets used were stacks of different materials covering also various proton ranges and energies. A systematic study on the performance of these two complementary imaging techniques is reported and the experimental results interpreted on the basis ofMonte Carlo calculations. The results demonstrate the possibility to combine both imaging techniques in a concomitant way, where high-efficiency prompt-gamma imaging is complemented with the high spatial accuracy of PET. Empowered by these results we suggest that a pulsed beam with a suitable duty cycle, in conjunction with in situ Compton- and PET-imaging may help to attain complementary information and quasi real-time range monitoring with high accuracy.
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Lerendegui-Marco, J., Balibrea-Correa, J., Babiano-Suarez, V., Ladarescu, I., & Domingo-Pardo, C. (2022). Towards machine learning aided real-time range imaging in proton therapy. Sci Rep, 12(1), 2735–17pp.
Abstract: Compton imaging represents a promising technique for range verification in proton therapy treatments. In this work, we report on the advantageous aspects of the i-TED detector for proton-range monitoring, based on the results of the first Monte Carlo study of its applicability to this field. i-TED is an array of Compton cameras, that have been specifically designed for neutron-capture nuclear physics experiments, which are characterized by gamma-ray energies spanning up to 5-6 MeV, rather low gamma-ray emission yields and very intense neutron induced gamma-ray backgrounds. Our developments to cope with these three aspects are concomitant with those required in the field of hadron therapy, especially in terms of high efficiency for real-time monitoring, low sensitivity to neutron backgrounds and reliable performance at the high gamma-ray energies. We find that signal-to-background ratios can be appreciably improved with i-TED thanks to its light-weight design and the low neutron-capture cross sections of its LaCl3 crystals, when compared to other similar systems based on LYSO, CdZnTe or LaBr3. Its high time-resolution (CRT similar to 500 ps) represents an additional advantage for background suppression when operated in pulsed HT mode. Each i-TED Compton module features two detection planes of very large LaCl3 monolithic crystals, thereby achieving a high efficiency in coincidence of 0.2% for a point-like 1 MeV gamma-ray source at 5 cm distance. This leads to sufficient statistics for reliable image reconstruction with an array of four i-TED detectors assuming clinical intensities of 10(8) protons per treatment point. The use of a two-plane design instead of three-planes has been preferred owing to the higher attainable efficiency for double time-coincidences than for threefold events. The loss of full-energy events for high energy gamma-rays is compensated by means of machine-learning based algorithms, which allow one to enhance the signal-to-total ratio up to a factor of 2.
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Plaza, J., Bécares, V., Cano-Ott, D., Gómez, C., Martínez, T., Mendoza, E., et al. (2023). CLYC as a neutron detector in low background conditions. Eur. Phys. J. C, 83(11), 1049–10pp.
Abstract: We report on the thermal neutron flux measurements carried out at the Laboratorio Subterraneo de Canfranc (LSC) with two commercial 2 '' x 2 '' CLYC detectors. The measurements were performed as part of an experimental campaign at LSC with He-3 detectors, for establishing the sensitivity limits and use of CLYCs in low background conditions. Acareful characterization of the intrinsic alpha and gamma-ray background in the detectors was required and done with dedicated measurements. It was found that the alpha activities in the two CLYC crystals differ by a factor of three, and the use of Monte Carlo simulations and a Bayesian unfolding method allowed us to determine the specific alpha activities from the U-238 and Th-232 decay chains. The simulations and unfolding also revealed that the gamma-ray background registered in the detectors is dominated by the intrinsic activity of the components of the detector such as the aluminum housing and photo-multiplier and that the activity within the crystal is low in comparison. The data from the neutron flux measurements with the two detectors were analyzed with different methodologies: one based on an innovative alpha/neutron pulse shape discrimination method and one based on the subtraction of the intrinsic alpha background that masks the neutron signals in the region of interest. The neutron sensitivity of the CLYCs was calculated by Monte Carlo simulations with MCNP6 and GEANT4. The resulting thermal neutron fluxes are in good agreement with complementary flux measurement performed with He-3 detectors, but close to the detection limit imposed by the intrinsic a activity.
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