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Author |
n_TOF Collaboration (Stamatopoulos, A. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Investigation of the Pu-240(n, f) reaction at the n_TOF/EAR2 facility in the 9 meV-6 MeV range |
Type |
Journal Article |
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Year |
2020 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
102 |
Issue |
1 |
Pages |
014616 - 23pp |
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Keywords |
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Abstract |
Background: Nuclear waste management is considered amongst the major challenges in the field of nuclear energy. A possible means of addressing this issue is waste transmutation in advanced nuclear systems, whose operation requires a fast neutron spectrum. In this regard, the accurate knowledge of neutron-induced reaction cross sections of several (minor) actinide isotopes is essential for design optimization and improvement of safety margins of such systems. One such case is Pu-240, due to its accumulation in spent nuclear fuel of thermal reactors and its usage in fast reactor fuel. The measurement of the Pu-240(n, f) cross section was previously attempted at the CERN nTOF facility EAR1 measuring station using the time-of-flight technique. Due to the low amount of available material and the given flux at EAR1, the measurement had to last several months to achieve a sufficient statistical accuracy. This long duration led to detector deterioration due to the prolonged exposure to the high alpha activity of the fission foils, therefore the measurement could not be successfully completed. Purpose: It is aimed to determine whether it is feasible to study neutron-induced fission at nTOF/EAR2 and provide data on the Pu-240(n, f) reaction in energy regions requested for applications. Methods: The study of the Pu-240(n, f) reaction was made at a new experimental area (EAR2) with a shorter flight path which delivered on average 30 times higher flux at fast neutron energies. This enabled the measurement to be performed much faster, thus limiting the exposure of the detectors to the intrinsic activity of the fission foils. The experimental setup was based on microbulk Micromegas detectors and the time-of-flight data were analyzed with an optimized pulse-shape analysis algorithm. Special attention was dedicated to the estimation of the non-negligible counting loss corrections with the development of a new methodology, and other corrections were estimated via Monte Carlo simulations of the experimental setup. Results: This new measurement of the Pu-240(n, f) cross section yielded data from 9 meV up to 6 MeV incident neutron energy and fission resonance kernels were extracted up to 10 keV. Conclusions: Neutron-induced fission of high activity samples can be successfully studied at the n_TOF/EAR2 facility at CERN covering a wide range of neutron energies, from thermal to a few MeV. |
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Address |
[Stamatopoulos, A.; Tsinganis, A.; Kokkoris, M.; Vlastou, R.; Diakaki, M.] Natl Tech Univ Athens, Athens, Greece, Email: athanasios.stamatopoulos@cern.ch |
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Amer Physical Soc |
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English |
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ISSN  |
0556-2813 |
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Expedition |
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Conference |
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Notes |
WOS:000551057500002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4466 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Balibrea-Correa, J. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Measurement of the alpha ratio and (n, gamma) cross section of U-235 from 0.2 to 200 eV at n_TOF |
Type |
Journal Article |
| |
Year |
2020 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
102 |
Issue |
4 |
Pages |
044615 - 18pp |
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Keywords |
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Abstract |
We measured the neutron capture-to-fission cross-section ratio (alpha ratio) and the capture cross section of U-235 between 0.2 and 200 eV at the nTOF facility at CERN. The simultaneous measurement of neutron-induced capture and fission rates was performed by means of the nTOF BaF2 Total Absorption Calorimeter (TAC), used for detection of gamma rays, in combination with a set of micromegas detectors used as fission tagging detectors. The energy dependence of the capture cross section was obtained with help of the Li-6(n, t) standard reaction determining the n_TOF neutron fluence; the well-known integral of the U-235(n, f) cross section between 7.8 and 11 eV was then used for its absolute normalization. The alpha ratio, obtained with slightly higher statistical fluctuations, was determined directly, without need for any reference cross section. To perform the analysis of this measurement we developed a new methodology to correct the experimentally observed effect that the probabilities of detecting a fission reaction in the TAC and the micromegas detectors are not independent. The results of this work have been used in a new evaluation of U-235 performed within the scope of the Collaborative International Evaluated Library Organisation (CIELO) Project, and are consistent with the ENDF/B-VIII.0 and JEFF-3.3 capture cross sections below 4 eV and above 100 eV. However, the measured capture cross section is on average 10% larger between 4 and 100 eV. |
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Address |
[Balibrea-Correa, J.; Mendoza, E.; Cano-Ott, D.] Ctr Invest Energet Medioambientales & Tecnol, CIEMAT, Madrid, Spain, Email: emilio.mendoza@ciemat.es |
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Amer Physical Soc |
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English |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0556-2813 |
ISBN |
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Expedition |
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Conference |
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Notes |
WOS:000579839000003 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4575 |
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Author |
n_TOF Collaboration (Gawlik, A. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Radiative Neutron Capture Cross-Section Measurement of Ge Isotopes at n_TOF CERN Facility and Its Importance for Stellar Nucleosynthesis |
Type |
Journal Article |
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Year |
2021 |
Publication |
Acta Physica Polonica A |
Abbreviated Journal |
Acta Phys. Pol. A |
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Volume |
139 |
Issue |
4 |
Pages |
383-388 |
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Keywords |
n_TOF; neutron time-of-flight; neutron capture cross-section; MACS |
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Abstract |
This manuscript summarizes the results of radiative neutron capture cross-section measurements on two stable germanium isotopes, Ge-70 and Ge-73. Experiments were performed at the n_TOF facility at CERN via the time-of-flight technique, over a wide neutron energy range, for all stable germanium isotopes (70,72,73,74, and 76). Results for Ge-70 [Phys. Rev. C 100, 045804 (2019)] and Ge-73 [Phys. Lett. B 790, 458 (2019)] are already published. In the field of nuclear structure, such measurements allow to study excited levels close to the neutron binding energy and to obtain information on nuclear properties. In stellar nucleosynthesis research, neutron induced reactions on germanium are of importance for nucleosynthesis in the weak component of the slow neutron capture processes. |
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Address |
[Gawlik, A.; Andrzejewski, J.; Perkowski, J.] Univ Lodz, Lodz, Poland, Email: aleksandra.gawlik@uni.lodz.pl |
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Polish Acad Sciences Inst Physics |
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English |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0587-4246 |
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Conference |
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Notes |
WOS:000653413700004 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4840 |
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Author |
Domingo-Pardo, C. |
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Title |
Beta-delayed neutron emission: first measurements in the heavy mass region and future prospects |
Type |
Journal Article |
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Year |
2016 |
Publication |
Acta Physica Polonica B |
Abbreviated Journal |
Acta Phys. Pol. B |
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Volume |
47 |
Issue |
3 |
Pages |
729-737 |
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Keywords |
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Abstract |
Beta-delayed neutrons play a key role in the formation of heavy elements in explosive stellar environments. The final r-process abundance distribution, including the rare-earth peak, is tailored to a large extent by the neutrons released after the beta decay of very exotic neutron-rich nuclei encountered along the r-process path and during the freeze-out phase. Such scenarios involve a vast amount of – yet undiscovered – nuclei, and most of them are expected to be neutron emitters. In this respect, existing beta-delayed neutron emission data is rather scarce, spanning from the lightest isotopes up to the region of the fission-fragments with masses up to A similar to 150. This contribution gives an overview on the latest measurements of neutron branching ratios in the heavy mass region around N = 126, which was practically unexplored in the past. Present plans to access very exotic nuclei at the RIB-facility of RIKEN in the framework of the BRIKEN project, are presented, together with the expected impact in r-process nucleosynthesis studies. |
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Address |
[Domingo-Pardo, C.; S410 GSI Collaboration; BRIKEN Collaboration] Univ Valencia, CSIC, IFIC, Valencia, Spain |
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Publisher |
Wydawnictwo Uniwersytetu Jagiellonskiego |
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English |
Summary Language |
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Original Title |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0587-4254 |
ISBN |
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Area |
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Conference |
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Notes |
WOS:000373495500015 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
no |
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Call Number |
IFIC @ pastor @ |
Serial |
2623 |
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Author |
Jordan, D.; Tain, J.L.; Algora, A.; Agramunt, J.; Domingo-Pardo, C.; Gomez-Hornillos, M.B.; Caballero-Folch, R.; Cortes, G.; Cano-Ott, D.; Mendoza, E.; Bandac, I.; Bettini, A.; Fraile, L.M.; Domingo, C. |
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Title |
Measurement of the neutron background at the Canfranc Underground Laboratory LSC |
Type |
Journal Article |
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Year |
2013 |
Publication |
Astroparticle Physics |
Abbreviated Journal |
Astropart Phys. |
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Volume |
42 |
Issue |
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Pages |
1-6 |
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Keywords |
Neutron background; Underground physics; He-3 proportional counters |
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Abstract |
The energy distribution of the neutron background was measured for the first time at Hall A of the Canfranc Underground Laboratory. For this purpose we used a novel approach based on the combination of the information obtained with six large high-pressure He-3 proportional counters embedded in individual polyethylene blocks of different size. In this way not only the integral value but also the flux distribution as a function of neutron energy was determined in the range from 1 eV to 10 MeV. This information is of importance because different underground experiments show different neutron background energy dependence. The high sensitivity of the setup allowed to measure a neutron flux level which is about four orders of magnitude smaller that the neutron background at sea level. The integral value obtained is Phi(Hall A) = (3.44 +/- 0.35) x 10(-6) cm(-2) s(-1). |
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Address |
[Jordan, D.; Tain, J. L.; Algora, A.; Agramunt, J.; Domingo-Pardo, C.] Univ Valencia, CSIC, Inst Fis Corpuscular, Valencia, Spain, Email: jordan@ific.uv.es |
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Publisher |
Elsevier Science Bv |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0927-6505 |
ISBN |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000315371900001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
1351 |
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Author |
AGATA Collaboration (Lalovic, N. et al); Gadea, A.; Domingo-Pardo, C. |
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Title |
Study of isomeric states in Pb-198, Pb-200, Pb-202, Pb-206 and Hg-206 populated in fragmentation reactions |
Type |
Journal Article |
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Year |
2018 |
Publication |
Journal of Physics G |
Abbreviated Journal |
J. Phys. G |
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Volume |
45 |
Issue |
3 |
Pages |
035105 - 27pp |
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Keywords |
gamma-ray spectroscopy; relativistic projectile fragmentation; direct reactions; isomeric decays; electromagnetic transitions; nuclear shell model |
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Abstract |
Isomeric states in isotopes in the vicinity of doubly-magic Pb-208 were populated following reactions of a relativistic Pb-208 primary beam impinging on a Be-9 fragmentation target. Secondary beams of Pb-198,Pb-200,Pb-202,Pb-206 and Hg-206 were isotopically separated and implanted in a passive stopper positioned in the focal plane of the GSI Fragment Separator. Delayed gamma rays were detected with the Advanced Gamma Tracking Array (AGATA). Decay schemes were reevaluated and interpreted with shell-model calculations. The momentum-dependent population of isomeric states in the two-nucleon hole nuclei Pb-206/Hg-206 was found to differ from the population of multi neutron-hole isomeric states in Pb-198,Pb-200,Pb-202. |
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Address |
[Lalovic, N.; Rudolph, D.; Sarmiento, L. G.; Golubev, P.; Fahlander, C.; Gellanki, J.] Lund Univ, Dept Phys, SE-22100 Lund, Sweden, Email: Natasa.Lalovic@nuclear.lu.se |
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Corporate Author |
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Publisher |
Iop Publishing Ltd |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0954-3899 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000424906600001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3488 |
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Author |
n_TOF Collaboration (Alcayne, V. et al); Balibrea-Correa, J.; Domingo-Pardo, C.; Lerendegui-Marco, J.; Babiano-Suarez, V.; Ladarescu, I. |
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Title |
A Segmented Total Energy Detector (sTED) optimized for (n,γ) cross-section measurements at n_TOF EAR2 |
Type |
Journal Article |
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Year |
2024 |
Publication |
Radiation Physics and Chemistry |
Abbreviated Journal |
Radiat. Phys. Chem. |
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Volume |
217 |
Issue |
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Pages |
11pp |
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Keywords |
Neutron capture; PHWT; Scintillation detectors; Monte Carlo simulation |
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Abstract |
The neutron time-of-flight facility nTOF at CERN is a spallation source dedicated to measurements of neutroninduced reaction cross-sections of interest in nuclear technologies, astrophysics, and other applications. Since 2014, Experimental ARea 2 (EAR2) is operational and delivers a neutron fluence of similar to 4 center dot 10(7) neutrons per nominal proton pulse, which is similar to 50 times higher than the one of Experimental ARea 1 (EAR1) of similar to 8 center dot 10(5) neutrons per pulse. The high neutron flux at EAR2 results in high counting rates in the detectors that challenged the previously existing capture detection systems. For this reason, a Segmented Total Energy Detector (sTED) has been developed to overcome the limitations in the detector's response, by reducing the active volume per module and by using a photo-multiplier (PMT) optimized for high counting rates. This paper presents the main characteristics of the sTED, including energy and time resolution, response to gamma-rays, and provides as well details of the use of the Pulse Height Weighting Technique (PHWT) with this detector. The sTED has been validated to perform neutron-capture cross-section measurements in EAR2 in the neutron energy range from thermal up to at least 400 keV. The detector has already been successfully used in several measurements at nTOF EAR2. |
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Address |
[Alcayne, V.; Cano-Ott, D.; Garcia, J.; Gonzalez-Romero, E.; Martinez, T.; de Rada, A. Perez; Plaza, J.; Sanchez-Caballero, A.; Mendoza, E.] Ctr Invest Energet Medioambient & Tecnol CIEMAT, Madrid, Spain, Email: victor.alcayne@ciemat.es |
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Corporate Author |
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Publisher |
Pergamon-Elsevier Science Ltd |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0969-806x |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:001185584800001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5999 |
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Author |
n_TOF Collaboration (Belloni, F. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Neutron-induced fission cross-section of U-233 in the energy range 0.5 < E-n < 20 MeV |
Type |
Journal Article |
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Year |
2011 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
47 |
Issue |
1 |
Pages |
2 - 7pp |
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Keywords |
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Abstract |
The neutron-induced fission cross-section of U-233 has been measured at the CERN nTOF facility relative to the standard fission cross-section of U-235 between 0.5 and 20MeV. The experiment was performed with a fast ionization chamber for the detection of the fission fragments and to discriminate against alpha-particles from the natural radioactivity of the samples. The high instantaneous flux and the low background of the nTOF facility result in data with uncertainties of approximate to 3%, which were found in good agreement with previous experiments. The high quality of the present results allows to improve the evaluation of the U-233(n, f) cross-section and, consequently, the design of energy systems based on the Th/U cycle. |
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Address |
[Belloni, F.; Milazzo, P. M.; Abbondanno, U.; Fujii, K.; Moreau, C.] Ist Nazl Fis Nucl INFN, Trieste, Italy, Email: paolo.milazzo@ts.infn.it |
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Corporate Author |
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Thesis |
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Publisher |
Springer |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1434-6001 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
ISI:000288550800006 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
539 |
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Author |
n_TOF Collaboration (Belloni, F. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Measurement of the neutron-induced fission cross-section of Am-243 relative to U-235 from 0.5 to 20 MeV |
Type |
Journal Article |
| |
Year |
2011 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
47 |
Issue |
12 |
Pages |
160 - 8pp |
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Keywords |
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Abstract |
The ratio of the neutron-induced fission cross-sections of Am-243 and U-235 was measured in the energy range from 0.5 to 20 MeV with uncertainties of approximate to 4%. The experiment was performed at the CERN n_TOF facility using a fast ionization chamber. With the good counting statistics that could be achieved thanks to the high instantaneous flux and the low backgrounds, the present results are useful for resolving discrepancies in previous data sets and are important for future reactors with improved fuel burn-up. |
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Address |
[Belloni, F.; Calviani, M.; Mastinu, P.; Milazzo, P. M.; Abbondanno, U.; Fujii, K.; Gramegna, F.; Moreau, C.] Ist Nazl Fis Nucl INFN, Lab Nazl Legnaro, Trieste, Italy, Email: paolo.milazzo@ts.infn.it |
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Corporate Author |
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Thesis |
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Publisher |
Springer |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1434-6001 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000300285100005 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
904 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Guerrero, C. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L. |
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Title |
Performance of the neutron time-of-flight facility n_TOF at CERN |
Type |
Journal Article |
| |
Year |
2013 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
49 |
Issue |
2 |
Pages |
27 - 15pp |
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Keywords |
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Abstract |
The neutron time-of-flight facility n_TOF features a white neutron source produced by spallation through 20 GeV/c protons impinging on a lead target. The facility, aiming primarily at the measurement of neutron-induced reaction cross sections, was operating at CERN between 2001 and 2004, and then underwent a major upgrade in 2008. This paper presents in detail all the characteristics of the new neutron beam in the currently available configurations, which correspond to two different collimation systems and two choices of neutron moderator. The characteristics discussed include the intensity and energy dependence of the neutron flux, the spatial profile of the beam, the in-beam background components and the energy resolution/broadening. The discussion of these features is based on dedicated measurements and Monte Carlo simulations, and includes estimations of the systematic uncertainties of the mentioned quantities. |
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Address |
[Guerrero, C.; Tsinganis, A.; Berthoumieux, E.; Weiss, C.; Chiaveri, E.; Calviani, M.; Vlachoudis, V.; Andriamonje, S.; Boccone, V.; Brugger, M.; Cerutti, F.; Chin, M.; Ferrari, A.; Hernandez-Prieto, A.; Kadi, Y.; Losito, R.; Roman, F.; Rubbia, C.; Versaci, R.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland, Email: carlos.guerrero@cern.ch |
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Corporate Author |
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Thesis |
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Publisher |
Springer |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1434-6001 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000315601600011 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
1358 |
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