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n_TOF Collaboration(Mastromarco, M. et al), Domingo-Pardo, C., & Tain, J. L. (2022). High accuracy, high resolution U-235(n,f) cross section from n_TOF (CERN) from 18 meV to 10 keV. Eur. Phys. J. A, 58(8), 147–13pp.
Abstract: The U-235(n,f) cross section was measured in a wide energy range (18 meV-170 keV) at the nTOF facility at CERN, relative to Li-6(n,t) and B-10(n,alpha) standard reactions, with high resolution and accuracy, with a setup based on a stack of six samples and six silicon detectors placed in the neutron beam. In this paper we report on the results in the region between 18 meV and 10 keV neutron energy. A resonance analysis has been performed up to 200 eV, with the code SAMMY. The resulting fission kernels are compared with the ones extracted on the basis of the resonance parameters of the most recent major evaluated data libraries. A comparison of the nTOF data with the evaluated cross sections is also performed from thermal to 10 keV neutron energy for the energy-averaged cross section in energy groups of suitably chosen width. A good agreement, within 0.5%, is found on average between the new results and the latest evaluated data files ENDF/B-VIII.0 and JEFF-3.3, as well as with respect to the broad group average fission cross section established in the framework of the standard working group of IAEA (the so-called reference file). However, some discrepancies, of up to 4%, are still present in some specific energy regions. The new dataset here presented, characterized by a unique combination of high resolution and accuracy, low background and wide energy range, can help to improve the evaluations from the Resolved Resonance Region up to 10 keV, also reducing the uncertainties that affect this region.
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n_TOF Collaboration(Lederer-Woods, C. et al), Domingo-Pardo, C., Tain, J. L., & Tarifeño-Saldivia, A. (2022). Ge-74(n, gamma) cross section below 70 keV measured at n_TOF CERN. Eur. Phys. J. A, 58(12), 239–9pp.
Abstract: Neutron capture reaction cross sections on Ge-74 are of importance to determine Ge-74 production during the astrophysical slow neutron capture process. We present new resonance data on Ge-74(n, gamma ) reactions below 70 keV neutron energy. We calculate Maxwellian averaged cross sections, combining our data below 70 keV with evaluated cross sections at higher neutron energies. Our stellar cross sections are in agreement with a previous activation measurement performed at Forschungszentrum Karlsruhe by Marganiec et al., once their data has been re-normalised to account for an update in the reference cross section used in that experiment.
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n_TOF Collaboration(Domingo-Pardo, C. et al), Babiano-Suarez, V., Balibrea-Correa, J., Caballero, L., Ladarescu, I., Lerendegui-Marco, J., et al. (2023). Advances and new ideas for neutron-capture astrophysics experiments at CERN n_TOF. Eur. Phys. J. A, 59(1), 8–11pp.
Abstract: This article presents a few selected developments and future ideas related to the measurement of (n, gamma ) data of astrophysical interest at CERN n_TOF. The MC-aided analysis methodology for the use of low-efficiency radiation detectors in time-of-flight neutron-capture measurements is discussed, with particular emphasis on the systematic accuracy. Several recent instrumental advances are also presented, such as the development of total-energy detectors with gamma- ray imaging capability for background suppression, and the development of an array of small-volume organic scintilla tors aimed at exploiting the high instantaneous neutron-flux of EAR2. Finally, astrophysics prospects related to the intermediate i neutron-capture process of nucleosynthesis are discussed in the context of the new NEAR activation area.
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Pasqualato, G. et al, Domingo-Pardo, C., & Gadea, A. (2023). Shape evolution in even-mass 98-104Zr isotopes via lifetime measurements using the γ γ-coincidence technique. Eur. Phys. J. A, 59(11), 276–13pp.
Abstract: The Zirconium (Z = 40) isotopic chain has attracted interest for more than four decades. The abrupt lowering of the energy of the first 2(+) state and the increase in the transition strength B(E2; 2(1)(+) -> 0(1)(+) ) going from Zr-98 to Zr-100 has been the first example of “quantum phase transition” in nuclear shapes, which has few equivalents in the nuclear chart. Although a multitude of experiments have been performed to measure nuclear properties related to nuclear shapes and collectivity in the region, none of the measured lifetimes were obtained using the Recoil Distance Doppler Shift method in the gamma gamma-coincidence mode where a gate on the direct feeding transition of the state of interest allows a strict control of systematical errors. This work reports the results of lifetime measurements for the first yrast excited states in Zr98-104 carried out to extract reduced transition probabilities. The new lifetime values in gamma gamma-coincidence and gamma-single mode are compared with the results of former experiments. Recent predictions of the Interacting Boson Model with Configuration Mixing, the Symmetry Conserving Configuration Mixing model based on the Hartree-Fock- Bogoliubov approach and the Monte Carlo Shell Model are presented and compared with the experimental data.
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Tagliente, G. et al, Babiano-Suarez, V., Domingo-Pardo, C., Ladarescu, I., & Tain, J. L. (2024). High-resolution cross section measurements for neutron interactions on 89Y with incident neutron energies up to 95 keV. Eur. Phys. J. A, 60(1), 21–18pp.
Abstract: The cross section of the Y-89(n,gamma) reaction has important implications in nuclear astrophysics and for advanced nuclear technology. Given its neutron magic number N = 50 and a consequent small neutron capture crosssection,89Y represents one of the key nuclides for the stellars-process. It acts as a bottleneck in the neutron capture chain between the Fe seed and the heavier elements. Moreover, it is located at the overlapping region, where both the weak and mains-process components take place.Y-89, the only stable yttrium isotope, is also used in innovative nuclear reactors. Neutron capture and transmission measurements were per-formed at the time-of-flight facilities n_TOF at CERN and GELINA at JRC-Geel. Resonance parameters of individual resonances were extracted from a resonance analysis of the experimental transmission and capture yields, up to a neutron incident energy of 95 keV. Even though a comparison with results reported in the literature shows differences in resonance parameters, the present data are consistent with the Maxwellian averaged cross section suggested by the astro-physical database KADoNiS.
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n_TOF Collaboration(Wright, T. et al), Domingo-Pardo, C., & Tain, J. L. (2024). Measurement of the prompt fission γ-rays from slow neutron-induced fission of 235U with STEFF. Eur. Phys. J. A, 60(3), 70–11pp.
Abstract: The amount of energy carried by gamma-rays during the fission process is an important consideration when developing new reactor designs. Many studies of gamma-ray energy and multiplicity, from a multitude of fissioning systems, were measured during the 1970s. However the data from such experiments largely underestimates the heating effect caused by gamma-rays in the structure of a reactor. It is therefore essential to obtain more accurate measurements of the energy carried during gamma-ray emission. As such, the OECD Nuclear Energy Agency has put out a high priority request [1] for measurements of the mean gamma-ray energy and multiplicity to an accuracy better than 7.5 percent from several fissioning systems; including U-235(n(thermal)). Measurements of the rays from these fissioning nuclei were performed with the SpecTrometer for Exotic Fission Fagments (STEFF).
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BRIKEN Collaboration(Tarifeño-Saldivia, A. et al), Tain, J. L., Domingo-Pardo, C., Agramunt, J., Algora, A., Morales, A. I., et al. (2017). Conceptual design of a hybrid neutron-gamma detector for study of beta-delayed neutrons at the RIB facility of RIKEN. J. Instrum., 12, P04006–22pp.
Abstract: BRIKEN is a complex detection system to be installed at the RIB-facility of the RIKEN Nishina Center. It is aimed at the detection of heavy-ion implants, β-particles, γ-rays and β-delayed neutrons. The whole detection setup involves the Advanced Implantation Detection Array (AIDA), two HPGe Clover detectors and a large set of 166 counters of 3He embedded in a high-density polyethylene matrix. This article reports on a novel methodology developed for the conceptual design and optimisation of the 3He-tubes array, aiming at the best possible performance in terms of neutron detection. The algorithm is based on a geometric representation of two selected parameters of merit, namely, average neutron detection efficiency and efficiency flatness, as a function of a reduced number of geometric variables. The response of the detection system itself, for each configuration, is obtained from a systematic MC-simulation implemented realistically in Geant4. This approach has been found to be particularly useful. On the one hand, due to the different types and large number of 3He-tubes involved and, on the other hand, due to the additional constraints introduced by the ancillary detectors for charged particles and gamma-rays. Empowered by the robustness of the algorithm, we have been able to design a versatile detection system, which can be easily re-arranged into a compact mode in order to maximize the neutron detection performance, at the cost of the gamma-ray sensitivity. In summary, we have designed a system which shows, for neutron energies up to 1(5) MeV, a rather flat and high average efficiency of 68.6%(64%) and 75.7%(71%) for the hybrid and compact modes, respectively. The performance of the BRIKEN system has been also quantified realistically by means of MC-simulations made with different neutron energy distributions.
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Caballero, L., Albiol, F., Corbi Bellot, A., Domingo-Pardo, C., Leganes Nieto, J. L., Agramunt Ros, J., et al. (2018). Gamma-ray imaging system for real-time measurements in nuclear waste characterisation. J. Instrum., 13, P03016–23pp.
Abstract: Acompact, portable and large field-of-viewgamma camera that is able to identify, locate and quantify gamma-ray emitting radioisotopes in real-time has been developed. The device delivers spectroscopic and imaging capabilities that enable its use it in a variety of nuclear waste characterisation scenarios, such as radioactivity monitoring in nuclear power plants and more specifically for the decommissioning of nuclear facilities. The technical development of this apparatus and some examples of its application in field measurements are reported in this article. The performance of the presented gamma-camera is also benchmarked against other conventional techniques.
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Olleros, P., Caballero, L., Domingo-Pardo, C., Babiano, V., Ladarescu, I., Calvo, D., et al. (2018). On the performance of large monolithic LaCl3(Ce) crystals coupled to pixelated silicon photosensors. J. Instrum., 13, P03014–17pp.
Abstract: We investigate the performance of large area radiation detectors, with high energy-and spatial-resolution, intended for the development of a Total Energy Detector with gamma-ray imaging capability, so-called i-TED. This new development aims for an enhancement in detection sensitivity in time-of-flight neutron capture measurements, versus the commonly used C6D6 liquid scintillation total-energy detectors. In this work, we study in detail the impact of the readout photosensor on the energy response of large area (50 x 50 mm(2)) monolithic LaCl3(Ce) crystals, in particular when replacing a conventional mono-cathode photomultiplier tube by an 8 x 8 pixelated silicon photomultiplier. Using the largest commercially available monolithic SiPM array (25 cm(2)), with a pixel size of 6 x 6 mm(2), we have measured an average energy resolution of 3.92% FWHM at 662 keV for crystal thick-nesses of 10, 20 and 30 mm. The results are confronted with detailed Monte Carlo (MC) calculations, where optical processes and properties have been included for the reliable tracking of the scintillation photons. After the experimental validation of the MC model, we use our MC code to explore the impact of a smaller photosensor segmentation on the energy resolution. Our optical MC simulations predict only a marginal deterioration of the spectroscopic performance for pixels of 3 x 3 mm(2).
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Colonna, N., Belloni, F., Berthoumieux, E., Calviani, M., Domingo-Pardo, C., Guerrero, C., et al. (2010). Advanced nuclear energy systems and the need of accurate nuclear data: the n_TOF project at CERN. Energy Environ. Sci., 3(12), 1910–1917.
Abstract: To satisfy the world's constantly increasing demand for energy, a suitable mix of different energy sources has to be devised. In this scenario, an important role could be played by nuclear energy, provided that major safety, waste and proliferation issues affecting current nuclear reactors are satisfactorily addressed. To this purpose, a large effort has been under way for a few years towards the development of advanced nuclear systems with the aim of closing the fuel cycle. Generation IV reactors, with full or partial waste recycling capability, accelerator driven systems, as well as new fuel cycles are the main options being investigated. The design of advanced systems requires improvements in basic nuclear data, such as cross-sections for neutron-induced reactions on actinides. In this paper, the main concepts of advanced reactor systems are described, together with the related needs of new and accurate nuclear data. The present activity in this field at the neutron facility n_TOF at CERN is discussed.
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