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Author |
n_TOF Collaboration (Lerendegui-Marco, J. et al.); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Radiative neutron capture on Pu-242 in the resonance region at the CERN n_TOF-EAR1 facility |
Type |
Journal Article |
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Year |
2018 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
97 |
Issue |
2 |
Pages |
024605 - 21pp |
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Abstract |
The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with uranium to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. However, an extensive use of MOX fuels, in particular in fast reactors, requires more accurate capture and fission cross sections for some Pu isotopes. In the case of Pu-242 there are sizable discrepancies among the existing capture cross-section measurements included in the evaluations (all from the 1970s) resulting in an uncertainty as high as 35% in the fast energy region. Moreover, postirradiation experiments evaluated with JEFF-3.1 indicate an overestimation of 14% in the capture cross section in the fast neutron energy region. In this context, the Nuclear Energy Agency (NEA) requested an accuracy of 8% in this cross section in the energy region between 500 meV and 500 keV. This paper presents a new time-of-flight capture measurement on Pu-242 carried out at nTOF-EAR1 (CERN), focusing on the analysis and statistical properties of the resonance region, below 4 keV. The Pu-242(n, gamma) reaction on a sample containing 95(4) mg enriched to 99.959% was measured with an array of four C6D6 detectors and applying the total energy detection technique. The high neutron energy resolution of nTOF-EAR1 and the good statistics accumulated have allowed us to extend the resonance analysis up to 4 keV, obtaining new individual and average resonance parameters from a capture cross section featuring a systematic uncertainty of 5%, fulfilling the request of the NEA. |
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Address |
[Lerendegui-Marco, J.; Guerrero, C.; Quesada, J. M.; Cortes-Giraldo, M. A.; Praena, J.; Sabate-Gilarte, M.] Univ Seville, Dept Fis Atom Mol & Nucl, E-41012 Seville, Spain, Email: cguerrero4@us.es |
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Publisher |
Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
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Notes |
WOS:000424190700001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration ![sorted by International Collaboration field, descending order (down)](img/sort_desc.gif) |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3474 |
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Author |
AGATA Collaboration (Lalovic, N. et al); Gadea, A.; Domingo-Pardo, C. |
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Title |
Study of isomeric states in Pb-198, Pb-200, Pb-202, Pb-206 and Hg-206 populated in fragmentation reactions |
Type |
Journal Article |
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Year |
2018 |
Publication |
Journal of Physics G |
Abbreviated Journal |
J. Phys. G |
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Volume |
45 |
Issue |
3 |
Pages |
035105 - 27pp |
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Keywords |
gamma-ray spectroscopy; relativistic projectile fragmentation; direct reactions; isomeric decays; electromagnetic transitions; nuclear shell model |
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Abstract |
Isomeric states in isotopes in the vicinity of doubly-magic Pb-208 were populated following reactions of a relativistic Pb-208 primary beam impinging on a Be-9 fragmentation target. Secondary beams of Pb-198,Pb-200,Pb-202,Pb-206 and Hg-206 were isotopically separated and implanted in a passive stopper positioned in the focal plane of the GSI Fragment Separator. Delayed gamma rays were detected with the Advanced Gamma Tracking Array (AGATA). Decay schemes were reevaluated and interpreted with shell-model calculations. The momentum-dependent population of isomeric states in the two-nucleon hole nuclei Pb-206/Hg-206 was found to differ from the population of multi neutron-hole isomeric states in Pb-198,Pb-200,Pb-202. |
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Address |
[Lalovic, N.; Rudolph, D.; Sarmiento, L. G.; Golubev, P.; Fahlander, C.; Gellanki, J.] Lund Univ, Dept Phys, SE-22100 Lund, Sweden, Email: Natasa.Lalovic@nuclear.lu.se |
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Iop Publishing Ltd |
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English |
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ISSN |
0954-3899 |
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Notes |
WOS:000424906600001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration ![sorted by International Collaboration field, descending order (down)](img/sort_desc.gif) |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3488 |
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Author |
n_TOF Collaboration (Barbagallo, M. et al); Domingo-Pardo, C.; Tain, J.L. |
![goto web page (via DOI) doi](img/doi.gif)
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Title |
Experimental setup and procedure for the measurement of the Be-7(n,p)Li-7 reaction at n_TOF |
Type |
Journal Article |
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Year |
2018 |
Publication |
Nuclear Instruments & Methods in Physics Research A |
Abbreviated Journal |
Nucl. Instrum. Methods Phys. Res. A |
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Volume |
887 |
Issue |
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Pages |
27-33 |
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Keywords |
Cosmological Lithium problem; Big bang nucleosynthesis; Be-7(n,p)Li-7 reaction; n_TOF spallation neutron source |
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Abstract |
Following the completion of the second neutron beam line and the related experimental area (EAR2) at the n_TOF spallation neutron source at CERN, several experiments were planned and performed. The high instantaneous neutron flux available in EAR2 allows to investigate neutron induced reactions with charged particles in the exit channel even employing targets made out of small amounts of short-lived radioactive isotopes. After the successful measurement of the Be-7(n,alpha)alpha cross section, the Be-7(n,p)Li-7 reaction was studied in order to provide still missing cross section data of relevance for Big Bang Nucleosynthesis (BBN), in an attempt to find a solution to the cosmological Lithium abundance problem. This paper describes the experimental setup employed in such a measurement and its characterization. |
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Address |
[Barbagallo, M.; Mastromarco, M.; Damone, L. A.; Mazzone, A.; Colonna, N.; Tagliente, G.; Variale, V.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: finocchiaro@lns.infn.ir |
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Publisher |
Elsevier Science Bv |
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English |
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Edition |
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ISSN |
0168-9002 |
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Notes |
WOS:000427814400005 |
Approved |
no |
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Is ISI |
yes |
International Collaboration ![sorted by International Collaboration field, descending order (down)](img/sort_desc.gif) |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3528 |
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Permanent link to this record |
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Author |
n_TOF Collaboration (Praena, J. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Preparation and characterization of S-33 samples for S-33(n,alpha)Si-30 cross-section measurements at the n_TOF facility at CERN |
Type |
Journal Article |
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Year |
2018 |
Publication |
Nuclear Instruments & Methods in Physics Research A |
Abbreviated Journal |
Nucl. Instrum. Methods Phys. Res. A |
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Volume |
890 |
Issue |
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Pages |
142-147 |
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Keywords |
Neutron induced alpha emission; Thermal evaporation; Rutherford backscattering |
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Abstract |
Thin S-33 samples for the study of the S-33(n,alpha)Si-30 cross-section at the n_TOF facility at CERN were made by thermal evaporation of S-33 powder onto a dedicated substrate made of kapton covered with thin layers of copper, chromium and titanium. This method has provided for the first time bare sulfur samples a few centimeters in diameter. The samples have shown an excellent adherence with no mass loss after few years and no sublimation in vacuum at room temperature. The determination of the mass thickness of S-33 has been performed by means of Rutherford backscattering spectrometry. The samples have been successfully tested under neutron irradiation. |
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Address |
[Praena, J.; Porras, I.] Univ Granada, Granada, Spain, Email: jpraena@ugr.es |
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Publisher |
Elsevier Science Bv |
Place of Publication |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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ISSN |
0168-9002 |
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Conference |
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Notes |
WOS:000427814900020 |
Approved |
no |
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Is ISI |
yes |
International Collaboration ![sorted by International Collaboration field, descending order (down)](img/sort_desc.gif) |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3537 |
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Permanent link to this record |
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Author |
n_TOF Collaboration (Praena, J. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Measurement and resonance analysis of the S-33(n,alpha)Si-30 cross section at the CERN n_TOF facility in the energy region from 10 to 300 keV |
Type |
Journal Article |
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Year |
2018 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
97 |
Issue |
6 |
Pages |
064603 - 10pp |
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Keywords |
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Abstract |
The (33)(n , alpha)Si-30 cross section has been measured at the neutron time-of-flight (n_TOF) facility at CERN in the neutron energy range from 10 to 300 keV relative to the B-10(n, alpha)(7) Li cross-section standard. Both reactions were measured simultaneously with a set of micromegas detectors. The flight path of 185 m has allowed us to obtain the cross section with high-energy resolution. An accurate description of the resonances has been performed by means of the multilevel multichannel R-matrix code SAMMY. The results show a significantly higher area of the biggest resonance (13.45 keV) than the unique high-resolution (n , alpha) measurement. The new parametrization of the 13.45-keV resonance is similar to that of the unique transmission measurement. This resonance is a matter of research in neutron-capture therapy. The S-33(n, alpha)Si-30 cross section has been studied in previous works because of its role in the production of S-36 in stars, which is currently overproduced in stellar models compared to observations. |
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Address |
[Praena, J.; Porras, I] Univ Granada, Granada, Spain, Email: jpraena@ugr.es |
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Corporate Author |
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Thesis |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
2469-9985 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000434017300004 |
Approved |
no |
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Is ISI |
yes |
International Collaboration ![sorted by International Collaboration field, descending order (down)](img/sort_desc.gif) |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3597 |
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Permanent link to this record |