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Yokoyama, R. et al, Tain, J. L., Algora, A., Agramunt, J., Domingo-Pardo, C., Morales, A. I., et al. (2023). β-delayed neutron emissions from N > 50 gallium isotopes. Phys. Rev. C, 108(6), 064307–15pp.
Abstract: beta-delayed gamma-neutron spectroscopy has been performed on the decay of A=84 to 87 gallium isotopes at the RI-beam Factory at the RIKEN Nishina Center using a high-efficiency array of 3He neutron counters (BRIKEN). beta-2n-gamma events were measured in the decays of all of the four isotopes for the first time, which is direct evidence for populating the excited states of two-neutron daughter nuclei. Detailed decay schemes with the gamma branching ratios were obtained for these isotopes, and the neutron emission probabilities (P-xn) were updated from the previous study. Hauser-Feshbach statistical model calculations were performed to understand the experimental branching ratios. We found that the P-1n and P-2n values are sensitive to the nuclear level densities of 1n daughter nuclei and showed that the statistical model reproduced the P-2n/P-1n ratio better when experimental levels plus shell-model level densities fit by the Gilbert-Cameron formula were used as the level-density input. We also showed the neutron and gamma branching ratios are sensitive to the ground-state spin of the parent nucleus. Our statistical model analysis suggested J <= 3 for the unknown ground-state spin of the odd-odd nucleus Ga-86, from the I gamma(4(+)-> 2(+))/I-gamma(2(+)-> 0(+)) ratio of Ga-84 and the P-2n/P-1n ratio. These results show the necessity of detailed understanding of the decay scheme, including data from neutron spectroscopy, in addition to gamma measurements of the multineutron emitters.
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Tagliente, G. et al, Babiano-Suarez, V., Domingo-Pardo, C., Ladarescu, I., & Tain, J. L. (2024). High-resolution cross section measurements for neutron interactions on 89Y with incident neutron energies up to 95 keV. Eur. Phys. J. A, 60(1), 21–18pp.
Abstract: The cross section of the Y-89(n,gamma) reaction has important implications in nuclear astrophysics and for advanced nuclear technology. Given its neutron magic number N = 50 and a consequent small neutron capture crosssection,89Y represents one of the key nuclides for the stellars-process. It acts as a bottleneck in the neutron capture chain between the Fe seed and the heavier elements. Moreover, it is located at the overlapping region, where both the weak and mains-process components take place.Y-89, the only stable yttrium isotope, is also used in innovative nuclear reactors. Neutron capture and transmission measurements were per-formed at the time-of-flight facilities n_TOF at CERN and GELINA at JRC-Geel. Resonance parameters of individual resonances were extracted from a resonance analysis of the experimental transmission and capture yields, up to a neutron incident energy of 95 keV. Even though a comparison with results reported in the literature shows differences in resonance parameters, the present data are consistent with the Maxwellian averaged cross section suggested by the astro-physical database KADoNiS.
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Zanon, I. et al, Domingo-Pardo, C., & Gadea, A. (2023). High-Precision Spectroscopy of O-20 Benchmarking Ab Initio Calculations in Light Nuclei. Phys. Rev. Lett., 131(26), 262501–7pp.
Abstract: The excited states of unstable O-20 were investigated via.-ray spectroscopy following the O-19(d, p)O-20 reaction at 8 AMeV. By exploiting the Doppler shift attenuation method, the lifetimes of the 2(2)(+) and 3(1)(+) states were firmly established. From the gamma-ray branching and E2/M1 mixing ratios for transitions deexciting the 2(2)(+) and 3(1)(+) states, the B(E2) and B(M1) were determined. Various chiral effective field theory Hamiltonians, describing the nuclear properties beyond ground states, along with a standard USDB interaction, were compared with the experimentally obtained data. Such a comparison for a large set of gamma-ray transition probabilities with the valence space in medium similarity renormalization group ab initio calculations was performed for the first time in a nucleus far from stability. It was shown that the ab initio approaches using chiral effective field theory forces are challenged by detailed high-precision spectroscopic properties of nuclei. The reduced transition probabilities were found to be a very constraining test of the performance of the ab initio models.
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n_TOF Collaboration(Alcayne, V. et al), Balibrea-Correa, J., Domingo-Pardo, C., Lerendegui-Marco, J., Babiano-Suarez, V., & Ladarescu, I. (2024). A Segmented Total Energy Detector (sTED) optimized for (n,γ) cross-section measurements at n_TOF EAR2. Radiat. Phys. Chem., 217, 11pp.
Abstract: The neutron time-of-flight facility nTOF at CERN is a spallation source dedicated to measurements of neutroninduced reaction cross-sections of interest in nuclear technologies, astrophysics, and other applications. Since 2014, Experimental ARea 2 (EAR2) is operational and delivers a neutron fluence of similar to 4 center dot 10(7) neutrons per nominal proton pulse, which is similar to 50 times higher than the one of Experimental ARea 1 (EAR1) of similar to 8 center dot 10(5) neutrons per pulse. The high neutron flux at EAR2 results in high counting rates in the detectors that challenged the previously existing capture detection systems. For this reason, a Segmented Total Energy Detector (sTED) has been developed to overcome the limitations in the detector's response, by reducing the active volume per module and by using a photo-multiplier (PMT) optimized for high counting rates. This paper presents the main characteristics of the sTED, including energy and time resolution, response to gamma-rays, and provides as well details of the use of the Pulse Height Weighting Technique (PHWT) with this detector. The sTED has been validated to perform neutron-capture cross-section measurements in EAR2 in the neutron energy range from thermal up to at least 400 keV. The detector has already been successfully used in several measurements at nTOF EAR2.
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n_TOF Collaboration(Wright, T. et al), Domingo-Pardo, C., & Tain, J. L. (2024). Measurement of the prompt fission γ-rays from slow neutron-induced fission of 235U with STEFF. Eur. Phys. J. A, 60(3), 70–11pp.
Abstract: The amount of energy carried by gamma-rays during the fission process is an important consideration when developing new reactor designs. Many studies of gamma-ray energy and multiplicity, from a multitude of fissioning systems, were measured during the 1970s. However the data from such experiments largely underestimates the heating effect caused by gamma-rays in the structure of a reactor. It is therefore essential to obtain more accurate measurements of the energy carried during gamma-ray emission. As such, the OECD Nuclear Energy Agency has put out a high priority request [1] for measurements of the mean gamma-ray energy and multiplicity to an accuracy better than 7.5 percent from several fissioning systems; including U-235(n(thermal)). Measurements of the rays from these fissioning nuclei were performed with the SpecTrometer for Exotic Fission Fagments (STEFF).
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