Abstract: We report on spectroscopic information and lifetime measurements in the neutron-rich I-135,I-137,I-139 isotopes. This is the first lifetime data on iodine isotopes beyond N = 82. Excited states were populated in fast neutron-induced fission of U-238 at the ALTO facility of IJCLab with the LICORNE neutron source and detected using the hybrid nu-ball spectrometer. The level schemes of the I-135,I-137,I-139 isotopes are revised in terms of excited states with up to maximum spin-parity of (33/2(+)), populated for the first time in fast neutron-induced fission. We provide first results on the lifetimes of the (9/2(1)(+)) and (13/2(1)(+)) states in I-137 and I-139, and the (17/2(1)(+)) state in 137I. In addition, we give upper lifetime limits for the (11/2(1)(+)) states in I135-139, the (15/2(1)(+)) state in I-137, the (17/2(1)(+)) state in I-139, and reexamine the (29/2(1)(+)) state in I-137. The isomeric data in I-13(5) are reinvestigated, such as the previously known (15/2(1)(+)) and (23/21) isomers with T-1/2 of 1.64(14) and 4.6(7) ns, respectively, as obtained in this work. The new spectroscopic information is compared to that from spontaneous or thermal-neutron induced fission and discussed in the context of large scale shell-model (LSSM) calculations for the region beyond Sn-132, indicating the behavior of collectivity for the three valence-proton iodine chain with N = 82, 84, 86.

Abstract: In order to study the Gamow-Teller (GT) transitions from the T-z = +2 nucleus Ca-44 to the T-z = +1 nucleus Sc-44, where T-z is the z component of isospin T, we performed the (p, n)-type (He-3, t) charge-exchange (CE) reaction at 140 MeV/nucleon and the scattering angles 0 degrees and 2.5 degrees. An energy resolution of 28 keV, that was realized by applying matching techniques to the magnetic spectrometer system, allowed the study of fragmented states. The GT transition strengths, B(GT), were derived up to the excitation energy (E-x) of 13.7 MeV assuming the proportionality between cross sections and B(GT) values. The total sum of B(GT) values in discrete states was 3.7, which was 31% of the sum-rule-limit value of 12. Shell model calculations using the GXPF1J interaction could reproduce the gross features of the experimental B(GT) distribution, but not the fragmentation of the strength. By introducing the concepts of isospin, properties of isospin analogous transitions and states were investigated. (i) Assuming isospin symmetry, the T-z = +2 -> +1 and T-z = -2 -> -1 mirror GT transitions should have the same properties, where the latter can be studied in the beta decay of Cr-44 to V-44. First, we confirmed that the beta-decay half-life T-1/2 of Cr-44 can be reproduced using the B(GT) distribution from the Ca-44(He-3, t) measurement. Then, the 0 degrees, (3He, t) spectrum was modified to deduce the “beta-decay spectrum” and it was compared with the delayed-proton spectrum from the Cr-44 beta decay. The two spectra were mostly in agreement for the GT excitations, but suppression of the proton decay was found for the T = 2 isobaric analog state (IAS). (ii) Starting from the T = 2 ground state of 44Ca, the (3He, t) can excite GT states (state populated by GT transitions) with T = 1, 2, and 3. On the other hand, the Ca-44(p, p') reaction can excite spin-M1 states (states populated by spin-M1 transitions) with T = 2 and 3 that are analogous to the T = 2 and 3 GT states, respectively. By comparing the spectra from these two reactions, a T value of 2 is suggested for several GT states in the E-x = 11.5-13.7 MeV region. (iii) It has been suggested that the T = 2, J(pi) = 0(+) double isobaric analog state (DIAS) at 9.338 MeV in the T-z = 0 nucleus Ti-44 forms an isospin-mixed doublet with a subsidiary 0(+) state at 9.298 MeV. Since no corresponding state was found in the T-z = +1 nucleus Sc-44, we suggest T = 0 for the subsidiary state.

Abstract: The ss decays of the ground state (gs) and isomeric state (m) of Y-96 have been studied with the total absorption gamma-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility. The separation of the 8(+) isomeric state from the 0(-) ground state was achieved thanks to the purification capabilities of the JYFLTRAP double Penning trap system. The ss-intensity distributions of both decays have been independently determined. In the analyses the deexcitation of the 1581.6 keV level in Zr-96, in which conversion electron emission competes with pair production, has been carefully considered and found to have significant impact on the ss-detector efficiency, influencing the ss-intensity distribution obtained. Our results for Y-96gs (0(-)) confirm the large ground state to ground state ss-intensity probability, although a slightly larger value than reported in previous studies was obtained, amounting to 96.6(-2.1)(+0.3) % of the total ss intensity. Given that the decay of Y-96gs is the second most important contributor to the reactor antineutrino spectrum between 5 and 7 MeV, the impact of the present results on reactor antineutrino summation calculations has been evaluated. In the decay of Y-96m (8(+)), previously undetected ss intensity in transitions to states above 6 MeV has been observed. This shows the importance of total absorption gamma-ray spectroscopy measurements of ss decays with highly fragmented deexcitation patterns. Y-96m (8(+)) is a major contributor to reactor decay heat in uranium-plutonium and thorium-uranium fuels around 10 s after fission pulses, and the newly measured average ss and gamma energies differ significantly from the previous values in evaluated databases. The discrepancy is far above the previously quoted uncertainties. Finally, we also report on the successful implementation of an innovative total absorption gamma-ray spectroscopy analysis of the module-multiplicity gated spectra, as a first proof of principle to distinguish between decaying states with very different spin-parity values.

Abstract: The beta-delayed neutron emission probabilities of neutron rich Hg and Tl nuclei have been measured together with beta-decay half-lives for 20 isotopes of Au, Hg, Tl, Pb, and Bi in the mass region N greater than or similar to 126. These are the heaviest species where neutron emission has been observed so far. These measurements provide key information to evaluate the performance of nuclear microscopic and phenomenological models in reproducing the high-energy part of the beta-decay strength distribution. This provides important constraints on global theoretical models currently used in r-process nucleosynthesis.

Abstract: We report on the observation of a microsecond isomeric state in the single-proton-hole, three-neutron-particle nucleus In-134. The nuclei of interest were produced by in-flight fission of a U-238 beam at the Radioactive Isotope Beam Factory at RIKEN. The isomer depopulates through a gamma ray of energy 56.7(1) keV and with a half-life of T-1/2 = 3.5(4) μs. Based on the comparison with shell-model calculations, we interpret the isomer as the I-pi = 5(-) member of the pi 0g(9/2)(-1) circle times nu 1f(7/2)(3) multiplet, decaying to the I-pi = 7(-) ground state with a reduced-transition probability of B(E2; 5(-) -> 7(-)) = 0.53(6) W.u. Observation of this isomer, and lack of evidence in the current work for a I-pi = 5(-) isomer decay in In-132, provides a benchmark of the proton-neutron interaction in the region of the nuclear chart “southeast” of Sn-132, where experimental information on excited states is sparse.