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Author |
n_TOF Collaboration (Lerendegui-Marco, J. et al.); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Radiative neutron capture on Pu-242 in the resonance region at the CERN n_TOF-EAR1 facility |
Type |
Journal Article |
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Year |
2018 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
97 |
Issue |
2 |
Pages ![sorted by First Page field, descending order (down)](img/sort_desc.gif) |
024605 - 21pp |
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Abstract |
The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with uranium to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. However, an extensive use of MOX fuels, in particular in fast reactors, requires more accurate capture and fission cross sections for some Pu isotopes. In the case of Pu-242 there are sizable discrepancies among the existing capture cross-section measurements included in the evaluations (all from the 1970s) resulting in an uncertainty as high as 35% in the fast energy region. Moreover, postirradiation experiments evaluated with JEFF-3.1 indicate an overestimation of 14% in the capture cross section in the fast neutron energy region. In this context, the Nuclear Energy Agency (NEA) requested an accuracy of 8% in this cross section in the energy region between 500 meV and 500 keV. This paper presents a new time-of-flight capture measurement on Pu-242 carried out at nTOF-EAR1 (CERN), focusing on the analysis and statistical properties of the resonance region, below 4 keV. The Pu-242(n, gamma) reaction on a sample containing 95(4) mg enriched to 99.959% was measured with an array of four C6D6 detectors and applying the total energy detection technique. The high neutron energy resolution of nTOF-EAR1 and the good statistics accumulated have allowed us to extend the resonance analysis up to 4 keV, obtaining new individual and average resonance parameters from a capture cross section featuring a systematic uncertainty of 5%, fulfilling the request of the NEA. |
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Address |
[Lerendegui-Marco, J.; Guerrero, C.; Quesada, J. M.; Cortes-Giraldo, M. A.; Praena, J.; Sabate-Gilarte, M.] Univ Seville, Dept Fis Atom Mol & Nucl, E-41012 Seville, Spain, Email: cguerrero4@us.es |
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Publisher |
Amer Physical Soc |
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English |
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Abbreviated Series Title |
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Series Volume |
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ISSN |
2469-9985 |
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Notes |
WOS:000424190700001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3474 |
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Permanent link to this record |
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Author |
n_TOF Collaboration (Paradela, C. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L. |
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Title |
High-accuracy determination of the U-238/U-235 fission cross section ratio up to approximate to 1 GeV at n_TOF at CERN |
Type |
Journal Article |
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Year |
2015 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
91 |
Issue |
2 |
Pages ![sorted by First Page field, descending order (down)](img/sort_desc.gif) |
024602 - 11pp |
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Abstract |
The U-238 to U-235 fission cross section ratio has been determined at nTOF up to approximate to 1 GeV, with two different detection systems, in different geometrical configurations. A total of four datasets has been collected and compared. They are all consistent to each other within the relative systematic uncertainty of 3-4%. The data collected at nTOF have been suitably combined to yield a unique fission cross section ratio as a function of neutron energy. The result confirms current evaluations up to 200 MeV. Good agreement is also observed with theoretical calculations based on the INCL++ /Gemini++ combination up to the highest measured energy. The n_TOF results may help solve a long-standing discrepancy between the two most important experimental datasets available so far above 20 MeV, while extending the neutron energy range for the first time up to approximate to 1 GeV. |
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Address |
[Paradela, C.; Tarrio, D.; Leal-Cidoncha, E.; Duran, I.; Alvarez, H.] Univ Santiago de Compostela, Santiago De Compostela, Spain, Email: nicola.colonna@ba.infn.it |
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Amer Physical Soc |
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English |
Summary Language |
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ISSN |
0556-2813 |
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Notes |
WOS:000350174000004 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
2139 |
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Permanent link to this record |
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Author |
n_TOF Collaboration (Lederer-Woods, C. et al.); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Destruction of the cosmic gamma-ray emitter Al-26 in massive stars: Study of the key Al-26(n, p) reaction |
Type |
Journal Article |
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Year |
2021 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
104 |
Issue |
2 |
Pages ![sorted by First Page field, descending order (down)](img/sort_desc.gif) |
L022803 - 7pp |
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Abstract |
The Al-26(n, p) Mg-26 reaction is the key reaction impacting on the abundances of the cosmic gamma-ray emitter Al-26 produced in massive stars and impacts on the potential pollution of the early solar system with Al-26 by asymptotic giant branch stars. We performed a measurement of the Al-26(n, p) Mg-26 cross section at the high-flux beam line EAR-2 at the n_TOF facility (CERN). We report resonance strengths for eleven resonances, nine being measured for the first time, while there is only one previous measurement for the other two. Our resonance strengths are significantly lower than the only previous values available. Our cross-section data range to 150 keV neutron energy, which is sufficient for a reliable determination of astrophysical reactivities up to 0.5 GK stellar temperature. |
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Address |
[Lederer-Woods, C.; Woods, P. J.; Davinson, T.; Kahl, D.; Lonsdale, S. J.] Univ Edinburgh, Sch Phys & Astron, Peter Guthrie Tait Rd, Edinburgh EH9 3FD, Midlothian, Scotland, Email: claudia.lederer-woods@ed.ac.uk |
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Publisher |
Amer Physical Soc |
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English |
Summary Language |
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ISSN |
2469-9985 |
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Notes |
WOS:000691442700005 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4949 |
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Permanent link to this record |
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Author |
n_TOF Collaboration (Lederer, C. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L. |
![goto web page (via DOI) doi](img/doi.gif)
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Title |
Neutron Capture Cross Section of Unstable Ni-63: Implications for Stellar Nucleosynthesis |
Type |
Journal Article |
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Year |
2013 |
Publication |
Physical Review Letters |
Abbreviated Journal |
Phys. Rev. Lett. |
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Volume |
110 |
Issue |
2 |
Pages ![sorted by First Page field, descending order (down)](img/sort_desc.gif) |
022501 - 5pp |
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Abstract |
The Ni-63(n, gamma) cross section has been measured for the first time at the neutron time-of-flight facility n_TOF at CERN from thermal neutron energies up to 200 keV. In total, capture kernels of 12 (new) resonances were determined. Maxwellian averaged cross sections were calculated for thermal energies from kT = 5-100 keV with uncertainties around 20%. Stellar model calculations for a 25M(circle dot) star show that the new data have a significant effect on the s-process production of Cu-63, Ni-64, and Zn-64 in massive stars, allowing stronger constraints on the Cu yields from explosive nucleosynthesis in the subsequent supernova. |
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Address |
[Lederer, C.; Paradela, C.; Wallner, A.] Univ Vienna, Fac Phys, A-1090 Vienna, Austria |
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Publisher |
Amer Physical Soc |
Place of Publication |
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English |
Summary Language |
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Series Editor |
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0031-9007 |
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Notes |
WOS:000313336500005 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
1305 |
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Permanent link to this record |
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Author |
n_TOF Collaboration (Zugec, P. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L. |
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Title |
Measurement of the C-12(n, p)B-12 cross section at n_TOF at CERN by in-beam activation analysis |
Type |
Journal Article |
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Year |
2014 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
90 |
Issue |
2 |
Pages ![sorted by First Page field, descending order (down)](img/sort_desc.gif) |
021601 - 5pp |
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Keywords |
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Abstract |
The integral cross section of the C-12(n, p)B-12 reaction has been determined for the first time in the neutron energy range from threshold to several GeV at the n_TOF facility at CERN. The measurement relies on the activation technique with the beta decay of B-12 measured over a period of four half-lives within the same neutron bunch in which the reaction occurs. The results indicate that model predictions, used in a variety of applications, are mostly inadequate. The value of the integral cross section reported here can be used as a benchmark for verifying or tuning model calculations. |
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Address |
[Zugec, P.; Bosnar, D.] Univ Zagreb, Fac Sci, Dept Phys, Zagreb 41000, Croatia, Email: nicola.colonna@ba.infn.it |
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Corporate Author |
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Thesis |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0556-2813 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000340744900001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
1894 |
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Permanent link to this record |