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Mistry, A. K. et al, Tain, J. L., Agramunt, J., Algora, A., Guadilla, V., Morales, A. I., et al. (2022). The DESPEC setup for GSI and FAIR. Nucl. Instrum. Methods Phys. Res. A, 1033, 166662–18pp.
Abstract: The DEcay SPECtroscopy (DESPEC) setup for nuclear structure investigations was developed and commissioned at GSI, Germany in preparation for a full campaign of experiments at the FRS and Super-FRS. In this paper, we report on the first employment of the setup in the hybrid configuration with the AIDA implanter coupled to the FATIMA LaBr3(Ce) fast-timing array, and high-purity germanium detectors. Initial results are shown from the first experiments carried out with the setup. An overview of the setup and function is discussed, including technical advancements along the path.
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Goigoux, T. et al, Algora, A., Guadilla, V., Montaner-Piza, A., Morales, A. I., Orrigo, S. E. A., et al. (2016). Two-Proton Radioactivity of Kr-67. Phys. Rev. Lett., 117(16), 162501–6pp.
Abstract: In an experiment with the BigRIPS separator at the RIKEN Nishina Center, we observed two-proton (2p) emission from Kr-67. At the same time, no evidence for 2p emission of Ge-59 and Se-63, two other potential candidates for this exotic radioactivity, could be observed. This observation is in line with Q value predictions which pointed to Kr-67 as being the best new candidate among the three for two-proton radioactivity. Kr-67 is only the fourth 2p ground-state emitter to be observed with a half-life of the order of a few milliseconds. The decay energy was determined to be 1690(17) keV, the 2p emission branching ratio is 37(14)%, and the half-life of Kr-67 is 7.4(30) ms.
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Vitez-Sveiczer, A. et al, Algora, A., Morales, A. I., Rubio, B., Agramunt, J., Guadilla, V., et al. (2022). The beta-decay of Kr-70 into Br-70: Restoration of the pseudo-SU(4) symmetry. Phys. Lett. B, 830, 137123–8pp.
Abstract: The beta-decay of the even-even nucleus Kr-70 with Z=N+2, has been investigated at the Radioactive Ion Beam Factory (RIBF) of the RIKEN Nishina Center using the BigRIPS fragment separator, the ZeroDegree Spectrometer, the WAS3ABI implantation station and the EURICA HPGe cluster array. Fifteen gamma-rays associated with the beta-decay of( 70)Kr into Br-70 have been identified for the first time, defining ten populated states below E-exc=3300 keV. The half-life of Kr-70 was derived with increased precision and found to be t(1/2)=45.19 +/- 0.14 ms. The beta-delayed proton emission probability has also been determined as epsilon(p)=0.545(23)%. An increase in the beta-strength to the yrast 1(+) state in comparison with the heaviest Z=N+2 system studied so far (Ge-62 decay) is observed that may indicate increased np correlations in the T=0 channel. The beta-decay strength deduced from the results is interpreted in terms of the proton-neutron quasiparticle random-phase approximation (pnQRPA) and also with a schematic model that includes isoscalar and isovector pairing in addition to quadrupole deformation. The application of this last model indicates an approximate realization of pseudo-SU(4) symmetry in this system.
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Algora, A., Ganioglu, E., Sarriguren, P., Guadilla, V., Fraile, L. M., Nacher, E., et al. (2021). Total absorption gamma-ray spectroscopy study of the beta-decay of Hg-186. Phys. Lett. B, 819, 136438–7pp.
Abstract: The Gamow-Teller strength distribution of the decay of Hg-186 into Au-186 has been determined for the first time using the total absorption gamma spectroscopy technique and has been compared with theoretical QRPA calculations using the SLy4 Skyrme force. The measured Gamow-Teller strength distribution and the half-life are described by mixing oblate and prolate configurations independently in the parent and daughter nuclei. In this theoretical framework the best description of the experimental beta strength is obtained with dominantly prolate components for both parent Hg-186 and daughter Au-186. The approach also allowed us to determine an upper limit of the oblate component in the parent state. The complexity of the analysis required the development of a new approach in the analysis of the X-ray gated total absorption spectrum.
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Morales, A. I. et al, Algora, A., Rubio, B., Orrigo, S. E. A., Agramunt, J., Gelletly, W., et al. (2017). Simultaneous investigation of the T=1(J(pi)=0(+)) and T=0(J(pi)=9(+)) beta decays in Br-70. Phys. Rev. C, 95(6), 064327–11pp.
Abstract: The beta decay of the odd-odd nucleus Br-70 has been investigated with the BigRIPS and EURICA setups at the Radioactive Ion Beam Factory (RIBF) of the RIKEN Nishina Center. The T = 0(J(pi) = 9(+)) and T = 1(J(pi) = 0(+)) isomers have both been produced in in-flight fragmentation of Kr-78 with ratios of 41.6(8)% and 58.4(8)%, respectively. A half-life of t(1/2) = 2157(-49)(+53) ms has been measured for the J pi = 9(+) isomer from gamma-ray time decay analysis. Based on this result, we provide a new value of the half-life for the J pi = 0(+) ground state of Br-70, t(1/2) = 78.42 +/- 0.51 ms, which is slightly more precise, and in excellent agreement, with the best measurement reported hitherto in the literature. For this decay, we provide the first estimate of the total branching fraction decaying through the 2(1)(+) state in the daughter nucleus Se-70, R(2(1)(+)) = 1.3 +/- 1.1%. We also report four new low-intensity gamma-ray transitions at 661, 1103, 1561, and 1749 keV following the beta decay of the J pi = 9(+) isomer. Based on their coincidence relationships, we tentatively propose two new excited states at 3945 and 4752 keV in 70Se with most probable spins and parities of J(pi) = (6(+)) and (8(+)), respectively. The observed structure is interpreted with the help of shell-model calculations, which predict a complex interplay between oblate and prolate configurations at low excitation energies.
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Guadilla, V. et al, Tain, J. L., Algora, A., Agramunt, J., Jordan, D., Monserrate, M., et al. (2020). Determination of beta-decay ground state feeding of nuclei of importance for reactor applications. Phys. Rev. C, 102(6), 064304–12pp.
Abstract: In beta-decay studies the determination of the decay probability to the ground state (g.s.) of the daughter nucleus often suffers from large systematic errors. The difficulty of the measurement is related to the absence of associated delayed gamma-ray emission. In this work we revisit the 4 pi gamma – beta method proposed by Greenwood and collaborators in the 1990s, which has the potential to overcome some of the experimental difficulties. Our interest is driven by the need to determine accurately the beta-intensity distributions of fission products that contribute significantly to the reactor decay heat and to the antineutrinos emitted by reactors. A number of such decays have large g.s. branches. The method is relevant for nuclear structure studies as well. Pertinent formulas are revised and extended to the special case of beta-delayed neutron emitters, and the robustness of the method is demonstrated with synthetic data. We apply it to a number of measured decays that serve as test cases and discuss the features of the method. Finally, we obtain g.s. feeding intensities with reduced uncertainty for four relevant decays that will allow future improvements in antineutrino spectrum and decay heat calculations using the summation method.
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Blank, B. et al, Agramunt, J., Algora, A., Guadilla, V., Montaner-Piza, A., Morales, A. I., et al. (2016). New neutron-deficient isotopes from Kr-78 fragmentation. Phys. Rev. C, 93(6), 061301–5pp.
Abstract: In an experiment with the RIKEN projectile fragment separator called BigRIPS at the RIKEN Nishina Center, the fragmentation of a Kr-78 beam allowed the observation of new neutron-deficient isotopes at the proton drip line. Clean identification spectra could be produced and Se-63, Kr-67, and Kr-68 were identified for the first time. In addition, Ge-59 was also observed. Three of these isotopes, Ge-59, Se-63, and Kr-67, are potential candidates for ground-state two-proton radioactivity. In addition, the isotopes Ge-58, Se-62, and Kr-66 were also sought but without success. The present experiment also allowed the determination of production cross sections for some of the most exotic isotopes. These measurements confirm the trend already observed that the empirical parametrization of fragmentation cross sections, EPAX, significantly overestimates experimental cross sections in this mass region.
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Guadilla, V. et al, Tain, J. L., Algora, A., Agramunt, J., Jordan, D., Monserrate, M., et al. (2019). Total absorption gamma-ray spectroscopy of the beta-delayed neutron emitters I-137 and Rb-95. Phys. Rev. C, 100(4), 044305–17pp.
Abstract: The decays of the beta-delayed neutron emitters( 137)I and Rb-95 have been studied with the total absorption gamma-ray spectroscopy technique. The purity of the beams provided by the JYFLTRAP Penning trap at the ion guide isotope separator on-line facility in Jyvaskyla allowed us to carry out a campaign of isotopically pure measurements with the decay total absorption gamma-ray spectrometer, a segmented detector composed of 18 NaI(T1) modules. The contamination coming from the interaction of neutrons with the spectrometer has been carefully studied, and we have tested the use of time differences between prompt gamma rays and delayed neutron interactions to eliminate this source of contamination. Due to the sensitivity of our spectrometer, we have found a significant amount of beta intensity to states above the neutron separation energy that deexcite by gamma rays, comparable to the neutron emission probability. The competition between gamma deexcitation and neutron emission has been compared with Hauser-Feshbach calculations, and it can be understood as a nuclear structure effect. In addition, we have studied the impact of the beta-intensity distributions determined in this work on reactor decay heat and reactor antineutrino spectrum summation calculations. The robustness of our results is demonstrated by a thorough study of uncertainties and with the reproduction of the spectra of the individual modules and the module-multiplicity gated spectra. This work represents the state-of-the-art of our analysis methodology for segmented total absorption spectrometers.
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Guadilla, V. et al, Algora, A., Tain, J. L., Agramunt, J., Aysto, J., Jordan, D., et al. (2019). Large Impact of the Decay of Niobium Isomers on the Reactor (v)over-bar(e) Summation Calculations. Phys. Rev. Lett., 122(4), 042502–6pp.
Abstract: Even mass neutron-rich niobium isotopes are among the principal contributors to the reactor antineutrino energy spectrum. They are also among the most challenging to measure due to the refractory nature of niobium, and because they exhibit isomeric states lying very close in energy. The beta-intensity distributions of Nb-100gs,Nb-100m and Nb-102gs,Nb-02m beta decays have been determined using the total absorption.-ray spectroscopy technique. The measurements were performed at the upgraded Ion Guide Isotope Separator On-Line facility at the University of Jyvaskyla. Here, the double Penning trap system JYFLTRAP was employed to disentangle the beta decay of the isomeric states. The new data obtained in this challenging measurement have a large impact in antineutrino summation calculations. For the first time the discrepancy between the summation model and the reactor antineutrino measurements in the region of the shape distortion has been reduced.
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Caballero-Folch, R. et al, Agramunt, J., Tain, J. L., Algora, A., Domingo-Pardo, C., Guadilla, V., et al. (2018). First determination of beta-delayed multiple neutron emission beyond A=100 through direct neutron measurement: The P-2n value of Sb-136. Phys. Rev. C, 98(3), 034310–10pp.
Abstract: Background: beta-delayed multiple neutron emission has been observed for some nuclei with A <= 100 being the Rb-100 the heaviest beta 2n emitter measured to date. So far only 25 P-2n values have been determined for the approximate to 300 nuclei that may decay in this way. Accordingly it is of interest to measure P-2n values for the other possible multiple neutron emitters throughout the chart of the nuclides. It is of particular interest to make such a measurement for nuclei with A > 100 to test the predictions of theoretical models and simulation tools for the decays of heavy nuclei in the region of very neutron-rich nuclei. In addition the decay properties of these nuclei are fundamental for the understanding of astrophysical nucleosynthesis processes such as the r-process and safety inputs for nuclear reactors. Purpose: To determine for the first time the two-neutron branching ratio the P-2n value for Sb-136 through a direct neutron measurement and to provide precise P-1n values for Sb-136 and Te-136. Method: A pure beam of each isotope of interest was provided by the JYFLTRAP Penning trap at the Ion Guide Isotope Separator On-Line (IGISOL) facility of the University of Jyvaskyla Finland. The purified ions were implanted into a moving tape at the end of the beam line. The detection setup consisted of a plastic scintillator placed right behind the implantation point after the tape to register the beta decays and the BELEN detector based on neutron counters embedded in a polyethylene matrix. The analysis was based on the study of the beta- and neutron-growth-and-decay curves and the beta-one-neutron and beta-two-neutron time correlations which allowed us the determination of the neutron branching ratios. Results: The P-2n value of Sb-136 was found to be 0.14(3)% and the measured P-1n values for Sb-136 and Te-136 were found to be 32.2(15)% and 1.47(6)% respectively. Conclusions: The measured P-2n value is a factor 44 smaller than predicted by the finite-range droplet model plus the quasiparticle random-phase approximation (FRDM+QRPA) model used for r-process calculations.
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