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Gjestvang, D. et al, & Algora, A. (2023). Examination of how properties of a fissioning system impact isomeric yield ratios of the fragments. Phys. Rev. C, 108(6), 064602–12pp.
Abstract: The population of isomeric states in the prompt decay of fission fragments-so-called isomeric yield ratios (IYRs)-is known to be sensitive to the angular momentum J that the fragment emerged with, and may therefore contain valuable information on the mechanism behind the fission process. In this work, we investigate how changes in the fissioning system impact the measured IYRs of fission fragments to learn more about what parameters affect angular momentum generation. To enable this, a new technique for measuring IYRs is first demonstrated. It is based on the time of arrival of discrete gamma rays, and has the advantage that it enables the study of the IYR as a function of properties of the partner nucleus. This technique is used to extract the IYR of 134Te, strongly populated in actinide fission, from the three different fissioning systems: 232Th(n, f), 238U(n, f), at two different neutron energies, as well as 252Cf(sf). The impacts of changing the fissioning system, the compound nuclear excitation energy, the minimum J of the binary partner, and the number of neutrons emitted on the IYR of 134Te are determined. The decay code TALYS is used in combination with the fission simulation code FREYA to calculate the primary fragment angular momentum from the IYR. We find that the IYR of 134Te has a slope of 0.004 +/- 0.002 with increase in compound nucleus (CN) mass. When investigating the impact on the IYR of increased CN excitation energy, we find no change with an energy increase similar to the difference between thermal and fast fission. By varying the mass of the partner fragment emerging with 134Te, it is revealed that the IYR of 134Te is independent of the total amount of prompt neutrons emitted from the fragment pair. This indicates that neutrons carry minimal angular momentum away from the fission fragments. Comparisons with the FREYA+TALYS simulations reveal that the average angular momentum in 134Te following 238U(n, f) is 6.0 h over bar . This is not consistent with the value deduced from recent CGMF calculations. Finally, the IYR sensitivity to the angular momentum of the primary fragment is discussed. These results are not only important to help understanding the underlying mechanism in nuclear fission, but can also be used to constrain and benchmark fission models, and are relevant to the gamma -ray heating problem of reactors.
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Yue, Z. et al, Algora, A., & Nacher, E. (2024). Magnetic moments of thallium isotopes in the vicinity of magic N=126. Phys. Lett. B, 849, 138452–7pp.
Abstract: The magnetic dipole moments (mu) of Tl-209(g)(N =128) and Tl-207(m)(N = 126) have been measured for the first time using the in -source laser resonance -ionization spectroscopy technique with the Laser Ion Source and Trap (LIST) at ISOLDE (CERN). The application of the LIST suppresses the usually overwhelming background of the isobaric francium isotopes and allows access to heavy thallium isotopes with >207. The self -consistent theory of finite Fermi systems based on the energy density functional by Fayans et al. well describes the N dependence of μfor 1/2(+) thallium ground states, as well as μfor the 11/2(-) isomeric states in europium, gold and thallium isotopes. The inclusion of particle-vibration coupling leads to a better agreement between the theory and experiment for mu(Tl-g , I-pi = 1/2(+)). It is shown that beyond mean-field contributions tocannot be neglected at least for thallium isotopes with I-pi = 1/2(+).
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Guadilla, V., Algora, A., Estienne, M., Fallot, M., Gelletly, W., Porta, A., et al. (2024). First measurements with a new fl-electron detector for spectral shape studies. J. Instrum., 19(2), P02027–21pp.
Abstract: The shape of the electron spectrum emitted in /3 decay carries a wealth of information about nuclear structure and fundamental physics. In spite of that, few dedicated measurements have been made of /3 -spectrum shapes. In this work we present a newly developed detector for /3 electrons based on a telescope concept. A thick plastic scintillator is employed in coincidence with a thin silicon detector. The first measurements employing this detector have been carried out with mono -energetic electrons from the high-energy resolution electron -beam spectrometer at Bordeaux. Here we report on the good reproduction of the experimental spectra of mono -energetic electrons using Monte Carlo simulations. This is a crucial step for future experiments, where a detailed Monte Carlo characterization of the detector is needed to determine the shape of the /3 -electron spectra by deconvolution of the measured spectra with the response function of the detector. A chamber to contain two telescope assemblies has been designed for future /3 -decay experiments at the Ion Guide Isotope Separator On -Line facility in Jyvaskyla, aimed at improving our understanding of reactor antineutrino spectra.
Keywords: Detector modelling and simulations I (interaction of radiation with matter; interaction of photons with matter; interaction of hadrons with matter; etc); Instrumentation for radioactive beams (fragmentation devices; fragment and isotope; separators incl. ISOL; isobar separators; ion and atom traps; weak-beam diagnostics; radioactive-beam ion sources); Hybrid detectors; Spectrometers
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Jungclaus, A., Doornenbal, P., Acosta, J., Vaquero, V., Browne, F., Cortes, M. L., et al. (2024). Position of the single-particle 3/2- state in 135Sn and the N = 90 subshell closure. Phys. Lett. B, 851, 138561–5pp.
Abstract: The decay of excited states of the nucleus Sn-135, with three neutrons outside the doubly-magic Sn-132 core, was studied in an experiment performed at the Radioactive Isotope Beam Factory at RIKEN. Several gamma rays emitted from excited Sn-135 ions were observed following one-neutron and one-neutron-one-proton removal from Sn-136 and Sb-137 beams, respectively, on a beryllium target at relativistic energies. Based on the analogy to 133Sn populated via one-neutron removal from Sn-134, an excitation energy of 695(15) keV is assigned to the 3/2(-) state with strongest single-particle character in 135Sn. This result provides the first direct information about the evolution of the neutron shell structure beyond N = 82 and thus allows for a crucial test of shellmodel calculations in this region. The experimental findings are in full agreement with calculations performed employing microscopic effective two-body interactions derived from CD-Bonn and N3LO nucleon-nucleon potentials, which do not predict a pronounced subshell gap at neutron number N=90. The occurrence of such a gap in Sn-140, i.e., when the 1f(7/2) orbital is completely filled, had been proposed in the past, in analogy to the magicity of Ca-48, featuring a completely filled 0f(7/2) orbital one harmonic oscillator shell below.
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Das, B. et al, & Algora, A. (2024). Broken seniority symmetry in the semimagic proton mid-shell nucleus 95Rh. Phys. Rev. Res., 6(2), L022038–7pp.
Abstract: Lifetime measurements of low-lying excited states in the semimagic ( N = 50) nucleus 95 Rh have been performed by means of the fast -timing technique. The experiment was carried out using gamma -ray detector arrays consisting of LaBr 3 (Ce) scintillators and germanium detectors integrated into the DESPEC experimental setup commissioned for the Facility for Antiproton and Ion Research ( FAIR ) Phase -0, Darmstadt, Germany. The excited states in 95 Rh were populated primarily via the /3 decays of 95 Pd nuclei, produced in the projectile fragmentation of a 850 MeV / nucleon 124 Xe beam impinging on a 4 g / cm 2 9 Be target. The deduced electromagnetic E2 transition strengths for the gamma -ray cascade within the multiplet structure depopulating from the isomeric I pi = 21 / 2 + state are found to exhibit strong deviations from predictions of standard shell model calculations which feature approximately conserved seniority symmetry. In particular, the observation of a strongly suppressed E2 strength for the 13 / 2 + -> 9 / 2 + ground state transition cannot be explained by calculations employing standard interactions. This remarkable result may require revision of the nucleon-nucleon interactions employed in state-of-the-art theoretical model calculations, and might also point to the need for including three-body forces in the Hamiltonian.
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IDS Collaboration(Andel, B. et al), Algora, A., & Nacher, E. (2024). β decay of the ground state and of a low-lying isomer in Bi-216. Phys. Rev. C, 109(6), 064321–18pp.
Abstract: A detailed beta -decay study of the low- and high -spin states in 216 Bi has been performed at the ISOLDE Decay Station at the CERN-ISOLDE facility. In total, 48 new levels and 83 new transitions in the beta -decay daughter 216 Po were identified. Shell -model calculations for excited states in 216 Bi and 216 Po were performed using the H208 and the modified Kuo-Herling particle effective interactions. Based on the experimental observations and the shell -model calculations, the most likely spin and parity assignments for the beta -decaying states in 216 Bi are (3 – ) and (8 – ), respectively.
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Yaneva, A. et al, & Algora, A. (2024). The shape of the Tz =+1 nucleus 94Pd and the role of proton-neutron interactions on the structure of its excited states. Phys. Lett. B, 855, 138805–7pp.
Abstract: Reduced transition probabilities have been extracted between excited, yrast states in the N = Z + 2 nucleus Pd-94. The transitions of interest were observed following decays of the I-pi = 14(+), E-x = 2129-keV isomeric state, which was populated following the projectile fragmentation of a Xe-124 primary beam at the GSI Helmholtzzentrum fur Schwerionenforschung accelerator facility as part of FAIR Phase-0. Experimental information regarding the reduced E2 transition strengths for the decays of the yrast 8(+) and 6(+) states was determined following isomer-delayed E-gamma 1 – E-gamma 2 – Delta T-2,T-1 coincidence method, using the LaBr3(Ce)-based FATIMA fast-timing coincidence gamma-ray array, which allowed direct determination of lifetimes of states in Pd-94 using the Generalized Centroid Difference (GCD) method. The experimental value for the half-life of the yrast 8(+) state of 755(106) ps results in a reduced transition probability of B(E2:8(+)-> 6(+)) = 205(-25)(+34) e(2) fm(4), which enables a precise verification of shell-model calculations for this unique system, lying directly between the N = Z line and the N = 50 neutron shell closure. The determined B(E2) value provides an insight into the purity of (g(9/2))(n) configurations in competition with admixtures from excitations between the (lower) N = 3pf and (higher) N = 4gds orbitals for the first time. The results indicate weak collectivity expected for near-zero quadrupole deformation and an increasing importance of the T = 0 proton-neutron interaction at N = 48.
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Yeung, T. T. et al, Morales, A. I., Tain, J. L., Alcala, G., Algora, A., Agramunt, J., et al. (2024). First Exploration of Monopole-Driven Shell Evolution above the N=126 Shell Closure: New Millisecond Isomers in Tl-213 and Tl-215. Phys. Rev. Lett., 133(7), 072501–7pp.
Abstract: Isomer spectroscopy of heavy neutron-rich nuclei beyond the N = 126 closed shell has been performed for the first time at the Radioactive Isotope Beam Factory of the RIKEN Nishina Center. New millisecond isomers have been identified at low excitation energies, 985.3(19) keV in Tl-213 and 874(5) keV in Tl-215. The measured half-lives of 1.34(5) ms in Tl-213 and 3.0(3) ms in Tl-215 suggest spins and parities 11/2(-) with the single proton-hole configuration pi h(11/2) as leading component. They are populated via E1 transitions by the decay of higher-lying isomeric states with proposed spin and parity 17/2(+), interpreted as arising from a single pi s(1/2) proton hole coupled to the 8(+) seniority isomer in the PbA + 1 cores. The lowering of the 11/2(-) states is ascribed to an increase of the pi h(11/2) proton effective single-particle energy as the second nu g(9/2) orbital is filled by neutrons, owing to a significant reduction of the proton-neutron monopole interaction between the pi h(11/2) and nu g(9/2) orbitals. The new ms isomers provide the first experimental observation of shell evolution in the almost unexplored N > 126 nuclear region below doubly magic Pb-208.
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IDS Collaboration(Yue, Z. et al), Algora, A., & Nacher, E. (2024). Charge radii of thallium isotopes near the N=126 shell closure. Phys. Rev. C, 110(3), 034315–9pp.
Abstract: The changes in the mean-squared charge radius of Tl-209(g )(N=128) and Tl-207(m) (N=126) relative to Tl-205 have been measured for the first time using the in-source laser resonance-ionization spectroscopy technique with the Laser Ion Source and Trap (LIST) at ISOLDE (CERN). The application of the LIST suppresses the dominant background from isobaric francium isotopes and allows access to thallium nuclides with A >= 207. The characteristic kink in the charge radii at the N=126 neutron shell closure, as well as the odd-even effect similar to that in the adjacent bismuth, lead, and mercury isotopic chains, have been observed. The self-consistent theory of finite Fermi systems based on the energy density functional by Fayans et al. reproduces the behavior of charge radii in these isotopic chains near N=126. The comparison with calculations in the framework of the relativistic mean field (RMF) approach is also presented. In the case of the Fayans functional it is a specific form of pairing interaction with the dependence on the density gradient that is essential to provide agreement with the experimental charge radii. In particular, the kink is reproduced without the inversion of g(9/2) and i(11/2) neutron single-particle states, which is a prerequisite to correctly describe the kink in the RMF models.
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Rochman, D. et al, & Algora, A. (2024). An introduction to Spent Nuclear Fuel decay heat for Light Water Reactors: a review from the NEA WPNCS. EPJ Nucl. Sci. Technol., 10, 9–83pp.
Abstract: This paper summarized the efforts performed to understand decay heat estimation from existing spent nuclear fuel (SNF), under the auspices of the Working Party on Nuclear Criticality Safety (WPNCS) of the OECD Nuclear Energy Agency. Needs for precise estimations are related to safety, cost, and optimization of SNF handling, storage, and repository. The physical origins of decay heat (a more correct denomination would be decay power) are then introduced, to identify its main contributors (fission products and actinides) and time-dependent evolution. Due to limited absolute prediction capabilities, experimental information is crucial; measurement facilities and methods are then presented, highlighting both their relevance and our need for maintaining the unique current full-scale facility and developing new ones. The third part of this report is dedicated to the computational aspect of the decay heat estimation: calculation methods, codes, and validation. Different approaches and implementations currently exist for these three aspects, directly impacting our capabilities to predict decay heat and to inform decision-makers. Finally, recommendations from the expert community are proposed, potentially guiding future experimental and computational developments. One of the most important outcomes of this work is the consensus among participants on the need to reduce biases and uncertainties for the estimated SNF decay heat. If it is agreed that uncertainties (being one standard deviation) are on average small (less than a few percent), they still substantially impact various applications when one needs to consider up to three standard deviations, thus covering more than 95% of cases. The second main finding is the need of new decay heat measurements and validation for cases corresponding to more modern fuel characteristics: higher initial enrichment, higher average burnup, as well as shorter and longer cooling time. Similar needs exist for fuel types without public experimental data, such as MOX, VVER, or CANDU fuels. A third outcome is related to SNF assemblies for which no direct validation can be performed, representing the vast majority of cases (due to the large number of SNF assemblies currently stored, or too short or too long cooling periods of interest). A few solutions are possible, depending on the application. For the final repository, systematic measurements of quantities related to decay heat can be performed, such as neutron or gamma emission. This would provide indications of the SNF decay heat at the time of encapsulation. For other applications (short- or long-term cooling), the community would benefit from applying consistent and accepted recommendations on calculation methods, for both decay heat and uncertainties. This would improve the understanding of the results and make comparisons easier.
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