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Author |
Colonna, N.; Belloni, F.; Berthoumieux, E.; Calviani, M.; Domingo-Pardo, C.; Guerrero, C.; Karadimos, D.; Lederer, C.; Massimi, C.; Paradela, C.; Plag, R.; Praena, J.; Sarmento, R. |
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Title |
Advanced nuclear energy systems and the need of accurate nuclear data: the n_TOF project at CERN |
Type |
Journal Article |
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Year |
2010 |
Publication |
Energy & Environmental Science |
Abbreviated Journal |
Energy Environ. Sci. |
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Volume |
3 |
Issue |
12 |
Pages |
1910-1917 |
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Keywords |
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Abstract |
To satisfy the world's constantly increasing demand for energy, a suitable mix of different energy sources has to be devised. In this scenario, an important role could be played by nuclear energy, provided that major safety, waste and proliferation issues affecting current nuclear reactors are satisfactorily addressed. To this purpose, a large effort has been under way for a few years towards the development of advanced nuclear systems with the aim of closing the fuel cycle. Generation IV reactors, with full or partial waste recycling capability, accelerator driven systems, as well as new fuel cycles are the main options being investigated. The design of advanced systems requires improvements in basic nuclear data, such as cross-sections for neutron-induced reactions on actinides. In this paper, the main concepts of advanced reactor systems are described, together with the related needs of new and accurate nuclear data. The present activity in this field at the neutron facility n_TOF at CERN is discussed. |
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Address |
[Colonna, N.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy, Email: nicola.colonna@ba.infn.it |
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Publisher |
Royal Soc Chemistry |
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English |
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Edition |
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ISSN |
1754-5692 |
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Conference |
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Notes |
ISI:000284590900007 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number  |
IFIC @ elepoucu @ |
Serial |
319 |
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Author |
n_TOF Collaboration (Paradela, C. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Neutron-induced fission cross section of U-234 and Np-237 measured at the CERN Neutron Time-of-Flight (n_TOF) facility |
Type |
Journal Article |
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Year |
2010 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
82 |
Issue |
3 |
Pages |
034601 - 11pp |
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Keywords |
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Abstract |
A high-resolution measurement of the neutron-induced fission cross section of U-234 and Np-237 has been performed at the CERN Neutron Time-of-Flight facility. The cross sections have been determined in a wide energy range from 1 eV to 1 GeV using the evaluated U-235 cross section as reference. In these measurements the energy determination for the U-234 resonances could be improved, whereas previous discrepancies for the Np-237 resonances were confirmed. New cross-section data are provided for high neutron energies that go beyond the limits of prior evaluations, obtaining important differences in the case of Np-237. |
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Address |
[Paradela, C.; Duran, I.; Tarrio, D.; Alvarez, H.] Univ Santiago de Compostela, Santiago De Compostela, Spain, Email: carlos.paradela@usc.es |
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Corporate Author |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0556-2813 |
ISBN |
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Expedition |
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Conference |
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Notes |
ISI:000281651400002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
382 |
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Author |
n_TOF Collaboration (Mosconi, M. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Neutron physics of the Re/Os clock. I. Measurement of the (n, gamma) cross sections of Os-186,Os-187,Os-188 at the CERN n_TOF facility |
Type |
Journal Article |
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Year |
2010 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
82 |
Issue |
1 |
Pages |
015802 - 10pp |
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Keywords |
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Abstract |
The precise determination of the neutron capture cross sections of Os-186 and Os-187 is important to define the s-process abundance of Os-187 at the formation of the solar system. This quantity can be used to evaluate the radiogenic component of the abundance of Os-187 due to the decay of the unstable Re-187 (t(1/2) = 41.2 Gyr) and from this to infer the time duration of the nucleosynthesis in our galaxy (Re/Os cosmochronometer). The neutron capture cross sections of Os-186, Os-187, and Os-188 have been measured at the CERN n_TOF facility from 1 eV to 1 MeV, covering the entire energy range of astrophysical interest. The measurement has been performed by time-of-flight technique using isotopically enriched samples and two C6D6 scintillation detectors for recording the prompt. rays emitted in the capture events. Maxwellian averaged capture cross sections have been determined for thermal energies between kT = 5 and 100 keV corresponding to all possible s-process scenarios. The estimated uncertainties for the values at 30 keV are 4.1, 3.3, and 4.7% for Os-186, Os-187, and Os-188, respectively. |
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Address |
[Mosconi, M.; Domingo-Pardo, C.; Kaeppeler, F.; Audouin, L.; Bisterzo, S.; Dillmann, I.; Heil, M.; Plag, R.; Voss, F.; Walter, S.; Wisshak, K.] KIT, Inst Kernphys, D-76021 Karlsruhe, Germany, Email: Marita.Mosconi@ptb.de |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0556-2813 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
ISI:000279940200007 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
409 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Fujii, K. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Neutron physics of the Re/Os clock. III. Resonance analyses and stellar (n, gamma) cross sections of Os-186,Os-187,Os-188 |
Type |
Journal Article |
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Year |
2010 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
82 |
Issue |
1 |
Pages |
015804 - 18pp |
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Keywords |
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Abstract |
Neutron resonance analyses have been performed for the capture cross sections of Os-186, Os-187, and Os-188 measured at the n_TOF facility at CERN. Resonance parameters have been extracted up to 5, 3, and 8 keV, respectively, using the SAMMY code for a full R-matrix fit of the capture yields. From these results average resonance parameters were derived by a statistical analysis to provide a comprehensive experimental basis for modeling of the stellar neutron capture rates of these isotopes in terms of the Hauser-Feshbach statistical model. Consistent calculations for the capture and inelastic reaction channels are crucial for the evaluation of stellar enhancement factors to correct the Maxwellian averaged cross sections obtained from experimental data for the effect of thermally populated excited states. These factors have been calculated for the full temperature range of current scenarios of s-process nucleosynthesis using the combined information of the experimental data in the region of resolved resonances and in the continuum. The consequences of this analysis for the s-process component of the Os-187 abundance and the related impact on the evaluation of the time duration of galactic nucleosynthesis via the Re/Os cosmochronometer are discussed. |
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Address |
[Fujii, K.; Abbondanno, U.; Belloni, F.; Milazzo, P. M.; Moreau, C.] Ist Nazl Fis Nucl, I-34149 Trieste, Italy, Email: Kaori.Fujii@ts.infn.it |
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Corporate Author |
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Thesis |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0556-2813 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
ISI:000279940200009 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
410 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Tagliente, G. et al.); Domingo-Pardo, C.; Tain, J.L. |
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Title |
The Zr-92(n,gamma) reaction and its implications for stellar nucleosynthesis |
Type |
Journal Article |
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Year |
2010 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
81 |
Issue |
5 |
Pages |
055801 - 9pp |
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Keywords |
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Abstract |
Because the relatively small neutron capture cross sections of the zirconium isotopes are difficult to measure, the results of previous measurements are often not adequate for a number of problems in astrophysics and nuclear technology. Therefore, the Zr-92(n,gamma) cross section has been remeasured at the CERN n_TOF facility, providing a set of improved parameters for 44 resonances in the neutron energy range up to 40 keV. With this information the cross-section uncertainties in the keV region could be reduced to 5% as required for s-process nucleosynthesis studies and technological applications. |
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Address |
[Tagliente, G.; Colonna, N.; Marrone, S.; Terlizzi, R.] Ist Nazl Fis Nucl, I-70126 Bari, Italy, Email: giuseppe.tagliente@ba.infn.it |
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Corporate Author |
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Thesis |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0556-2813 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
ISI:000278144800074 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
444 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Massimi, C. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Au-197(n,gamma) cross section in the resonance region |
Type |
Journal Article |
| |
Year |
2010 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
81 |
Issue |
4 |
Pages |
044616 - 22pp |
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Keywords |
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Abstract |
The (n,gamma) cross section of Au-197 has been measured at nTOF in the resolved resonance region, up to 5 keV, with the aim of improving the accuracy in an energy range where it is not yet considered standard. The measurements were performed with two different experimental setup and detection techniques, the total energy method based on C6D6 detectors, and the total absorption calorimetry based on a 4 pi BaF2 array. By comparing the data collected with the two techniques, two accurate sets of neutron-capture yields have been obtained, which could be the basis for a new evaluation leading to an extended cross-section standard. Overall good agreement is found between the n_TOF results and evaluated cross sections, with some significant exceptions for small resonances. A few resonances not included in the existing databases have also been observed. |
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Address |
[Domingo-Pardo, C.] GSI Helmholtzzentrum Schwerionenforsch GmbH, Darmstadt, Germany, Email: c.domingopardo@gsi.de |
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Corporate Author |
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Thesis |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0556-2813 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
ISI:000277209500051 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
463 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Guerrero, C. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Study of Photon Strength Function of Actinides: the Case of (235)U, (238)Np and (241)Pu |
Type |
Journal Article |
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Year |
2011 |
Publication |
Journal of the Korean Physical Society |
Abbreviated Journal |
J. Korean Phys. Soc. |
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Volume |
59 |
Issue |
2 |
Pages |
1510-1513 |
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Keywords |
Photon/Gamma strength functions; Pygmy; Scissor mode; n_TOF; Total absorption calorimeter; TAC; Neutron capture |
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Abstract |
The decay from excited levels in medium and heavy nuclei can be described in a statistical approach by means of Photon Strength Functions and Level Density distributions. The study of electromagnetic cascades following neutron capture based on the use of high efficiency detectors has been shown to be well suited for probing the properties of the Photon Strength Function of heavy (high level density) and/or radioactive (high background) nuclei. In this work we have investigated for the first time the validity of the recommended PSF of actinides, in particular (235)U, (238)Np and (241)Pu. Our study includes the search for resonance structures in the PSF below S(n) and draws conclusions regarding their existence and their characteristics in terms of energy, width and electromagnetic nature. |
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Address |
[Guerrero, C; Alvarez-Velarde, F; Ano-Ott, DC; Martinez, T; Mendoza, E; Villamarin, D] Ctr Invest Energet Medioambientales & Technol CIE, Madrid, Spain, Email: carlos.guerrero@ciemat.es |
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Corporate Author |
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Thesis |
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Publisher |
Korean Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0374-4884 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000294080700013 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
731 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration; Gunsing, F.; Berthoumieux, E.; Borella, A.; Belgya, T.; Szentmiklosi, L.; Schillebeeckx, P.; Drohe, J.C.; Wynants, R.; Colonna, N.; Marrone, S.; Tagliente, G.; Terlizzi, R.; Domingo-Pardo, C.; Tain, J.L.; Martinez, T.; Massimi, C.; Mastinu, P.M.; Milazzo, P.M. |
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Title |
Neutron Capture on (209)Bi: Determination of the Production Ratio of (210m)Bi/(210g)Bi |
Type |
Journal Article |
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Year |
2011 |
Publication |
Journal of the Korean Physical Society |
Abbreviated Journal |
J. Korean Phys. Soc. |
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Volume |
59 |
Issue |
2 |
Pages |
1670-1675 |
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Keywords |
ND2010; Nuclear data; Neutron capture; Branching ratio; Statistical decay; (209)Bi; (210)Bi; (210)Po |
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Abstract |
Neutron capture on (209)Bi produces either an isomeric state (210m)Bi with a half life of 3 x 106 years, or the ground state (210g)Bi which decays with a half life of 5 days to the alpha emitter (210)Po. Therefore the neutron capture cross section ratio (209)Bi(n,gamma)(210m)Bi/(210g)Bi plays an important role in predicting the short- and long-term radio-toxicity produced by (209)Bi under neutron irradiation. This ratio is dependent on the neutron energy. We have measured this ratio for cold neutrons at the cold neutron beam facility of the Budapest Neutron Centre by observing the population of the ground-and the metastable state using high resolution gamma-ray spectroscopy. The same technique has been used at the pulsed white neutron source GELINA of the IRMM, Geel in combination with the neutron time-of-flight technique. Results for the neutron-energy dependent branching ratio will be presented. In addition we performed simulations using a statistical decay code. |
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Address |
[Gunsing, F; Berthoumieux, E; Borella, A] CEA Saclay, IRFU, SPhN, F-91911 Gif Sur Yvette, France, Email: gunsing@cea.fr |
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Corporate Author |
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Thesis |
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Publisher |
Korean Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0374-4884 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000294080700051 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
736 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Cano-Ott, D. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Neutron Capture Measuremetns on Minor Actinides at the n_TOF Facility at CERN: Past, Present and Future |
Type |
Journal Article |
| |
Year |
2011 |
Publication |
Journal of the Korean Physical Society |
Abbreviated Journal |
J. Korean Phys. Soc. |
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Volume |
59 |
Issue |
2 |
Pages |
1809-1812 |
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Keywords |
n_TOF; Total Absorption Calorimeter; TAC; Neutron capture; Cross section; Nuclear waste; Transmutation; Generation IV; Accelerator driven system; ADS; Nuclear reactor; Nuclear energy; Nuclear data; Barium fluoride; Actinides; Plutonium; Americium; Uranium |
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Abstract |
The successful development of advanced nuclear systems for sustainable energy production and nuclear waste management depends on high quality nuclear data libraries. Recent sensitivity studies and reports [1-3] have identified the need for substantially improving the accuracy of neutron cross-section data for minor actinides. The n_TOF collaboration has initiated an ambitious experimental program for the measurement of neutron capture cross sections of minor actinides. Two experimental setups have been constructed for this purpose: a Total Absorption Calorimeter (TAC) [4] for measuring neutron capture cross-sections of low-mass and/or radioactive samples and a set of two low neutron sensitivity C(6)D(6) detectors for the less radioactive materials. |
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Address |
[Cano-Ott, D; Alvarez-Velarde, F; Gonzalez-Romero, E; Guerrero, C; Martinez, T; Mendoza, E; Villamarin, D; Vicente, MC] Ctr Invest Energet Medioambientales & Technol CIE, Madrid, Spain, Email: daniel.cano@ciemat.es |
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Corporate Author |
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Thesis |
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Publisher |
Korean Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0374-4884 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000294080700085 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
737 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Tarrio, D. et al); Domingo-Pardo, C.; Plag, R.; Plompen, A.; Tain, J.L. |
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Title |
High-energy Neutron-induced Fission Cross Sections of Natural Lead and Bismuth-209 |
Type |
Journal Article |
| |
Year |
2011 |
Publication |
Journal of the Korean Physical Society |
Abbreviated Journal |
J. Korean Phys. Soc. |
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Volume |
59 |
Issue |
2 |
Pages |
1904-1907 |
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Keywords |
Nuclear data; Neutron-induced fission reactions; Pb-nat(n,f); Bi-209(n,f); Spallation neutron source; n_TOF facility |
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Abstract |
The CERN Neutron Time-Of-Flight (n_TOF) facility is well suited to measure small neutron-induced fission cross sections, as those of subactinides. The cross section ratios of (nat)Pb and (209)Bi relative to (235)U and (238)U were measured using PPAC detectors. The fragment coincidence method allows to unambiguously identify the fission events. The present experiment provides the first results for neutron-induced fission up to 1 GeV for (nat)Pb and (209)Bi. A good agreement with previous experimental data below 200 MeV is shown. The comparison with proton-induced fission indicates that the limiting regime where neutron-induced and proton-induced fission reach equal cross section is close to 1 GeV. |
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Address |
[Tarrio, D] Univ Santiago de Compostela, Fac Fis, Santiago De Compostela 15782, Spain, Email: diego.tarrio@usc.es |
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Corporate Author |
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Thesis |
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Publisher |
Korean Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0374-4884 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000294080700109 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
739 |
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| Permanent link to this record |
