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n_TOF Collaboration(Tarrio, D. et al), Domingo-Pardo, C., Plag, R., Plompen, A., & Tain, J. L. (2011). High-energy Neutron-induced Fission Cross Sections of Natural Lead and Bismuth-209. J. Korean Phys. Soc., 59(2), 1904–1907.
Abstract: The CERN Neutron Time-Of-Flight (n_TOF) facility is well suited to measure small neutron-induced fission cross sections, as those of subactinides. The cross section ratios of (nat)Pb and (209)Bi relative to (235)U and (238)U were measured using PPAC detectors. The fragment coincidence method allows to unambiguously identify the fission events. The present experiment provides the first results for neutron-induced fission up to 1 GeV for (nat)Pb and (209)Bi. A good agreement with previous experimental data below 200 MeV is shown. The comparison with proton-induced fission indicates that the limiting regime where neutron-induced and proton-induced fission reach equal cross section is close to 1 GeV.
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n_TOF Collaboration(Tarrio D. et al.), Domingo-Pardo, C., & Tain, J. L. (2011). Neutron-induced fission cross section of Pb-nat and Bi-209 from threshold to 1 GeV: An improved parametrization. Phys. Rev. C, 83(4), 044620–9pp.
Abstract: Neutron-induced fission cross sections for Pb-nat and Bi-209 were measured with a white-spectrum neutron source at the CERN Neutron Time-of-Flight (n_TOF) facility. The experiment, using neutrons from threshold up to 1 GeV, provides the first results for these nuclei above 200 MeV. The cross sections were measured relative to U-235 and U-238 in a dedicated fission chamber with parallel plate avalanche counter detectors. Results are compared with previous experimental data. Upgraded parametrizations of the cross sections are presented, from threshold energy up to 1 GeV. The proposed new sets of fitting parameters improve former results along the whole energy range.
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n_TOF Collaboration(Tagliente, G. et al.), Domingo-Pardo, C., & Tain, J. L. (2011). Neutron capture on (94)Zr: Resonance parameters and Maxwellian-averaged cross sections. Phys. Rev. C, 84(1), 015801–9pp.
Abstract: The neutron capture cross sections of the Zr isotopes play an important role in nucleosynthesis studies. The s-process reaction flow between the Fe seed and the heavier isotopes passes through the neutron magic nucleus (90)Zr and through (91,92,93,94)Zr, but only part of the flow extends to (96)Zr because of the branching point at (95)Zr. Apart from their effect on the s-process flow, the comparably small isotopic (n, gamma) cross sections make Zr also an interesting structural material for nuclear reactors. The (94)Zr (n, gamma) cross section has been measured with high resolution at the spallation neutron source n_TOF at CERN and resonance parameters are reported up to 60 keV neutron energy.
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n_TOF Collaboration(Tagliente, G. et al.), Domingo-Pardo, C., & Tain, J. L. (2011). (96)Zr(n,gamma) measurement at the n_TOF facility at CERN. Phys. Rev. C, 84(5), 055802–8pp.
Abstract: The (n,gamma) cross section of (96)Zr has been investigated at the CERN n_TOF spallation neutron source. High-resolution time-of-flight measurements using an enriched ZrO(2) sample allowed us to analyze 15 resonances below 40 keV with improved accuracy. On average, the capture widths were found to be 25% smaller than reported in earlier experiments. If complemented with the contribution by direct radiative capture, the derived Maxwellian averaged cross sections are consistent with activation data at kT = 25 keV. The present results confirm the astrophysical implications for the s-process branching at (95)Zr.
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n_TOF Collaboration(Sarmento, R. et al), Domingo-Pardo, C., & Tain, J. L. (2011). Measurement of the (236)U(n, f) cross section from 170 meV to 2 MeV at the CERN n_TOF facility. Phys. Rev. C, 84(4), 044618–10pp.
Abstract: The neutron-induced fission cross section of (236)U was measured at the neutron Time-of-Flight (nTOF) facility at CERN relative to the standard (235)U(n, f) cross section for neutron energies ranging from above thermal to several MeV. The measurement, covering the full range simultaneously, was performed with a fast ionization chamber, taking advantage of the high resolution of the nTOF spectrometer. The n_TOF results confirm that the first resonance at 5.45 eV is largely overestimated in some nuclear data libraries. The resonance triplet around 1.2 keV was measured with high resolution and resonance parameters were determined with good accuracy. Resonances at high energy have also been observed and characterized and different values for the cross section are provided for the region between 10 keV and the fission threshold. The present work indicates various shortcomings of the current nuclear data libraries in the subthreshold region and provides the basis for an accurate re-evaluation of the (236)U(n, f) cross section, which is of great relevance for the development of emerging or innovative nuclear reactor technologies.
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n_TOF Collaboration(Paradela, C. et al), Domingo-Pardo, C., Plag, R., Plompen, A., & Tain, J. L. (2011). (237)Np(n,f) Cross Section: New Data and Present Status. J. Korean Phys. Soc., 59(2), 1908–1911.
Abstract: In this document, we present the final result obtained at the nTOF experiment; for the neutron-induced fission cross section of the (237)Np, from the fission threshold up to 1 GeV. The method applied to get tins result is briefly discussed. nTOF data are compared to the last experimental measurements using other TOF facilities or the surrogate method, reported experiments performed with monoenergetic sources and the FISCAL systematic, including a discussion about the existing discrepancies.
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n_TOF Collaboration(Mendoza, E. et al), Giubrone, G., & Tain, J. L. (2011). Improved Neutron Capture Cross Section Measurements with the n_TOF Total Absorption Calorimeter. J. Korean Phys. Soc., 59(2), 1813–1816.
Abstract: The n_TOF collaboration operates a Total Absorption Calorimeter (TAC) [1] for measuring neutron capture cross-sections of low-mass and/or radioactive samples. The results obtained with the TAC have led to a substantial improvement of the capture cross sections of (237)Np and (240)Pu [2]. The experience acquired during the first measurements has allowed us to optimize the performance of the TAC and to improve the capture signal to background ratio, thus opening the way to more complex and demanding measurements on rare radioactive materials. The new design has been reached by a series of detailed Monte Carlo simulations of complete experiments and dedicated test measurements. The new capture setup will be presented and the main achievements highlighted.
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n_TOF Collaboration(Lederer, C. et al), Domingo-Pardo, C., & Tain, J. L. (2011). Au-197(n,gamma) cross section in the unresolved resonance region. Phys. Rev. C, 83(3), 034608–11pp.
Abstract: The cross section of the reaction Au-197(n,gamma) was measured with the time-of-flight technique at the n_TOF (neutron time-of-flight) facility in the unresolved resonance region between 5 and 400 keV using a pair of C6D6 (where D denotes H-2) liquid scintillators for the detection of prompt capture gamma rays. The results with a total uncertainty of 3.9%-6.7% for a resolution of 20 bins per energy decade show fair agreement with the Evaluated Nuclear Data File Version B-VII.0 (ENDF/B-VII.0), which contains the standard evaluation. The Maxwellian-averaged cross section (MACS) at 30 keV is in excellent agreement with the one according to the ENDF/B-VII.0 evaluation and 4.7% higher than the MACS measured independently by activation technique. Structures in the cross section, which had also been reported earlier, have been interpreted as being due to clusters of resonances.
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n_TOF Collaboration(Guerrero, C. et al), Giubrone, G., & Tain, J. L. (2011). Characterization of the New n_TOF Neutron Beam: Fluence, Profile and Resolution. J. Korean Phys. Soc., 59(2), 1624–1627.
Abstract: After a halt of four years, the nTOF spallation neutron facility at CERN has resumed operation in November 2008 with a new spallation target characterized by an improved safety and engineering design, resulting in a more robust overall performance and efficient cooling. The first measurement during the 2009 run has aimed at the full characterization of the neutron beam. Several detectors, such as calibrated fission chambers, the nTOF Silicon Monitor, a MicroMegas detector with (10)B and (235)U samples, as well as liquid and solid scintillators have been used in order to characterize the properties of the neutron fluence. The spatial profile of the beam has been studied with a specially designed “X-Y” MicroMegas which provided a 2D image of the beam as a function of neutron energy. Both properties have been compared with simulations performed. with the FLUKA code. The characterization of the resolution function is based on results from simulations which have been verified by the study of narrow capture resonances. of (56)Fe, which were measured as part of a new campaign of (n,gamma) measurements on Fe and Ni isotopes.
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n_TOF Collaboration(Guerrero, C. et al), Domingo-Pardo, C., & Tain, J. L. (2011). Study of Photon Strength Function of Actinides: the Case of (235)U, (238)Np and (241)Pu. J. Korean Phys. Soc., 59(2), 1510–1513.
Abstract: The decay from excited levels in medium and heavy nuclei can be described in a statistical approach by means of Photon Strength Functions and Level Density distributions. The study of electromagnetic cascades following neutron capture based on the use of high efficiency detectors has been shown to be well suited for probing the properties of the Photon Strength Function of heavy (high level density) and/or radioactive (high background) nuclei. In this work we have investigated for the first time the validity of the recommended PSF of actinides, in particular (235)U, (238)Np and (241)Pu. Our study includes the search for resonance structures in the PSF below S(n) and draws conclusions regarding their existence and their characteristics in terms of energy, width and electromagnetic nature.
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