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Author |
Caballero-Folch, R. et al; Domingo-Pardo, C.; Agramunt, J.; Algora, A.; Rubio, B.; Tain, J.L. |
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Title |
beta-decay half-lives and beta-delayed neutron emission probabilities for several isotopes of Au, Hg, Tl, Pb, and Bi, beyond N=126 |
Type |
Journal Article |
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Year |
2017 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
95 |
Issue |
6 |
Pages |
064322 - 16pp |
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Abstract |
Background: There have been measurements on roughly 230 nuclei that are beta-delayed neutron emitters. They range from He-8 up to La-150. Apart from 210Tl, with a branching ratio of only 0.007%, no other neutron emitter has been measured beyond A = 150. Therefore, new data are needed, particularly in the region of heavy nuclei around N = 126, in order to guide theoretical models and help understand the formation of the third r-process peak at A similar to 195. Purpose: To measure both beta-decay half-lives and neutron branching ratios of several neutron-rich Au, Hg, Tl, Pb, and Bi isotopes beyond N = 126. Method: Ions of interest were produced by fragmentation of a U-238 beam, selected and identified via the GSI-FRS fragment separator. A stack of segmented silicon detectors (SIMBA) was used to measure ion implants and beta decays. An array of 30 He-3 tubes embedded in a polyethylene matrix (BELEN) was used to detect neutrons with high efficiency and selectivity. A self-triggered digital system is employed to acquire data and to enable time correlations. The latter were analyzed with an analytical model and results for the half-lives and neutron-branching ratios were derived by using the binned maximum-likelihood method. Results: Twenty new beta-decay half-lives are reported for Au204-206, Hg208-211, Tl211-216, Pb215-218, and Bi218-220, nine of them for the first time. Neutron emission probabilities are reported for Hg-210,Hg-211 and Tl211-216. Conclusions: The new beta-decay half-lives are in good agreement with previous measurements on nuclei in this region. The measured neutron emission probabilities are comparable to or smaller than values predicted by global models such as relativistic Hartree Bogoliubov plus the relativistic quasi-particle random phase approximation (RHB + RQRPA). |
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Address |
[Caballero-Folch, R.; Calvino, F.; Cortes, G.; Gomez-Hornillos, M. B.; Riego, A.] Univ Politecn Cataluna, DFEN, INTE, E-08028 Barcelona, Spain, Email: rcaballero-folch@triumf.ca |
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Publisher |
Amer Physical Soc |
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English |
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Series Volume |
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Series Issue |
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ISSN |
2469-9985 |
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Expedition |
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Conference |
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Notes |
WOS:000404022100001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3176 |
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Permanent link to this record |
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Author |
Caballero-Folch, R. et al; Agramunt, J.; Tain, J.L.; Algora, A.; Domingo-Pardo, C.; Guadilla, V.; Montaner-Piza, A.; Orrigo, S.E.A.; Rubio, B.; Tarifeño-Saldivia, A.; Tolosa-Delgado, A. |
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Title |
First determination of beta-delayed multiple neutron emission beyond A=100 through direct neutron measurement: The P-2n value of Sb-136 |
Type |
Journal Article |
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Year |
2018 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
98 |
Issue |
3 |
Pages |
034310 - 10pp |
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Keywords |
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Abstract |
Background: beta-delayed multiple neutron emission has been observed for some nuclei with A <= 100 being the Rb-100 the heaviest beta 2n emitter measured to date. So far only 25 P-2n values have been determined for the approximate to 300 nuclei that may decay in this way. Accordingly it is of interest to measure P-2n values for the other possible multiple neutron emitters throughout the chart of the nuclides. It is of particular interest to make such a measurement for nuclei with A > 100 to test the predictions of theoretical models and simulation tools for the decays of heavy nuclei in the region of very neutron-rich nuclei. In addition the decay properties of these nuclei are fundamental for the understanding of astrophysical nucleosynthesis processes such as the r-process and safety inputs for nuclear reactors. Purpose: To determine for the first time the two-neutron branching ratio the P-2n value for Sb-136 through a direct neutron measurement and to provide precise P-1n values for Sb-136 and Te-136. Method: A pure beam of each isotope of interest was provided by the JYFLTRAP Penning trap at the Ion Guide Isotope Separator On-Line (IGISOL) facility of the University of Jyvaskyla Finland. The purified ions were implanted into a moving tape at the end of the beam line. The detection setup consisted of a plastic scintillator placed right behind the implantation point after the tape to register the beta decays and the BELEN detector based on neutron counters embedded in a polyethylene matrix. The analysis was based on the study of the beta- and neutron-growth-and-decay curves and the beta-one-neutron and beta-two-neutron time correlations which allowed us the determination of the neutron branching ratios. Results: The P-2n value of Sb-136 was found to be 0.14(3)% and the measured P-1n values for Sb-136 and Te-136 were found to be 32.2(15)% and 1.47(6)% respectively. Conclusions: The measured P-2n value is a factor 44 smaller than predicted by the finite-range droplet model plus the quasiparticle random-phase approximation (FRDM+QRPA) model used for r-process calculations. |
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Address |
[Caballero-Folch, R.; Dillmann, I] TRIUMF, Vancouver, BC V6T 2A3, Canada, Email: rcaballero-folch@triumf.ca |
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Publisher |
Amer Physical Soc |
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English |
Summary Language |
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Original Title |
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Abbreviated Series Title |
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Series Issue |
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Edition |
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ISSN |
2469-9985 |
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Expedition |
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Conference |
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Notes |
WOS:000444207600003 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3728 |
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Permanent link to this record |
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Author |
Caballero, L.; Albiol, F.; Corbi Bellot, A.; Domingo-Pardo, C.; Leganes Nieto, J.L.; Agramunt Ros, J.; Contreras, P.; Monserrate, M.; Olleros Rodriguez, P.; Perez Magan, D.L. |
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Title |
Gamma-ray imaging system for real-time measurements in nuclear waste characterisation |
Type |
Journal Article |
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Year |
2018 |
Publication |
Journal of Instrumentation |
Abbreviated Journal |
J. Instrum. |
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Volume |
13 |
Issue |
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Pages |
P03016 - 23pp |
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Keywords |
Inspection with gamma rays; Radiation monitoring |
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Abstract |
Acompact, portable and large field-of-viewgamma camera that is able to identify, locate and quantify gamma-ray emitting radioisotopes in real-time has been developed. The device delivers spectroscopic and imaging capabilities that enable its use it in a variety of nuclear waste characterisation scenarios, such as radioactivity monitoring in nuclear power plants and more specifically for the decommissioning of nuclear facilities. The technical development of this apparatus and some examples of its application in field measurements are reported in this article. The performance of the presented gamma-camera is also benchmarked against other conventional techniques. |
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Address |
[Caballero, L.] Univ Valencia, CSIC, Inst Fis Corpuscular, C Catedrat Jose Beltran 2, E-46980 Paterna, Spain, Email: Luis.Caballero@ific.uv.es |
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Publisher |
Iop Publishing Ltd |
Place of Publication |
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English |
Summary Language |
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Original Title |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1748-0221 |
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Expedition |
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Conference |
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Notes |
WOS:000428146300006 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
no |
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Call Number |
IFIC @ pastor @ |
Serial |
3540 |
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Permanent link to this record |
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Author |
BRIKEN Collaboration (Tolosa-Delgado, A. et al); Agramunt, J.; Tain, J.L.; Algora, A.; Domingo-Pardo, C.; Morales, A.I.; Rubio, B. |
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Title |
Commissioning of the BRIKEN detector for the measurement of very exotic beta-delayed neutron emitters |
Type |
Journal Article |
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Year |
2019 |
Publication |
Nuclear Instruments & Methods in Physics Research A |
Abbreviated Journal |
Nucl. Instrum. Methods Phys. Res. A |
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Volume |
925 |
Issue |
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Pages |
133-147 |
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Keywords |
Beta-delayed neutrons; Neutron and beta counters; Analysis methodology; Background correction |
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Abstract |
A new detection system has been installed at the RIKEN Nishina Center (Japan) to investigate decay properties of very neutron-rich nuclei. The setup consists of three main parts: a moderated neutron counter, a detection system sensitive to the implantation and decay of radioactive ions, and gamma-ray detectors. We describe here the setup, the commissioning experiment and some selected results demonstrating its performance for the measurement of half-lives and beta-delayed neutron emission probabilities. The methodology followed in the analysis of the data is described in detail. Particular emphasis is placed on the correction of the accidental neutron background. |
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Address |
[Tolosa-Delgado, A.; Agramunt, J.; Tain, J. L.; Algora, A.; Domingo-Pardo, C.; Morales, A., I; Rubio, B.] CSIC, Inst Fis Corpuscular, E-46980 Paterna, Spain, Email: tain@ific.uv.es |
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Publisher |
Elsevier Science Bv |
Place of Publication |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0168-9002 |
ISBN |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000460539400018 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3939 |
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Permanent link to this record |
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Author |
BRIKEN Collaboration (Tarifeño-Saldivia, A. et al); Tain, J.L.; Domingo-Pardo, C.; Agramunt, J.; Algora, A.; Morales, A.I.; Rubio, B.; Tolosa, A. |
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Title |
Conceptual design of a hybrid neutron-gamma detector for study of beta-delayed neutrons at the RIB facility of RIKEN |
Type |
Journal Article |
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Year |
2017 |
Publication |
Journal of Instrumentation |
Abbreviated Journal |
J. Instrum. |
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Volume |
12 |
Issue |
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Pages |
P04006 - 22pp |
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Keywords |
Detector modelling and simulations I (interaction of radiation with matter, interaction; of photons with matter, interaction of hadrons with matter, etc); Instrumentation for radioactive beams (fragmentation devices; fragment and isotope, separators incl. ISOL; isobar separators; ion and atom traps; weak-beam diagnostics; radioactive-beam ion sources); Neutron detectors (cold, thermal, fast neutrons) |
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Abstract |
BRIKEN is a complex detection system to be installed at the RIB-facility of the RIKEN Nishina Center. It is aimed at the detection of heavy-ion implants, β-particles, γ-rays and β-delayed neutrons. The whole detection setup involves the Advanced Implantation Detection Array (AIDA), two HPGe Clover detectors and a large set of 166 counters of 3He embedded in a high-density polyethylene matrix. This article reports on a novel methodology developed for the conceptual design and optimisation of the 3He-tubes array, aiming at the best possible performance in terms of neutron detection. The algorithm is based on a geometric representation of two selected parameters of merit, namely, average neutron detection efficiency and efficiency flatness, as a function of a reduced number of geometric variables. The response of the detection system itself, for each configuration, is obtained from a systematic MC-simulation implemented realistically in Geant4. This approach has been found to be particularly useful. On the one hand, due to the different types and large number of 3He-tubes involved and, on the other hand, due to the additional constraints introduced by the ancillary detectors for charged particles and gamma-rays. Empowered by the robustness of the algorithm, we have been able to design a versatile detection system, which can be easily re-arranged into a compact mode in order to maximize the neutron detection performance, at the cost of the gamma-ray sensitivity. In summary, we have designed a system which shows, for neutron energies up to 1(5) MeV, a rather flat and high average efficiency of 68.6%(64%) and 75.7%(71%) for the hybrid and compact modes, respectively. The performance of the BRIKEN system has been also quantified realistically by means of MC-simulations made with different neutron energy distributions. |
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Address |
[Tarifeno-Saldivia, A.] UPC, Barcelona, Spain, Email: ariel.esteban.tarifeno@upc.edu |
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Corporate Author |
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Thesis |
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Publisher |
Iop Publishing Ltd |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1748-0221 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000405067800006 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3209 |
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Permanent link to this record |