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Pedersen, L. G. et al, & Morales, A. I. (2023). First spectroscopic study of odd-odd 78Cu. Phys. Rev. C, 107(4), 044301–10pp.
Abstract: Nuclei in the vicinity of 78Ni are important benchmarks for nuclear structure, which can reveal changes in the shell structure far from stability. Spectroscopy of the odd-odd isotope 78Cu was performed for the first time in an experiment with the EURICA setup at the Radioactive Isotope Beam Factory at RIKEN Nishina Center. Excited states in the neutron-rich isotope were populated following the beta decay of 78Ni produced by in-flight fission and and separated by the BigRIPS separator. A level scheme based on the analysis of γ−γ coincidences is presented. Tentative spin and parity assignments were made when possible based on the β-decay feeding intensities and γ-decay properties of the excited states. Time correlations between β and γ decay show clear indications of an isomeric state with a half-life of 3.8(4) ms. Large-scale Monte Carlo shell-model calculations were performed using the A3DA-m interaction and a valence space comprising the full fp shell and the 1g9/2 and 2d5/2 orbitals for both protons and neutrons. The comparison of the experimental results with the shell-model calculations allows interpreting the excited states in terms of spin multiplets arising from the proton-neutron interaction. The results provide further insight into the evolution of the proton single-particle orbitals as a function of neutron number, and quantitative information about the proton-neutron interaction outside the doubly magic 78Ni core.
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Orrigo, S. E. A. et al, Rubio, B., Gelletly, W., Aguilera, P., Algora, A., Morales, A. I., et al. (2021). beta decay of the very neutron-deficient Ge-60 and Ge-62 nuclei. Phys. Rev. C, 103(1), 014324–12pp.
Abstract: We report here the results of a study of the beta decay of the proton-rich Ge isotopes, Ge-60 and Ge-62, produced in an experiment at the RIKEN Nishina Center. We have improved our knowledge of the half-lives of Ge-62 [73.5(1) ms] and Ge-60 [25.0(3) ms] and its daughter nucleus, Ga-60 [69.4(2) ms]. We measured individual beta-delayed proton and gamma emissions and their related branching ratios. Decay schemes and absolute Fermi and Gamow-Teller transition strengths have been determined. The mass excesses of the nuclei under study have been deduced. A total beta-delayed proton-emission branching ratio of 67(3)% has been obtained for Ge-60. New information has been obtained on the energy levels populated in Ga-60 and on the 1/2(-) excited state in the beta p daughter Zn-59. We extracted a ground state-to-ground state feeding of 85.3(3)% for the decay of Ge-62. Eight new y lines have been added to the deexcitation of levels populated in the Ga-62 daughter.
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Morales, A. I., & Tuzon, P. (2022). Misconceptions, Knowledge, and Attitudes Towards the Phenomenon of Radioactivity. Sci. Educ., 31, 405–426.
Abstract: The teaching of the phenomenon of radioactivity is considered a key ingredient in the path towards developing critical thinking skills in many secondary science education curricula. Despite being one of the basic concepts in general physics courses, the scientific teaching literature of the last 40 years reports a great deal of misconceptions and conceptual errors related to radioactivity that seemingly appear regardless of the educational level and context. This study reports the first cross-sectional diagnostic study in Spain to secondary education students and pre-service teachers. Data were collected in the year 2019 through a questionnaire adapted from a previously validated one to explore the main misconceptions, attitudes, and knowledge status on the topic on a sample of 191 secondary school students and 29 Physics-and-Chemistry trainee teachers in the Spanish region of Valencia. Open and closed questions were used to categorize the entity itself, its properties, and the main misconceptions related to radioactivity. The responses were analysed using conventional statistical methods. The results indicate an evolution from a widespread dissenting notion on the phenomenon, which is staunchly related to danger, hazard, and destruction in the lowest educational levels, towards a more rational, relative, and multidimensional perspective in the highest ones. On the other hand, the ideas, emotions, and attitudes of the inquired individuals are in good agreement with the main misconceptions reported in the literature.
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Morales, A. I., Algora, A., Molina, F., & Rubio, B. (2014). Half-Life Systematics across the N=126 Shell Closure: Role of First-Forbidden Transitions in the beta Decay of Heavy Neutron-Rich Nuclei. Phys. Rev. Lett., 113(2), 022702–5pp.
Abstract: This Letter reports on a systematic study of beta-decay half-lives of neutron-rich nuclei around doubly magic Pb-208. The lifetimes of the 126-neutron shell isotone Pt-204 and the neighboring Ir200-202, Pt-203, Au-204 are presented together with other 19 half-lives measured during the “stopped beam” campaign of the rare isotope investigations at GSI collaboration. The results constrain the main nuclear theories used in calculations of r-process nucleosynthesis. Predictions based on a statistical macroscopic description of the first-forbidden beta strength reveal significant deviations for most of the nuclei with N < 126. In contrast, theories including a fully microscopic treatment of allowed and first-forbidden transitions reproduce more satisfactorily the trend in the measured half-lives for the nuclei in this region, where the r-process pathway passes through during beta decay back to stability.
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Morales, A. I. et al, Gadea, A., & Algora, A. (2014). beta-decay studies of neutron-rich Tl, Pb, and Bi isotopes. Phys. Rev. C, 89(1), 014324–13pp.
Abstract: The fragmentation of relativistic uranium projectiles has been exploited at the Gesellschaft fur Schwerionenforschung laboratory to investigate the beta decay of neutron-rich nuclei just beyond Pb-208. This paper reports on beta-delayed gamma decays of Tl211-213, Pb-215, and Bi215-219 de-exciting states in the daughters Pb211-213, Bi-215, and Po215-219. The resulting partial level schemes, proposed with the help of systematics and shell-model calculations, are presented. The role of allowed Gamow-Teller and first-forbidden beta transitions in this mass region is discussed.
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Morales, A. I. et al, Algora, A., Rubio, B., Orrigo, S. E. A., Agramunt, J., Gelletly, W., et al. (2017). Simultaneous investigation of the T=1(J(pi)=0(+)) and T=0(J(pi)=9(+)) beta decays in Br-70. Phys. Rev. C, 95(6), 064327–11pp.
Abstract: The beta decay of the odd-odd nucleus Br-70 has been investigated with the BigRIPS and EURICA setups at the Radioactive Ion Beam Factory (RIBF) of the RIKEN Nishina Center. The T = 0(J(pi) = 9(+)) and T = 1(J(pi) = 0(+)) isomers have both been produced in in-flight fragmentation of Kr-78 with ratios of 41.6(8)% and 58.4(8)%, respectively. A half-life of t(1/2) = 2157(-49)(+53) ms has been measured for the J pi = 9(+) isomer from gamma-ray time decay analysis. Based on this result, we provide a new value of the half-life for the J pi = 0(+) ground state of Br-70, t(1/2) = 78.42 +/- 0.51 ms, which is slightly more precise, and in excellent agreement, with the best measurement reported hitherto in the literature. For this decay, we provide the first estimate of the total branching fraction decaying through the 2(1)(+) state in the daughter nucleus Se-70, R(2(1)(+)) = 1.3 +/- 1.1%. We also report four new low-intensity gamma-ray transitions at 661, 1103, 1561, and 1749 keV following the beta decay of the J pi = 9(+) isomer. Based on their coincidence relationships, we tentatively propose two new excited states at 3945 and 4752 keV in 70Se with most probable spins and parities of J(pi) = (6(+)) and (8(+)), respectively. The observed structure is interpreted with the help of shell-model calculations, which predict a complex interplay between oblate and prolate configurations at low excitation energies.
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Morales, A. I. et al, Algora, A., Molina, F., & Rubio, B. (2013). beta-delayed gamma-ray spectroscopy of Au-203,Au-204 and Pt200-202. Phys. Rev. C, 88(1), 014319–12pp.
Abstract: The beta decay of five heavy, neutron-rich nuclei, Pt-203,Pt-204 and Ir200-202, has been investigated following relativistic cold fragmentation reactions of lead projectiles using the FRS + RISING setup at GSI. This paper reports on the study of the low-lying states in the decay daughter nuclei Au-203,Au-204 and Pt200-202. The characteristic gamma rays for each nucleus have been determined using beta-delayed gamma-ray spectroscopy. Tentative level schemes, relative intensities, and apparent beta feedings are provided. These data are compared with shell-model calculations, which indicate a substantial contribution to the total beta strength from high-energy first-forbidden beta-decay transitions in this mass region.
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Morales, A. I. et al, Agramunt, J., Algora, A., Gadea, A., Molina, F., & Rubio, B. (2011). Synthesis of N=127 isotones through (p,n) charge-exchange reactions induced by relativistic (208)Pb projectiles. Phys. Rev. C, 84(1), 011601–5pp.
Abstract: The production cross sections of four N = 127 isotones ((207)Hg, (206)Au, (205)Pt, and (204)Ir) have been measured using (p,n) charge-exchange reactions, induced in collisions of a (208)Pb primary beam at 1 A GeV with a Be target. These data allow one to investigate the use of a reaction mechanism to extend the limits of the chart of nuclides toward the important r-process nuclei in the region of the third peak of elemental abundance distribution.
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Morales, A. I. et al. (2017). Type II shell evolution in A=70 isobars from the N >= 40 island of inversion. Phys. Lett. B, 765, 328–333.
Abstract: The level structures of Co-70 and Ni-70, populated from the Chi decay of Fe-70, have been investigated using beta-delayed gamma-ray spectroscopy following in-flight fission of a U-238 beam. The experimental results are compared to Monte-Carlo Shell-Model calculations including the pf + g(9/2) + d(5/2) orbitals. The strong population of a (1(+)) state at 274 keV in Co-70 is at variance with the expected excitation energy of 1 MeV from near spherical single-particle estimates. This observation indicates a dominance of prolate deformed intruder configurations in the low-lying levels, which coexist with the normal near spherical states. It is shown that the 13 decay of the neutron-rich A = 70 isobars from the new island of inversion to the Z = 28 closed-shell regime progresses in accordance with a newly reported type of shell evolution, the so-called Type II, which involves many particle-hole excitations across energy gaps.
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Morales, A. I. et al. (2018). Is seniority a partial dynamic symmetry in the first νg(9/2) shell? Phys. Lett. B, 781, 706–712.
Abstract: The low-lying structures of the midshell vg(9/2) Ni isotopes Ni-72 and Ni-74 have been investigated at the RIBF facility in RIKEN within the EURICA collaboration. Previously unobserved low-lying states were accessed for the first time following beta decay of the mother nuclei Co-72 and Co-74. As a result, we provide a complete picture in terms of the seniority scheme up to the first (8(+)) levels for both nuclei. The experimental results are compared to shell-model calculations in order to define to what extent the seniority quantum number is preserved in the first neutron g(9/2) shell. We find that the disappearance of the seniority isomerism in the (8(1)(+)) states can be explained by a lowering of the seniority-four (6(+)) levels as predicted years ago. For Ni-74, the internal de-excitation pattern of the newly observed (6(2)(+)) state supports a restoration of the normal seniority ordering up to spin J = 4. This property, unexplained by the shell-model calculations, is in agreement with a dominance of the single-particle spherical regime near Ni-78.
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