Yokoyama, R. et al, Tain, J. L., Algora, A., Agramunt, J., Domingo-Pardo, C., Morales, A. I., et al. (2019). Strong one-neutron emission from two-neutron unbound states in beta decays of the r-process nuclei Ga-86,Ga-87. Phys. Rev. C, 100(3), 031302–6pp.
Abstract: beta-delayed one-neutron and two-neutron branching ratios (P-1n and P-2n) have been measured in the decay of A = 84 to 87 Ga isotopes at the Radioactive-Isotope Beam Factory (RIBF) at the RIKEN Nishina Center using a high-efficiency array of He-3 neutron counters (BRIKEN). Two-neutron emission was observed in the decay of Ga-84,Ga-85,Ga-87 for the first time and the branching ratios were measured to be P-2n = 1.6(2)%, 1.3(2)%, and 10.2(28)(stat)(5)(sys)%, respectively. One-neutron branching ratio of Ga-87 (P-1n = 81(9)(stat)(8)(sys)%) and half-life of 29(4) ms were measured for the first time. The branching ratios of Ga-86 were also measured to be P-1n = 74(2)(stat)(8)(sys)% and 16.2(9)(stat)(6)(sys)% with better precision than a previous study. The observation that P-1n > P-2n for both Ga-86,Ga-87 was unexpected and is interpreted as a signature of dominating one-neutron emission from the two-neutron unbound excited states in Ge-86,Ge-87. In order to interpret the experimental results, shell-model and Hauser-Feshbach statistical model calculations of delayed particle and gamma-ray emission probabilities were performed. This model framework reproduces the experimental results. The shell model alone predicts P-2n significantly larger than P-1n for the Ga-87 decay, and it is necessary to invoke a statistical description to successfully explain the observation that P-1n > P-2n. Our new results demonstrate the relevance and importance of a statistical description of neutron emission for the prediction of the decay properties of multineutron emitters and that it must be included in the r-process modeling.
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Yokoyama, R. et al, Tain, J. L., Algora, A., Agramunt, J., Domingo-Pardo, C., Morales, A. I., et al. (2023). β-delayed neutron emissions from N > 50 gallium isotopes. Phys. Rev. C, 108(6), 064307–15pp.
Abstract: beta-delayed gamma-neutron spectroscopy has been performed on the decay of A=84 to 87 gallium isotopes at the RI-beam Factory at the RIKEN Nishina Center using a high-efficiency array of 3He neutron counters (BRIKEN). beta-2n-gamma events were measured in the decays of all of the four isotopes for the first time, which is direct evidence for populating the excited states of two-neutron daughter nuclei. Detailed decay schemes with the gamma branching ratios were obtained for these isotopes, and the neutron emission probabilities (P-xn) were updated from the previous study. Hauser-Feshbach statistical model calculations were performed to understand the experimental branching ratios. We found that the P-1n and P-2n values are sensitive to the nuclear level densities of 1n daughter nuclei and showed that the statistical model reproduced the P-2n/P-1n ratio better when experimental levels plus shell-model level densities fit by the Gilbert-Cameron formula were used as the level-density input. We also showed the neutron and gamma branching ratios are sensitive to the ground-state spin of the parent nucleus. Our statistical model analysis suggested J <= 3 for the unknown ground-state spin of the odd-odd nucleus Ga-86, from the I gamma(4(+)-> 2(+))/I-gamma(2(+)-> 0(+)) ratio of Ga-84 and the P-2n/P-1n ratio. These results show the necessity of detailed understanding of the decay scheme, including data from neutron spectroscopy, in addition to gamma measurements of the multineutron emitters.
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Wimmer, K. et al, Algora, A., & Rubio, B. (2018). Shape coexistence and isospin symmetry in A=70 nuclei: Spectroscopy of the T-z =-1 nucleus Kr-70. Phys. Lett. B, 785, 441–446.
Abstract: Excited states in the T-z = -1 nucleus Kr-70 have been populated using inelastic scattering of a radioactive Kr-70 beam as well as one- and two-neutron removal reactions from Kr-71,Kr-72 at intermediate beam energies. The level scheme of Kr-70 was constructed from the observed gamma-ray transitions and coincidences. Tentative spin and parity assignments were made based on comparison with the mirror nucleus Se-70. Asecond 2(+) state and a candidate for the corresponding 4(2)(+) state suggest shape coexistence in Kr-70.
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Wimmer, K. et al, Algora, A., & Rubio, B. (2019). Discovery of Br-68 in secondary reactions of radioactive beams. Phys. Lett. B, 795, 266–270.
Abstract: The proton-rich isotope Br-68 was discovered in secondary fragmentation reactions of fast radioactive beams. Proton-rich secondary beams of (70,71,72) Kr and Br-70, produced at the RIKEN Nishina Center and identified by the BigRIPS fragment separator, impinged on a secondary Be-9 target. Unambiguous particle identification behind the secondary target was achieved with the ZeroDegree spectrometer. Based on the expected direct production cross sections from neighboring isotopes, the lifetime of the ground or long-lived isomeric state of Br-68 was estimated. The results suggest that secondary fragmentation reactions, where relatively few nucleons are removed from the projectile, offer an alternative way to search for new isotopes, as these reactions populate preferentially low-lying states.
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Wimmer, K. et al, Algora, A., & Rubio, B. (2020). Shape coexistence revealed in the N = Z isotope Kr-72 through inelastic scattering. Eur. Phys. J. A, 56(6), 159–12pp.
Abstract: The N = Z = 36 nucleus Kr-72 has been studied by inelastic scattering at intermediate energies. Two targets, Be-9 and Au-197, were used to extract the nuclear deformation length, delta(N), and the reduced E2 transition probability, B(E2). The previously unknown non-yrast 2(+) and 4(+) states as well as a new candidate for the octupole 3(-) state have been observed in the scattering on the Be target and placed in the level scheme based on gamma – gamma coincidences. The second 2(+) state was also observed in the scattering on the Au target and the B(E2; 2(2)(+) -> 0(1)(+)) value could be determined for the first time. Analyzing the results in terms of a two-band mixing model shows clear evidence for a oblate-prolate shape coexistence and can be explained by a shape change from an oblate ground state to prolate deformed yrast band from the first 2+ state. This interpretation is corroborated by beyond mean field calculations using the Gogny D1S interaction.
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