Abstract: The population of isomeric states in the prompt decay of fission fragments-so-called isomeric yield ratios (IYRs)-is known to be sensitive to the angular momentum J that the fragment emerged with, and may therefore contain valuable information on the mechanism behind the fission process. In this work, we investigate how changes in the fissioning system impact the measured IYRs of fission fragments to learn more about what parameters affect angular momentum generation. To enable this, a new technique for measuring IYRs is first demonstrated. It is based on the time of arrival of discrete gamma rays, and has the advantage that it enables the study of the IYR as a function of properties of the partner nucleus. This technique is used to extract the IYR of 134Te, strongly populated in actinide fission, from the three different fissioning systems: 232Th(n, f), 238U(n, f), at two different neutron energies, as well as 252Cf(sf). The impacts of changing the fissioning system, the compound nuclear excitation energy, the minimum J of the binary partner, and the number of neutrons emitted on the IYR of 134Te are determined. The decay code TALYS is used in combination with the fission simulation code FREYA to calculate the primary fragment angular momentum from the IYR. We find that the IYR of 134Te has a slope of 0.004 +/- 0.002 with increase in compound nucleus (CN) mass. When investigating the impact on the IYR of increased CN excitation energy, we find no change with an energy increase similar to the difference between thermal and fast fission. By varying the mass of the partner fragment emerging with 134Te, it is revealed that the IYR of 134Te is independent of the total amount of prompt neutrons emitted from the fragment pair. This indicates that neutrons carry minimal angular momentum away from the fission fragments. Comparisons with the FREYA+TALYS simulations reveal that the average angular momentum in 134Te following 238U(n, f) is 6.0 h over bar . This is not consistent with the value deduced from recent CGMF calculations. Finally, the IYR sensitivity to the angular momentum of the primary fragment is discussed. These results are not only important to help understanding the underlying mechanism in nuclear fission, but can also be used to constrain and benchmark fission models, and are relevant to the gamma -ray heating problem of reactors.

Abstract: The beta decays of Nb-103,Nb-104m were studied with the Summing NaI(Tl) (SuN) detector at the National Superconducting Cyclotron Laboratory. The beta-decay feeding intensity distribution I-beta(E) for each isotope was extracted by measuring gamma rays in coincidence with an emitted electron. The I-beta(E) was extracted via the total absorption spectroscopy technique. The I-beta(E) for each nucleus was compared to predictions made by the quasiparticle random-phase approximation (QRPA) model which is commonly used to calculate beta-decay properties for astrophysical applications. The main goal was to provide experimental data for neutron-rich nuclei, relevant to the astrophysical r process. In addition, the extracted beta-decay feeding intensity distributions can lead to a better understanding of nuclear structure in a region of rapid structure changes around A = 100. Finally, experimental data for Nb-104m are also of interest to antineutrino studies of nuclear reactors.

Abstract: The structure of the neutron-rich bismuth isotope Bi-217 has been studied for the first time. The fragmentation of a primary U-238 beam at the FRS-RISING setup at GSI was exploited to perform gamma-decay spectroscopy, since μs isomeric states were expected in this nucleus. Gamma rays following the decay of a t(1/2) = 3 μs isomer were observed, allowing one to establish the low-lying structure of Bi-217. The level energies and the reduced electric quadrupole transition probability B(E2) from the isomeric state are compared to large-scale shell-model calculations.