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Author (up) n_TOF Collaboration (Mendoza, E. et al); Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A.
Title Measurement and analysis of the Am-241 neutron capture cross section at the n_TOF facility at CERN Type Journal Article
Year 2018 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 97 Issue 5 Pages 054616 - 21pp
Keywords
Abstract The Am-241(n, gamma) cross section has been measured at the nTOF facility at CERN with the nTOF BaF2 Total Absorption Calorimeter in the energy range between 0.2 eV and 10 keV. Our results are analyzed as resolved resonances up to 700 eV, allowing a more detailed description of the cross section than in the current evaluations, which contain resolved resonances only up to 150-160 eV. The cross section in the unresolved resonance region is perfectly consistent with the predictions based on the average resonance parameters deduced from the resolved resonances, thus obtaining a consistent description of the cross section in the full neutron energy range under study. Below 20 eV, our results are in reasonable agreement with JEFF-3.2 as well as with the most recent direct measurements of the resonance integral, and differ up to 20-30% with other experimental data. Between 20 eV and 1 keV, the disagreement with other experimental data and evaluations gradually decreases, in general, with the neutron energy. Above 1 keV, we find compatible results with previously existing values.
Address [Mendoza, E.; Cano-Ott, D.; Balibrea, J.; Becares, V; Garcia, A. R.; Gonzalez, E.; Lopez, D.; Martinez, T.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain, Email: emilio.mendoza@ciemat.es
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:000433032300001 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 3584
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Author (up) n_TOF Collaboration (Praena, J. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A.
Title Preparation and characterization of S-33 samples for S-33(n,alpha)Si-30 cross-section measurements at the n_TOF facility at CERN Type Journal Article
Year 2018 Publication Nuclear Instruments & Methods in Physics Research A Abbreviated Journal Nucl. Instrum. Methods Phys. Res. A
Volume 890 Issue Pages 142-147
Keywords Neutron induced alpha emission; Thermal evaporation; Rutherford backscattering
Abstract Thin S-33 samples for the study of the S-33(n,alpha)Si-30 cross-section at the n_TOF facility at CERN were made by thermal evaporation of S-33 powder onto a dedicated substrate made of kapton covered with thin layers of copper, chromium and titanium. This method has provided for the first time bare sulfur samples a few centimeters in diameter. The samples have shown an excellent adherence with no mass loss after few years and no sublimation in vacuum at room temperature. The determination of the mass thickness of S-33 has been performed by means of Rutherford backscattering spectrometry. The samples have been successfully tested under neutron irradiation.
Address [Praena, J.; Porras, I.] Univ Granada, Granada, Spain, Email: jpraena@ugr.es
Corporate Author Thesis
Publisher Elsevier Science Bv Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0168-9002 ISBN Medium
Area Expedition Conference
Notes WOS:000427814900020 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 3537
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Author (up) n_TOF Collaboration (Praena, J. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A.
Title Measurement and resonance analysis of the S-33(n,alpha)Si-30 cross section at the CERN n_TOF facility in the energy region from 10 to 300 keV Type Journal Article
Year 2018 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 97 Issue 6 Pages 064603 - 10pp
Keywords
Abstract The (33)(n , alpha)Si-30 cross section has been measured at the neutron time-of-flight (n_TOF) facility at CERN in the neutron energy range from 10 to 300 keV relative to the B-10(n, alpha)(7) Li cross-section standard. Both reactions were measured simultaneously with a set of micromegas detectors. The flight path of 185 m has allowed us to obtain the cross section with high-energy resolution. An accurate description of the resonances has been performed by means of the multilevel multichannel R-matrix code SAMMY. The results show a significantly higher area of the biggest resonance (13.45 keV) than the unique high-resolution (n , alpha) measurement. The new parametrization of the 13.45-keV resonance is similar to that of the unique transmission measurement. This resonance is a matter of research in neutron-capture therapy. The S-33(n, alpha)Si-30 cross section has been studied in previous works because of its role in the production of S-36 in stars, which is currently overproduced in stellar models compared to observations.
Address [Praena, J.; Porras, I] Univ Granada, Granada, Spain, Email: jpraena@ugr.es
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:000434017300004 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 3597
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Author (up) n_TOF Collaboration (Sabate-Gilarte et al.); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A.
Title High-accuracy determination of the neutron flux in the new experimental area n_TOF-EAR2 at CERNx Type Journal Article
Year 2017 Publication European Physical Journal A Abbreviated Journal Eur. Phys. J. A
Volume 53 Issue 10 Pages 210 - 13pp
Keywords
Abstract A new high flux experimental area has recently become operational at the nTOF facility at CERN. This new measuring station, nTOF-EAR2, is placed at the end of a vertical beam line at a distance of approximately 20m from the spallation target. The characterization of the neutron beam, in terms of flux, spatial profile and resolution function, is of crucial importance for the feasibility study and data analysis of all measurements to be performed in the new area. In this paper, the measurement of the neutron flux, performed with different solid-state and gaseous detection systems, and using three neutronconverting reactions considered standard in different energy regions is reported. The results of the various measurements have been combined, yielding an evaluated neutron energy distribution in a wide energy range, from 2meV to 100MeV, with an accuracy ranging from 2%, at low energy, to 6% in the high-energy region. In addition, an absolute normalization of the n_TOF-EAR2 neutron flux has been obtained by means of an activation measurement performed with 197 Au foils in the beam.
Address [Sabate-Gilarte, M.; Vlachoudis, V.; Aberle, O.; Bacak, M.; Brugger, M.; Calviani, M.; Cardella, R.; Cerutti, F.; Chiaveri, E.; Ferrari, A.; Hernandez-Prieto, A.; Kadi, Y.; Losito, R.; Macina, D.; Mingrone, F.; Montesano, S.; Rubbia, C.; Weiss, C.] CERN, European Org Nucl Res, Geneva, Switzerland, Email: massimo.barbagallo@ba.infn.it
Corporate Author Thesis
Publisher Springer Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 1434-6001 ISBN Medium
Area Expedition Conference
Notes WOS:000413766400002 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 3350
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Author (up) n_TOF Collaboration (Stamatopoulos, A. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A.
Title Investigation of the Pu-240(n, f) reaction at the n_TOF/EAR2 facility in the 9 meV-6 MeV range Type Journal Article
Year 2020 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 102 Issue 1 Pages 014616 - 23pp
Keywords
Abstract Background: Nuclear waste management is considered amongst the major challenges in the field of nuclear energy. A possible means of addressing this issue is waste transmutation in advanced nuclear systems, whose operation requires a fast neutron spectrum. In this regard, the accurate knowledge of neutron-induced reaction cross sections of several (minor) actinide isotopes is essential for design optimization and improvement of safety margins of such systems. One such case is Pu-240, due to its accumulation in spent nuclear fuel of thermal reactors and its usage in fast reactor fuel. The measurement of the Pu-240(n, f) cross section was previously attempted at the CERN nTOF facility EAR1 measuring station using the time-of-flight technique. Due to the low amount of available material and the given flux at EAR1, the measurement had to last several months to achieve a sufficient statistical accuracy. This long duration led to detector deterioration due to the prolonged exposure to the high alpha activity of the fission foils, therefore the measurement could not be successfully completed. Purpose: It is aimed to determine whether it is feasible to study neutron-induced fission at nTOF/EAR2 and provide data on the Pu-240(n, f) reaction in energy regions requested for applications. Methods: The study of the Pu-240(n, f) reaction was made at a new experimental area (EAR2) with a shorter flight path which delivered on average 30 times higher flux at fast neutron energies. This enabled the measurement to be performed much faster, thus limiting the exposure of the detectors to the intrinsic activity of the fission foils. The experimental setup was based on microbulk Micromegas detectors and the time-of-flight data were analyzed with an optimized pulse-shape analysis algorithm. Special attention was dedicated to the estimation of the non-negligible counting loss corrections with the development of a new methodology, and other corrections were estimated via Monte Carlo simulations of the experimental setup. Results: This new measurement of the Pu-240(n, f) cross section yielded data from 9 meV up to 6 MeV incident neutron energy and fission resonance kernels were extracted up to 10 keV. Conclusions: Neutron-induced fission of high activity samples can be successfully studied at the n_TOF/EAR2 facility at CERN covering a wide range of neutron energies, from thermal to a few MeV.
Address [Stamatopoulos, A.; Tsinganis, A.; Kokkoris, M.; Vlastou, R.; Diakaki, M.] Natl Tech Univ Athens, Athens, Greece, Email: athanasios.stamatopoulos@cern.ch
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0556-2813 ISBN Medium
Area Expedition Conference
Notes WOS:000551057500002 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 4466
Permanent link to this record