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n_TOF Collaboration(Zugec, P. et al), Domingo-Pardo, C., Giubrone, G., & Tain, J. L. (2014). GEANT4 simulation of the neutron background of the C6D6 set-up for capture studies at n_TOF. Nucl. Instrum. Methods Phys. Res. A, 760, 57–67.
Abstract: The neutron sensitivity of the Cr6D6 detector setup used at nTOF facility for capture measurements has been studied by means of detailed GEANT4 simulations. A realistic software replica of the entire nTOF experimental hall, including the neutron beam line, sample, detector supports and the walls of the experimental area has been implemented in the simulations. The simulations have been analyzed in the same manner as experimental data, in particular by applying the Pulse Height Weighting Technique. The simulations have been validated against a measurement of the neutron background performed with a(nat)-C sample, showing an excellent agreement above 1 keV. At lower energies, an additional component in the measured C-nat yield has been discovered, which prevents the use of C-nat data for neutron background estimates at neutron energies below a few hundred eV. The origin and time structure of the neutron background have been derived from the simulations. Examples of the neutron background for two different samples are demonstrating the important role of accurate simulations of the neutron background in capture cross-section measurements.
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n_TOF Collaboration(Zugec, P. et al), Domingo-Pardo, C., Giubrone, G., & Tain, J. L. (2014). Experimental neutron capture data of Ni-58 from the CERN n_TOF facility. Phys. Rev. C, 89(1), 014605–9pp.
Abstract: The Ni-58(n,gamma) cross section has been measured at the neutron time of flight facility n_TOF at CERN, in the energy range from 27 meV up to 400 keV. In total, 51 resonances have been analyzed up to 122 keV. Maxwellian averaged cross sections (MACS) have been calculated for stellar temperatures of kT = 5-100 keV with uncertainties of less than 6%, showing fair agreement with recent experimental and evaluated data up to kT = 50 keV. The MACS extracted in the present work at 30 keV is 34.2 +/- 0.6(stat) +/- 1.8(sys) mb, in agreement with latest results and evaluations, but 12% lower relative to the recent KADoNIS compilation of astrophysical cross sections. When included in models of the s-process nucleosynthesis in massive stars, this change results in a 60% increase of the abundance of Ni-58, with a negligible propagation on heavier isotopes. The reason is that, using both the old or the new MACS, Ni-58 is efficiently depleted by neutron captures.
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n_TOF Collaboration(Zugec, P. et al), Domingo-Pardo, C., Giubrone, G., & Tain, J. L. (2014). Measurement of the C-12(n, p)B-12 cross section at n_TOF at CERN by in-beam activation analysis. Phys. Rev. C, 90(2), 021601–5pp.
Abstract: The integral cross section of the C-12(n, p)B-12 reaction has been determined for the first time in the neutron energy range from threshold to several GeV at the n_TOF facility at CERN. The measurement relies on the activation technique with the beta decay of B-12 measured over a period of four half-lives within the same neutron bunch in which the reaction occurs. The results indicate that model predictions, used in a variety of applications, are mostly inadequate. The value of the integral cross section reported here can be used as a benchmark for verifying or tuning model calculations.
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n_TOF Collaboration, Gunsing, F., Berthoumieux, E., Borella, A., Belgya, T., Szentmiklosi, L., et al. (2011). Neutron Capture on (209)Bi: Determination of the Production Ratio of (210m)Bi/(210g)Bi. J. Korean Phys. Soc., 59(2), 1670–1675.
Abstract: Neutron capture on (209)Bi produces either an isomeric state (210m)Bi with a half life of 3 x 106 years, or the ground state (210g)Bi which decays with a half life of 5 days to the alpha emitter (210)Po. Therefore the neutron capture cross section ratio (209)Bi(n,gamma)(210m)Bi/(210g)Bi plays an important role in predicting the short- and long-term radio-toxicity produced by (209)Bi under neutron irradiation. This ratio is dependent on the neutron energy. We have measured this ratio for cold neutrons at the cold neutron beam facility of the Budapest Neutron Centre by observing the population of the ground-and the metastable state using high resolution gamma-ray spectroscopy. The same technique has been used at the pulsed white neutron source GELINA of the IRMM, Geel in combination with the neutron time-of-flight technique. Results for the neutron-energy dependent branching ratio will be presented. In addition we performed simulations using a statistical decay code.
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Olleros, P., Caballero, L., Domingo-Pardo, C., Babiano, V., Ladarescu, I., Calvo, D., et al. (2018). On the performance of large monolithic LaCl3(Ce) crystals coupled to pixelated silicon photosensors. J. Instrum., 13, P03014–17pp.
Abstract: We investigate the performance of large area radiation detectors, with high energy-and spatial-resolution, intended for the development of a Total Energy Detector with gamma-ray imaging capability, so-called i-TED. This new development aims for an enhancement in detection sensitivity in time-of-flight neutron capture measurements, versus the commonly used C6D6 liquid scintillation total-energy detectors. In this work, we study in detail the impact of the readout photosensor on the energy response of large area (50 x 50 mm(2)) monolithic LaCl3(Ce) crystals, in particular when replacing a conventional mono-cathode photomultiplier tube by an 8 x 8 pixelated silicon photomultiplier. Using the largest commercially available monolithic SiPM array (25 cm(2)), with a pixel size of 6 x 6 mm(2), we have measured an average energy resolution of 3.92% FWHM at 662 keV for crystal thick-nesses of 10, 20 and 30 mm. The results are confronted with detailed Monte Carlo (MC) calculations, where optical processes and properties have been included for the reliable tracking of the scintillation photons. After the experimental validation of the MC model, we use our MC code to explore the impact of a smaller photosensor segmentation on the energy resolution. Our optical MC simulations predict only a marginal deterioration of the spectroscopic performance for pixels of 3 x 3 mm(2).
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Orrigo, S. E. A., Tain, J. L., Mont-Geli, N., Tarifeño-Saldivia, A., Fraile, L. M., Grieger, M., et al. (2022). Long-term evolution of the neutron rate at the Canfranc Underground Laboratory. Eur. Phys. J. C, 82(9), 814–11pp.
Abstract: We report results on the long-term variation of the neutron counting rate at the Canfranc Underground Laboratory, of importance for several low-background experiments installed there, including rare-event searches. The measurement campaign was performed employing the High Efficiency Neutron Spectrometry Array (HENSA) mounted in Hall A and lasted 412 live days. The present study is the first long-term measurement of the neutron rate with sensitivity over a wide range of neutron energies (from thermal up to 0.1 GeV and beyond) performed in any underground laboratory so far. Data on the environmental variables inside the experimental hall (radon concentration, air temperature, air pressure and humidity) were also acquired during all the measurement campaign. We have investigated for the first time the evolution of the neutron rate for different energies of the neutrons and its correlation with the ambient variables.
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Perez-Cerdan, A. B., Rubio, B., Gelletly, W., Algora, A., Agramunt, J., Nacher, E., et al. (2013). Deformation of Sr and Rb isotopes close to the N = Z line via beta-decay studies using the total absorption technique. Phys. Rev. C, 88(1), 014324–15pp.
Abstract: A study of the Gamow-Teller strength distributions B(GT) in the beta decay of Sr-78 and Rb-76,Rb-78 has been made using a total absorption spectrometer (TAS). Following the success in deducing the sign of the deformation for Sr-76, a similar approach is adopted for Sr-78 based on a comparison of the measured B(GT) with quasiparticle random-phase approximation calculations. This work confirms its previously expected prolate deformation in the ground state. Conclusions about the structure of the odd-odd Rb-76,Rb-78 isotopes have been drawn based on their measured B(GT) distributions.
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Phong, V. H. et al, Agramunt, J., Algora, A., Domingo-Pardo, C., Morales, A. I., Rubio, B., et al. (2022). Beta-Delayed One and Two Neutron Emission Probabilities South-East of Sn-132 and the Odd-Even Systematics in r-Process Nuclide Abundances. Phys. Rev. Lett., 129(18), 172701–7pp.
Abstract: The beta-delayed one- and two-neutron emission probabilities (P-1n and P-2n) of 20 neutron-rich nuclei with N >= 82 have been measured at the RIBF facility of the RIKEN Nishina Center. P-1n of Ag-130;131, Cd-133;134, In-135;136, and (138;13)9Sn were determined for the first time, and stringent upper limits were placed on P-2n for nearly all cases. beta-delayed two-neutron emission (beta 2n) was unambiguously identified in Cd-133 and In-135;136, and their P-2n were measured. Weak beta 2n was also detected from Sn-137;138. Our results highlight the effect of the N = 82 and Z = 50 shell closures on beta-delayed neutron emission probability and provide stringent benchmarks for newly developed macroscopic-microscopic and self-consistent global models with the inclusion of a statistical treatment of neutron and. emission. The impact of our measurements on r-process nucleosynthesis was studied in a neutron star merger scenario. Our P-1n and P-2n have a direct impact on the
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Phong, V. H. et al, Agramunt, J., Algora, A., Domingo-Pardo, C., Morales, A. I., Tain, J. L., et al. (2019). Observation of a μs isomer in In-134(49)85: Proton-neutron coupling “southeast” of Sn-132(50)82. Phys. Rev. C, 100(1), 011302–6pp.
Abstract: We report on the observation of a microsecond isomeric state in the single-proton-hole, three-neutron-particle nucleus In-134. The nuclei of interest were produced by in-flight fission of a U-238 beam at the Radioactive Isotope Beam Factory at RIKEN. The isomer depopulates through a gamma ray of energy 56.7(1) keV and with a half-life of T-1/2 = 3.5(4) μs. Based on the comparison with shell-model calculations, we interpret the isomer as the I-pi = 5(-) member of the pi 0g(9/2)(-1) circle times nu 1f(7/2)(3) multiplet, decaying to the I-pi = 7(-) ground state with a reduced-transition probability of B(E2; 5(-) -> 7(-)) = 0.53(6) W.u. Observation of this isomer, and lack of evidence in the current work for a I-pi = 5(-) isomer decay in In-132, provides a benchmark of the proton-neutron interaction in the region of the nuclear chart “southeast” of Sn-132, where experimental information on excited states is sparse.
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Rasco, B. C., Brewer, N. T., Yokoyama, R., Grzywacz, R., Rykaczewski, K. P., Tolosa-Delgado, A., et al. (2018). The ORNL analysis technique for extracting beta-delayed multi-neutron branching ratios with BRIKEN. Nucl. Instrum. Methods Phys. Res. A, 911, 79–86.
Abstract: Many choices are available in order to evaluate large radioactive decay networks. There are many parameters that influence the calculated beta-decay delayed single and multi-neutron emission branching fractions. We describe assumptions about the decay model, background, and other parameters and their influence on beta-decay delayed multi-neutron emission analysis. An analysis technique, the ORNL BRIKEN analysis procedure, for determining beta-delayed multi-neutron branching ratios in beta-neutron precursors produced by means of heavy-ion fragmentation is presented. The technique is based on estimating the initial activities of zero, one, and two neutrons occurring in coincidence with an ion-implant and beta trigger. The technique allows one to extract beta-delayed multi-neutron decay branching ratios measured with the He-3 BRIKEN neutron counter. As an example, two analyses of the beta-neutron emitter Cu-77 based on different a priori assumptions are presented along with comparisons to literature values.
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