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n_TOF Collaboration(Tagliente, G. et al), Domingo-Pardo, C., Giubrone, G., Tain, J. L., & Tarifeño-Saldivia, A. (2022). Zr-92(n, gamma) and (n,tot) measurements at the GELINA and n_TOF facilities. Phys. Rev. C, 105(2), 025805–14pp.
Abstract: Background: Stellar nucleosynthesis of elements heavier than iron is driven by neutron capture processes. Zr-92 is positioned at a strategic point along the slow nucleosynthesis path, given its proximity to the neutron magic number N = 50 and its position at the matching region between the weak and main slow processes. Purpose: In parallel with recent improved astronomical data, the extraction of accurate Maxwellian averaged cross sections (MACSs) derived from a more complete and accurate set of resonance parameters should allow for a better understanding of the stellar conditions at which nucleosynthesis takes place. Methods: Transmission and capture cross section measurements using enriched Zr-92 metallic samples were performed at the time-of flight facilities GELINA of JRC-Geel (BE) and nTOF of CERN (CH). The neutron beam passing through the samples was investigated in transmission measurements at GELINA using a Li-glass scintillator. The gamma rays emitted during the neutron capture reactions were detected by C6D6 detectors at both GELINA and nTOF. Results: Resonance parameters of individual resonances up to 81 keV were extracted from a combined resonance shape analysis of experimental transmissions and capture yields. For the majority of the resonances the parity was determined from an analysis of the transmission data obtained with different sample thicknesses. Average resonance parameters were calculated. Conclusions: Maxwellian averaged cross sections were extracted from resonances observed up to 81 keV. The MACS for kT = 30 keV is fully consistent with experimental data reported in the literature. The MACSs for kT less than or similar to 15 keV are in good agreement with those derived from the ENDF/B-VIII.0 library and recommended in the KADoNTS database. For kT higher than 30 keV differences are observed. A comparison with MACSs obtained with the cross sections recommended in the JEFF-3.3 and JENDL-4.0 libraries shows discrepancies even for kT less than or similar to 15 keV.
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n_TOF Collaboration(Tagliente, G. et al.), Domingo-Pardo, C., & Tain, J. L. (2010). The Zr-92(n,gamma) reaction and its implications for stellar nucleosynthesis. Phys. Rev. C, 81(5), 055801–9pp.
Abstract: Because the relatively small neutron capture cross sections of the zirconium isotopes are difficult to measure, the results of previous measurements are often not adequate for a number of problems in astrophysics and nuclear technology. Therefore, the Zr-92(n,gamma) cross section has been remeasured at the CERN n_TOF facility, providing a set of improved parameters for 44 resonances in the neutron energy range up to 40 keV. With this information the cross-section uncertainties in the keV region could be reduced to 5% as required for s-process nucleosynthesis studies and technological applications.
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n_TOF Collaboration(Tagliente, G. et al.), Domingo-Pardo, C., & Tain, J. L. (2013). The Zr-93(n, gamma) reaction up to 8 keV neutron energy. Phys. Rev. C, 87(1), 014622–7pp.
Abstract: The (n, gamma) reaction of the radioactive isotope Zr-93 has been measured at the n_TOF high-resolution time-of-flight facility at CERN. Resonance parameters have been extracted in the neutron energy range up to 8 keV, yielding capture widths smaller (14%) than reported in an earlier experiment. These results are important for detailed nucleosynthesis calculations and for refined studies of waste transmutation concepts. DOI: 10.1103/PhysRevC.87.014622
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n_TOF Collaboration(Tagliente, G. et al.), Domingo-Pardo, C., & Tain, J. L. (2011). Neutron capture on (94)Zr: Resonance parameters and Maxwellian-averaged cross sections. Phys. Rev. C, 84(1), 015801–9pp.
Abstract: The neutron capture cross sections of the Zr isotopes play an important role in nucleosynthesis studies. The s-process reaction flow between the Fe seed and the heavier isotopes passes through the neutron magic nucleus (90)Zr and through (91,92,93,94)Zr, but only part of the flow extends to (96)Zr because of the branching point at (95)Zr. Apart from their effect on the s-process flow, the comparably small isotopic (n, gamma) cross sections make Zr also an interesting structural material for nuclear reactors. The (94)Zr (n, gamma) cross section has been measured with high resolution at the spallation neutron source n_TOF at CERN and resonance parameters are reported up to 60 keV neutron energy.
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n_TOF Collaboration(Tagliente, G. et al.), Domingo-Pardo, C., & Tain, J. L. (2011). (96)Zr(n,gamma) measurement at the n_TOF facility at CERN. Phys. Rev. C, 84(5), 055802–8pp.
Abstract: The (n,gamma) cross section of (96)Zr has been investigated at the CERN n_TOF spallation neutron source. High-resolution time-of-flight measurements using an enriched ZrO(2) sample allowed us to analyze 15 resonances below 40 keV with improved accuracy. On average, the capture widths were found to be 25% smaller than reported in earlier experiments. If complemented with the contribution by direct radiative capture, the derived Maxwellian averaged cross sections are consistent with activation data at kT = 25 keV. The present results confirm the astrophysical implications for the s-process branching at (95)Zr.
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