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Azevedo, C. D. R., Baeza, A., Chauveau, E., Corbacho, J. A., Diaz, J., Domange, J., et al. (2023). Development of a real-time tritium-in-water monitor. J. Instrum., 18(12), T12008–14pp.
Abstract: In this paper, we report the development and performance of a detector module envisaging a tritium-in-water real-time activity monitor. The monitor is based on modular detection units whose number can be chosen according to the required sensitivity. The full system is being designed to achieve a Minimum Detectable Activity (MDA) of 100 Bq/L of tritium-in-water activity which is the limit established by the E.U. Council Directive 2013/51/Euratom for water intended for human consumption. The same system can be used as a real-time pre-alert system for nuclear power plant regarding tritium-in water environmental surveillance. The first detector module was characterized, commissioned and installed immediately after the discharge channel of the Arrocampo dam (Almaraz nuclear power plant, Spain) on the Tagus river. Due to the high sensitivity of the single detection modules, the system requires radioactive background mitigation techniques through the use of active and passive shielding. We have extrapolated a MDA of 3.6 kBq/L for a single module being this value limited by the cosmic background. The obtained value for a single module is already compatible with a real-time environmental surveillance and pre-alert system. Further optimization of the single-module sensitivity will imply the reduction of the number of modules and the cost of the detector system.
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Azevedo, C. D. R., Baeza, A., Chauveau, E., Corbacho, J. A., Diaz, J., Domange, J., et al. (2023). Design, setup and routine operation of a water treatment system for the monitoring of low activities of tritium in water. Nucl. Eng. Technol., 55(7), 2349–2355.
Abstract: In the TRITIUM project, an on-site monitoring system is being developed to measure tritium (3H) levels in water near nuclear power plants. The quite low-energy betas emitted by 3H have a very short average path in water (5 mm as shown by simulations for 18 keV electrons). This path would be further reduced by impurities present in the water, resulting in a significant reduction of the detection efficiency. Therefore, one of the essential requirements of the project is the elimination of these impurities through a filtration process and the removal of salts in solution. This paper describes a water treatment system developed for the project that meets the following requirements: the water produced should be of nearpure water quality according to ISO 3696 grade 3 standard (conductivity < 10 mS/cm); the system should operate autonomously and be remotely monitored.
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Azevedo, C. D. R., Baeza, A., Chauveau, E., Corbacho, J. A., Diaz, J., Domange, J., et al. (2020). Simulation results of a real-time in water tritium monitor. Nucl. Instrum. Methods Phys. Res. A, 982, 164555–7pp.
Abstract: In this work we present simulation results for a modular tritium in-water real-time monitor. The system allows for scalability in order to achieve the required sensitivity. The modules are composed by 340 uncladed scintillating fibers immersed in water and 2 photosensors in coincidence for light readout. Light yield and Birks' coefficient uncertainties for low energy beta particles is discussed. A study of the detection efficiency according to the fiber length is presented. Discussion on the system requirements and background mitigation for a device with sensitivity of 100 Bq/L, required to comply with the European directive 2013/51/Euratom, is presented. Due to the low energetic beta emission from tritium a detection efficiency close to 3.3% was calculated for a single 2 mm round fiber.
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