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Hall, O. et al, Agramunt, J., Algora, A., Domingo-Pardo, C., Morales, A. I., Rubio, B., et al. (2021). beta-delayed neutron emission of r-process nuclei at the N=82 shell closure. Phys. Lett. B, 816, 136266–7pp.
Abstract: Theoretical models of beta-delayed neutron emission are used as crucial inputs in r-process calculations. Benchmarking the predictions of these models is a challenge due to a lack of currently available experimental data. In this work the beta-delayed neutron emission probabilities of 33 nuclides in the important mass regions south and south-west of Sn-132 are presented, 16 for the first time. The measurements were performed at RIKEN using the Advanced Implantation Detector Array (AIDA) and the BRIKEN neutron detector array. The P-1n values presented constrain the predictions of theoretical models in the region, affecting the final abundance distribution of the second r-process peak at A approximate to 130.
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n_TOF Collaboration, Gunsing, F., Berthoumieux, E., Borella, A., Belgya, T., Szentmiklosi, L., et al. (2011). Neutron Capture on (209)Bi: Determination of the Production Ratio of (210m)Bi/(210g)Bi. J. Korean Phys. Soc., 59(2), 1670–1675.
Abstract: Neutron capture on (209)Bi produces either an isomeric state (210m)Bi with a half life of 3 x 106 years, or the ground state (210g)Bi which decays with a half life of 5 days to the alpha emitter (210)Po. Therefore the neutron capture cross section ratio (209)Bi(n,gamma)(210m)Bi/(210g)Bi plays an important role in predicting the short- and long-term radio-toxicity produced by (209)Bi under neutron irradiation. This ratio is dependent on the neutron energy. We have measured this ratio for cold neutrons at the cold neutron beam facility of the Budapest Neutron Centre by observing the population of the ground-and the metastable state using high resolution gamma-ray spectroscopy. The same technique has been used at the pulsed white neutron source GELINA of the IRMM, Geel in combination with the neutron time-of-flight technique. Results for the neutron-energy dependent branching ratio will be presented. In addition we performed simulations using a statistical decay code.
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n_TOF Collaboration(Gunsing, F. et al), Domingo-Pardo, C., & Tain, J. L. (2012). Measurement of resolved resonances of Th-232(n, gamma) at the n_TOF facility at CERN. Phys. Rev. C, 85(6), 064601–17pp.
Abstract: The yield of the neutron capture reaction Th-232(n, gamma) has been measured at the neutron time-of-flight facility n_TOF at CERN in the energy range from 1 eV to 1 MeV. The reduction of the acquired data to the capture yield for resolved resonances from 1 eV to 4 keV is described and compared to a recent evaluated data set. The resonance parameters were used to assign an orbital momentum to each resonance. A missing level estimator was used to extract the s-wave level spacing of D-0 = 17.2 +/- 0.9 eV.
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n_TOF Collaboration(Gunsing, F. et al), Domingo-Pardo, C., Tain, J. L., & Tarifeño-Saldivia, A. (2016). Nuclear data activities at the n_TOF facility at CERN. Eur. Phys. J. Plus, 131(10), 371–13pp.
Abstract: Nuclear data in general, and neutron-induced reaction cross sections in particular, are important for a wide variety of research fields. They play a key role in the safety and criticality assessment of nuclear technology, not only for existing power reactors but also for radiation dosimetry, medical applications, the transmutation of nuclear waste, accelerator-driven systems, fuel cycle investigations and future reactor systems as in Generation IV. Applications of nuclear data are also related to research fields as the study of nuclear level densities and stellar nucleosynthesis. Simulations and calculations of nuclear technology applications largely rely on evaluated nuclear data libraries. The evaluations in these libraries are based both on experimental data and theoretical models. Experimental nuclear reaction data are compiled on a worldwide basis by the international network of Nuclear Reaction Data Centres (NRDC) in the EXFOR database. The EXFOR database forms an important link between nuclear data measurements and the evaluated data libraries. CERN's neutron time-of-flight facility nTOF has produced a considerable amount of experimental data since it has become fully operational with the start of the scientific measurement programme in 2001. While for a long period a single measurement station (EAR1) located at 185 m from the neutron production target was available, the construction of a second beam line at 20 m (EAR2) in 2014 has substantially increased the measurement capabilities of the facility. An outline of the experimental nuclear data activities at CERN's neutron time-of-flight facility nTOF will be presented.
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n_TOF Collaboration(Guerrero, C. et al), Giubrone, G., & Tain, J. L. (2011). Characterization of the New n_TOF Neutron Beam: Fluence, Profile and Resolution. J. Korean Phys. Soc., 59(2), 1624–1627.
Abstract: After a halt of four years, the nTOF spallation neutron facility at CERN has resumed operation in November 2008 with a new spallation target characterized by an improved safety and engineering design, resulting in a more robust overall performance and efficient cooling. The first measurement during the 2009 run has aimed at the full characterization of the neutron beam. Several detectors, such as calibrated fission chambers, the nTOF Silicon Monitor, a MicroMegas detector with (10)B and (235)U samples, as well as liquid and solid scintillators have been used in order to characterize the properties of the neutron fluence. The spatial profile of the beam has been studied with a specially designed “X-Y” MicroMegas which provided a 2D image of the beam as a function of neutron energy. Both properties have been compared with simulations performed. with the FLUKA code. The characterization of the resolution function is based on results from simulations which have been verified by the study of narrow capture resonances. of (56)Fe, which were measured as part of a new campaign of (n,gamma) measurements on Fe and Ni isotopes.
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n_TOF Collaboration(Guerrero, C. et al), Domingo-Pardo, C., & Tain, J. L. (2011). Study of Photon Strength Function of Actinides: the Case of (235)U, (238)Np and (241)Pu. J. Korean Phys. Soc., 59(2), 1510–1513.
Abstract: The decay from excited levels in medium and heavy nuclei can be described in a statistical approach by means of Photon Strength Functions and Level Density distributions. The study of electromagnetic cascades following neutron capture based on the use of high efficiency detectors has been shown to be well suited for probing the properties of the Photon Strength Function of heavy (high level density) and/or radioactive (high background) nuclei. In this work we have investigated for the first time the validity of the recommended PSF of actinides, in particular (235)U, (238)Np and (241)Pu. Our study includes the search for resonance structures in the PSF below S(n) and draws conclusions regarding their existence and their characteristics in terms of energy, width and electromagnetic nature.
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n_TOF Collaboration(Guerrero, C. et al), Domingo-Pardo, C., Giubrone, G., & Tain, J. L. (2013). Performance of the neutron time-of-flight facility n_TOF at CERN. Eur. Phys. J. A, 49(2), 27–15pp.
Abstract: The neutron time-of-flight facility n_TOF features a white neutron source produced by spallation through 20 GeV/c protons impinging on a lead target. The facility, aiming primarily at the measurement of neutron-induced reaction cross sections, was operating at CERN between 2001 and 2004, and then underwent a major upgrade in 2008. This paper presents in detail all the characteristics of the new neutron beam in the currently available configurations, which correspond to two different collimation systems and two choices of neutron moderator. The characteristics discussed include the intensity and energy dependence of the neutron flux, the spatial profile of the beam, the in-beam background components and the energy resolution/broadening. The discussion of these features is based on dedicated measurements and Monte Carlo simulations, and includes estimations of the systematic uncertainties of the mentioned quantities.
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n_TOF Collaboration(Guerrero, C. et al), Domingo-Pardo, C., & Tain, J. L. (2020). Neutron Capture on the s-Process Branching Point Tm-171 via Time-of-Flight and Activation. Phys. Rev. Lett., 125(14), 142701–8pp.
Abstract: The neutron capture cross sections of several unstable nuclides acting as branching points in the s process are crucial for stellar nucleosynthesis studies. The unstable Tm-171 (t(1/2) = 1.92 yr) is part of the branching around mass A similar to 170 but its neutron capture cross section as a function of the neutron energy is not known to date. In this work, following the production for the first time of more than 5 mg of Tm-171 at the high-flux reactor Institut Laue-Langevin in France, a sample was produced at the Paul Scherrer Institute in Switzerland. Two complementary experiments were carried out at the neutron time-of-flight facility (nTOF) at CERN in Switzerland and at the SARAF liquid lithium target facility at Soreq Nuclear Research Center in Israel by time of flight and activation, respectively. The result of the time -of-flight experiment consists of the first ever set of resonance parameters and the corresponding average resonance parameters, allowing us to make an estimation of the Maxwellian-averaged cross sections (MACS) by extrapolation. The activation measurement provides a direct and more precise measurement of the MACS at 30 keV: 384 (40) mb, with which the estimation from the nTOF data agree at the limit of 1 standard deviation. This value is 2.6 times lower than the JEFF-3.3 and ENDF/B-VIII evaluations, 25% lower than that of the Bao et al. compilation, and 1.6 times larger than the value recommended in the KAlloNiS (v1) database, based on the only previous experiment. Our result affects the nucleosynthesis at the A similar to 170 branching, namely, the Yb-171 abundance increases in the material lost by asymptotic giant branch stars, providing a better match to the available pre-solar SiC grain measurements compared to the calculations based on the current JEFF-3.3 model-based evaluation.
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Guerrero, C., Cano-Ott, D., Mendoza, E., Tain, J. L., Algora, A., Berthoumieux, E., et al. (2012). Monte Carlo simulation of the n_TOF Total Absorption Calorimeter. Nucl. Instrum. Methods Phys. Res. A, 671, 108–117.
Abstract: The n_TOF Total Absorption Calorimeter (TAC) is a 4 pi BaF2 segmented detector used at CERN for measuring neutron capture cross-sections of importance for the design of advanced nuclear reactors. This work presents the simulation code that has been developed in GEANT4 for the accurate determination of the detection efficiency of the TAC for neutron capture events. The code allows to calculate the efficiency of the TAC for every neutron capture state, as a function of energy, crystal multiplicity, and counting rate. The code includes all instrumental effects such as the single crystal detection threshold and energy resolution, finite size of the coincidence time window, and signal pile-up. The results from the simulation have been validated with experimental data for a large set of electromagnetic de-excitation patterns: beta-decay of well known calibration sources, neutron capture reactions in light nuclei with well known level schemes like Ti-nat, reference samples used in (n,gamma) measurements like Au-197 and experimental data from an actinide sample like Pu-240. The systematic uncertainty in the determination of the detection efficiency has been estimated for all the cases. As a representative example, the accuracy reached for the case of Au-197(n,gamma) ranges between 0.5% and 2%, depending on the experimental and analysis conditions. Such a value matches the high accuracy required for the nuclear cross-section data needed in advanced reactor design.
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n_TOF Collaboration(Guerrero, C. et al), Domingo-Pardo, C., & Tain, J. L. (2012). Measurement and resonance analysis of the Np-237 neutron capture cross section. Phys. Rev. C, 85(4), 044616–15pp.
Abstract: The neutron capture cross section of Np-237 was measured between 0.7 and 500 eV at the CERN n_TOF facility using the 4 pi BaF2 Total Absorption Calorimeter. The experimental capture yield was extracted minimizing all the systematic uncertainties and was analyzed together with the most reliable transmission data available using the SAMMY code. The result is a complete set of individual as well as average resonance parameters [D-0 = 0.56(2) eV, <Gamma(gamma)> = 40.9(18) meV, 10(4)S(0) = 0.98(6), R' = 9.8(6) fm]. The capture cross section obtained in this work is in overall agreement with the evaluations and the data of Weston and Todd [Nucl. Sci. Eng. 79, 184 (1981)], thus showing sizable differences with respect to previous data from Scherbakov et al. [J. Nucl. Sci. Technol. 42, 135 (2005)] and large discrepancies with data Kobayashi et al. [J. Nucl. Sci. Technol. 39, 111 (2002)]. The results indicate that a new evaluation combining the present capture data with reliable transmission data would allow reaching an accuracy better than 4%, in line with the uncertainty requirements of the nuclear data community for the design and operation of current and future nuclear devices.
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