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Nichols, A. L., Dimitriou, P., Algora, A., Fallot, M., Giot, L., Kondev, F. G., et al. (2023). Improving fission-product decay data for reactor applications: part I-decay heat. Eur. Phys. J. A, 59(4), 78–78pp.
Abstract: Effort has been expended to assess the relative merits of undertaking further decay-data measurements of the main fission-product contributors to the decay heat of neutron-irradiated fissionable fuel and related actinides by means of Total Absorption Gamma-ray Spectroscopy (TAGS – sometimes abbreviated to TAS) and Discrete Gamma-ray Spectroscopy (DGS). This review has been carried out following similar work performed under the auspices of OECD/WPEC-Subgroup 25 (2005-2007) and the International Atomic Energy Agency (2009, 2014), and various highly relevant TAGS measurements completed as a consequence of such assessments. We present our recommendations for new decay-data evaluations, along with possible requirements for total absorption and discrete high-resolution gamma-ray spectroscopy studies that cover approximately 120 fission products and various isomeric states.
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Nacher, E., Rubio, B., Algora, A., Cano-Ott, D., Tain, J. L., Gadea, A., et al. (2016). Observations of the Gamow-Teller resonance in the rare-earth nuclei above Gd-146 populated in beta decay. Phys. Rev. C, 93(1), 014308–13pp.
Abstract: The rare-earth region of the nuclear table around the quasi-doubly magic nucleus Gd-146 is one of the very few places in which the Gamow-Teller (GT) resonance can be populated in beta decay. The appropriate technique to study such a phenomenon is total absorption spectroscopy, thanks to which one can measure the B(GT) distribution in beta-decay experiments even when it is very fragmented and lies at high excitation energy in the daughter nucleus. Results on the GT resonance measured in the beta decay of the odd-Z, N = 83 nuclei Tb-148, Ho-150, and Tm-152 are presented in this work and compared with shell-model calculations. The tail of the resonance is clearly observed up to the limit imposed by the Q value. This observation is important in the context of the understanding of the “quenching” of the GT strength.
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n_TOF Collaboration(Mosconi, M. et al), Domingo-Pardo, C., & Tain, J. L. (2010). Neutron physics of the Re/Os clock. I. Measurement of the (n, gamma) cross sections of Os-186,Os-187,Os-188 at the CERN n_TOF facility. Phys. Rev. C, 82(1), 015802–10pp.
Abstract: The precise determination of the neutron capture cross sections of Os-186 and Os-187 is important to define the s-process abundance of Os-187 at the formation of the solar system. This quantity can be used to evaluate the radiogenic component of the abundance of Os-187 due to the decay of the unstable Re-187 (t(1/2) = 41.2 Gyr) and from this to infer the time duration of the nucleosynthesis in our galaxy (Re/Os cosmochronometer). The neutron capture cross sections of Os-186, Os-187, and Os-188 have been measured at the CERN n_TOF facility from 1 eV to 1 MeV, covering the entire energy range of astrophysical interest. The measurement has been performed by time-of-flight technique using isotopically enriched samples and two C6D6 scintillation detectors for recording the prompt. rays emitted in the capture events. Maxwellian averaged capture cross sections have been determined for thermal energies between kT = 5 and 100 keV corresponding to all possible s-process scenarios. The estimated uncertainties for the values at 30 keV are 4.1, 3.3, and 4.7% for Os-186, Os-187, and Os-188, respectively.
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n_TOF Collaboration(Moreno-Soto, J. et al), Babiano-Suarez, V., Caballero-Ontanaya, L., Domingo-Pardo, C., Ladarescu, I., & Tain, J. L. (2022). Constraints on the dipole photon strength for the odd uranium isotopes. Phys. Rev. C, 105(2), 024618–14pp.
Abstract: Background: The photon strength functions (PSFs) and nuclear level density (NLD) are key ingredients for calculation of the photon interaction with nuclei, in particular the reaction cross sections. These cross sections are important especially in nuclear astrophysics and in the development of advanced nuclear technologies. Purpose: The role of the scissors mode in the M1 PSF of (well-deformed) actinides was investigated by several experimental techniques. The analyses of different experiments result in significant differences, especially on the strength of the mode. The shape of the low-energy tail of the giant electric dipole resonance is uncertain as well. In particular, some works proposed a presence of the E1 pygmy resonance just above 7 MeV. Because of these inconsistencies additional information on PSFs in this region is of great interest. Methods: The gamma-ray spectra from neutron-capture reactions on the U-234, U-236, and U-238 nuclei have been measured with the total absorption calorimeter of the n_TOF facility at CERN. The background-corrected sum-energy and multi-step-cascade spectra were extracted for several isolated s-wave resonances up to about 140 eV. Results: The experimental spectra were compared to statistical model predictions coming from a large selection of models of photon strength functions and nuclear level density. No combination of PSF and NLD models from literature is able to globally describe our spectra. After extensive search we were able to find model combinations with modified generalized Lorentzian (MGLO) E1 PSF, which match the experimental spectra as well as the total radiative widths. Conclusions: The constant temperature energy dependence is favored for a NLD. The tail of giant electric dipole resonance is well described by the MGLO model of the E1 PSF with no hint of pygmy resonance. The M1 PSF must contain a very strong, relatively wide, and likely double-resonance scissors mode. The mode is responsible for about a half of the total radiative width of neutron resonances and significantly affects the radiative cross section.
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Molina, F. et al, Rubio, B., Agramunt, J., Algora, A., Domingo-Pardo, C., Gadea, A., et al. (2015). T-z =-1 -> 0 beta decays of Ni-54, Fe-50, Cr-46, and Ti-42 and comparison with mirror (He-3,t) measurements. Phys. Rev. C, 91(1), 014301–19pp.
Abstract: We have studied the beta decay of the T-z = -1, f(7/2) shell nuclei Ni-54, Fe-50, Cr-46, and Ti-42 produced in fragmentation reactions. The proton separation energies in the daughter T-z = 0 nuclei are relatively large (approximate to 4-5 MeV) so studies of the. rays are essential. The experiments were performed at GSI as part of the Stopped-beam campaign with the RISING setup consisting of 15 Euroball Cluster Ge detectors. From the newly obtained high precision beta-decay half-lives, excitation energies, and beta branching ratios, we were able to extract Fermi and Gamow-Teller transition strengths in these beta decays. With these improved results it was possible to compare in detail the Gamow-Teller (GT) transition strengths observed in beta decay including a sensitivity limit with the strengths of the T-z = +1 to T-z = 0 transitions derived from high resolution (He-3,t) reactions on the mirror target nuclei at RCNP, Osaka. The accumulated B(GT) strength obtained from both experiments looks very similar although the charge exchange reaction provides information on a broader energy range. Using the “merged analysis” one can obtain a full picture of the B(GT) over the full Q(beta) range. Looking at the individual transitions some differences are observed, especially for the weak transitions. Their possible origins are discussed.
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n_TOF Collaboration(Mingrone, F. et al), Domingo-Pardo, C., Giubrone, G., & Tain, J. L. (2017). Neutron capture cross section measurement of U-238 at the CERN n_TOF facility in the energy region from 1 eV to 700 keV. Phys. Rev. C, 95(3), 034604–14pp.
Abstract: The aim of this work is to provide a precise and accurate measurement of the U-238(n,gamma) reaction cross section in the energy region from 1 eV to 700 keV. This reaction is of fundamental importance for the design calculations of nuclear reactors, governing the behavior of the reactor core. In particular, fast reactors, which are experiencing a growing interest for their ability to burn radioactive waste, operate in the high energy region of the neutron spectrum. In this energy region most recent evaluations disagree due to inconsistencies in the existing measurements of up to 15%. In addition, the assessment of nuclear data uncertainty performed for innovative reactor systems shows that the uncertainty in the radiative capture cross section of U-238 should be further reduced to 1-3% in the energy region from 20 eV to 25 keV. To this purpose, addressed by the Nuclear Energy Agency as a priority nuclear data need, complementary experiments, one at the GELINA and two at the nTOF facility, were proposed and carried out within the 7th Framework Project ANDES of the European Commission. The results of one of these U-238(n, gamma) measurements performed at the nTOF CERN facility are presented in this work. The gamma-ray cascade following the radiative neutron capture has been detected exploiting a setup of two C6D6 liquid scintillators. Resonance parameters obtained from this work are on average in excellent agreement with the ones reported in evaluated libraries. In the unresolved resonance region, this work yields a cross section in agreement with evaluated libraries up to 80 keV, while for higher energies our results are significantly higher.
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n_TOF Collaboration(Michalopoulou, V. et al), Babiano-Suarez, V., Caballero, L., Domingo-Pardo, C., Ladarescu, I., & Tain, J. L. (2023). Measurement of the neutron-induced fission cross section of Th-230 at the CERN n_TOF facility. Phys. Rev. C, 108(1), 014616–15pp.
Abstract: The neutron-induced fission cross section of Th-230 has been measured at the neutron time-of-flight facility n_TOF located at CERN. The experiment was performed at the experimental area EAR-1 with a neutron flight path of 185 m, using Micromegas detectors for the detection of the fission fragments. The Th-230(n, f ) cross section was determined relative to the U-235(n, f ) one, covering the energy range from the fission threshold up to 400 MeV. The results from the present work are compared with existing cross-section datasets and the observed discrepancies are discussed and analyzed. Finally, using the code EMPIRE 3.2.3 a theoretical study, based on the statistical model, was performed leading to a satisfactory reproduction of the experimental results with the proper tuning of the respective parameters, while for incident neutron energy beyond 200 MeV the fission of( 230)Th was described by Monte Carlo simulations.
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n_TOF Collaboration(Mendoza, E. et al), Giubrone, G., & Tain, J. L. (2011). Improved Neutron Capture Cross Section Measurements with the n_TOF Total Absorption Calorimeter. J. Korean Phys. Soc., 59(2), 1813–1816.
Abstract: The n_TOF collaboration operates a Total Absorption Calorimeter (TAC) [1] for measuring neutron capture cross-sections of low-mass and/or radioactive samples. The results obtained with the TAC have led to a substantial improvement of the capture cross sections of (237)Np and (240)Pu [2]. The experience acquired during the first measurements has allowed us to optimize the performance of the TAC and to improve the capture signal to background ratio, thus opening the way to more complex and demanding measurements on rare radioactive materials. The new design has been reached by a series of detailed Monte Carlo simulations of complete experiments and dedicated test measurements. The new capture setup will be presented and the main achievements highlighted.
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n_TOF Collaboration(Mendoza, E. et al), Domingo-Pardo, C., & Tain, J. L. (2014). Measurement and analysis of the Am-243 neutron capture cross section at the n_TOF facility at CERN. Phys. Rev. C, 90(3), 034608–16pp.
Abstract: Background: The design of new nuclear reactors and transmutation devices requires to reduce the present neutron cross section uncertainties of minor actinides. Purpose: Improvement of the Am-243(n, gamma) cross section uncertainty. Method: The Am-243(n, gamma) cross section has been measured at the n_TOF facility at CERN with a BaF2 total absorption calorimeter, in the energy range between 0.7 eV and 2.5 keV. Results: The Am-243(n, gamma) cross section has been successfully measured in the mentioned energy range. The resolved resonance region has been extended from 250 eV up to 400 eV. In the unresolved resonance region our results are compatible with one of the two incompatible capture data sets available below 2.5 keV. The data available in EXFOR and in the literature have been used to perform a simple analysis above 2.5 keV. Conclusions: The results of this measurement contribute to reduce the Am-243(n, gamma) cross section uncertainty and suggest that this cross section is underestimated up to 25% in the neutron energy range between 50 eV and a few keV in the present evaluated data libraries.
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n_TOF Collaboration(Mendoza, E. et al), Giubrone, G., Tain, J. L., & Tarifeño-Saldivia, A. (2018). Measurement and analysis of the Am-241 neutron capture cross section at the n_TOF facility at CERN. Phys. Rev. C, 97(5), 054616–21pp.
Abstract: The Am-241(n, gamma) cross section has been measured at the nTOF facility at CERN with the nTOF BaF2 Total Absorption Calorimeter in the energy range between 0.2 eV and 10 keV. Our results are analyzed as resolved resonances up to 700 eV, allowing a more detailed description of the cross section than in the current evaluations, which contain resolved resonances only up to 150-160 eV. The cross section in the unresolved resonance region is perfectly consistent with the predictions based on the average resonance parameters deduced from the resolved resonances, thus obtaining a consistent description of the cross section in the full neutron energy range under study. Below 20 eV, our results are in reasonable agreement with JEFF-3.2 as well as with the most recent direct measurements of the resonance integral, and differ up to 20-30% with other experimental data. Between 20 eV and 1 keV, the disagreement with other experimental data and evaluations gradually decreases, in general, with the neutron energy. Above 1 keV, we find compatible results with previously existing values.
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