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Author |
Caballero-Folch, R. et al; Domingo-Pardo, C.; Agramunt, J.; Algora, A.; Rubio, B.; Tain, J.L. |
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Title |
beta-decay half-lives and beta-delayed neutron emission probabilities for several isotopes of Au, Hg, Tl, Pb, and Bi, beyond N=126 |
Type |
Journal Article |
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Year |
2017 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
95 |
Issue |
6 |
Pages |
064322 - 16pp |
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Abstract |
Background: There have been measurements on roughly 230 nuclei that are beta-delayed neutron emitters. They range from He-8 up to La-150. Apart from 210Tl, with a branching ratio of only 0.007%, no other neutron emitter has been measured beyond A = 150. Therefore, new data are needed, particularly in the region of heavy nuclei around N = 126, in order to guide theoretical models and help understand the formation of the third r-process peak at A similar to 195. Purpose: To measure both beta-decay half-lives and neutron branching ratios of several neutron-rich Au, Hg, Tl, Pb, and Bi isotopes beyond N = 126. Method: Ions of interest were produced by fragmentation of a U-238 beam, selected and identified via the GSI-FRS fragment separator. A stack of segmented silicon detectors (SIMBA) was used to measure ion implants and beta decays. An array of 30 He-3 tubes embedded in a polyethylene matrix (BELEN) was used to detect neutrons with high efficiency and selectivity. A self-triggered digital system is employed to acquire data and to enable time correlations. The latter were analyzed with an analytical model and results for the half-lives and neutron-branching ratios were derived by using the binned maximum-likelihood method. Results: Twenty new beta-decay half-lives are reported for Au204-206, Hg208-211, Tl211-216, Pb215-218, and Bi218-220, nine of them for the first time. Neutron emission probabilities are reported for Hg-210,Hg-211 and Tl211-216. Conclusions: The new beta-decay half-lives are in good agreement with previous measurements on nuclei in this region. The measured neutron emission probabilities are comparable to or smaller than values predicted by global models such as relativistic Hartree Bogoliubov plus the relativistic quasi-particle random phase approximation (RHB + RQRPA). |
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Address  |
[Caballero-Folch, R.; Calvino, F.; Cortes, G.; Gomez-Hornillos, M. B.; Riego, A.] Univ Politecn Cataluna, DFEN, INTE, E-08028 Barcelona, Spain, Email: rcaballero-folch@triumf.ca |
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Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
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Notes |
WOS:000404022100001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3176 |
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Author |
Caballero-Folch, R. et al; Domingo-Pardo, C.; Tain, J.L.; Agramunt, J.; Algora, A.; Rubio, B. |
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Title |
beta-decay and beta-delayed Neutron Emission Measurements at GSI-FRS Beyond N=126, for r-process Nucleosynthesis |
Type |
Journal Article |
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Year |
2014 |
Publication |
Nuclear Data Sheets |
Abbreviated Journal |
Nucl. Data Sheets |
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Volume |
120 |
Issue |
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Pages |
81-83 |
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Abstract |
New measurements of very exotic nuclei in the neutron-rich region beyond N=126 have been performed at the GSI facility with the fragment separator (FRS). The aim of the experiment is to determine half-lives and beta-delayed neutron emission branching ratios of isotopes of Hg, Tl and Pb in this region. This contribution summarizes final counting statistics for identification and for implantation, as well as the present status of the data analysis of the half-lives. In summary, isotopes of Pt, Au, Hg, Ti, Pb, Bi, Po, At, Rn and Fr were clearly identified and several of them (Hg208-211, Tl211-215, Pb214-218) were implanted with enough statistics to determine their half-lives. About half of them are expected to be neutron emitters, in such cases it will become possible to obtain the neutron emission probabilities, P-n. |
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Address |
[Caballero-Folch, R.; Cortes, G.; Calvino, F.; Gomez-Hornillos, M. B.; Riego, A.] Univ Politecn Cataluna, Dept Fis Enginyeria Nucl, E-08028 Barcelona, Spain, Email: roger.caballero@upc.edu |
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Academic Press Inc Elsevier Science |
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English |
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ISSN |
0090-3752 |
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Notes |
WOS:000339860100022 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
1873 |
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Author |
Caballero-Folch, R. et al; Agramunt, J.; Tain, J.L.; Algora, A.; Domingo-Pardo, C.; Guadilla, V.; Montaner-Piza, A.; Orrigo, S.E.A.; Rubio, B.; Tarifeño-Saldivia, A.; Tolosa-Delgado, A. |
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Title |
First determination of beta-delayed multiple neutron emission beyond A=100 through direct neutron measurement: The P-2n value of Sb-136 |
Type |
Journal Article |
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Year |
2018 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
98 |
Issue |
3 |
Pages |
034310 - 10pp |
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Keywords |
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Abstract |
Background: beta-delayed multiple neutron emission has been observed for some nuclei with A <= 100 being the Rb-100 the heaviest beta 2n emitter measured to date. So far only 25 P-2n values have been determined for the approximate to 300 nuclei that may decay in this way. Accordingly it is of interest to measure P-2n values for the other possible multiple neutron emitters throughout the chart of the nuclides. It is of particular interest to make such a measurement for nuclei with A > 100 to test the predictions of theoretical models and simulation tools for the decays of heavy nuclei in the region of very neutron-rich nuclei. In addition the decay properties of these nuclei are fundamental for the understanding of astrophysical nucleosynthesis processes such as the r-process and safety inputs for nuclear reactors. Purpose: To determine for the first time the two-neutron branching ratio the P-2n value for Sb-136 through a direct neutron measurement and to provide precise P-1n values for Sb-136 and Te-136. Method: A pure beam of each isotope of interest was provided by the JYFLTRAP Penning trap at the Ion Guide Isotope Separator On-Line (IGISOL) facility of the University of Jyvaskyla Finland. The purified ions were implanted into a moving tape at the end of the beam line. The detection setup consisted of a plastic scintillator placed right behind the implantation point after the tape to register the beta decays and the BELEN detector based on neutron counters embedded in a polyethylene matrix. The analysis was based on the study of the beta- and neutron-growth-and-decay curves and the beta-one-neutron and beta-two-neutron time correlations which allowed us the determination of the neutron branching ratios. Results: The P-2n value of Sb-136 was found to be 0.14(3)% and the measured P-1n values for Sb-136 and Te-136 were found to be 32.2(15)% and 1.47(6)% respectively. Conclusions: The measured P-2n value is a factor 44 smaller than predicted by the finite-range droplet model plus the quasiparticle random-phase approximation (FRDM+QRPA) model used for r-process calculations. |
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Address |
[Caballero-Folch, R.; Dillmann, I] TRIUMF, Vancouver, BC V6T 2A3, Canada, Email: rcaballero-folch@triumf.ca |
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Amer Physical Soc |
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English |
Summary Language |
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Original Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
2469-9985 |
ISBN |
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Notes |
WOS:000444207600003 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3728 |
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Author |
n_TOF Collaboration (Calviani, M. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Fission Cross-section Measurements of (233)U, (245)Cm and (241,243)Am at CERN n_TOF Facility |
Type |
Journal Article |
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Year |
2011 |
Publication |
Journal of the Korean Physical Society |
Abbreviated Journal |
J. Korean Phys. Soc. |
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Volume |
59 |
Issue |
2 |
Pages |
1912-1915 |
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Keywords |
ND2010; Nuclear data; ENDF; n_TOF; Neutron-induced fission reactions; Am; Cm; U |
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Abstract |
Neutron-induced fission cross-sections of minor actinides have been measured using the nTOF white neutron source at CERN. Geneva, as part of a large experimental program aiming at collecting new data relevant for nuclear astrophysics and for the design of advanced reactor systems. The measurements at nTOF take advantage of the innovative features of the n_TOF facility, namely the wide energy range, high instantaneous neutron flux and good energy resolution. Final results on the fission cross-section of (233)U, (245)cm and (243)Am from thermal to 20 MeV are here reported, together with preliminary results for (241)Am. The measurement have been performed with a dedicated Fast Ionization Chamber (FIC), a fission fragment detector with a very high efficiency, relative to the very well known cross-section of (235)U, measured simultaneously with the same detector. |
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Address |
[Calviani, M; Andriamonje, S; Chiaveri, E; Vlachoudis, V] CERN, Geneva, Switzerland, Email: marco.calviani@cern.ch |
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Korean Physical Soc |
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English |
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ISSN |
0374-4884 |
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Notes |
WOS:000294080700111 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
741 |
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Author |
n_TOF Collaboration (Cano-Ott, D. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Neutron Capture Measuremetns on Minor Actinides at the n_TOF Facility at CERN: Past, Present and Future |
Type |
Journal Article |
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Year |
2011 |
Publication |
Journal of the Korean Physical Society |
Abbreviated Journal |
J. Korean Phys. Soc. |
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Volume |
59 |
Issue |
2 |
Pages |
1809-1812 |
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Keywords |
n_TOF; Total Absorption Calorimeter; TAC; Neutron capture; Cross section; Nuclear waste; Transmutation; Generation IV; Accelerator driven system; ADS; Nuclear reactor; Nuclear energy; Nuclear data; Barium fluoride; Actinides; Plutonium; Americium; Uranium |
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Abstract |
The successful development of advanced nuclear systems for sustainable energy production and nuclear waste management depends on high quality nuclear data libraries. Recent sensitivity studies and reports [1-3] have identified the need for substantially improving the accuracy of neutron cross-section data for minor actinides. The n_TOF collaboration has initiated an ambitious experimental program for the measurement of neutron capture cross sections of minor actinides. Two experimental setups have been constructed for this purpose: a Total Absorption Calorimeter (TAC) [4] for measuring neutron capture cross-sections of low-mass and/or radioactive samples and a set of two low neutron sensitivity C(6)D(6) detectors for the less radioactive materials. |
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Address |
[Cano-Ott, D; Alvarez-Velarde, F; Gonzalez-Romero, E; Guerrero, C; Martinez, T; Mendoza, E; Villamarin, D; Vicente, MC] Ctr Invest Energet Medioambientales & Technol CIE, Madrid, Spain, Email: daniel.cano@ciemat.es |
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Corporate Author |
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Publisher |
Korean Physical Soc |
Place of Publication |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0374-4884 |
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Conference |
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Notes |
WOS:000294080700085 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
737 |
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