| Records |
| Author |
n_TOF Collaboration (Stamatopoulos, A. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
| Title |
Investigation of the Pu-240(n, f) reaction at the n_TOF/EAR2 facility in the 9 meV-6 MeV range |
Type |
Journal Article |
| Year |
2020 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
| Volume |
102 |
Issue |
1 |
Pages |
014616 - 23pp |
| Keywords |
|
| Abstract |
Background: Nuclear waste management is considered amongst the major challenges in the field of nuclear energy. A possible means of addressing this issue is waste transmutation in advanced nuclear systems, whose operation requires a fast neutron spectrum. In this regard, the accurate knowledge of neutron-induced reaction cross sections of several (minor) actinide isotopes is essential for design optimization and improvement of safety margins of such systems. One such case is Pu-240, due to its accumulation in spent nuclear fuel of thermal reactors and its usage in fast reactor fuel. The measurement of the Pu-240(n, f) cross section was previously attempted at the CERN nTOF facility EAR1 measuring station using the time-of-flight technique. Due to the low amount of available material and the given flux at EAR1, the measurement had to last several months to achieve a sufficient statistical accuracy. This long duration led to detector deterioration due to the prolonged exposure to the high alpha activity of the fission foils, therefore the measurement could not be successfully completed. Purpose: It is aimed to determine whether it is feasible to study neutron-induced fission at nTOF/EAR2 and provide data on the Pu-240(n, f) reaction in energy regions requested for applications. Methods: The study of the Pu-240(n, f) reaction was made at a new experimental area (EAR2) with a shorter flight path which delivered on average 30 times higher flux at fast neutron energies. This enabled the measurement to be performed much faster, thus limiting the exposure of the detectors to the intrinsic activity of the fission foils. The experimental setup was based on microbulk Micromegas detectors and the time-of-flight data were analyzed with an optimized pulse-shape analysis algorithm. Special attention was dedicated to the estimation of the non-negligible counting loss corrections with the development of a new methodology, and other corrections were estimated via Monte Carlo simulations of the experimental setup. Results: This new measurement of the Pu-240(n, f) cross section yielded data from 9 meV up to 6 MeV incident neutron energy and fission resonance kernels were extracted up to 10 keV. Conclusions: Neutron-induced fission of high activity samples can be successfully studied at the n_TOF/EAR2 facility at CERN covering a wide range of neutron energies, from thermal to a few MeV. |
Address  |
[Stamatopoulos, A.; Tsinganis, A.; Kokkoris, M.; Vlastou, R.; Diakaki, M.] Natl Tech Univ Athens, Athens, Greece, Email: athanasios.stamatopoulos@cern.ch |
| Corporate Author |
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Thesis |
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| Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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| Language |
English |
Summary Language |
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Original Title |
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| Series Editor |
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Series Title |
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Abbreviated Series Title |
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| Series Volume |
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Series Issue |
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Edition |
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| ISSN |
0556-2813 |
ISBN |
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Medium |
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| Area |
|
Expedition |
|
Conference |
|
| Notes |
WOS:000551057500002 |
Approved |
no |
| Is ISI |
yes |
International Collaboration |
yes |
| Call Number |
IFIC @ pastor @ |
Serial |
4466 |
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| |
| Author |
n_TOF Collaboration (Tagliente, G. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A. |
| Title |
Zr-92(n, gamma) and (n,tot) measurements at the GELINA and n_TOF facilities |
Type |
Journal Article |
| Year |
2022 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
| Volume |
105 |
Issue |
2 |
Pages |
025805 - 14pp |
| Keywords |
|
| Abstract |
Background: Stellar nucleosynthesis of elements heavier than iron is driven by neutron capture processes. Zr-92 is positioned at a strategic point along the slow nucleosynthesis path, given its proximity to the neutron magic number N = 50 and its position at the matching region between the weak and main slow processes. Purpose: In parallel with recent improved astronomical data, the extraction of accurate Maxwellian averaged cross sections (MACSs) derived from a more complete and accurate set of resonance parameters should allow for a better understanding of the stellar conditions at which nucleosynthesis takes place. Methods: Transmission and capture cross section measurements using enriched Zr-92 metallic samples were performed at the time-of flight facilities GELINA of JRC-Geel (BE) and nTOF of CERN (CH). The neutron beam passing through the samples was investigated in transmission measurements at GELINA using a Li-glass scintillator. The gamma rays emitted during the neutron capture reactions were detected by C6D6 detectors at both GELINA and nTOF. Results: Resonance parameters of individual resonances up to 81 keV were extracted from a combined resonance shape analysis of experimental transmissions and capture yields. For the majority of the resonances the parity was determined from an analysis of the transmission data obtained with different sample thicknesses. Average resonance parameters were calculated. Conclusions: Maxwellian averaged cross sections were extracted from resonances observed up to 81 keV. The MACS for kT = 30 keV is fully consistent with experimental data reported in the literature. The MACSs for kT less than or similar to 15 keV are in good agreement with those derived from the ENDF/B-VIII.0 library and recommended in the KADoNTS database. For kT higher than 30 keV differences are observed. A comparison with MACSs obtained with the cross sections recommended in the JEFF-3.3 and JENDL-4.0 libraries shows discrepancies even for kT less than or similar to 15 keV. |
| Address |
[Tagliente, G.; Barbagallo, M.; Colonna, N.; Mastromarco, M.; Variale, V.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: giuseppe.tagliente@ba.infn.it |
| Corporate Author |
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Thesis |
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| Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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| Language |
English |
Summary Language |
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Original Title |
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| Series Editor |
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Series Title |
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Abbreviated Series Title |
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| Series Volume |
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Series Issue |
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Edition |
|
| ISSN |
2469-9985 |
ISBN |
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Medium |
|
| Area |
|
Expedition |
|
Conference |
|
| Notes |
WOS:000766732800002 |
Approved |
no |
| Is ISI |
yes |
International Collaboration |
yes |
| Call Number |
IFIC @ pastor @ |
Serial |
5163 |
| Permanent link to this record |
| |
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| |
| Author |
n_TOF Collaboration (Tagliente, G. et al.); Domingo-Pardo, C.; Tain, J.L. |
| Title |
The Zr-92(n,gamma) reaction and its implications for stellar nucleosynthesis |
Type |
Journal Article |
| Year |
2010 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
| Volume |
81 |
Issue |
5 |
Pages |
055801 - 9pp |
| Keywords |
|
| Abstract |
Because the relatively small neutron capture cross sections of the zirconium isotopes are difficult to measure, the results of previous measurements are often not adequate for a number of problems in astrophysics and nuclear technology. Therefore, the Zr-92(n,gamma) cross section has been remeasured at the CERN n_TOF facility, providing a set of improved parameters for 44 resonances in the neutron energy range up to 40 keV. With this information the cross-section uncertainties in the keV region could be reduced to 5% as required for s-process nucleosynthesis studies and technological applications. |
| Address |
[Tagliente, G.; Colonna, N.; Marrone, S.; Terlizzi, R.] Ist Nazl Fis Nucl, I-70126 Bari, Italy, Email: giuseppe.tagliente@ba.infn.it |
| Corporate Author |
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Thesis |
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| Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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| Language |
English |
Summary Language |
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Original Title |
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| Series Editor |
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Series Title |
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Abbreviated Series Title |
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| Series Volume |
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Series Issue |
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Edition |
|
| ISSN |
0556-2813 |
ISBN |
|
Medium |
|
| Area |
|
Expedition |
|
Conference |
|
| Notes |
ISI:000278144800074 |
Approved |
no |
| Is ISI |
yes |
International Collaboration |
yes |
| Call Number |
IFIC @ elepoucu @ |
Serial |
444 |
| Permanent link to this record |
| |
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| |
| Author |
n_TOF Collaboration (Tagliente, G. et al.); Domingo-Pardo, C.; Tain, J.L. |
| Title |
The Zr-93(n, gamma) reaction up to 8 keV neutron energy |
Type |
Journal Article |
| Year |
2013 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
| Volume |
87 |
Issue |
1 |
Pages |
014622 - 7pp |
| Keywords |
|
| Abstract |
The (n, gamma) reaction of the radioactive isotope Zr-93 has been measured at the n_TOF high-resolution time-of-flight facility at CERN. Resonance parameters have been extracted in the neutron energy range up to 8 keV, yielding capture widths smaller (14%) than reported in an earlier experiment. These results are important for detailed nucleosynthesis calculations and for refined studies of waste transmutation concepts. DOI: 10.1103/PhysRevC.87.014622 |
| Address |
[Tagliente, G.; Colonna, N.; Marrone, S.; Terlizzi, R.] Ist Nazl Fis Nucl, I-70126 Bari, Italy, Email: giuseppe.tagliente@ba.infn.it |
| Corporate Author |
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Thesis |
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| Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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| Language |
English |
Summary Language |
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Original Title |
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| Series Editor |
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Series Title |
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Abbreviated Series Title |
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| Series Volume |
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Series Issue |
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Edition |
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| ISSN |
0556-2813 |
ISBN |
|
Medium |
|
| Area |
|
Expedition |
|
Conference |
|
| Notes |
WOS:000314335800003 |
Approved |
no |
| Is ISI |
yes |
International Collaboration |
yes |
| Call Number |
IFIC @ pastor @ |
Serial |
1322 |
| Permanent link to this record |
| |
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| |
| Author |
Tagliente, G. et al; Babiano-Suarez, V.; Domingo-Pardo, C.; Ladarescu, I.; Tain, J.L. |
| Title |
High-resolution cross section measurements for neutron interactions on 89Y with incident neutron energies up to 95 keV |
Type |
Journal Article |
| Year |
2024 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
| Volume |
60 |
Issue |
1 |
Pages |
21 - 18pp |
| Keywords |
|
| Abstract |
The cross section of the Y-89(n,gamma) reaction has important implications in nuclear astrophysics and for advanced nuclear technology. Given its neutron magic number N = 50 and a consequent small neutron capture crosssection,89Y represents one of the key nuclides for the stellars-process. It acts as a bottleneck in the neutron capture chain between the Fe seed and the heavier elements. Moreover, it is located at the overlapping region, where both the weak and mains-process components take place.Y-89, the only stable yttrium isotope, is also used in innovative nuclear reactors. Neutron capture and transmission measurements were per-formed at the time-of-flight facilities n_TOF at CERN and GELINA at JRC-Geel. Resonance parameters of individual resonances were extracted from a resonance analysis of the experimental transmission and capture yields, up to a neutron incident energy of 95 keV. Even though a comparison with results reported in the literature shows differences in resonance parameters, the present data are consistent with the Maxwellian averaged cross section suggested by the astro-physical database KADoNiS. |
| Address |
[Tagliente, G.; Damone, L. A.; Barbagallo, M.; Colonna, N.; Mastromarco, M.; Mazzone, A.; Variale, V.] Ist Nazl Fis Nucl, Bari, Italy, Email: giuseppe.tagliente@ba.infn.it |
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Thesis |
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| Publisher |
Springer |
Place of Publication |
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Editor |
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| Language |
English |
Summary Language |
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Original Title |
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| Series Editor |
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Series Title |
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Abbreviated Series Title |
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| Series Volume |
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Series Issue |
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Edition |
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| ISSN |
1434-6001 |
ISBN |
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Medium |
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| Area |
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Expedition |
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Conference |
|
| Notes |
WOS:001157129400001 |
Approved |
no |
| Is ISI |
yes |
International Collaboration |
yes |
| Call Number |
IFIC @ pastor @ |
Serial |
5946 |
| Permanent link to this record |
| |
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| |
| Author |
n_TOF Collaboration (Tagliente, G. et al.); Domingo-Pardo, C.; Tain, J.L. |
| Title |
Neutron capture on (94)Zr: Resonance parameters and Maxwellian-averaged cross sections |
Type |
Journal Article |
| Year |
2011 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
| Volume |
84 |
Issue |
1 |
Pages |
015801 - 9pp |
| Keywords |
|
| Abstract |
The neutron capture cross sections of the Zr isotopes play an important role in nucleosynthesis studies. The s-process reaction flow between the Fe seed and the heavier isotopes passes through the neutron magic nucleus (90)Zr and through (91,92,93,94)Zr, but only part of the flow extends to (96)Zr because of the branching point at (95)Zr. Apart from their effect on the s-process flow, the comparably small isotopic (n, gamma) cross sections make Zr also an interesting structural material for nuclear reactors. The (94)Zr (n, gamma) cross section has been measured with high resolution at the spallation neutron source n_TOF at CERN and resonance parameters are reported up to 60 keV neutron energy. |
| Address |
[Tagliente, G; Colonna, N; Marrone, S; Terlizzi, R] Ist Nazl Fis Nucl, I-70126 Bari, Italy, Email: giuseppe.tagliente@ba.infn.it |
| Corporate Author |
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Thesis |
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| Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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| Language |
English |
Summary Language |
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Original Title |
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| Series Editor |
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Series Title |
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Abbreviated Series Title |
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| Series Volume |
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Series Issue |
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Edition |
|
| ISSN |
0556-2813 |
ISBN |
|
Medium |
|
| Area |
|
Expedition |
|
Conference |
|
| Notes |
WOS:000292767200010 |
Approved |
no |
| Is ISI |
yes |
International Collaboration |
yes |
| Call Number |
IFIC @ pastor @ |
Serial |
687 |
| Permanent link to this record |
| |
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| |
| Author |
n_TOF Collaboration (Tagliente, G. et al.); Domingo-Pardo, C.; Tain, J.L. |
| Title |
(96)Zr(n,gamma) measurement at the n_TOF facility at CERN |
Type |
Journal Article |
| Year |
2011 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
| Volume |
84 |
Issue |
5 |
Pages |
055802 - 8pp |
| Keywords |
|
| Abstract |
The (n,gamma) cross section of (96)Zr has been investigated at the CERN n_TOF spallation neutron source. High-resolution time-of-flight measurements using an enriched ZrO(2) sample allowed us to analyze 15 resonances below 40 keV with improved accuracy. On average, the capture widths were found to be 25% smaller than reported in earlier experiments. If complemented with the contribution by direct radiative capture, the derived Maxwellian averaged cross sections are consistent with activation data at kT = 25 keV. The present results confirm the astrophysical implications for the s-process branching at (95)Zr. |
| Address |
[Tagliente, G; Colonna, N; Marrone, S; Terlizzi, R] Ist Nazl Fis Nucl, I-70126 Bari, Italy, Email: giuseppe.tagliente@ba.infn.it |
| Corporate Author |
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Thesis |
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| Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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| Language |
English |
Summary Language |
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Original Title |
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| Series Editor |
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Series Title |
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Abbreviated Series Title |
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| Series Volume |
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Series Issue |
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Edition |
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| ISSN |
0556-2813 |
ISBN |
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Medium |
|
| Area |
|
Expedition |
|
Conference |
|
| Notes |
WOS:000297121100005 |
Approved |
no |
| Is ISI |
yes |
International Collaboration |
yes |
| Call Number |
IFIC @ elepoucu @ |
Serial |
812 |
| Permanent link to this record |
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| Author |
Tain, J.L.; Agramunt, J.; Algora, A.; Aprahamian, A.; Cano-Ott, D.; Fraile, L.M.; Guerrero, C.; Jordan, M.D.; Mach, H.; Martinez, T.; Mendoza, E.; Mosconi, M.; Nolte, R. |
| Title |
The sensitivity of LaBr3:Ce scintillation detectors to low energy neutrons: Measurement and Monte Carlo simulation |
Type |
Journal Article |
| Year |
2015 |
Publication |
Nuclear Instruments & Methods in Physics Research A |
Abbreviated Journal |
Nucl. Instrum. Methods Phys. Res. A |
| Volume |
774 |
Issue |
|
Pages |
17-24 |
| Keywords |
Neutron sensitivity; Scintillation detectors; Lanthanum bromide; Geant4 simulations; Nuclear data libraries |
| Abstract |
The neutron sensitivity of a cylindrical circle minus 1.5 in x 1.5 in LaBr3:Ce scintillation detector was measured using quasi-monoenergetic neutron beams in the energy range from 40 keV to 2.5 MeV. In this energy range the detector is sensitive to gamma-rays generated in neutron inelastic and capture processes. The experimental energy response was compared with Monte Carlo simulations performed with the Geant4 simulation toolkit using the so-called High Precision Neutron Models. These models rely on relevant information stored in evaluated nuclear data libraries. The performance of the Geant4 Neutron Data Library as well as several standard nuclear data libraries was investigated. In the latter case this was made possible by the use of a conversion tool that allowed the direct use of the data from other libraries in Geant4. Overall it was found that there was good agreement with experiment for some of the neutron data bases like ENDF/B-VII.0 or JENDL-3.3 but not with the others such as ENDF/B-VI.8 or JEFF-3.1. |
| Address |
[Tain, J. L.; Agramunt, J.; Algora, A.; Jordan, M. D.] Univ Valencia, CSIC, Inst Fis Corpuscular, E-28040 Valencia, Spain, Email: tain@ific.uv.es |
| Corporate Author |
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Thesis |
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| Publisher |
Elsevier Science Bv |
Place of Publication |
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Editor |
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| Language |
English |
Summary Language |
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Original Title |
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| Series Editor |
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Series Title |
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Abbreviated Series Title |
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| Series Volume |
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Series Issue |
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Edition |
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| ISSN |
0168-9002 |
ISBN |
|
Medium |
|
| Area |
|
Expedition |
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Conference |
|
| Notes |
WOS:000347407800003 |
Approved |
no |
| Is ISI |
yes |
International Collaboration |
yes |
| Call Number |
IFIC @ pastor @ |
Serial |
2076 |
| Permanent link to this record |
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| Author |
Tain, J.L.; Algora, A.; Agramunt, J.; Guadilla, V.; Jordan, M.D.; Montaner-Piza, A.; Rubio, B.; Valencia, E.; Cano-Ott, D.; Gelletly, W.; Martinez, T.; Mendoza, E.; Podolyak, Z.; Regan, P.; Simpson, J.; Smith, A.J.; Strachan, J. |
| Title |
A decay total absorption spectrometer for DESPEC at FAIR |
Type |
Journal Article |
| Year |
2015 |
Publication |
Nuclear Instruments & Methods in Physics Research A |
Abbreviated Journal |
Nucl. Instrum. Methods Phys. Res. A |
| Volume |
803 |
Issue |
|
Pages |
36-46 |
| Keywords |
Total absorption gamma-ray spectrometer; Scintillation detectors; Beta decay; High-energy beam fragmentation facilities |
| Abstract |
This paper presents the design of a total absorption gamma-ray spectrometer for the determination of beta-decay intensity distributions of exotic nuclear species at the focal plane of the FAIR-NUSTAR Super Fragment Separator. The spectrometer is a key instrument in the DESPEC experiment and the proposed implementation follows extensive design studies and prototype tests. Two options were contemplated, based on Nal(TI) and LaBr3:Ce inorganic scintillation crystals respectively. Monte Carlo simulations and technical considerations determined the optimal configurations consisting of sixteen 15 x 15 x 25 cm(3) crystals for the Nal(Tl) option and one hundred and twenty-eight 5.5 x 5.5 x 11 cm(3) crystals for the LaBr3:Ce option. Minimization of dead material was crucial for maximizing the spectrometer full-energy peak efficiency. Module prototypes were build to verify constructional details and characterize their performance. The measured energy and timing resolution was found to agree rather well with estimates based on simulations of scintillation light transport and collection. The neutron sensitivity of the spectrometer, important when measuring beta-delayed neutron emitters, was investigated by means of Monte Carlo simulations. |
| Address |
[Tain, J. L.; Algora, A.; Agramunt, J.; Guadilla, V.; Jordan, M. D.; Montaner-Piza, A.; Rubio, B.; Valencia, E.] Univ Valencia, Inst Fis Corpuscular, CSIC, E-46071 Valencia, Spain, Email: tain@ific.uv.es |
| Corporate Author |
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Thesis |
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| Publisher |
Elsevier Science Bv |
Place of Publication |
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Editor |
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| Language |
English |
Summary Language |
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Original Title |
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| Series Editor |
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Series Title |
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Abbreviated Series Title |
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| Series Volume |
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Series Issue |
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Edition |
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| ISSN |
0168-9002 |
ISBN |
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Medium |
|
| Area |
|
Expedition |
|
Conference |
|
| Notes |
WOS:000363464600007 |
Approved |
no |
| Is ISI |
yes |
International Collaboration |
yes |
| Call Number |
IFIC @ pastor @ |
Serial |
2431 |
| Permanent link to this record |
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| Author |
Tain, J.L. et al; Valencia, E.; Algora, A.; Agramunt, J.; Rubio, B.; Estevez, E.; Jordan, M.D. |
| Title |
Enhanced gamma-Ray Emission from Neutron Unbound States Populated in beta Decay |
Type |
Journal Article |
| Year |
2015 |
Publication |
Physical Review Letters |
Abbreviated Journal |
Phys. Rev. Lett. |
| Volume |
115 |
Issue |
6 |
Pages |
062502 - 5pp |
| Keywords |
|
| Abstract |
Total absorption spectroscopy is used to investigate the beta-decay intensity to states above the neutron separation energy followed by gamma-ray emission in Br-87,Br-88 and Rb-94. Accurate results are obtained thanks to a careful control of systematic errors. An unexpectedly large. intensity is observed in all three cases extending well beyond the excitation energy region where neutron penetration is hindered by low neutron energy. The gamma branching as a function of excitation energy is compared to Hauser-Feshbach model calculations. For Br-87 and Br-88 the gamma branching reaches 57% and 20%, respectively, and could be explained as a nuclear structure effect. Some of the states populated in the daughter can only decay through the emission of a large orbital angular momentum neutron with a strongly reduced barrier penetrability. In the case of neutron-rich Rb-94 the observed 4.5% branching is much larger than the calculations performed with standard nuclear statistical model parameters, even after proper correction for fluctuation effects on individual transition widths. The difference can be reconciled by introducing an enhancement of 1 order of magnitude in the photon strength to neutron strength ratio. An increase in the photon strength function of such magnitude for very neutron-rich nuclei, if it proves to be correct, leads to a similar increase in the (n, gamma) cross section that would have an impact on r process abundance calculations. |
| Address |
[Tain, J. L.; Valencia, E.; Algora, A.; Agramunt, J.; Rubio, B.; Estevez, E.; Jordan, M. D.] Univ Valencia, CSIC, Inst Fis Corpuscular, E-46071 Valencia, Spain, Email: tain@ific.uv.es |
| Corporate Author |
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Thesis |
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| Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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| Language |
English |
Summary Language |
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Original Title |
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| Series Editor |
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Series Title |
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Abbreviated Series Title |
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| Series Volume |
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Series Issue |
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Edition |
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| ISSN |
0031-9007 |
ISBN |
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Medium |
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| Area |
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Expedition |
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Conference |
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| Notes |
WOS:000359059100002 |
Approved |
no |
| Is ISI |
yes |
International Collaboration |
yes |
| Call Number |
IFIC @ pastor @ |
Serial |
2319 |
| Permanent link to this record |
