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Vijande, J., Tedgren, A. C., Ballester, F., Baltas, D., Papagiannis, P., Rivard, M. J., et al. (2021). Source strength determination in iridium-192 and cobalt-60 brachytherapy: A European survey on the level of agreement between clinical measurements and manufacturer certificates. Phys. Imag. Radiat. Oncol., 19, 108–111.
Abstract: Background and purpose: Brachytherapy treatment outcomes depend on the accuracy of the delivered dose distribution, which is proportional to the reference air-kerma rate (RAKR). Current societal recommendations require the medical physicist to compare the measured RAKR values to the manufacturer source calibration certificate. The purpose of this work was to report agreement observed in current clinical practice in the European Union. Materials and methods: A European survey was performed for high- and pulsed-dose-rate (HDR and PDR) highenergy sources (Ir-192 and Co-60), to quantify observed RAKR differences. Medical physicists at eighteen hospitals from eight European countries were contacted, providing 1,032 data points from 2001 to 2020. Results: Over the survey period, 77% of the Ir-192 measurements used a well chamber instead of the older Krieger phantom method. Mean differences with the manufacturer calibration certificate were 0.01% +/- 1.15% for Ir-192 and -0.1% +/- 1.3% for Co-60. Over 95% of RAKR measurements in the clinic were within 3% of the manufacturer calibration certificate. Conclusions: This study showed that the agreement level was generally better than that reflected in prior societal recommendations positing 5%. Future recommendations on high-energy HDR and PDR source calibrations in the clinic may consider tightened agreements levels.
Keywords: RAKR; Calibration; HDR; PDR; Brachytherapy
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Albiol, A., Albiol, F., Paredes, R., Plasencia-Martinez, J. M., Blanco Barrio, A., Garcia Santos, J. M., et al. (2022). A comparison of Covid-19 early detection between convolutional neural networks and radiologists. Insights Imaging, 13(1), 122–12pp.
Abstract: Background The role of chest radiography in COVID-19 disease has changed since the beginning of the pandemic from a diagnostic tool when microbiological resources were scarce to a different one focused on detecting and monitoring COVID-19 lung involvement. Using chest radiographs, early detection of the disease is still helpful in resource-poor environments. However, the sensitivity of a chest radiograph for diagnosing COVID-19 is modest, even for expert radiologists. In this paper, the performance of a deep learning algorithm on the first clinical encounter is evaluated and compared with a group of radiologists with different years of experience. Methods The algorithm uses an ensemble of four deep convolutional networks, Ensemble4Covid, trained to detect COVID-19 on frontal chest radiographs. The algorithm was tested using images from the first clinical encounter of positive and negative cases. Its performance was compared with five radiologists on a smaller test subset of patients. The algorithm's performance was also validated using the public dataset COVIDx. Results Compared to the consensus of five radiologists, the Ensemble4Covid model achieved an AUC of 0.85, whereas the radiologists achieved an AUC of 0.71. Compared with other state-of-the-art models, the performance of a single model of our ensemble achieved nonsignificant differences in the public dataset COVIDx. Conclusion The results show that the use of images from the first clinical encounter significantly drops the detection performance of COVID-19. The performance of our Ensemble4Covid under these challenging conditions is considerably higher compared to a consensus of five radiologists. Artificial intelligence can be used for the fast diagnosis of COVID-19.
Keywords: Deep learning; Covid-19; Radiology
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Bello Garrote, F. L. et al, & Morales, A. I. (2020). beta decay of Ni-75 and the systematics of the low-lying level structure of neutron-rich odd-A Cu isotopes. Phys. Rev. C, 102(3), 034314–13pp.
Abstract: Background: Detailed spectroscopy of neutron-rich odd-A Cu isotopes is of great importance for studying the shell evolution in the region of Ni-78. While there is experimental information on excited states in 69-73,77,79CU isotopes, the information concerning Cu-75 is very limited. Purpose: Experimentally observed single-particle, core-coupling, and proton-hole intruder states in Cu-75, will complete the systematics of these states in the chain of isotopes. Method: Excited states in Cu-75 were populated in the beta decay of Ni-75 isotopes. The Ni nuclei were produced by the in-flight fission of U-238 projectiles, and were separated, identified, and implanted in a highly segmented Si detector array for the detection of the beta-decay electrons. The beta-delayed gamma rays were detected in a HPGe cluster array. Monte Carlo shell model calculations were performed using the A3DA interaction built on the pf g(9/2)d(5/2) model space for both neutrons and protons. Results: A level scheme of Cu-75 was built up to approximate to 4 MeV by performing a gamma-gamma coincidence analysis. The excited states below 2 MeV were interpreted based on the systematics of neutron-rich odd-A Cu isotopes and the results of the shell model calculations. Conclusions: The evolution of the single-particle, core-coupling, and proton-hole intruder states in the chain of neutron-rich odd-A Cu isotopes is discussed in the present work, in connection with the newly observed level structure of Cu-75.
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Biswas, S. et al, Perez-Vidal, R. M., & Domingo-Pardo, C. (2019). Effects of one valence proton on seniority and angular momentum of neutrons in neutron-rich(51)( 122-)(131)Sb isotopes. Phys. Rev. C, 99(6), 064302–21pp.
Abstract: Background: Levels fulfilling the seniority scheme and relevant isomers are commonly observed features in semimagic nuclei; for example, in Sn isotopes (Z = 50). Seniority isomers in Sn, with dominantly pure neutron configurations, directly probe the underlying neutron-neutron (vv) interaction. Furthermore, an addition of a valence proton particle or hole, through neutron-proton (v pi) interaction, affects the neutron seniority as well as the angular momentum. Purpose: Benchmark the reproducibility of the experimental observables, like the excitation energies (E-x) and the reduced electric-quadrupole transition probabilities [B(E2)], with the results obtained from shell-model interactions for neutron-rich Sn and Sb isotopes with N < 82. Study the sensitivity of the aforementioned experimental observables to the model interaction components. Furthermore, explore from a microscopic point of view the structural similarity between the isomers in Sn and Sb, and thus the importance of the valence proton. Methods: The neutron-rich Sb122-131 isotopes were produced as fission fragments in the reaction Be-9(U-238, f) with 6.2 MeV/u beam energy. A unique setup, consisting of AGATA, VAMOS++, and EXOGAM detectors, was used which enabled the prompt-delayed gamma-ray spectroscopy of fission fragments in the time range of 100 ns to 200 μs. Results: New isomers and prompt and delayed transitions were established in the even-A Sb122-131 isotopes. In the odd-A Sb122-131 isotopes, new prompt and delayed gamma-ray transitions were identified, in addition to the confirmation of the previously known isomers. The half-lives of the isomeric states and the B(E2) transition probabilities of the observed transitions depopulating these isomers were extracted. Conclusions: The experimental data was compared with the theoretical results obtained in the framework of large-scale shell-model (LSSM) calculations in a restricted model space. Modifications of several components of the shell-model interaction were introduced to obtain a consistent agreement with the excitation energies and the B(E2) transition probabilities in neutron-rich Sn and Sb isotopes. The isomeric configurations in Sn and Sb were found to be relatively pure. Furthermore, the calculations revealed that the presence of a single valence proton, mainly in the g(7/2) orbital in Sb isotopes, leads to significant mixing (due to the v pi interaction) of (i) the neutron seniorities (upsilon(v)) and (ii) the neutron angular momentum (I-v). The above features have a weak impact on the excitation energies, but have an important impact on the B(E2) transition probabilities. In addition, a constancy of the relative excitation energies irrespective of neutron seniority and neutron number in Sn and Sb was observed.
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n_TOF Collaboration(Stamatopoulos, A. et al), Domingo-Pardo, C., Tain, J. L., & Tarifeño-Saldivia, A. (2020). Investigation of the Pu-240(n, f) reaction at the n_TOF/EAR2 facility in the 9 meV-6 MeV range. Phys. Rev. C, 102(1), 014616–23pp.
Abstract: Background: Nuclear waste management is considered amongst the major challenges in the field of nuclear energy. A possible means of addressing this issue is waste transmutation in advanced nuclear systems, whose operation requires a fast neutron spectrum. In this regard, the accurate knowledge of neutron-induced reaction cross sections of several (minor) actinide isotopes is essential for design optimization and improvement of safety margins of such systems. One such case is Pu-240, due to its accumulation in spent nuclear fuel of thermal reactors and its usage in fast reactor fuel. The measurement of the Pu-240(n, f) cross section was previously attempted at the CERN nTOF facility EAR1 measuring station using the time-of-flight technique. Due to the low amount of available material and the given flux at EAR1, the measurement had to last several months to achieve a sufficient statistical accuracy. This long duration led to detector deterioration due to the prolonged exposure to the high alpha activity of the fission foils, therefore the measurement could not be successfully completed. Purpose: It is aimed to determine whether it is feasible to study neutron-induced fission at nTOF/EAR2 and provide data on the Pu-240(n, f) reaction in energy regions requested for applications. Methods: The study of the Pu-240(n, f) reaction was made at a new experimental area (EAR2) with a shorter flight path which delivered on average 30 times higher flux at fast neutron energies. This enabled the measurement to be performed much faster, thus limiting the exposure of the detectors to the intrinsic activity of the fission foils. The experimental setup was based on microbulk Micromegas detectors and the time-of-flight data were analyzed with an optimized pulse-shape analysis algorithm. Special attention was dedicated to the estimation of the non-negligible counting loss corrections with the development of a new methodology, and other corrections were estimated via Monte Carlo simulations of the experimental setup. Results: This new measurement of the Pu-240(n, f) cross section yielded data from 9 meV up to 6 MeV incident neutron energy and fission resonance kernels were extracted up to 10 keV. Conclusions: Neutron-induced fission of high activity samples can be successfully studied at the n_TOF/EAR2 facility at CERN covering a wide range of neutron energies, from thermal to a few MeV.
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Siciliano, M. et al, & Gadea, A. (2020). Shape coexistence in neutron-deficient Hg-188 investigated via lifetime measurements. Phys. Rev. C, 102(1), 014318–16pp.
Abstract: Background: Shape coexistence in the Z approximate to 82 region has been established in mercury, lead, and polonium isotopes. For even-even mercury isotopes with 100 <= N <= 106 multiple fingerprints of this phenomenon are observed, which seems to be no longer present for N >= 110. According to a number of theoretical calculations, shape coexistence is predicted in the Hg-188 isotope. Purpose: The aim of this work was to measure lifetimes of excited states in Hg-188 to infer their collective properties, such as the deformation. Extending the investigation to higher-spin states, which are expected to be less affected by band-mixing effects, can provide additional information on the coexisting structures. Methods: The Hg-188 nucleus was populated using two different fusion-evaporation reactions with two targets, Gd-158 and Gd-160, and a beam of S-34 provided by the Tandem-ALPI accelerator complex at the Laboratori Nazionali di Legnaro. The channels of interest were selected using the information from the Neutron Wall array, while the gamma rays were detected using the GALILEO gamma-ray spectrometer. Lifetimes of excited states were determined using the recoil-distance Doppler-shift method, employing the dedicated GALILEO plunger device. Results: Lifetimes of the states up to spin 16 (h) over bar were measured and the corresponding reduced transition probabilities were calculated. Assuming two-band mixing and adopting, as done commonly, the rotational model, the mixing strengths and the deformation parameters of the unperturbed structures were obtained from the experimental results. In order to shed light on the nature of the observed configurations in the Hg-188 nucleus, the extracted transition strengths were compared with those resulting from state-of-the-art beyond-mean-field calculations using the symmetry-conserving configuration-mixing approach, limited to axial shapes, and the five-dimensional collective Hamiltonian, including the triaxial degree of freedom. Conclusions: The first lifetime measurement for states with spin >= 6 suggested the presence of an almost spherical structure above the 12(1)(+) isomer and allowed elucidating the structure of the intruder band. The comparison of the extracted B(E2) strengths with the two-band mixing model allowed the determination of the ground-state band deformation. Both beyond-mean-field calculations predict coexistence of a weakly deformed band with a strongly prolate-deformed one, characterized by elongation parameters similar to those obtained experimentally, but the calculated relative position of the bands and their mixing strongly differ.
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n_TOF Collaboration(Tagliente, G. et al), Domingo-Pardo, C., Giubrone, G., Tain, J. L., & Tarifeño-Saldivia, A. (2022). Zr-92(n, gamma) and (n,tot) measurements at the GELINA and n_TOF facilities. Phys. Rev. C, 105(2), 025805–14pp.
Abstract: Background: Stellar nucleosynthesis of elements heavier than iron is driven by neutron capture processes. Zr-92 is positioned at a strategic point along the slow nucleosynthesis path, given its proximity to the neutron magic number N = 50 and its position at the matching region between the weak and main slow processes. Purpose: In parallel with recent improved astronomical data, the extraction of accurate Maxwellian averaged cross sections (MACSs) derived from a more complete and accurate set of resonance parameters should allow for a better understanding of the stellar conditions at which nucleosynthesis takes place. Methods: Transmission and capture cross section measurements using enriched Zr-92 metallic samples were performed at the time-of flight facilities GELINA of JRC-Geel (BE) and nTOF of CERN (CH). The neutron beam passing through the samples was investigated in transmission measurements at GELINA using a Li-glass scintillator. The gamma rays emitted during the neutron capture reactions were detected by C6D6 detectors at both GELINA and nTOF. Results: Resonance parameters of individual resonances up to 81 keV were extracted from a combined resonance shape analysis of experimental transmissions and capture yields. For the majority of the resonances the parity was determined from an analysis of the transmission data obtained with different sample thicknesses. Average resonance parameters were calculated. Conclusions: Maxwellian averaged cross sections were extracted from resonances observed up to 81 keV. The MACS for kT = 30 keV is fully consistent with experimental data reported in the literature. The MACSs for kT less than or similar to 15 keV are in good agreement with those derived from the ENDF/B-VIII.0 library and recommended in the KADoNTS database. For kT higher than 30 keV differences are observed. A comparison with MACSs obtained with the cross sections recommended in the JEFF-3.3 and JENDL-4.0 libraries shows discrepancies even for kT less than or similar to 15 keV.
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n_TOF Collaboration(Torres-Sanchez, P. et al), Babiano-Suarez, V., Caballero, L., Domingo-Pardo, C., Ladarescu, I., & Tain, J. L. (2023). Measurement of the 14N(n, p) 14C cross section at the CERN n_TOF facility from subthermal energy to 800 keV. Phys. Rev. C, 107(6), 064617–15pp.
Abstract: Background: The 14N(n, p) 14C reaction is of interest in neutron capture therapy, where nitrogen-related dose is the main component due to low-energy neutrons, and in astrophysics, where 14N acts as a neutron poison in the s process. Several discrepancies remain between the existing data obtained in partial energy ranges: thermal energy, keV region, and resonance region. Purpose: We aim to measure the 14N(n, p) 14C cross section from thermal to the resonance region in a single measurement for the first time, including characterization of the first resonances, and provide calculations of Maxwellian averaged cross sections (MACS). Method: We apply the time-of-flight technique at Experimental Area 2 (EAR-2) of the neutron time-of-flight (n_TOF) facility at CERN. 10B(n, & alpha;) 7Li and 235U(n, f ) reactions are used as references. Two detection systems are run simultaneously, one on beam and another off beam. Resonances are described with the R-matrix code SAMMY. Results: The cross section was measured from subthermal energy to 800 keV, resolving the first two resonances (at 492.7 and 644 keV). A thermal cross section was obtained (1.809 & PLUSMN; 0.045 b) that is lower than the two most recent measurements by slightly more than one standard deviation, but in line with the ENDF/B-VIII.0 and JEFF-3.3 evaluations. A 1/v energy dependence of the cross section was confirmed up to tens of keV neutron energy. The low energy tail of the first resonance at 492.7 keV is lower than suggested by evaluated values, while the overall resonance strength agrees with evaluations. Conclusions: Our measurement has allowed determination of the 14N(n, p) cross section over a wide energy range for the first time. We have obtained cross sections with high accuracy (2.5%) from subthermal energy to 800 keV and used these data to calculate the MACS for kT = 5 to kT = 100 keV.
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Escrig, S. et al, & Morales, A. I. (2021). Persistence of the Z=28 shell gap in A=75 isobars: Identification of a possible (1/2(-)) μs isomer in Co-75 and beta decay to Ni-75. Phys. Rev. C, 103(6), 064328–12pp.
Abstract: Background: The evolution of shell structure around doubly magic exotic nuclei is of great interest in nuclear physics and astrophysics. In the 'southwest' region of Ni-78, the development of deformation might trigger a major shift in our understanding of explosive nucleosynthesis. To this end, new spectroscopic information on key close-lying nuclei is very valuable. Purpose: We intend to measure the isomeric and beta decay of Co-75, with one-proton and two-neutron holes relative to Ni-78, to access new nuclear structure information in Co-75 and its beta-decay daughters Ni-75 and Ni-74. Methods: The nucleus Co-75 is produced in relativistic in-flight fission reactions of U-238 at the Radioactive Ion Beam Factory in the RIKEN Nishina Center. Its isomeric and f decay are studied exploiting the BigRIPS and EURICA setups. Results: We obtain partial beta-decay spectra for Ni-75 and Ni-74, and report a new isomeric transition in Co-75. The energy [E-gamma = 1914(2) keV] and half-life [t(1/2) = 13(6) μs] of the delayed gamma ray lend support for the existence of aJ(pi) = (1/2(-)) isomeric state at 1914(2) keV. A comparison with PFSDG-U shell-model calculations provides a good account for the observed states in Ni-75, but the first calculated 1/2(-) level in Co-75, a prolate K = 1/2 state, is predicted about 1 MeV below the observed (1/2(-)) level. Conclusions: The spherical-like structure of the lowest-lying excited states in Ni-75 is proved. In the case of Co-75, the results suggest that the dominance of the spherical configurations over the deformed ones might be stronger than expected below Ni-78. Further experimental efforts to discern the nature of the J(pi) = (1/2(-)) isomer are necessary.
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Siciliano, M. et al, Gadea, A., & Perez-Vidal, R. M. (2021). Lifetime measurements in the even-even Cd102-108 isotopes. Phys. Rev. C, 104(3), 034320–16pp.
Abstract: Background: The heaviest T-z = 0 doubly-magic nucleus, Sn-100, and the neighboring nuclei offer unique opportunities to investigate the properties of nuclear interaction. For instance, the structure of light-Sn nuclei has been shown to be affected by the delicate balance between nuclear-interaction components, such as pairing and quadrupole correlations. From Cd to Te, many common features and phenomena have been observed experimentally along the isotopic chains, leading to theoretical studies devoted to a more general and comprehensive study of the region. In this context, having only two proton holes in the Z = 50 shell, the Cd isotopes are expected to present properties similar to those found in the Sn isotopic chain. Purpose: The aim of this work was to measure lifetimes of excited states in neutron-deficient nuclei in the vicinity of Sn-100. Methods: The neutron-deficient nuclei in the N approximate to Z approximate to 50 region were populated using a multinucleon transfer reaction with a Cd-106 beam and a Mo-92 target. The beamlike products were identified by the VAMOS++ spectrometer, while the gamma rays were detected using the AGATA array. Lifetimes of excited states were determined using the recoil distance Doppler-shift method, employing the Cologne differential plunger. Results: Lifetimes of low-lying states were measured in the even-mass Cd-102-(108) isotopes. In particular, multiple states with excitation energy up to MeV, belonging to various bands, were populated in approximate to 3 Cd-106 via inelastic scattering. The transition strengths corresponding to the measured lifetimes were compared with those resulting from state-of-the-art beyond-mean-field calculations using the symmetry-conserving configuration-mixing approach. Conclusions: Despite the similarities in the electromagnetic properties of the low-lying states, there is a fundamental structural difference between the ground-state bands in the Z = 48 and Z = 50 isotopes. The comparison between experimental and theoretical results revealed a rotational character of the Cd nuclei, which have prolate-deformed ground states with beta(2) approximate to 0.2. At this deformation Z = 48 becomes a closed-shell configuration, which is favored with respect to the spherical one.
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