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Siciliano, M. et al, & Gadea, A. (2020). Shape coexistence in neutron-deficient Hg-188 investigated via lifetime measurements. Phys. Rev. C, 102(1), 014318–16pp.
Abstract: Background: Shape coexistence in the Z approximate to 82 region has been established in mercury, lead, and polonium isotopes. For even-even mercury isotopes with 100 <= N <= 106 multiple fingerprints of this phenomenon are observed, which seems to be no longer present for N >= 110. According to a number of theoretical calculations, shape coexistence is predicted in the Hg-188 isotope. Purpose: The aim of this work was to measure lifetimes of excited states in Hg-188 to infer their collective properties, such as the deformation. Extending the investigation to higher-spin states, which are expected to be less affected by band-mixing effects, can provide additional information on the coexisting structures. Methods: The Hg-188 nucleus was populated using two different fusion-evaporation reactions with two targets, Gd-158 and Gd-160, and a beam of S-34 provided by the Tandem-ALPI accelerator complex at the Laboratori Nazionali di Legnaro. The channels of interest were selected using the information from the Neutron Wall array, while the gamma rays were detected using the GALILEO gamma-ray spectrometer. Lifetimes of excited states were determined using the recoil-distance Doppler-shift method, employing the dedicated GALILEO plunger device. Results: Lifetimes of the states up to spin 16 (h) over bar were measured and the corresponding reduced transition probabilities were calculated. Assuming two-band mixing and adopting, as done commonly, the rotational model, the mixing strengths and the deformation parameters of the unperturbed structures were obtained from the experimental results. In order to shed light on the nature of the observed configurations in the Hg-188 nucleus, the extracted transition strengths were compared with those resulting from state-of-the-art beyond-mean-field calculations using the symmetry-conserving configuration-mixing approach, limited to axial shapes, and the five-dimensional collective Hamiltonian, including the triaxial degree of freedom. Conclusions: The first lifetime measurement for states with spin >= 6 suggested the presence of an almost spherical structure above the 12(1)(+) isomer and allowed elucidating the structure of the intruder band. The comparison of the extracted B(E2) strengths with the two-band mixing model allowed the determination of the ground-state band deformation. Both beyond-mean-field calculations predict coexistence of a weakly deformed band with a strongly prolate-deformed one, characterized by elongation parameters similar to those obtained experimentally, but the calculated relative position of the bands and their mixing strongly differ.
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n_TOF Collaboration(Tagliente, G. et al), Domingo-Pardo, C., Giubrone, G., Tain, J. L., & Tarifeño-Saldivia, A. (2022). Zr-92(n, gamma) and (n,tot) measurements at the GELINA and n_TOF facilities. Phys. Rev. C, 105(2), 025805–14pp.
Abstract: Background: Stellar nucleosynthesis of elements heavier than iron is driven by neutron capture processes. Zr-92 is positioned at a strategic point along the slow nucleosynthesis path, given its proximity to the neutron magic number N = 50 and its position at the matching region between the weak and main slow processes. Purpose: In parallel with recent improved astronomical data, the extraction of accurate Maxwellian averaged cross sections (MACSs) derived from a more complete and accurate set of resonance parameters should allow for a better understanding of the stellar conditions at which nucleosynthesis takes place. Methods: Transmission and capture cross section measurements using enriched Zr-92 metallic samples were performed at the time-of flight facilities GELINA of JRC-Geel (BE) and nTOF of CERN (CH). The neutron beam passing through the samples was investigated in transmission measurements at GELINA using a Li-glass scintillator. The gamma rays emitted during the neutron capture reactions were detected by C6D6 detectors at both GELINA and nTOF. Results: Resonance parameters of individual resonances up to 81 keV were extracted from a combined resonance shape analysis of experimental transmissions and capture yields. For the majority of the resonances the parity was determined from an analysis of the transmission data obtained with different sample thicknesses. Average resonance parameters were calculated. Conclusions: Maxwellian averaged cross sections were extracted from resonances observed up to 81 keV. The MACS for kT = 30 keV is fully consistent with experimental data reported in the literature. The MACSs for kT less than or similar to 15 keV are in good agreement with those derived from the ENDF/B-VIII.0 library and recommended in the KADoNTS database. For kT higher than 30 keV differences are observed. A comparison with MACSs obtained with the cross sections recommended in the JEFF-3.3 and JENDL-4.0 libraries shows discrepancies even for kT less than or similar to 15 keV.
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n_TOF Collaboration(Torres-Sanchez, P. et al), Babiano-Suarez, V., Caballero, L., Domingo-Pardo, C., Ladarescu, I., & Tain, J. L. (2023). Measurement of the 14N(n, p) 14C cross section at the CERN n_TOF facility from subthermal energy to 800 keV. Phys. Rev. C, 107(6), 064617–15pp.
Abstract: Background: The 14N(n, p) 14C reaction is of interest in neutron capture therapy, where nitrogen-related dose is the main component due to low-energy neutrons, and in astrophysics, where 14N acts as a neutron poison in the s process. Several discrepancies remain between the existing data obtained in partial energy ranges: thermal energy, keV region, and resonance region. Purpose: We aim to measure the 14N(n, p) 14C cross section from thermal to the resonance region in a single measurement for the first time, including characterization of the first resonances, and provide calculations of Maxwellian averaged cross sections (MACS). Method: We apply the time-of-flight technique at Experimental Area 2 (EAR-2) of the neutron time-of-flight (n_TOF) facility at CERN. 10B(n, & alpha;) 7Li and 235U(n, f ) reactions are used as references. Two detection systems are run simultaneously, one on beam and another off beam. Resonances are described with the R-matrix code SAMMY. Results: The cross section was measured from subthermal energy to 800 keV, resolving the first two resonances (at 492.7 and 644 keV). A thermal cross section was obtained (1.809 & PLUSMN; 0.045 b) that is lower than the two most recent measurements by slightly more than one standard deviation, but in line with the ENDF/B-VIII.0 and JEFF-3.3 evaluations. A 1/v energy dependence of the cross section was confirmed up to tens of keV neutron energy. The low energy tail of the first resonance at 492.7 keV is lower than suggested by evaluated values, while the overall resonance strength agrees with evaluations. Conclusions: Our measurement has allowed determination of the 14N(n, p) cross section over a wide energy range for the first time. We have obtained cross sections with high accuracy (2.5%) from subthermal energy to 800 keV and used these data to calculate the MACS for kT = 5 to kT = 100 keV.
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n_TOF Collaboration(Mendoza, E. et al), Domingo-Pardo, C., & Tain, J. L. (2014). Measurement and analysis of the Am-243 neutron capture cross section at the n_TOF facility at CERN. Phys. Rev. C, 90(3), 034608–16pp.
Abstract: Background: The design of new nuclear reactors and transmutation devices requires to reduce the present neutron cross section uncertainties of minor actinides. Purpose: Improvement of the Am-243(n, gamma) cross section uncertainty. Method: The Am-243(n, gamma) cross section has been measured at the n_TOF facility at CERN with a BaF2 total absorption calorimeter, in the energy range between 0.7 eV and 2.5 keV. Results: The Am-243(n, gamma) cross section has been successfully measured in the mentioned energy range. The resolved resonance region has been extended from 250 eV up to 400 eV. In the unresolved resonance region our results are compatible with one of the two incompatible capture data sets available below 2.5 keV. The data available in EXFOR and in the literature have been used to perform a simple analysis above 2.5 keV. Conclusions: The results of this measurement contribute to reduce the Am-243(n, gamma) cross section uncertainty and suggest that this cross section is underestimated up to 25% in the neutron energy range between 50 eV and a few keV in the present evaluated data libraries.
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Escrig, S. et al, & Morales, A. I. (2021). Persistence of the Z=28 shell gap in A=75 isobars: Identification of a possible (1/2(-)) μs isomer in Co-75 and beta decay to Ni-75. Phys. Rev. C, 103(6), 064328–12pp.
Abstract: Background: The evolution of shell structure around doubly magic exotic nuclei is of great interest in nuclear physics and astrophysics. In the 'southwest' region of Ni-78, the development of deformation might trigger a major shift in our understanding of explosive nucleosynthesis. To this end, new spectroscopic information on key close-lying nuclei is very valuable. Purpose: We intend to measure the isomeric and beta decay of Co-75, with one-proton and two-neutron holes relative to Ni-78, to access new nuclear structure information in Co-75 and its beta-decay daughters Ni-75 and Ni-74. Methods: The nucleus Co-75 is produced in relativistic in-flight fission reactions of U-238 at the Radioactive Ion Beam Factory in the RIKEN Nishina Center. Its isomeric and f decay are studied exploiting the BigRIPS and EURICA setups. Results: We obtain partial beta-decay spectra for Ni-75 and Ni-74, and report a new isomeric transition in Co-75. The energy [E-gamma = 1914(2) keV] and half-life [t(1/2) = 13(6) μs] of the delayed gamma ray lend support for the existence of aJ(pi) = (1/2(-)) isomeric state at 1914(2) keV. A comparison with PFSDG-U shell-model calculations provides a good account for the observed states in Ni-75, but the first calculated 1/2(-) level in Co-75, a prolate K = 1/2 state, is predicted about 1 MeV below the observed (1/2(-)) level. Conclusions: The spherical-like structure of the lowest-lying excited states in Ni-75 is proved. In the case of Co-75, the results suggest that the dominance of the spherical configurations over the deformed ones might be stronger than expected below Ni-78. Further experimental efforts to discern the nature of the J(pi) = (1/2(-)) isomer are necessary.
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