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Guadilla, V. et al, Tain, J. L., Algora, A., Agramunt, J., Gelletly, W., Jordan, D., et al. (2018). Characterization and performance of the DTAS detector. Nucl. Instrum. Methods Phys. Res. A, 910, 79–89.
Abstract: DTAS is a segmented total absorption y-ray spectrometer developed for the DESPEC experiment at FAIR. It is composed of up to eighteen NaI(Tl) crystals. In this work we study the performance of this detector with laboratory sources and also under real experimental conditions. We present a procedure to reconstruct offline the sum of the energy deposited in all the crystals of the spectrometer, which is complicated by the effect of NaI(Tl) light-yield non-proportionality. The use of a system to correct for time variations of the gain in individual detector modules, based on a light pulse generator, is demonstrated. We describe also an event-based method to evaluate the summing-pileup electronic distortion in segmented spectrometers. All of this allows a careful characterization of the detector with Monte Carlo simulations that is needed to calculate the response function for the analysis of total absorption gamma-ray spectroscopy data. Special attention was paid to the interaction of neutrons with the spectrometer, since they are a source of contamination in studies of beta-delayed neutron emitting nuclei.
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Nichols, A. L., Dimitriou, P., Algora, A., Fallot, M., Giot, L., Kondev, F. G., et al. (2023). Improving fission-product decay data for reactor applications: part I-decay heat. Eur. Phys. J. A, 59(4), 78–78pp.
Abstract: Effort has been expended to assess the relative merits of undertaking further decay-data measurements of the main fission-product contributors to the decay heat of neutron-irradiated fissionable fuel and related actinides by means of Total Absorption Gamma-ray Spectroscopy (TAGS – sometimes abbreviated to TAS) and Discrete Gamma-ray Spectroscopy (DGS). This review has been carried out following similar work performed under the auspices of OECD/WPEC-Subgroup 25 (2005-2007) and the International Atomic Energy Agency (2009, 2014), and various highly relevant TAGS measurements completed as a consequence of such assessments. We present our recommendations for new decay-data evaluations, along with possible requirements for total absorption and discrete high-resolution gamma-ray spectroscopy studies that cover approximately 120 fission products and various isomeric states.
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Guadilla, V. et al, Algora, A., Tain, J. L., Agramunt, J., Aysto, J., Jordan, D., et al. (2019). Large Impact of the Decay of Niobium Isomers on the Reactor (v)over-bar(e) Summation Calculations. Phys. Rev. Lett., 122(4), 042502–6pp.
Abstract: Even mass neutron-rich niobium isotopes are among the principal contributors to the reactor antineutrino energy spectrum. They are also among the most challenging to measure due to the refractory nature of niobium, and because they exhibit isomeric states lying very close in energy. The beta-intensity distributions of Nb-100gs,Nb-100m and Nb-102gs,Nb-02m beta decays have been determined using the total absorption.-ray spectroscopy technique. The measurements were performed at the upgraded Ion Guide Isotope Separator On-Line facility at the University of Jyvaskyla. Here, the double Penning trap system JYFLTRAP was employed to disentangle the beta decay of the isomeric states. The new data obtained in this challenging measurement have a large impact in antineutrino summation calculations. For the first time the discrepancy between the summation model and the reactor antineutrino measurements in the region of the shape distortion has been reduced.
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n_TOF Collaboration(Barbagallo, M. et al), Domingo-Pardo, C., & Tain, J. L. (2018). Experimental setup and procedure for the measurement of the Be-7(n,p)Li-7 reaction at n_TOF. Nucl. Instrum. Methods Phys. Res. A, 887, 27–33.
Abstract: Following the completion of the second neutron beam line and the related experimental area (EAR2) at the n_TOF spallation neutron source at CERN, several experiments were planned and performed. The high instantaneous neutron flux available in EAR2 allows to investigate neutron induced reactions with charged particles in the exit channel even employing targets made out of small amounts of short-lived radioactive isotopes. After the successful measurement of the Be-7(n,alpha)alpha cross section, the Be-7(n,p)Li-7 reaction was studied in order to provide still missing cross section data of relevance for Big Bang Nucleosynthesis (BBN), in an attempt to find a solution to the cosmological Lithium abundance problem. This paper describes the experimental setup employed in such a measurement and its characterization.
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n_TOF Collaboration(Lederer-Woods, C. et al), Domingo-Pardo, C., Tain, J. L., & Tarifeño-Saldivia, A. (2019). Measurement of Ge-73(n, gamma) cross sections and implications for stellar nucleosynthesis. Phys. Lett. B, 790, 458–465.
Abstract: Ge-73(n, gamma) cross sections were measured at the neutron time-of-flight facility n_TOF at CERN up to neutron energies of 300 keV, providing for the first time experimental data above 8 keV. Results indicate that the stellar cross section at kT = 30 keV is 1.5 to 1.7 times higher than most theoretical predictions. The new cross sections result in a substantial decrease of Ge-73 produced in stars, which would explain the low isotopic abundance of Ge-73 in the solar system.
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Rubio, B., Gelletly, W., Algora, A., Nacher, E., & Tain, J. L. (2017). Beta decay studies with total absorption spectroscopy and the Lucrecia spectrometer at ISOLDE. J. Phys. G, 44(8), 084004–25pp.
Abstract: Here we present the experimental activities carried out at ISOLDE with the total absorption spectrometer Lucrecia, a large 4 pi scintillator detector designed to absorb a full gamma cascade following beta decay. This spectrometer is designed to measure beta-feeding to excited states without the systematic error called Pandemonium. The set up allows the measurement of decays of very short half life. Experimental results from several campaigns, that focus on the determination of the shapes of beta-decaying nuclei by measuring their beta decay strength distributions as a function of excitation energy in the daughter nucleus, are presented.
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Guadilla, V. et al, Tain, J. L., Algora, A., Agramunt, J., Jordan, D., Monserrate, M., et al. (2020). Determination of beta-decay ground state feeding of nuclei of importance for reactor applications. Phys. Rev. C, 102(6), 064304–12pp.
Abstract: In beta-decay studies the determination of the decay probability to the ground state (g.s.) of the daughter nucleus often suffers from large systematic errors. The difficulty of the measurement is related to the absence of associated delayed gamma-ray emission. In this work we revisit the 4 pi gamma – beta method proposed by Greenwood and collaborators in the 1990s, which has the potential to overcome some of the experimental difficulties. Our interest is driven by the need to determine accurately the beta-intensity distributions of fission products that contribute significantly to the reactor decay heat and to the antineutrinos emitted by reactors. A number of such decays have large g.s. branches. The method is relevant for nuclear structure studies as well. Pertinent formulas are revised and extended to the special case of beta-delayed neutron emitters, and the robustness of the method is demonstrated with synthetic data. We apply it to a number of measured decays that serve as test cases and discuss the features of the method. Finally, we obtain g.s. feeding intensities with reduced uncertainty for four relevant decays that will allow future improvements in antineutrino spectrum and decay heat calculations using the summation method.
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n_TOF Collaboration(Bacak, M. et al), Domingo-Pardo, C., & Tain, J. L. (2020). A compact fission detector for fission-tagging neutron capture experiments with radioactive fissile isotopes. Nucl. Instrum. Methods Phys. Res. A, 969, 163981–10pp.
Abstract: In the measurement of neutron capture cross-sections of fissile isotopes, the fission channel is a source of background which can be removed efficiently using the so-called fission-tagging or fission-veto technique. For this purpose a new compact and fast fission chamber has been developed. The design criteria and technical description of the chamber are given within the context of a measurement of the U-233(n, gamma) cross-section at the nTOF facility at CERN, where it was coupled to the nTOF Total Absorption Calorimeter. For this measurement the fission detector was optimized for time resolution, minimization of material in the neutron beam and for alpha-fission discrimination. The performance of the fission chamber and its application as a fission tagging detector are discussed.
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n_TOF Collaboration(Paradela, C. et al), Domingo-Pardo, C., Plag, R., Plompen, A., & Tain, J. L. (2011). (237)Np(n,f) Cross Section: New Data and Present Status. J. Korean Phys. Soc., 59(2), 1908–1911.
Abstract: In this document, we present the final result obtained at the nTOF experiment; for the neutron-induced fission cross section of the (237)Np, from the fission threshold up to 1 GeV. The method applied to get tins result is briefly discussed. nTOF data are compared to the last experimental measurements using other TOF facilities or the surrogate method, reported experiments performed with monoenergetic sources and the FISCAL systematic, including a discussion about the existing discrepancies.
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Fallot, M., Cormon, S., Estienne, M., Algora, A., Bui, V. M., Cucoanes, A., et al. (2012). New Antineutrino Energy Spectra Predictions from the Summation of Beta Decay Branches of the Fission Products. Phys. Rev. Lett., 109(20), 202504–5pp.
Abstract: In this Letter, we study the impact of the inclusion of the recently measured beta decay properties of the Tc-102;104;105;106;107, Mo-105, and Nb-101 nuclei in an updated calculation of the antineutrino energy spectra of the four fissible isotopes U-235,U-238 and Pu-239,Pu-241. These actinides are the main contributors to the fission processes in pressurized water reactors. The beta feeding probabilities of the above-mentioned Tc, Mo, and Nb isotopes have been found to play a major role in the gamma component of the decay heat of Pu-239, solving a large part of the gamma discrepancy in the 4-3000 s range. They have been measured by using the total absorption technique, insensitive to the pandemonium effect. The calculations are performed by using the information available nowadays in the nuclear databases, summing all the contributions of the beta decay branches of the fission products. Our results provide a new prediction of the antineutrino energy spectra of U-235, Pu-239,Pu-241, and, in particular, U-238 for which no measurement has been published yet. We conclude that new total absorption technique measurements are mandatory to improve the reliability of the predicted spectra.
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