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AGATA Collaboration (Louchart, C. et al); Gadea, A.; Huyuk, T. |
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Title |
Collective nature of low-lying excitations in 70,72,74Zn from lifetime measurements using the AGATA spectrometer demonstrator |
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Journal Article |
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Year |
2013 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
87 |
Issue |
5 |
Pages |
054302 - 10pp |
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Background: Neutron-rich nuclei with protons in the fp shell show an onset of collectivity around N=40. Spectroscopic information is required to understand the underlying mechanism and to determine the relevant terms of the nucleon-nucleon interaction that are responsible for the evolution of the shell structure in this mass region. Methods: We report on the lifetime measurement of the first 2+ and 4+ states in 70,72,74Zn and the first 6+ state in 72Zn using the recoil distance Doppler shift method. The experiment was carried out at the INFN Laboratory of Legnaro with the AGATA demonstrator, first phase of the Advanced Gamma Tracking Array of highly segmented, high-purity germanium detectors coupled to the PRISMA magnetic spectrometer. The excited states of the nuclei of interest were populated in the deep inelastic scattering of a 76Ge beam impinging on a 238U target. Results: The maximum of collectivity along the chain of Zn isotopes is observed for 72Zn at N=42. An unexpectedly long lifetime of 20−5.2+1.8 ps was measured for the 4+ state in 74Zn. Conclusions: Our results lead to small values of the B(E2;41+→21+)/B(E2;21+→01+) ratio for 72,74Zn, suggesting a significant noncollective contribution to these excitations. These experimental results are not reproduced by state-of-the-art microscopic models and call for lifetime measurements beyond the first 2+ state in heavy zinc and nickel isotopes. |
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no |
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yes |
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yes |
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IFIC @ pastor @ |
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1638 |
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Birkenbach, B. et al; Gadea, A. |
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Title |
Spectroscopy of the neutron-rich actinide nucleus U-240 following multinucleon-transfer reactions |
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Journal Article |
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Year |
2015 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
92 |
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4 |
Pages |
044319 - 9pp |
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Background: Nuclear structure information for the neutron-rich actinide nuclei is important since it is the benchmark for theoretical models that provide predictions for the heaviest nuclei. Purpose: gamma-ray spectroscopy of neutron-rich heavy nuclei in the actinide region. Method: Multinucleon-transfer reactions in Zn-70 + U-238 and Xe-136 + U-238 have been measured in two experiments performed at the INFN Legnaro, Italy. In the Zn-70 experiment the high-resolution HPGe Clover Array (CLARA) coupled to the magnetic spectrometer PRISMA was employed. In the Xe-136 experiment the high-resolution Advanced Gamma Tracking Array (AGATA) was used in combination with PRISMA and the Detector Array for Multinucleon Transfer Ejectiles (DANTE). Results: The ground-state band (g.s. band) of U-240 was measured up to the 20(+) level and a tentative assignment was made up to the (24(+)) level. Results from gamma gamma coincidence and from particle coincidence analyses are shown. Moments of inertia (MoI) show a clear upbend. Evidence for an extended first negative-parity band of U-240 is found. Conclusions: A detailed comparison with latest calculations shows best agreement with cranked relativistic Hartree-Bogoliubov (CRHB) calculations for the g.s. band properties. The negative-parity band shows the characteristics of a K-pi = 0 band based on an octupole vibration. |
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[Birkenbach, B.; Vogt, A.; Geibel, K.; Reiter, P.; Eberth, J.; Hess, H.; Jolie, J.; Radeck, F.; Steinbach, T.; Wiens, A.] Univ Cologne, Inst Kernphys, D-50937 Cologne, Germany, Email: birkenbach@ikp.uni-koeln.de |
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Amer Physical Soc |
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0556-2813 |
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WOS:000363236900001 |
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no |
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yes |
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yes |
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Call Number |
IFIC @ pastor @ |
Serial |
2421 |
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n_TOF Collaboration (Stamatopoulos, A. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Investigation of the Pu-240(n, f) reaction at the n_TOF/EAR2 facility in the 9 meV-6 MeV range |
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Journal Article |
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2020 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
102 |
Issue |
1 |
Pages |
014616 - 23pp |
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Background: Nuclear waste management is considered amongst the major challenges in the field of nuclear energy. A possible means of addressing this issue is waste transmutation in advanced nuclear systems, whose operation requires a fast neutron spectrum. In this regard, the accurate knowledge of neutron-induced reaction cross sections of several (minor) actinide isotopes is essential for design optimization and improvement of safety margins of such systems. One such case is Pu-240, due to its accumulation in spent nuclear fuel of thermal reactors and its usage in fast reactor fuel. The measurement of the Pu-240(n, f) cross section was previously attempted at the CERN nTOF facility EAR1 measuring station using the time-of-flight technique. Due to the low amount of available material and the given flux at EAR1, the measurement had to last several months to achieve a sufficient statistical accuracy. This long duration led to detector deterioration due to the prolonged exposure to the high alpha activity of the fission foils, therefore the measurement could not be successfully completed. Purpose: It is aimed to determine whether it is feasible to study neutron-induced fission at nTOF/EAR2 and provide data on the Pu-240(n, f) reaction in energy regions requested for applications. Methods: The study of the Pu-240(n, f) reaction was made at a new experimental area (EAR2) with a shorter flight path which delivered on average 30 times higher flux at fast neutron energies. This enabled the measurement to be performed much faster, thus limiting the exposure of the detectors to the intrinsic activity of the fission foils. The experimental setup was based on microbulk Micromegas detectors and the time-of-flight data were analyzed with an optimized pulse-shape analysis algorithm. Special attention was dedicated to the estimation of the non-negligible counting loss corrections with the development of a new methodology, and other corrections were estimated via Monte Carlo simulations of the experimental setup. Results: This new measurement of the Pu-240(n, f) cross section yielded data from 9 meV up to 6 MeV incident neutron energy and fission resonance kernels were extracted up to 10 keV. Conclusions: Neutron-induced fission of high activity samples can be successfully studied at the n_TOF/EAR2 facility at CERN covering a wide range of neutron energies, from thermal to a few MeV. |
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[Stamatopoulos, A.; Tsinganis, A.; Kokkoris, M.; Vlastou, R.; Diakaki, M.] Natl Tech Univ Athens, Athens, Greece, Email: athanasios.stamatopoulos@cern.ch |
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Amer Physical Soc |
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0556-2813 |
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WOS:000551057500002 |
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no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4466 |
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Author |
Siciliano, M. et al; Gadea, A. |
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Title |
Shape coexistence in neutron-deficient Hg-188 investigated via lifetime measurements |
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Journal Article |
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Year |
2020 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
102 |
Issue |
1 |
Pages |
014318 - 16pp |
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Background: Shape coexistence in the Z approximate to 82 region has been established in mercury, lead, and polonium isotopes. For even-even mercury isotopes with 100 <= N <= 106 multiple fingerprints of this phenomenon are observed, which seems to be no longer present for N >= 110. According to a number of theoretical calculations, shape coexistence is predicted in the Hg-188 isotope. Purpose: The aim of this work was to measure lifetimes of excited states in Hg-188 to infer their collective properties, such as the deformation. Extending the investigation to higher-spin states, which are expected to be less affected by band-mixing effects, can provide additional information on the coexisting structures. Methods: The Hg-188 nucleus was populated using two different fusion-evaporation reactions with two targets, Gd-158 and Gd-160, and a beam of S-34 provided by the Tandem-ALPI accelerator complex at the Laboratori Nazionali di Legnaro. The channels of interest were selected using the information from the Neutron Wall array, while the gamma rays were detected using the GALILEO gamma-ray spectrometer. Lifetimes of excited states were determined using the recoil-distance Doppler-shift method, employing the dedicated GALILEO plunger device. Results: Lifetimes of the states up to spin 16 (h) over bar were measured and the corresponding reduced transition probabilities were calculated. Assuming two-band mixing and adopting, as done commonly, the rotational model, the mixing strengths and the deformation parameters of the unperturbed structures were obtained from the experimental results. In order to shed light on the nature of the observed configurations in the Hg-188 nucleus, the extracted transition strengths were compared with those resulting from state-of-the-art beyond-mean-field calculations using the symmetry-conserving configuration-mixing approach, limited to axial shapes, and the five-dimensional collective Hamiltonian, including the triaxial degree of freedom. Conclusions: The first lifetime measurement for states with spin >= 6 suggested the presence of an almost spherical structure above the 12(1)(+) isomer and allowed elucidating the structure of the intruder band. The comparison of the extracted B(E2) strengths with the two-band mixing model allowed the determination of the ground-state band deformation. Both beyond-mean-field calculations predict coexistence of a weakly deformed band with a strongly prolate-deformed one, characterized by elongation parameters similar to those obtained experimentally, but the calculated relative position of the bands and their mixing strongly differ. |
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[Siciliano, M.; Zanon, I; Cicerchia, M.; de Angelis, G.; Galtarossa, F.; Gozzelino, A.; Hadynska-Klek, K.; Jaworski, G.; Napoli, D. R.; Valiente-Dobon, J. J.] INFN, Lab Nazl Legnaro, I-35020 Legnaro, Italy, Email: marco.siciliano@lnl.infn.it |
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Amer Physical Soc |
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0556-2813 |
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WOS:000551404600001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4471 |
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Author |
n_TOF Collaboration (Tagliente, G. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Zr-92(n, gamma) and (n,tot) measurements at the GELINA and n_TOF facilities |
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Journal Article |
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2022 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
105 |
Issue |
2 |
Pages |
025805 - 14pp |
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Background: Stellar nucleosynthesis of elements heavier than iron is driven by neutron capture processes. Zr-92 is positioned at a strategic point along the slow nucleosynthesis path, given its proximity to the neutron magic number N = 50 and its position at the matching region between the weak and main slow processes. Purpose: In parallel with recent improved astronomical data, the extraction of accurate Maxwellian averaged cross sections (MACSs) derived from a more complete and accurate set of resonance parameters should allow for a better understanding of the stellar conditions at which nucleosynthesis takes place. Methods: Transmission and capture cross section measurements using enriched Zr-92 metallic samples were performed at the time-of flight facilities GELINA of JRC-Geel (BE) and nTOF of CERN (CH). The neutron beam passing through the samples was investigated in transmission measurements at GELINA using a Li-glass scintillator. The gamma rays emitted during the neutron capture reactions were detected by C6D6 detectors at both GELINA and nTOF. Results: Resonance parameters of individual resonances up to 81 keV were extracted from a combined resonance shape analysis of experimental transmissions and capture yields. For the majority of the resonances the parity was determined from an analysis of the transmission data obtained with different sample thicknesses. Average resonance parameters were calculated. Conclusions: Maxwellian averaged cross sections were extracted from resonances observed up to 81 keV. The MACS for kT = 30 keV is fully consistent with experimental data reported in the literature. The MACSs for kT less than or similar to 15 keV are in good agreement with those derived from the ENDF/B-VIII.0 library and recommended in the KADoNTS database. For kT higher than 30 keV differences are observed. A comparison with MACSs obtained with the cross sections recommended in the JEFF-3.3 and JENDL-4.0 libraries shows discrepancies even for kT less than or similar to 15 keV. |
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[Tagliente, G.; Barbagallo, M.; Colonna, N.; Mastromarco, M.; Variale, V.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: giuseppe.tagliente@ba.infn.it |
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Amer Physical Soc |
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2469-9985 |
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WOS:000766732800002 |
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no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5163 |
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