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Caballero-Folch, R. et al; Domingo-Pardo, C.; Agramunt, J.; Algora, A.; Rubio, B.; Tain, J.L. |
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Title |
beta-decay half-lives and beta-delayed neutron emission probabilities for several isotopes of Au, Hg, Tl, Pb, and Bi, beyond N=126 |
Type |
Journal Article |
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Year |
2017 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
95 |
Issue |
6 |
Pages |
064322 - 16pp |
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Abstract  |
Background: There have been measurements on roughly 230 nuclei that are beta-delayed neutron emitters. They range from He-8 up to La-150. Apart from 210Tl, with a branching ratio of only 0.007%, no other neutron emitter has been measured beyond A = 150. Therefore, new data are needed, particularly in the region of heavy nuclei around N = 126, in order to guide theoretical models and help understand the formation of the third r-process peak at A similar to 195. Purpose: To measure both beta-decay half-lives and neutron branching ratios of several neutron-rich Au, Hg, Tl, Pb, and Bi isotopes beyond N = 126. Method: Ions of interest were produced by fragmentation of a U-238 beam, selected and identified via the GSI-FRS fragment separator. A stack of segmented silicon detectors (SIMBA) was used to measure ion implants and beta decays. An array of 30 He-3 tubes embedded in a polyethylene matrix (BELEN) was used to detect neutrons with high efficiency and selectivity. A self-triggered digital system is employed to acquire data and to enable time correlations. The latter were analyzed with an analytical model and results for the half-lives and neutron-branching ratios were derived by using the binned maximum-likelihood method. Results: Twenty new beta-decay half-lives are reported for Au204-206, Hg208-211, Tl211-216, Pb215-218, and Bi218-220, nine of them for the first time. Neutron emission probabilities are reported for Hg-210,Hg-211 and Tl211-216. Conclusions: The new beta-decay half-lives are in good agreement with previous measurements on nuclei in this region. The measured neutron emission probabilities are comparable to or smaller than values predicted by global models such as relativistic Hartree Bogoliubov plus the relativistic quasi-particle random phase approximation (RHB + RQRPA). |
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Address |
[Caballero-Folch, R.; Calvino, F.; Cortes, G.; Gomez-Hornillos, M. B.; Riego, A.] Univ Politecn Cataluna, DFEN, INTE, E-08028 Barcelona, Spain, Email: rcaballero-folch@triumf.ca |
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Amer Physical Soc |
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English |
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2469-9985 |
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Notes |
WOS:000404022100001 |
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no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3176 |
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Author |
n_TOF Collaboration (Moreno-Soto, J. et al); Babiano-Suarez, V.; Caballero-Ontanaya, L.; Domingo-Pardo, C.; Ladarescu, I.; Tain, J.L. |
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Title |
Constraints on the dipole photon strength for the odd uranium isotopes |
Type |
Journal Article |
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Year |
2022 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
105 |
Issue |
2 |
Pages |
024618 - 14pp |
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Keywords |
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Abstract |
Background: The photon strength functions (PSFs) and nuclear level density (NLD) are key ingredients for calculation of the photon interaction with nuclei, in particular the reaction cross sections. These cross sections are important especially in nuclear astrophysics and in the development of advanced nuclear technologies. Purpose: The role of the scissors mode in the M1 PSF of (well-deformed) actinides was investigated by several experimental techniques. The analyses of different experiments result in significant differences, especially on the strength of the mode. The shape of the low-energy tail of the giant electric dipole resonance is uncertain as well. In particular, some works proposed a presence of the E1 pygmy resonance just above 7 MeV. Because of these inconsistencies additional information on PSFs in this region is of great interest. Methods: The gamma-ray spectra from neutron-capture reactions on the U-234, U-236, and U-238 nuclei have been measured with the total absorption calorimeter of the n_TOF facility at CERN. The background-corrected sum-energy and multi-step-cascade spectra were extracted for several isolated s-wave resonances up to about 140 eV. Results: The experimental spectra were compared to statistical model predictions coming from a large selection of models of photon strength functions and nuclear level density. No combination of PSF and NLD models from literature is able to globally describe our spectra. After extensive search we were able to find model combinations with modified generalized Lorentzian (MGLO) E1 PSF, which match the experimental spectra as well as the total radiative widths. Conclusions: The constant temperature energy dependence is favored for a NLD. The tail of giant electric dipole resonance is well described by the MGLO model of the E1 PSF with no hint of pygmy resonance. The M1 PSF must contain a very strong, relatively wide, and likely double-resonance scissors mode. The mode is responsible for about a half of the total radiative width of neutron resonances and significantly affects the radiative cross section. |
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[Moreno-Soto, J.; Berthoumieux, E.; Dupont, E.; Gunsing, F.; Bacak, M.] Univ Paris Saclay, CEA Irfu, F-91191 Gif Sur Yvette, France, Email: jmoreno53@us.es; |
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Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
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Notes |
WOS:000810791100001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5278 |
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Author |
n_TOF Collaboration (Mendoza, E. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Measurement and analysis of the Am-243 neutron capture cross section at the n_TOF facility at CERN |
Type |
Journal Article |
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Year |
2014 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
90 |
Issue |
3 |
Pages |
034608 - 16pp |
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Abstract |
Background: The design of new nuclear reactors and transmutation devices requires to reduce the present neutron cross section uncertainties of minor actinides. Purpose: Improvement of the Am-243(n, gamma) cross section uncertainty. Method: The Am-243(n, gamma) cross section has been measured at the n_TOF facility at CERN with a BaF2 total absorption calorimeter, in the energy range between 0.7 eV and 2.5 keV. Results: The Am-243(n, gamma) cross section has been successfully measured in the mentioned energy range. The resolved resonance region has been extended from 250 eV up to 400 eV. In the unresolved resonance region our results are compatible with one of the two incompatible capture data sets available below 2.5 keV. The data available in EXFOR and in the literature have been used to perform a simple analysis above 2.5 keV. Conclusions: The results of this measurement contribute to reduce the Am-243(n, gamma) cross section uncertainty and suggest that this cross section is underestimated up to 25% in the neutron energy range between 50 eV and a few keV in the present evaluated data libraries. |
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[Mendoza, E.; Cano-Ott, D.; Guerrero, C.; Alvarez-Velarde, F.; Balibrea, J.; Gonzalez-Romero, E.; Martinez, T.; Villamarin, D.; Vicente, M. C.] CIEMAT, E-28040 Madrid, Spain |
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Amer Physical Soc |
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English |
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ISSN |
0556-2813 |
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Notes |
WOS:000341912100005 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
1935 |
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Author |
n_TOF Collaboration (Torres-Sanchez, P. et al); Babiano-Suarez, V.; Caballero, L.; Domingo-Pardo, C.; Ladarescu, I.; Tain, J.L. |
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Title |
Measurement of the 14N(n, p) 14C cross section at the CERN n_TOF facility from subthermal energy to 800 keV |
Type |
Journal Article |
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Year |
2023 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
107 |
Issue |
6 |
Pages |
064617 - 15pp |
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Keywords |
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Abstract |
Background: The 14N(n, p) 14C reaction is of interest in neutron capture therapy, where nitrogen-related dose is the main component due to low-energy neutrons, and in astrophysics, where 14N acts as a neutron poison in the s process. Several discrepancies remain between the existing data obtained in partial energy ranges: thermal energy, keV region, and resonance region. Purpose: We aim to measure the 14N(n, p) 14C cross section from thermal to the resonance region in a single measurement for the first time, including characterization of the first resonances, and provide calculations of Maxwellian averaged cross sections (MACS). Method: We apply the time-of-flight technique at Experimental Area 2 (EAR-2) of the neutron time-of-flight (n_TOF) facility at CERN. 10B(n, & alpha;) 7Li and 235U(n, f ) reactions are used as references. Two detection systems are run simultaneously, one on beam and another off beam. Resonances are described with the R-matrix code SAMMY. Results: The cross section was measured from subthermal energy to 800 keV, resolving the first two resonances (at 492.7 and 644 keV). A thermal cross section was obtained (1.809 & PLUSMN; 0.045 b) that is lower than the two most recent measurements by slightly more than one standard deviation, but in line with the ENDF/B-VIII.0 and JEFF-3.3 evaluations. A 1/v energy dependence of the cross section was confirmed up to tens of keV neutron energy. The low energy tail of the first resonance at 492.7 keV is lower than suggested by evaluated values, while the overall resonance strength agrees with evaluations. Conclusions: Our measurement has allowed determination of the 14N(n, p) cross section over a wide energy range for the first time. We have obtained cross sections with high accuracy (2.5%) from subthermal energy to 800 keV and used these data to calculate the MACS for kT = 5 to kT = 100 keV. |
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Address |
[Torres-Sanchez, Pablo; Praena, Javier; Porras, Ignacio; Ogallar, Francisco] Univ Granada, Granada, Spain, Email: pablotorres@ugr.es |
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Amer Physical Soc |
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English |
Summary Language |
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Original Title |
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ISSN |
2469-9985 |
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Notes |
WOS:001063209900001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5701 |
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Author |
n_TOF Collaboration (Tagliente, G. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Zr-92(n, gamma) and (n,tot) measurements at the GELINA and n_TOF facilities |
Type |
Journal Article |
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Year |
2022 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
105 |
Issue |
2 |
Pages |
025805 - 14pp |
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Keywords |
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Abstract |
Background: Stellar nucleosynthesis of elements heavier than iron is driven by neutron capture processes. Zr-92 is positioned at a strategic point along the slow nucleosynthesis path, given its proximity to the neutron magic number N = 50 and its position at the matching region between the weak and main slow processes. Purpose: In parallel with recent improved astronomical data, the extraction of accurate Maxwellian averaged cross sections (MACSs) derived from a more complete and accurate set of resonance parameters should allow for a better understanding of the stellar conditions at which nucleosynthesis takes place. Methods: Transmission and capture cross section measurements using enriched Zr-92 metallic samples were performed at the time-of flight facilities GELINA of JRC-Geel (BE) and nTOF of CERN (CH). The neutron beam passing through the samples was investigated in transmission measurements at GELINA using a Li-glass scintillator. The gamma rays emitted during the neutron capture reactions were detected by C6D6 detectors at both GELINA and nTOF. Results: Resonance parameters of individual resonances up to 81 keV were extracted from a combined resonance shape analysis of experimental transmissions and capture yields. For the majority of the resonances the parity was determined from an analysis of the transmission data obtained with different sample thicknesses. Average resonance parameters were calculated. Conclusions: Maxwellian averaged cross sections were extracted from resonances observed up to 81 keV. The MACS for kT = 30 keV is fully consistent with experimental data reported in the literature. The MACSs for kT less than or similar to 15 keV are in good agreement with those derived from the ENDF/B-VIII.0 library and recommended in the KADoNTS database. For kT higher than 30 keV differences are observed. A comparison with MACSs obtained with the cross sections recommended in the JEFF-3.3 and JENDL-4.0 libraries shows discrepancies even for kT less than or similar to 15 keV. |
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Address |
[Tagliente, G.; Barbagallo, M.; Colonna, N.; Mastromarco, M.; Variale, V.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: giuseppe.tagliente@ba.infn.it |
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Publisher |
Amer Physical Soc |
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English |
Summary Language |
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Original Title |
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Abbreviated Series Title |
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ISSN |
2469-9985 |
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Notes |
WOS:000766732800002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5163 |
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